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Electron scattering by Friedel oscillations in carbon nanotubes

Nano research 2022年第2期15卷 889-897页

作者： Takumi Inaba Takahiro Morimoto Satoshi Yamazaki Toshiya Okazaki CNT-Application Research Center National Institute of Advanced Industrial Science and TechnologyTsukuba 305-8565Japan Research Association of High-Throughput Design and Development for Advanced Functional Materials Tsukuba 305-8565Japan

Multi-walled carbon nanotube networks were confirmed to exhibit a linear decrease in resistivity with increasing temperature from 100 to above 400 *** linearity was explained using a defect scattering model that involved Friedel oscillations(that is,electron-electron interactions).The applicability of this model,which was originally proposed for graphene,to carbon nanotubes was assessed based on a comparison of various experimental *** in the slopes of the resistivity-temperature plots following the introduction of defects,as well as an effect of charge concentration on the slope were key predictions of this *** results obtained from few-walled carbon nanotube networks are also *** the literature,linear resistivity-temperature plots were obtained from other graphene derivatives,indicating that the linearity originates from the hexagonal symmetry of these *** present work also indicated a relationship between the appearance of linearity and negative magnetoresistance above 100 *** on a mechanism incorporating scattering in association with Friedel oscillations and conventional electron conduction models,the universality of resistivity-temperature plots obtained from carbon nanotube networks is introduced.

关键词： carbon nanotube electron transport electron-electron interaction Friedel oscillations magnetoresistance

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Micro and Macroscopic Structure Evolution of Few-Walled Carbon Nanotube Bundled Network by high Temperature Anneal

SSRN

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SSRN 2022年

作者： Kobashi, Kazufumi Yamazaki, Satoshi Michishio, Koji Nakajima, Hideaki Muroga, Shun Morimoto, Takahiro Oshima, Nagayasu Okazaki, Toshiya Tsukuba Central 5 1-1-1 Higashi Ibaraki Tsukuba305-8565 Japan Research Association of High-Throughput Design and Development for Advanced Functional Materials Ibaraki Tsukuba305-8565 Japan Tsukuba Central 2 1-1-1 Umezono Ibaraki Tsukuba305-8568 Japan

high temperature anneal is of importance to create nanocarbon-based materials with excellent functions and performances. However, a comprehensive understanding on annealed nanocarbon assembly structures has been challenging. We successfully propose the micro and macroscopic structural analysis of 0.8-3.4 nm diameter few-walled carbon nanotube (CNT) bundled network by a multifaceted characterization, which was annealed over 1200-3000oC in the form of a film as the case study. Up to 1800oC carbonaceous impurities were removed to secure nanospace among nanotubes, i.e. interstitial channels important to design multiple functions. Beyond 1900oC nanoscale graphitic particles were generated on the nanotube bundles, then grown to be micro-meter scale toward 3000oC. Parallel to the particle growth, small diameter ( © 2022, The Authors. All rights reserved.

关键词： Annealing

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Number Density Descriptor on Extended-Connectivity Fingerprints Combined with Machine Learning Approaches for Predicting Polymer Properties

Number Density Descriptor on Extended-Connectivity Fingerpri...

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MRS Advances

作者： Minami, Takuya Okuno, Yoshishige Research Association of High-Throughput Design Development for Advanced Functional Materials Ibaraki Japan

Abstract We developed a new type of polymer descriptor based on Extended Connectivity Fingerprints. The number densities, that are substructure numbers divided by the number of atoms in a polymer model, were employed. We found that this approach is superior in accurately predicting linear polymer properties, compared to the conventional approach, where just the substructure numbers are used as descriptors. In addition, dimension reduction and multiple replication of repeat unit were found to improve prediction accuracy. As a result, the novel descriptor based on the Extended Connectivity Fingerprints with machine learning approaches was found to achieve accurate prediction of the refractive indices of linear polymers, which is comparable to that by ab initio density functional theory. Although process-dependent properties such as mechanical properties were difficult to predict, the present approach was found to be applicable to prediction of substructure-dependent properties, for example, optical properties, thermal stabilities. Copyright © materials research Society 2018Â.

关键词： Refractive index

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Prediction of repeat unit of optimal polymer by Bayesian optimization

Prediction of repeat unit of optimal polymer by Bayesian opt...

