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Stretchable and self-healable spoof plasmonic meta-waveguide for wearable wireless communication system

Light(science & Applications) 2022年第11期11卷 2725-2737页

作者： Bu-Yun Yu De-Wei Yue Ke-Xin Hou Lu JU Hao Chen Cong Ding Zhen-Guo Liu Yun-Qian Dai Hari Krishna Bisoyi Ying-Shi Guan Wei-Bing Lu Cheng-Hui Li Quan Li State Key Laboratory of Millimeter Waves School of Information Science and EngineeringSoutheast UniversityNanjing 210096China Center for Flexible RF Technology Frontiers Science Center for Mobile Information Communication and SecuritySoutheast UniversityNanjing 210096China Purple Mountain Laboratories Nanjing 21111China State Key Laboratory of Coordination Chemistry School of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China Institute of Advanced Materials and School of Chemistry and Chemical Engineering Southeast UniversityNanjing 211189China Advanced Materials and Liquid Crystal Institute and Chemical Physics Interdisciplinary Program Kent State UniversityKentOH 44242USA

Microwave transmission lines in wearable systems are easily damaged after frequent mechanical deformation,posing a severe threat to wireless ***,we report a new strategy to achieve stretchable microwave transmission lines with superior reliability and durability by integrating a self-healable elastomer with serpentine-geometry plasmonic meta-waveguide to support the spoof surface plasmon polariton(SSPP).After mechanical damage,the self-healable elastomer can autonomously repair itself to maintain the electromagnetic performance and mechanical ***,the specially designed SSPP structure exhibits excellent stability and damage *** if the self-healing process has not been completed or the eventual repair effect is not ideal,the spoof plasmonic meta-waveguide Can still maintain reliable ***-healing material enhances strength and durability,while the SSPP improves stability and gives more tolerance to the self-healing *** design coordinates the structural design with material synthesis to maximize the advantages of the SSPP and self-healing material,signifcantly improving the relability and durability of stretchable microwave transmission *** also perform communication quality experiments to demonstrate the potential of the proposed meta-waveguide as interconnects in future body area network systems.

关键词： process durability maintain

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Polyetheretherketone with citrate potentiated influx of copper boosts osteogenesis,angiogenesis,and bacteria-triggered antibacterial abilities

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Journal of materials science & Technology 2021年第12期71卷 31-43页

作者： Jianglong Yan Dandan Xiab Pan Xionga Yangyang Li Wenhao Zhou Qiyao Li Pei Wang Yufeng Zheng Yan Cheng Academy for Advanced Interdisciplinary Studies Peking UniversityBeijing 100871China Department of Materials Science and Engineering College of EngineeringPeking UniversityBeijing 100871China Department of Biomedical Engineering Materials Research InstituteHuck Institutes of the Life SciencesThe Pennsylvania State UniversityUniversity ParkPA 16802USA The Science and Technology Bureau of Chengdu Chengdu Administration of Foreign Experts AffairsChengdu 610042China

A well designed coating for polyetheretherketone(PEEK)implants can provide enough support to overcome crucial medical challenges,which are insufficient osseointegration and high rate of ***,we utilize the co-deposition of polydopamine(PDA)and copper-citrate nanoclusters to construct a p H-responsive coating on porous PEEK for synergistic bone regeneration,vascular formation and ***,this PDA coating released high dose of copper and citrate at lower p H value,which increased intracellular copper content,boosted production of reactive oxygen species and severe damage of protein,leading to killing of 93%planktonic bacterial and eradication of adherent *** p H of 7.4,the release of copper and citrate were in a slow and sustained behavior,synergistically enhanced vascular formation potential and osteodiffereration of Ad-MSC in *** implanted in rabbit tibia for 6 and 12 weeks,the micro-CT evaluation and histological analysis consistently highlighted the ability of this PDA coating to increase new bone formation adjacent to coated PEEK implant and enhance bone-implant interfacial *** results were proven to be related to the synergistic effect that citrate facilitated a 2-fold influx of copper into cells,which not only enhanced the bacteria-killing ability but also encouraged bone regeneration of *** present work provides an effective method to control infections while promoting osseointegration simultaneously,which will show tremendous clinical application and can be a solution to current challenges facing orthopedics.

