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Strong enhancement of spin-orbit torques in ferrimagnetic Ptx(Si3N4)1–x/CoTb bilayers by Si3N4 doping

Physical Review B 2022年第14期106卷 L140407-L140407页

作者： Xin Lin Jingwei Li Lujun Zhu Xinyue Xie Qianbiao Liu Dahai Wei Guodong Yuan Lijun Zhu State Key Laboratory of Superlattices and Microstructures Institute of Semiconductors Chinese Academy of Sciences Beijing 100083 China College of Materials Science and Opto-Electronic Technology University of Chinese Academy of Sciences Beijing 100049 China Multi-scale Porous Materials Center Institute of Advanced Interdisciplinary Studies and School of Chemistry and Chemical Engineering Chongqing University Chongqing 400044 China College of Physics and Information Technology Shaanxi Normal University Xi'an 710062 China

We report strong enhancement of spin-orbit torques by incorporating Si3N4 impurities into the dirty metal Pt. We find that the Si3N4 impurities lower the spin Hall conductivity and the charge conductivity of the Pt host at different rates, leading to a twofold increase in the dampinglike spin-orbit torque per unit current density for ferrimagnetic Ptx(Si3N4)1–x/Co0.65Tb0.35 bilayers. This torque enhancement is attributed to the optimized trade-off between the intrinsic spin Hall conductivity and the spin carrier lifetime in the dirty limit. We also find that only 58% of the angular momentum of the spin current entering the ferrimagnetic Co0.65Tb0.35 relaxes via exchange interaction and thus makes a contribution to spin torque generation. This work establishes Pt0.7(Si3N4)0.3 with a high spin Hall ratio of 0.8 and a high charge conductivity of 1.2×106Ω−1m−1 as a compelling spin Hall metal for spin-orbitronics. This work also reaffirms the variation of the spin-orbit torque with relative spin relaxation rates within the magnetic layer.

关键词： Bilayers Spin Hall effect Spin-orbit torque Ferrimagnets

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Effect of double coating on microencapsulation of levofloxacin using the particles from gas-saturated solutions process as a controlled-release system

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Discover Chemistry 2025年第1期2卷 1-13页

作者： Sharmin, Tanjina Takeshita, Toshihiro Ouchi, Mikio Yoshida, Koji Znad, Hussein Saptoro, Agus Sarker, Zaidul Islam Irie, Keiichi Satho, Tomomitsu Nioh, Atsushi Masuda, Takaaki Muneyoshi, Yuuki Terayama, Suzuko Mishima, Kenji Department of Chemical Engineering Faculty of Engineering Fukuoka University Fukuoka Japan Research Institute of Composite Materials Fukuoka University Fukuoka Japan Resource Circulation Faculty of Environmental Engineering Fukuoka University Fukuoka Japan Faculty of Sciences Fukuoka University Fukuoka Japan Western Australian School of Mines: Minerals Energy and Chemical Engineering Faculty of Science and Engineering Curtin University Perth Australia Department of Chemical Engineering Faculty of Engineering Curtin Malaysia Graduate School Miri Sarawak Malaysia Department of State Program and Food Science Northern Marianas College Saipan USA Faculty of Pharmaceutical Sciences Fukuoka University Fukuoka Japan Yokohama Research Center Pola Chemical Industries Yokohama Japan

A novel double-coating technique was employed to encapsulate levofloxacin (LVF), a potent antibacterial drug, using the particles from gas-saturated solutions (PGSS) process to achieve extended release. The primary coating utilized glyceryl tristearate (GT), a lipid with a high melting point (72 °C), followed by a secondary coating with trimyristin (TM), a lipid with a lower melting point (52 °C). For comparison, a single-coating approach was also explored, using the biocompatible polymer poly-(ε-caprolactone) (PCL). The resulting particles were characterized for their shape, size, and LVF encapsulation efficiency, with confirmation of LVF entrapment provided by Fourier transform infrared (FTIR) spectroscopy, and X‐ray powder diffraction (XRD) analysis. The particles, with an average diameter of 95.3 ± 16.5 μm, exhibited an encapsulation efficiency of up to 92.1 ± 2.5%. Furthermore, in vitro release studies revealed that the double-coated microcapsules effectively suppressed the initial burst release and provided controlled, extended release of LVF (t30D = 36.3%), demonstrating the efficiency of this encapsulation method for prolonged drug delivery.

