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Design and fabrication of photovoltaics based on MFS (Ag/BaTiO3/silicon p-type) structure

materials science for Energy Technologies 2024年第1期7卷 29-34页

作者： Irzaman Dahrul, M. Rahmani, M. Rukyati, A.M. Samsidar Nurhidayah Deswardani, F. Peslinof, M. Jenie, R.P. Iskandar, J. Wahyuni, Y. Priandana, K. Siskandar, R. Department of Physics Faculty of Mathematics and Natural Sciences IPB University Bogor16680 Indonesia Department of Physics Faculty of Sciences and Technology Jambi University Jambi36361 Indonesia Department of Nutrition Faculty of Health Science and Technology Binawan University East Jakarta13630 Indonesia Department of Computer Engineering Pakuan University Bogor16142 Indonesia Department of Computer Science IPB University Bogor16680 Indonesia Computer Engineering Technology Study Program College of Vocational Studies IPB University West Java Bogor16151 Indonesia

The experiment was carried out by growing BaTiO3 (Undoped or Li-doped) on p-type Si(1 0 0) substrates using the Chemical Solution Deposition (CSD) method and spin coating at a rotational speed of 3000 rpm for 60 s, followed by heating at 850 °C. The characterization results show that the bandgap energy value of the thin film due to lithium doping reduces the bandgap energy value. This is presumably because the donor atom added to a semiconductor causes the allowable energy level to be slightly below the conduction band. The presence of this new band causes the thin film bandgap energy to decrease with a five-valent tantalum dip. The morphological properties showed that the BaTiO3/Si(1 0 0) thin film particles in the deposited lithium had a fairly homogeneous grain. With the addition of lithium acetate as a binder into barium titanate, the grain size is getting smaller because it is suspected that the lithium-ion radius is smaller than the barium-ion radius. Measurement of I-V on the thin film shows that the output voltage value increases with more light intensity hitting the surface of the thin film. The greater the light intensity, the greater the energy of the photons, so the electrons are easier to jump. The three things above (both electrical and morphological properties) conclude that the thin films grown have the potential for photovoltaics. © 2023

关键词： Thin films

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Electronic structure and optical spectra of MSi2N4 (M = Mo, Ta, V) materials with single-atom decoration: a first-principles study

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Journal of materials Chemistry C 2023年第43期11卷 15097-15105页

作者： Wu, Tzu-Cheng Liao, Yin-Song Kao, Jui-Cheng Chou, Jyh-Pin Department of Physics National Tsing Hua University Hsinchu300044 Taiwan The Affiliated Senior High School of National Taiwan Normal University Taipei10658 Taiwan Tsing Hua Interdisciplinary Program National Tsing Hua University Hsinchu300044 Taiwan Department of Materials Science and Engineering National Tsing Hua University Hsinchu300044 Taiwan Department of Materials Science and Engineering National Yang Ming Chiao Tung University Hsinchu30010 Taiwan Department of Physics National Changhua University of Education Changhua50007 Taiwan

MoSi2N4 has outstanding potential for applications in electronics, spintronics, and semiconducting fabrication. This attractive scenario can be attributed to its remarkable electronic properties. In this study, we investigate the electronic structure and optical spectra of the MSi2N4 (M = Mo, Ta, and V) materials with single atom (H, N, and O) decoration using first-principles calculations. Pristine MoSi2N4 and VSi2N4 are semiconductors, and TaSi2N4 shows the half-metal properties. Decorating MoSi2N4 with single hydrogen and nitrogen atoms induces a magnetic moment. Single oxygen decorated TaSi2N4 does not change its intrinsic electronic properties, which is suitable for spintronic applications. On top of that, the semiconductor VSi2N4 can be turned into a half-metal via single hydrogen atom decoration. The absorption spectra demonstrate an enhancement in optical absorption for VSi2N4 after the decoration with a single nitrogen atom. Single atom decoration is one of the effective methods of tailoring the electronic properties of the two-dimensional MoSi2N4 family. Our findings can accelerate the development of the advanced electronic devices. © 2023 The Royal Society of Chemistry.