关键词： Citrate Copper Potentiated influx Bone regeneration Angiogenesis Bacteria-triggered coating

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Marine macro-litter sources and ecological impact: a review

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Environmental Chemistry Letters 2024年第3期22卷 1257-1273页

作者： Le, Van-Giang Nguyen, Hoang-Lam Nguyen, Minh-Ky Lin, Chitsan Hung, Nguyen T. Quang Khedulkar, Akhil P. Hue, Nguyen K. Trang, Phung T. Thu Mungray, Arvind Kumar Nguyen, D. Duc Central Institute for Natural Resources and Environmental Studies Vietnam National University Hanoi111000 Viet Nam Department of Civil Engineering McGill University MontrealQC Canada Faculty of Environment and Natural Resources Nong Lam University Hamlet 6 Linh Trung Ward Thu Duc City Ho Chi Minh City700000 Viet Nam Ph.D. Program in Maritime Science and Technology National Kaohsiung University of Science and Technology Kaohsiung81157 Taiwan Department of Marine Environmental Engineering National Kaohsiung University of Science and Technology Kaohsiung81157 Taiwan Department of Biomedical Engineering and Environmental Science National Tsing Hua University Hsinchu30013 Taiwan Environmental Research Center Institute of Hydrology and Meteorology Science and Climate Change Hanoi111000 Viet Nam Department of Chemical Engineering Sardar Vallabhbhai National Institute of Technology Gujarat Surat395007 India Department of Civil and Energy System Engineering Kyonggi University Suwon16227 Korea Republic of Institute of Applied and Sustainable Technology Nguyen Tat Thanh University Ho Chi Minh City700000 Viet Nam

Marine pollution by various debris is rising in the context of increasing urbanization, industrialization and worldwide trade. Here, we review marine macro-litter with focus on sources, abundance, distribution, and impact on aquatic wildlife, human health, and the economy. We observe that about 75–80% of marine litter originates from land-based sources, including poorly managed landfills and improper disposal. Macro-litter ingestion by marine life is of growing concern, in particular concerning the presence of plastics and associated pollutants, e.g., bisphenol A and phthalates, in fishes. These pollutants are accumulated and transferred to human via seafood. Marine plastic pollution induces a substantial rise of economic costs due to the decline of ecosystem services. Mitigation of marine plastic pollution should be done by following the ten Rs principles of refuse, rethink, reduce, re-use, repair, refurbish, remanufacture, repurpose, recycle, and recover. © The Author(s), under exclusive licence to Springer Nature Switzerland AG 2024.

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An expandable chamber for safe brain retraction: new technologies in the field of transcranial endoscopic surgery

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Journal of Zhejiang University-science B(Biomedicine & Biotechnology) 2023年第4期24卷 326-335页

作者： Elena ROCA Anna GOBETTI Giovanna CORNACCHIA Oscar VIVALDI Barbara BUFFOLI Giorgio RAMORINO Head and Neck Department NeurosurgeryIstituto Ospedaliero Fondazione Poliambulanza25124 BresciaItaly Technology for Health PhD Program University of Brescia25124 BresciaItaly Materials Science and Technology at Department of Mechanical and Industrial Engineering University of Brescia25123 BresciaItaly Metallurgy at Department of Mechanical and Industrial Engineering University of Brescia25123 BresciaItaly Anatomy and Physiopathology Division Department of Clinical and Experimental SciencesUniversity of Brescia25123 BresciaItaly

Neurosurgery is a highly specialized field:it often involves surgical manipulation of noble structures and cerebral retraction is frequently necessary to reach deep-seated brain *** are still no reliable methods preventing possible retraction *** objective of this study was to design work chambers well suited for transcranial endoscopic surgery while providing safe retraction of the surrounding brain *** chamber is designed to be inserted close to the intracranial point of interest;once it is best placed it can be *** should guarantee an appreciable workspace similar to that of current neurosurgical *** experimental aspect of this study involved the use of a force sensor to evaluate the pressures exerted on the brain tissue during the retraction *** pterional craniotomy,pressure measurements were made during retraction with the use of a conventional metal spatula with different *** that,although the force values necessary for retraction and exerted on the spatula by the neurosurgeon are the same,the local pressure exerted on the parenchyma at the edge of the spatula at different inclinations varied greatly.A new method of cerebral retraction using a chamber retractor(CR)has been designed to avoid any type of complication due to spatula edge overpressures and to maintain acceptable pressure values exerted on the parenchyma.

关键词： Brain retraction Spatula Brain retractor design Brain retraction injury Retraction complication Transcranial endoscopic surgery

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Impact of fabrication methods on binder distribution and charge transport in composite cathodes of all-solid-state batteries

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materials Futures 2023年第4期2卷 127-135页

作者： Benjamin Emley Chaoshan Wu Lihong Zhao Qing Ai Yanliang Liang Zhaoyang Chen Liqun Guo Tanguy Terlier Jun Lou Zheng Fan Yan Yao Materials Science and Engineering Program and Texas Center for Superconductivity at the University of Houston University of Houston4726 Calhoun RdHoustonTX 77204United States of America Department of Electrical and Computer Engineering University of Houston4726 Calhoun RdHoustonTX 77204United States of America Department of Materials Science and Nano Engineering Rice University6100 Main StreetHoustonTX 77005United States of America SIMS Laboratory Shared Equipment AuthorityRice UniversityHoustonTX 77005United States of America Department of Engineering Technology University of HoustonHoustonTX 77204United States of America