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Challenges of measuring spin Seebeck noise

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Physical Review B 2024年第10期109卷 104429-104429页

作者： Renjie Luo Xuanhan Zhao Tanner J. Legvold Liyang Chen Changjiang Liu Deshun Hong Anand Bhattacharya Douglas Natelson Department of Physics and Astronomy Rice University Houston Texas 77005 USA Applied Physics Program Smalley-Curl Institute Rice University Houston Texas 77005 USA Materials Science Division Argonne National Laboratory Lemont Illinois 60439 USA Department of Electrical and Computer Engineering Rice University Houston Texas 77005 USA Department of Materials Science and NanoEngineering Rice University Houston Texas 77005 USA

Just as electronic shot noise in driven conductors results from the granularity of charge and the statistical variation in the arrival times of charge carriers, there are predictions for fundamental noise in magnon currents due to angular momentum being carried by discrete excitations. The inverse spin Hall effect as a transduction mechanism to convert spin current into charge current raises the prospect of experimental investigations of such magnon shot noise. Spin Seebeck effect measurements have demonstrated the electrical detection of thermally driven magnon currents and have been suggested as an avenue for accessing spin current fluctuations. Using spin Seebeck structures made from yttrium iron garnet on gadolinium gallium garnet, we demonstrate the technical challenges inherent in such noise measurements. While there is a small increase in voltage noise in the inverse spin Hall detector at low temperatures associated with adding a magnetic field, the dependence on field orientation implies that this is not due to magnon shot noise. We describe theoretical predictions for the expected magnitude of magnon shot noise, highlighting ambiguities that exist. Further, we show that magnon shot noise detection through the standard inverse spin Hall approach is likely impossible due to geometric factors. Implications for future attempts to measure magnon shot noise are discussed.

关键词： Spin Seebeck effect Spin current Magnetic insulators Noise measurements

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Cathode-Electrolyte Interphase engineering through Artificial Surface Coating in 4.55 V High-Voltage LiCoO2 Cathodes

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ACS applied materials & interfaces 2025年第22期17卷 2025 May 23页

作者： Xianbin Wei Qing Zhang Mei Shen Xiaobo Shi Duojie Wu Cheng Zhen Menghao Li Zhen Zhang Xuming Yang Jiangfeng Li M Danny Gu School of Materials Science and Engineering Harbin Institute of Technology Harbin 150001 China. Eastern Institute for Advanced Study Eastern Institute of Technology Ningbo 315200 Zhejiang P. R. China. Department of Materials Science and Engineering Southern University of Science and Technology (SUSTech) Shenzhen 518055 China. College of Integrated Circuits Shenzhen Polytechnic University Shenzhen 518052 China. Academy for Advanced Interdisciplinary Studies Southern University of Science and Technology (SUSTech) Shenzhen 518055 China. School and Hospital of Stomatology Hebei Medical University Shijiazhuang 050017 PR China. Graphene Composite Research Center College of Chemistry and Environmental Engineering Shenzhen University Shenzhen 518060 China.

Increasing the high cutoff potential of LiCoO (LCO) has proven challenging, due to lattice structure deterioration and cathode electrolyte interphase (CEI) instability. This work reports an effective strategy for tuning the CEI and stabilizing the cathode surface structure; we used atomic layer deposition (ALD) to synthesize AlO-capped LCO (ACLCO). Direct cryogenic transmission electron microscopy (cryo-TEM) characterization of the CEI reveals that, at 4.55 V voltage, ACLCO suppresses unstable CEI growth and enhances the stability of the layered LCO lattice. More specifically, as the cycling process drives electrolyte corrosion, the AlO surface coating partially transforms into a thermodynamically stable AlF layer, which inhibits continuous side reactions in the high oxidation state, protecting the layered crystal lattice from transformation to rock-salt phases. Our comprehensive study describes a new technique for direct visualization of the CEI, demonstrates the efficacy of ACLCO, and reveals the mechanism by which it stabilizes the LCO cathode.