关键词： Silicon compounds

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Comparative Study of Testing Indigenous Air Filters for Fine PM Removal 1st

Comparative Study of Testing Indigenous Air Filters for Fine...

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1st International Conference on Pollution Control for Clean Environment, ICPCCE 2023

作者： Nawale, Prashant Sahu, Manoranjan Aerosol and Nanoparticle Technology Laboratory Environmental Science and Engineering Department Indian Institute of Technology Bombay Mumbai400076 India Interdisciplinary Program in Climate Studies Indian Institute of Technology Bombay Mumbai400076 India Centre for Machine Intelligence and Data Science Indian Institute of Technology Bombay Mumbai400076 India

ISBN: (纸本)9789819778454

Air pollution has become a serious global issue, which has significant impacts on both human health and the environment. Over the past decade, air quality has deteriorated due to various anthropogenic activities including construction, urbanization and industrialization. These activities release hazardous particles and harmful gases into the atmosphere, contributing to poor air quality. Developing countries such as India have been particularly affected, with some of their cities among the most polluted worldwide. To address this serious concern, it is imperative to develop and implement air pollution control technologies for both indoor and outdoor environments. This study focuses on the structured investigation of the performance of locally available air filter media in terms of their removal efficiency for submicron and micron-size particles. Various indigenous air filter media are subjected to rigorous testing to evaluate their overall and size-specific filtration efficiency and corresponding differential pressure drop. The results of these performance evaluations are then compared to their effectiveness in removing coarse and fine particles from the air. This research aims to provide valuable insights into the development of effective air filtration systems to combat air pollution. © The Author(s), under exclusive license to Springer Nature Singapore Pte Ltd. 2025.

关键词： Air filters Air pollution control technology Air purification Coarse PM Fine PM

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New insights into the hardening and pitting corrosion mechanisms of thermally aged duplex stainless steel at 475℃:A comparative study between 2205 and 2101 steels

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Journal of materials science & Technology 2022年第3期98卷 123-135页

作者： R.Silva G.S.Vacchi C.L.Kugelmeier I.G.R.Santos A.A.Mendes Filho D.C.C.Magalhães C.R.M.Afonso V.L.Sordi C.A.D.Rovere Munir Rachid Corrosion Laboratory Department of Materials EngineeringFederal University of São CarlosRodovia Washington Luis Km 23513565-905 São CarlosSPBrazil Engineering Modeling and Applied Social Sciences Center(CECS)Federal University of ABCAvenida dos Estados 500109210580 Santo AndréSPBrazil Federal University of São Carlos Graduate Program in Materials Science and EngineeringBrazil

In this study,the relationship between spinodal decomposition and the formation of Ni-rich clusters and G-phase in the ferrite on hardening and pitting corrosion of two thermally aged duplex stainless steels(DSSs)at 475℃was *** indicate that,for 2205 DSS,pitting corrosion behavior is influenced by the presence and size of G-phase precipitates for longer aging times,but this contribution is masked by the advanced stage of spinodal decomposition in the ferritic *** the other hand,for 2101 DSS,the formation of Cr-richer nitrides impairs pitting corrosion resistance more than spinodal decomposition.

关键词： Duplex stainless steel Spinodal decomposition G-phase precipitation Pitting corrosion Hardening

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Construction of SiO_x/nitrogen-doped carbon superstructures derived from rice husks for boosted lithium storage

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Journal of Colloid and Interface science 2022年第Part1期606卷 784-792页

作者： Guo, Xiaotian Li, Wenting Geng, Pengbiao Zhang, Qinyi Pang, Huan Xu, Qiang School of Chemistry and Chemical Engineering Yangzhou University Yangzhou 225009 Jiangsu China Department of Materials Science and Engineering and SUSTech Academy for Advanced Interdisciplinary Studies Southern University of Science and Technology (SUSTech) Xueyuan Ave Nanshan Shenzhen 518055 Guangdong China

Silicon sub-oxides (SiOx) are increasingly becoming a prospective anode material for lithium-ion batteries (LIBs). Nevertheless, inferior electrical conductivity and drastic volume fluctuation upon cycling significant... 详细信息