The manufacturing process of all-solid-state batteries necessitates the use of polymer ***,these binders,being ionic insulators by nature,can adversely affect charge transport within composite cathodes,thereby impacting the rate performance of the *** this work,we aim to investigate the impact of fabrication methods,specifically the solvent-free dry process versus the slurry-cast wet process,on binder distribution and charge transport in composite cathodes of solid-state *** the dry process,the binder forms a fibrous network,while the wet process results in binder coverage on the surface of cathode active *** difference in microstructure leads to a notable 20-fold increase in ionic conductivity in the dry-processed ***,the cells processed via the dry method exhibit higher capacity retention of 89%and 83%at C/3 and C/2 rates,respectively,in comparison to 68%and 58%for the wet-processed cells at the same *** findings provide valuable insights into the influence of fabrication methods on binder distribution and charge transport,contributing to a better understanding of the binder’s role in manufacturing of all-solid-state batteries.

关键词： solid-state battery solvent-free dry process polymer binder lithium thiophosphate electrolyte

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Perceiving the connection between the bone healing process and biodegradation of biodegradable metal implants through precise bioadaptability principle

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Journal of materials science & Technology 2023年第16期147卷 132-144页

作者： Yufeng Zheng Xiao Liu Danni Shen Wenting Li Yan Cheng Ming Yang Yuhui Kou Baoguo Jiang Academy for Advanced Interdisciplinary Studies Peking UniversityBeijing 100871China School of Materials Science and Engineering Peking UniversityBeijing 100871China International Research Organization for Advanced Science and Technology(IROAST) Kumamoto UniversityKumamoto 860-8555Japan Department of Orthopaedics and Traumatology Peking University People’s HospitalBeijing 100044China Key Laboratory of Trauma and Neural Regeneration(Peking University) Ministry of EducationBeijing 100044China National Center for Trauma Medicine Beijing 100044China

The implants made of metallic biomaterials help healing the bone fracture but also affect the bone repair *** proposed in Matter 4(2021)2548–2650 by Wang et al.,a precisely adaptable biomaterial ought to recapitulate the targeted tissue with spatiotemporal precision and hierarchical accuracy,ranging from atoms and molecules(genes,proteins,etc.)to cells(including organelles)and to tissues and *** comparison to traditional bio-inert metallic bone implants such as Co-based alloys and Ti alloys,biodegradable metal(Mg and Zn alloys)bone implants had been developed and might arise many unexpected variables in the bone repair,due to their bioactive *** this paper,the bone repair without and with the presence of metallic implants is ***,the perspectives concerning the interactions between the bone tissues and biodegradable metal implants are put forward,and how to better mimic in vivo biodegradation by in vitro experiments is proposed for further research and development of biodegradable metals.

关键词： Biodegradable metals Magnesium Zinc Bone healing Precise bioadaptability

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Experimental realization of supergrowing fields

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Physical Review Research 2024年第3期6卷 L032043页

作者： Sethuraj K. R. Tathagata Karmakar S. A. Wadood Andrew N. Jordan A. Nick Vamivakas The Institute of Optics Center for Coherence and Quantum Optics Department of Physics and Astronomy Institute for Quantum Studies Currently with Department of Electrical Engineering Materials Science

Supergrowth refers to the local amplitude growth rate of a signal being faster than its fastest Fourier mode. In contrast, superoscillation pertains to the variation of the phase. Compared to the latter, supergrowth can have exponentially higher intensities and promises improvement over superoscillation-based superresolution imaging. Here, we demonstrate the experimental synthesis of controlled supergrowing fields with a maximum growth rate of ∼19.07 times the system bandlimit. Our work is an essential step toward realizing supergrowth-based far-field superresolution imaging.

关键词： Imaging & optical processing

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Imaging atomic-scale chemistry from fused multi-modal electron microscopy

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npj Computational materials 2022年第1期8卷 164-171页

作者： Jonathan Schwartz Zichao Wendy Di Yi Jiang Alyssa J.Fielitz Don-Hyung Ha Sanjaya D.Perera Ismail El Baggari Richard D.Robinson Jeffrey A.Fessler Colin Ophus Steve Rozeveld Robert Hovden Department of Materials Science and Engineering University of MichiganAnn ArborMIUSA Mathematics and Computer Science Division Argonne National LaboratoryLemontILUSA Advanced Photon Source Facility Argonne National LaboratoryLemontILUSA Dow Chemical Co. MidlandMIUSA Department of Material Science and Engineering Cornell UniversityIthacaNew YorkUSA School of Integrative Engineering Chung-Ang UniversitySeoulRepublic of Korea Department of Physics Cornell UniversityIthacaNYUSA The Rowland Institute at Harvard CambridgeMAUSA Department of Electrical Engineering and Computer Science University of MichiganAnn ArborMIUSA National Center for Electron Microscopy Lawrence Berkeley National LaboratoryMolecular FoundryBerkeleyCAUSA Applied Physics Program University of MIchiganAnn ArborMIUnited States