关键词： Li-ion Battery LiCoO2 atomic layer deposition cathode-electrolyte interphase cryo-TEM

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Spin transport of half-metal Mn_(2)X_(3) with high Curie temperature:An ideal giant magnetoresistance device from electrical and thermal drives

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Frontiers of physics 2024年第4期19卷 125-135页

作者： Bin Liu Xiaolin Zhang Jingxian Xiong Xiuyang Pang Sheng Liu Zixin Yang Qiang Yu Honggen Li Sicong Zhu Jian Wu Hubei Province Key Laboratory of Systems Science in Metallurgical Process The State Key Laboratory for Refractories and MetallurgyCollaborative Innovation Center for Advanced SteelsInternational Research Institute for Steel TechnologyWuhan University of Science and TechnologyWuhan 430081China Key Laboratory of Artificial Micro-and Nano-structures of Ministry of Education and School of Physical and Technology Wuhan UniversityWuhan 430072China College of Advanced Interdisciplinary Studies Nanhu Laser LaboratoryNational University of Defense TechnologyChangsha 410073China Department of Mechanical Engineering National University of SingaporeSingapore 117575Singapore i-Lab&Key Laboratory of Nanodevices and Applications&Key Laboratory of Nanophotonic Materials and Devices Suzhou Institute of Nano-Tech and NanoBionicsChinese Academy of SciencesSuzhou 215123China Institute of Optical Science and Technology School of Physics and AstronomyShanghai Jiao Tong UniversityShanghai 200240China

Currently,magnetic storage devices are encountering the problem of achieving lightweight and high integration in mobile computing devices during the information *** a result,there is a growing urgency for twodimensional half-metallic materials with a high Curie temperature(TC).This study presents a theoretical investigation of the fundamental electromagnetic properties of the monolayer hexagonal lattice of Mn_(2)X_(3)(X=S,Se,Te).Additionally,the potential application of Mn_(2)X_(3) as magneto-resistive components is *** three of them fall into the category of ferromagnetic *** particular,the Monte Carlo simulations indicate that the TC of Mn2S3 reachs 381 K,noticeably greater than room *** findings present notable advantages for the application of Mn2S3 in spintronic ***,a prominent spin filtering effect is apparent when employing non-equilibrium Green’s function simulations to examine the transport *** resulting current magnitude is approximately 2×10^(4) nA,while the peak gigantic magnetoresistance exhibits a substantial value of 8.36×10^(16)%.It is noteworthy that the device demonstrates a substantial spin Seebeck effect when the temperature differential between the electrodes is *** brief,Mn_(2)X_(3) exhibits outstanding features as a highTC half-metal,exhibiting exceptional capabilities in electrical and thermal drives spin ***,it holds great potential for usage in spintronics applications.

关键词： half-metals Mn_(2)X_(3) high Curie temperature electrical and thermal GMR

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Opto2P-FCM: A MEMS Based Miniature Two-Photon Microscope with Patterned Optogenetic Stimulation

Opto2P-FCM: A MEMS Based Miniature Two-Photon Microscope wit...

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Microscopy Histopathology and Analytics, Microscopy 2024 - Part of Optica Biophotonics Congress: Biomedical Optics

作者： Futia, Gregory L. Zohrabi, Mo McCullough, Connor Teel, Alec de Souza, Fabio Simoes Oroke, Ryan Bright, Victor M. Restrepo, Diego Gopinath, Juliet T. Gibson, Emily A. Department of Bioengineering University of Colorado Anschutz Medical Campus AuroraCO80045 United States Department of Cell and Developmental Biology University of Colorado Anschutz Medical Campus AuroraCO80045 United States Department of Electrical Computer and Energy Engineering University of Colorado BoulderCO80309 United States Department of Mechanical Engineering University of Colorado BoulderCO80309 United States Department of Physics University of Colorado BoulderCO80309 United States Materials Science and Engineering Program University of Colorado BoulderCO80309 United States

