Cytometry plays a crucial role in characterizing cell properties, but its restricted optical window (400-850 nm) limits the number of stained fluorophores that can be detected simultaneously and hampers the study and ...
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The side-chain has a significant influence on the optical properties and aggregation behaviors of the organic small molecule acceptors,which becomes an important strategy to optimize the photovoltaic performance of or...
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The side-chain has a significant influence on the optical properties and aggregation behaviors of the organic small molecule acceptors,which becomes an important strategy to optimize the photovoltaic performance of organic solar *** this work,we designed and synthesized three brand-new nonfused ring electron acceptors(NFREAs)OC4-4Cl-Ph,OC4-4Cl-Th,and OC4-4Cl-C8 with hexylbenzene,hexylthiophene,and octyl side chains on theπ-bridge *** with OC4-4Cl-Ph and OC4-4Cl-Th,OC4-4Cl-C8 with linear alkyl side chain has more red-shift absorption,which is conducive to obtaining higher short-circuit current ***,the OC4-4Cl-C8 film exhibits a longer exciton diffusion distance,and the D18:OC4-4Cl-C8 blend film displays faster hole transfer,weaker bimolecular recombination,and more efficient exciton ***,The D18:OC4-4Cl-C8 blend films may effectively form interpenetrating networks that resemble nanofibrils,which can facilitate exciton dissociation and charge ***,OC4-4Cl-C8-based devices can be created a marvellously power conversion efficiency(PCE)of 16.56%,which is much higher than OC4-4Cl-Ph(12.29%)-and OC4-4Cl-Th-based(11.00%)ones,being the highest PCE among the NFREA based binary *** in all,we have validated that side-chain engineering is an efficient way to achieve high-performance NFREAs.
Strong multiparticle interactions at room temperature (RT) lead to broadened homogeneous exciton linewidths in 2D semiconductors, degrading the quality of excitonic mode and emission. By coupling a Mie resonator with ...
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Electrochemical intercalation of lithium in titanium dioxide and silicon-based metasurfaces is used to initiate phase changes in a continuously tunable, reversible, and bistable manner for dynamic control over structu...
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Artificial intelligence has prevailed in all trades and professions due to the assistance of big data resources,advanced algorithms,and high-performance electronic ***,conventional computing hardware is inefficient at...
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Artificial intelligence has prevailed in all trades and professions due to the assistance of big data resources,advanced algorithms,and high-performance electronic ***,conventional computing hardware is inefficient at implementing complex tasks,in large part because the memory and processor in its computing architecture are separated,performing insufficiently in computing speed and energy *** recent years,optical neural networks(ONNs)have made a range of research progress in optical computing due to advantages such as subnanosecond latency,low heat dissipation,and high *** are in prospect to provide support regarding computing speed and energy consumption for the further development of artificial intelligence with a novel computing ***,we first introduce the design method and principle of ONNs based on various optical ***,we successively review the non-integrated ONNs consisting of volume optical components and the integrated ONNs composed of on-chip ***,we summarize and discuss the computational density,nonlinearity,scalability,and practical applications of ONNs,and comment on the challenges and perspectives of the ONNs in the future development trends.
Resistive random-access memory (RRAM) is one of the most promising candidates for next-generation nanoscale nonvolatile memory devices and neuromorphic computing applications. In this study, we developed a novel mixed...
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We report a split ring photonic crystal that demonstrates an order of magnitude larger peak energy density compared to traditional photonic crystals. The split ring offers highly focused optical energy in an accessibl...
Magnesium alloys containing biocompatible components show tremendous promise for applications as temporary biomedical devices. However, to ensure their safe use as biodegradeable implants, it is essential to control t...
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Magnesium alloys containing biocompatible components show tremendous promise for applications as temporary biomedical devices. However, to ensure their safe use as biodegradeable implants, it is essential to control their corrosion rates. In concentrated Mg alloys, a microgalvanic coupling between the α-Mg matrix and secondary precipitates exists which results in increased corrosion rate. To address this challenge, we engineered the microstructure of a biodegradable Mg-Zn-RE-Zr alloy by friction stir processing (FSP), improving its corrosion resistance and mechanical properties simultaneously. The FS processed alloy with refined grains and broken and uniformly distributed secondary precipitates showed a relatively uniform corrosion morphology accompanied with the formation of a stable passive layer on the alloy surface. In vivo corrosion evaluation of the processed alloy in a small animal model showed that the material was well-tolerated with no signs of inflammation or harmful by-products. Remarkably, the processed alloy supported bone until it healed till eight weeks with a low in vivo corrosion rate of 0.7 mm/year. Moreover, we analyzed blood and histology of the critical organs such as liver and kidney, which showed normal functionality and consistent ion and enzyme levels, throughout the 12- week study period. These results demonstrate that the processed Mg-Zn-RE-Zr alloy offers promising potential for osseointegration in bone tissue healing while also exhibiting controlled biodegradability due to its engineered microstructure. The results from the present study will have profound benefit for bone fracture management, particularly in pediatric and elderly patients.
Current-induced out of plane magnetization has been utilized for field-free switching of ferromagnets with perpendicular magnetic anisotropy. Identifying systems capable of energy-efficiently converting charge current...
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Current-induced out of plane magnetization has been utilized for field-free switching of ferromagnets with perpendicular magnetic anisotropy. Identifying systems capable of energy-efficiently converting charge currents into out of plane orbit- or spin-polarized currents is crucial for advancing magnetic memory technologies. Here we introduce the Berry curvature dipole as a key evaluation factor, directly measurable through nonlinear Hall effects. In the Weyl semimetal TaIrTe4 used in our experiments, applying a current parallel to the Berry curvature dipole results in out of plane orbital magnetization, which governs the field-free perpendicular magnetization switching in TaIrTe4/Fe3GaTe2 heterostructures. Notably, all-electric control of van der Waals magnetoresistive memory at room temperature has been achieved with a low critical current density ∼2×106A/cm2 for data writing. Our findings reveal the connection between nonlinear Hall effects and field-free magnetization switching, highlighting the potential of the Berry curvature dipole in advancing orbitronics.
We report on the observation of the linear anomalous Hall effect (AHE) in the nonmagnetic Weyl semimetal TaIrTe4. This is achieved by applying a direct current Idc and an alternating current Iω (Iω≪Idc) in TaIrTe4, ...
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We report on the observation of the linear anomalous Hall effect (AHE) in the nonmagnetic Weyl semimetal TaIrTe4. This is achieved by applying a direct current Idc and an alternating current Iω (Iω≪Idc) in TaIrTe4, where the former induces time-reversal symmetry breaking and the latter probes the triggered AHE. The anomalous Hall resistance VHω/Iω shows a linear dependence on Idc and changes sign with the polarity of Idc. In temperature-dependent measurements, VHω/Iω also experiences a sign reversal at ∼100 K, consistent with the temperature-dependent nonlinear Hall effect (NLHE). Furthermore, in measurements involving only dc transport, the dc Hall voltage exhibits a quadratic relationship with Idc. When the Idc direction is reversed, the Hall resistance changes sign, demonstrating a colossal nonreciprocal Hall effect (NRHE). Our theoretical calculations suggest that the observed linear AHE, NLHE, and NRHE all dominantly originate from the current-induced orbital magnetization compared to the minor spin contribution. This work provides deep insights into the orbital magnetoelectric effect and nonlinear Hall response, promising precise electric control of out-of-plane polarized orbit flow.
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