Efforts to map atomic-scale chemistry at low doses with minimal noise using electron microscopes are fundamentally limited by inelastic ***,fused multi-modal electron microscopy offers high signal-to-noise ratio(SNR)recovery of material chemistry at nano-and atomic-resolution by coupling correlated information encoded within both elastic scattering(high-angle annular dark-field(HAADF))and inelastic spectroscopic signals(electron energy loss(EELS)or energy-dispersive x-ray(EDX)).By linking these simultaneously acquired signals,or modalities,the chemical distribution within nanomaterials can be imaged at significantly lower doses with existing detector *** many cases,the dose requirements can be reduced by over one order of *** high SNR recovery of chemistry is tested against simulated and experimental atomic resolution data of heterogeneous nanomaterials.

关键词： materials chemistry fused

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Ultrathin carbon biphenylene network as an anisotropic thermoelectric material with high temperature stability under mechanical strain

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Physical Review materials 2025年第2期9卷 024003-024003页

作者： Gözde Özbal Sargin Salih Demirci Kai Gong V. Ongun Özçelik Faculty of Engineering and Natural Sciences Sabanci University Istanbul 34956 Turkey Materials Science and Nano Engineering Program Sabanci University Istanbul 34956 Turkey Department of Physics Kirikkale University Kirikkale 71450 Turkey Department of Civil and Environmental Engineering Rice University Texas 77005 USA

Carbon biphenylene network (C-BPN), which is an ultrathin material consisting of carbon atoms arranged in square-hexagonal-octagonal (4-6-8) periodic rings, has intriguing properties for nano-scale device design due to its unique crystal structure. Here, using the Landauer formalism in combination with first-principles calculations, we show that C-BPN is a highly stable thermoelectric material at elevated temperatures under mechanical strain, where its thermoelectric efficiency can be anisotropically engineered. Transport calculations reveal that C-BPN's transmission spectrum has significant degrees of directional anisotropy and it undergoes a metal-insulator transition under strain, which leads to an increase in its Seebeck coefficient. C-BPN's lattice thermal conductance can be selectively tuned up to 35% bidirectionally at room temperature by strain engineering. Enhancement in its power factor and the suppression of its lattice thermal conductance improves the p-type figure of merit up to 0.31 and 0.46 at 300 and 500 K, respectively. Our findings reveal that C-BPN has high potency to be used in thermoelectric nanodevices with selective anisotropic properties at elevated temperatures.

关键词： Metal insulator transition

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Study of the growth mechanism of a self‑assembled and ordered multi‑dimensional heterojunction at atomic resolution

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Frontiers of Optoelectronics 2023年第4期16卷 37-48页

作者： Zunyu Liu Chaoyu Zhao Shuangfeng Jia Weiwei Meng Pei Li Shuwen Yan Yongfa Cheng Jinshui Miao Lei Zhang Yihua Gao Jianbo Wang Luying Li Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074China Ministry-of-Education Key Laboratory for the Green Preparation and Application of Functional Materials Hubei Collaborative Innovation Center for Advanced Organic Chemical MaterialsSchool of Materials Science and EngineeringHubei UniversityWuhan 430061China Center for Electron Microscopy MOE Key Laboratory of Artificial Micro-and Nano-Structures and the Institute for Advanced StudiesSchool of Physics and TechnologyWuhan UniversityWuhan 430072China State Key Laboratory of Infrared Physics Shanghai Institute of Technical PhysicsChinese Academy of SciencesShanghai 200083China

Multi-dimensional heterojunction materials have attracted much attention due to their intriguing properties,such as high efciency,wide band gap regulation,low dimensional limitation,versatility and *** further improve the performance of materials,researchers have combined materials with various dimensions using a wide variety of ***,research on growth mechanism of such composite materials is still *** this paper,the growth mechanism of multidimensional heterojunction composite material is studied using quasi-two-dimensional(quasi-2D)antimonene and quasione-dimensional(quasi-1D)antimony sulfde as *** are synthesized by a simple thermal injection *** is observed that the consequent nanorods are oriented along six-fold symmetric directions on the nanoplate,forming ordered quasi-1D/quasi-2D *** transmission electron microscopy(TEM)characterizations confrm the chemical information and reveal orientational relationship between Sb2S3 nanorods and the Sb nanoplate as *** density functional theory calculations indicate that interfacial binding energy is the primary deciding factor for the self-assembly of ordered *** details may fll the gaps in the research on multi-dimensional composite materials with ordered structures,and promote their future versatile applications.

关键词： Multi-dimensional composite materials Ordered heterostructures-Self-assembly Growth mechanism

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