Silicon sub-oxides (SiO_x) are increasingly becoming a prospective anode material for lithium-ion batteries (LIBs). Nevertheless, inferior electrical conductivity and drastic volume fluctuation upon cycling significantly hamper the electrochemical performance of SiO_x. In this work, rice husks (RHs)-derived pitaya-like SiO_x/nitrogen-doped carbon (SNC) superstructures have been prepared by a simple electrospray-carbonization approach. SiO_x nanoparticles (NPs) are well-dispersed in a spherical nitrogen-doped carbon (NC) matrix. The carbon frameworks discourage the aggregation of SiO_x NPs, facilitating the kinetics for ion diffusion and charge transfer, and maintaining structural stability upon cycling, thus bringing about improved electrochemical performance. When the optimized SNC superstructures with SiO_x content of 64.3% are utilized as LIBs anodes, a stable specific capacity of 622.8 mA h g⁻¹ after 100 cycles at 0.1 A g⁻¹, and an excellent long cycle performance of 190.1 mA h g⁻¹ after 5000 cycles at 5 A g⁻¹ are obtained. This effective and universal synthetic strategy for fabricating controllable superstructures offers insights into the development of high-performance LIBs. © 2021 Elsevier Inc.

关键词： Electrospray Li-ion battery Nitrogen-doped carbon Rice husks-derived SiO2 Superstructure

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Rational construction and triethylamine sensing performance of foam shapedα-MoO_(3)@SnS_(2) nanosheets

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Chinese Chemical Letters 2022年第1期33卷 567-572页

作者： Xianhui Dong Qing Han Yaru Kang Haidong Li Xinyu Huang Zhengtao Fang Huimin Yuan Ahmed A.Elzatahry Zongtao Chi Guanglei Wu Wanfeng Xie School of Material Science&Engineering Institute of Materials for Energy and EnvironmentState Key Laboratory of Bio-Fibers and Eco-TextilesQingdao UniversityQingdao 266071China School of Electronics and Information Qingdao UniversityQingdao 266071China College of Physics and Electronic Engineering Qilu Normal UniversityJi'nan 250200China Materials Science and Technology Program College of Arts and SciencesQatar UniversityPO Box 2713DohaQatar

Owing to their high surface area,stable structure and easy fabrication,composite nanomaterials with encapsulation structures have attracted considerable research interest as sensing materials to detect volatile organic ***,a hydrothermal route is designed to prepare foam shapedα-MoO_(3)@SnS_(2)nanosheets that exhibit excellent sensing performance for triethylamine(TEA).The developed sensor,based onα-MoO_(3)@SnS_(2)nanosheets,displays a high response of 114.9 for 100 ppm TEA at a low working temperature of 175℃with sensitivity higher than many other reported *** addition,the device shows a wide concentration detection range(from 500 ppb to 500 ppm),good stability after exposure to air for 80 days,and excellent *** superior sensing characteristics of the developed sensor are attributed to the high crystallinity ofα-MoO_(3)/SnS_(2),excessive and accessible active sites provided by the good permeability of porous SnS_(2)shells,and the excellent conductivity of the encapsulation heterojunction ***,the foam shapedα-MoO_(3)@SnS_(2)nanosheets presented herein have promising practical applications in TEA gas sensing devices.

关键词： MoO_(3) SnS_(2) Encapsulation heterojunction Triethylamine Sensing performance

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Method for the extraction of circulating nucleic acids based on MOF reveals cell-free RNA signatures in liver cancer

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National science Review 2024年第1期11卷 94-106页