Miniaturized microscopes for monitoring neural activity are an indispensable tool for neuroscience research. We present a novel MEMS based miniature microscope with patterned optogenetic stimulation capabilities enabl... 详细信息

ISBN: (纸本)9781957171340

关键词： Microscopes

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Ultrafine-Grained Stainless Steel with Wear-Resistant Nanoborides Decorating Grain Boundaries Produced by Laser Powder Bed Fusion

SSRN

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SSRN 2024年

作者： Martins Freitas, Brenda Juliet Koga, Guilherme Yuuki Miguel Rodrigues, Luana Cristina Botta Filho, Walter José Amancio-Filho, Sergio de Traglia Bolfarini, Claudemiro Federal University of São Carlos Graduate Program in Materials Science and Engineering São Carlos13.565-905 Brazil Graz University of Technology Institute of Materials Science Joining and Forming Graz8010 Austria Federal University of São Carlos Department of Materials Engineering São Carlos13.565-905 Brazil Rod. Washington Luis São Carlos13565-905 Brazil

Stainless steel composites combine corrosion resistance and toughness of the metallic matrix with wear resistance granted by hard reinforcing nanoparticles. Given their near-net-shape manufacturing characteristics, additive manufacturing techniques are attractive to produce these hard and wear-resistant classes of materials with low machinability. In this work, from a SAF 2205 duplex stainless steel with boron addition, laser powder bed fusion (LBPF) was employed to produce an ultrafine-grained (~1 µm), dense (porosity ~0.1%), and crack-free ferritic-induced matrix composite with Cr2B-nanoborides reinforcing the grain boundaries (GBs) without formation of Cr-depleted regions. The composite showed significant higher hardness (up to 456 HV0.5) and wear resistance (4.4 x 10-5 mm3 N-1m-1) in sliding condition compared to a hot-rolled (225 HV0.5 and 2.9 x 10-3 mm3 N-1m-1) and a LPBF-produced SAF 2205 (314 HV0.5 and 3.3 x 10-4 mm3 N-1m-1). © 2024, The Authors. All rights reserved.

关键词： Wear of materials

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Optimizing Lpbf-Parameters by Box-Behnken Design Allows to Print Crack-Free and Dense High-Boron Alloyed Stainless Steels

SSRN

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SSRN 2024年

作者： Freitas, Brenda Juliet Martins Koga, Guilherme Yuuki Arneitz, Siegfried Bolfarini, Claudemiro de Traglia Amancio-Filho, Sergio Federal University of São Carlos Graduate Program in Materials Science and Engineering São Carlos13.565-905 Brazil Graz University of Technology Institute of Materials Science Joining and Forming Graz8010 Austria Federal University of São Carlos Department of Materials Engineering São Carlos13.565-905 Brazil Rod. Washington Luis São Carlos13565-905 Brazil

Boron has almost null solubility in iron, and its addition to stainless steels leads to the formation of hard borides, beneficial for increasing the wear resistance. However, these boron-containing steels have poor printability, with the occurrence of pronounced cracking, high porosity and risk of delamination. In this work Box-Behnken design coupled to analysis of variance (ANOVA) were used to optimize the LPBF (Laser Powder Bed Fusion) processing parameters of a highly boron-alloyed stainless steel reinforced with a boride network. The proposed models demonstrated to be accurate to determine the porosity percentage for the studied alloys, in which the laser power and scanning speed play the main role on the alloys’ densification, and absence of extensive defects. These results indicate that the use of design of experiments tools are essential to produce defect-free boron-modified stainless steel specimens with a relatively low number of experiments, identifying a narrow optimized processing window to build bulk composite materials. © 2024, The Authors. All rights reserved.

关键词： Design of experiments

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Multi Task Classification Using Deep Learning Approaches for Big Five Personality Traits Prediction: A Review

Multi Task Classification Using Deep Learning Approaches for...