作者： Yuqing Sun Haixin Yu Shaoqing Han Ruoxi Ran Ying Yang Yongling Tang Yuhao Wang Wenhao Zhang Heng Tang Boqiao Fu Boshi Fu Xiaocheng Weng Song-Mei Liu Hexiang Deng Shuang Peng Xiang Zhou College of Chemistry and Molecular Sciences Key Laboratory of Biomedical Polymers-Ministry of Education Wuhan University Department of Digestive Surgical Oncology Union Hospital Tongji Medical College Huazhong University of Science and Technology Cancer Center Union HospitalTongji Medical CollegeHuazhong University of Science and Technology Department of Clinical Laboratory Center for Gene Diagnosis and Program of Clinical Laboratory Zhongnan Hospital of Wuhan University College of Chemistry and Materials Science Hubei Engineering University Department of Pharmacology School of Pharmacy China Medical University Taikang Center for Life and Medical Sciences Wuhan University Department of Hematology Zhongnan Hospital of Wuhan University

Cell-free RNA(cf RNA) allows assessment of health, status, and phenotype of a variety of human organs and is a potential biomarker to non-invasively diagnose numerous diseases. Nevertheless, there is a lack of highly efficient and bias-free cf RNA isolation technologies due to the low abundance and instability of cf ***, we developed a reproducible and high-efficiency isolation technology for different types of cell-free nucleic acids(containing cf RNA and viral RNA) in serum/plasma based on the inclusion of nucleic acids by metal-organic framework(MOF) materials, which greatly improved the isolation efficiency and was able to preserve RNA integrity compared with the most widely used research kit method. Importantly, the quality of cf RNA extracted by the MOF method is about 10-fold that of the kit method, and the MOF method isolates more than three times as many different RNA types as the kit method. The whole transcriptome mapping characteristics of cf RNA in serum from patients with liver cancer was described and a cf RNA signature with six cf RNAs was identified to diagnose liver cancer with high diagnostic efficiency(area under curve = 0.905 in the independent validation cohort) using this MOF method. Thus, this new MOF isolation technique will advance the field of liquid biopsy, with the potential to diagnose liver cancer.

关键词： MOF circulating cell-free RNA biomarker liver cancer diagnosis

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CsBr Immersion for Organic-Inorganic Hybrid Perovskite-Based Memristors: Controllable Grain, Poole-Frenkel Emission, and Electrical Properties

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ACS Applied Electronic materials 2023年第11期5卷 5916-5927页

作者： Chen, Yen-Shuo Lin, Ching Chang Lin, Chih Wei Tsai, Shang Yu Ko, Fu-Hsiang Department of Materials Science and Engineering National Yang Ming Chiao Tung University 1001 University Road Hsinchu30010 Taiwan Department of General Systems Studies Graduate School of Arts and Sciences The University of Tokyo 3-8-1 Komaba Tokyo153-8902 Japan

Organic-inorganic hybrid perovskites (OIHPs) have emerged as potential candidates for active layers in resistive switching memory (RSM) devices and have recently attracted much interest in academia and industry. In RSM devices based on the OIHPs, grain boundaries play an important role in the formation of resistive switching paths because the grain boundary regions contain many defects that favor the formation of conducting filaments. In this study, the effect of methylammonium lead iodide (MAPbI3)/indium tin oxide (ITO) substrates with various post-treatments on RSM devices is demonstrated. To reduce the defect density, variation of the immersion time of the MAPbI3 surface in CsI, MABr, and CsBr solutions promotes grain size enlargement and decreases the number of grain boundaries. The largest average grain size of the OIHP film obtained with 10 s of CsBr solution immersion (CsBr-10 s) for RSM devices is 1386.5 nm, and the corresponding photoluminescence (PL) intensity demonstrates the highest signal. The grain size can be well controlled by varying the immersion time in the ionic solution, and the appropriate post-treatment time is 10 s. Compared to untreated OIHP devices (on/off current ratio ∼102), perovskite film (MAPbI3)-based RSM devices with CsBr-10 s achieve a > 105 on/off current ratio and >104 s data retention. The conduction mechanism of the RSM devices with proper immersion treatment switches from the space-charge-limited current (SCLC) mechanism to Poole-Frenkel (PF) emission. This observation confirms that a low density of defects from fewer grain boundaries for RSM devices makes the conducting filaments in the memristors more susceptible to activation. Most OIHP-based devices suffer from humidity damage issues;however, the device fabrication and storage in our experiment are performed in ambient air. The results indicate that perovskite memory based on suitable ionic solution immersion exhibits great potential for use in future high-performance memri

关键词： Memristors

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engineering of dendritic dopant-free hole transport molecules:enabling ultrahigh fill factor in perovskite solar cells with optimized dendron construction

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science China Chemistry 2021年第1期64卷 41-51页

作者： Wei Chen Yang Wang Bin Liu Yajun Gao Ziang Wu Yongqiang Shi Yumin Tang Kun Yang Yujie Zhang Weipeng Sun Xiyuan Feng Frédéric Laquai Han Young Woo Aleksandra B.Djurisic Xugang Guo Zhubing He Department of Materials Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Department of Physics The University of Hong KongPokfulamHong KongChina King Abdullah University of Science and Technology KAUST Solar CenterPhysical Sciences and Engineering DivisionMaterial Science and Engineering ProgramThuwal 23955-6900Kingdom of Saudi Arabia Department of Chemistry Korea UniversitySeoul 02841South Korea

Developing dopant-free hole-transporting materials(HTMs)for high-performance perovskite solar cells(PVSCs)has been a very active research topic in recent years since HTMs play a critical role in optimizing interfacial charge carrier kinetics and in turn determining device ***,a novel dendritic engineering strategy is first utilized to design HTMs with a D-A type molecular framework,and diphenylamine and/or carbazole is selected as the building block for constructing *** HTMs show good thermal stability and excellent film morphology,and the key optoelectronic properties could be fine-tuned by varying the dendron *** them,MPA-Cz-BTI and MCz-Cz-BTI exhibit an improved interfacial contact with the perovskite active layer,and non-radiative recombination loss and charge transport loss can be effectively ***,high power conversion efficiencies(PCEs)of 20.8%and 21.35%are achieved for MPA-Cz-BTI and MCz-Cz-BTI based devices,respectively,accompanied by excellent long-term storage *** encouragingly,ultrahigh fill factors of 85.2%and 83.5%are recorded for both devices,which are among the highest values reported to *** work demonstrates the great potential of dendritic materials as a new type of dopant-free HTMs for high-performance PVSCs with excellent FF.

关键词： dendritic molecules hole-transporting materials dopant-free ultrahigh fill factor perovskite solar cells

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Scaled-up synthesis of defect-rich layered double hydroxide monolayers without organic species for efficient oxygen evolution reaction

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Green Energy & Environment 2022年第5期7卷 975-982页

作者： Haoyuan Chi Jingwen Dong Tian Li Sha Bai Ling Tan Jikang Wang Tianyang Shen Guihao Liu Lihong Liu Luyi Sun Yufei Zhao Yu-Fei Song State Key Laboratory of Chemical Resource Engineering Beijing University of Chemical TechnologyBeijing100029China College of Chemistry Key Laboratory of Theoretical&Computational Photochemistry of Ministry of EducationBeijing Normal UniversityBeijing100875China Polymer Program Institute of Materials Science and Department of Chemical&Biomolecular EngineeringUniversity of ConnecticutStorrsConnecticut06269USA Beijing Advanced Innovation Center for Soft Matter Science and Engineering Beijing University of Chemical TechnologyBeijing100029China

The scaled-up synthesis of organic-free monolayer nanomaterials is highly desirable,especially in obtaining green energy by *** this study,a method for the scaled-up synthesis of the series of monolayer layered double hydroxides(LDHs)without the addition of organic solvents is reported via the separate nucleation and aging steps *** resulting monolayer LDHs with the thicknesses of less than 1 nm showed a narrow thickness distribution.X-ray absorption fine-structure revealed that monolayer NiFe-LDH nanosheets have a number of oxygen and metal vacancies *** a practical application,monolayer NiFe-LDH nanosheets containing defects showed an enhanced electrocatalytic water oxidation activity compared with that of bulk *** functional theory calculations uncovered that excellent catalytic activity is attributed to vacancies *** proposed method is an economical and universally applicable strategy for the scaled-up production of monolayer LDHs.

关键词： process synthesis monolayer

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