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International Conference on Information Technology, Computer and Electrical engineering (ICITACEE)

作者： Salamun Rohman Nudin Rahmat Gernowo Maman Somantri Adi Wibowo Doctoral Program of Information System School of Postgraduate Studies Diponegoro University Semarang Indonesia Department of Physics Faculty of Science and Mathematics Diponegoro University Semarang Indonesia Department of Electrical Engineering Faculty of Engineering Diponegoro University Semarang Indonesia Department of Informatics Faculty of Science and Mathematics Diponegoro University Semarang Indonesia

ISBN: (数字)9798350389302

ISBN: (纸本)9798350389319

This paper presents a comprehensive review of deep learning methods for the Big Five personality traits prediction using multi-task classification. The purpose of the review is to determine the performance of models developed in previous research to describe research opportunities and challenges in the future. The Big Five model is a framework in psychology that categorizes human personality into five dimensions: openness, conscientiousness, extraversion, agreeableness, and neuroticism. The review begins by analyzing 22 articles from the science Direct, IEEE Xplore, and Scopus databases by applying screening using the Big Five Personality keywords. Then study the concepts of deep learning for model development such as: input, architecture, method, dataset, and performance to identify the strengths and limitations of each approach. The review results of the highest average accuracy by modality such as unimodal text with essay dataset (80.98 % ), unimodal image with ImageNet dataset (95.36%), unimodal audio with SSPNet dataset (79.48%), bimodal image and audio with Chalearn Video First Impression dataset (91.67 % ), multimodal text, image, and audio with Chalearn Video First Impression dataset (91.88%). The average accuracy of the Big Five Personality traits was highest (95.36 % ) and lowest (59 % ). This highlights the need for standard benchmarks, interpretable models and interdisciplinary collaboration to improve the accuracy, reliability and ethical implications of personality prediction. Future research is expected to pave the way for advancements in understanding human personality through deep learning approaches using other modalities such as EEG, GSR, and PPG.

关键词： Deep learning Accuracy Reviews Psychology Predictive models Brain modeling Multitasking Reliability Information technology Standards

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Textured BaTiO3 nanorod arrays synthesized via hydrothermal method: Enhanced degradation of Rhodamine B with piezocatalysis

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Ceramics International 2025年

作者： Chiu, Yen-Lun Chang, Kao-Shuo Program on Key Materials Academy of Innovative Semiconductor and Sustainable Manufacturing National Cheng Kung University No.1 University Road Tainan City70101 Taiwan Department of Materials Science & Engineering National Cheng Kung University No.1 University Road Tainan City70101 Taiwan

This paper presents a hydrothermal method for fabricating textured BaTiO3 (BTO) nanorod arrays with high crystallinity on fluorine-doped tin oxide (FTO) substrates by applying a polarization treatment to the samples to explore the feasibility of enhancing their piezoelectric properties. The preparation of highly textured BTO nanorod arrays using a two-step hydrothermal process was investigated in detail, including the spin-coating process for depositing the TiO2 seed layer, the influence of solution acidity on the hydrothermal synthesis of TiO2 nanorod arrays, and the formation mechanism of textured BTO nanostructures. The piezoelectric constants (d33) of the samples were determined using piezoresponse force microscopy. S-BTO(P), which has high crystallinity and preferential orientation, achieves a d33 as high as 85.4 p.m./V after poling, which is 3.2 times higher than that without textured structures and poling. Our findings revealed that chemically controlling and inducing a preferential orientation in the crystal structure of piezoelectric materials with a seed layer and specific hydrothermal conditions can significantly enhance their piezoelectric properties after poling, making them excellent candidates for piezoelectric devices. Especially, this study confirms that the piezoelectric-enhanced charge separation in poled BTO nanorod arrays enables efficient generation of reactive species under ultrasonication, leading to effective degradation of RhB. The strong piezocatalytic performance highlights the material's potential for practical applications in environmental pollutant removal. © 2025 Elsevier Ltd and Techna Group S.r.l.

关键词： Piezoelectricity

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