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MRS Advances

作者： Minami, Takuya Kawata, Masaaki Fujita, Toshio Murofushi, Katsumi Uchida, Hiroshi Omori, Kazuhiro Okuno, Yoshishige Research Association of High-Throughput Design and Development for Advanced Functional Materials Tsukuba Ibaraki305-8568 Japan Showa Denko K.K. Minato-ku Tokyo105-8518 Japan Tsukuba Ibaraki305-8568 Japan

design processes of functional polymers were accelerated by adopting the Bayesian optimization;the number of trials in the process was substantially reduced. The optimization process was more than forty time accelerated to find out the target polymer compared to the random selection. The optimization efficiency was found to be successfully improved by utilizing the standard deviation of predicted probability distribution of objective function. The performance of the method was robust for dataset size in the analysis;the target polymer could be found even for a small training dataset. The proposed method is a promising tool for the high-performance polymer design, and a wide range of its applications will be expected in the polymer industry. Copyright © materials research Society 2019.

关键词： Probability distributions

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Contributory presentations/posters

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Journal of Biosciences 1999年第1期24卷 33-198页

作者： N. Manoj V. R. Srinivas A. Surolia M. Vijayan K. Suguna R. Ravishankar R. Schwarzenbacher K. Zeth Diederichs G. M. Kostner A. Gries P. Laggner R. Prassl Madhusudan Pearl Akamine Nguyen-huu Xuong Susan S. Taylor M. Bidva Sagar K. Saikrishnan S. Roy K. Purnapatre P. Handa U. Varshney B. K. Biswal N. Sukumar J. K. Mohana Rao A. Johnson Vasantha Pattabhi S. Sri Krishna Mira Sastri H. S. Savithri M. R. N. Murthy Bindu Pillai Kannan M. V. Hosur Mukesh Kumar Swati Patwardhan K. K. Kannan B. Padmanabhaa S. Sasaki-Sugio M. Nukaga T. Matsuzaki S. Karthikevan S. Sharma A. K. Sharma M. Paramasivam P. Kumar J. A. Khan S. Yadav A. Srinivasan T. P. Singh S. Gourinath Neelima Alam A. Srintvasan Vikas Chandra Punit Kaur Ch. Betzel S. Ghosh A. K. Bera S. Bhattacharya S. Chakraborty A. K. Pal B. P. Mukhopadhyay I. Dey U. Haldar Asok Baneriee Jozef Sevcik Adriana Solovicova K. Sekar M. Sundaralingam N. Genov Dong-cai Liang Tao Jiang Ji-ping Zhang Wen-rui Chang Wolfgang Jahnke Marcel Blommers S. C. Panchal R. V. Hosur Bindu Pillay Puniti Mathur S. Srivatsun Ratan Mani Joshi N. R. Jaganathan V. S. Chauhan H. S. Atreya S. C. Sahu K. V. R. Chary Girjesh Govil Elisabeth Adjadj Éric Quinjou Nadia Izadi-Pruneyre Yves Blouquit Joël Mispelter Bernadette Heyd Guilhem Lerat Philippe Milnard Michel Desmadreil Y. Lin B. D. Nageswara Rao Vidva Raghunathan Mei H. Chau Prashant Pesais Sudha Srivastava Evans Coutinho Anil Saran Leizl F. Sapico Jayson Gesme Herbert Lijima Raymond Paxton Thamarapu Srikrishnan C. R. Grace G. Nagenagowda A. M. Lynn Sudha M. Cowsik Sarata C. Sahu S. Chauhan A. Bhattacharya G. Govil Anil Kumar Maurizio Pellecchia Erik R. P. Zuiderweg Keiichi Kawano Tomoyasu Aizawa Naoki Fujitani Yoichi Hayakawa Atsushi Ohnishi Tadayasu Ohkubo Yasuhiro Kumaki Kunio Hikichi Katsutoshi Nitta V. Rani Parvathy R. M. Kini Takumi Koshiba Yoshihiro Kobashigawa Min Yao Makoto Demura Astushi Nakagawa Isao Tanaka Kunihiro Kuwajima Jens Linge Seán O. Donoghue Michael Nilges G. Chakshusmathi Girish S. Ratnaparkhi P. K. Madhu R. Varadarajan C. Tetreau Molecular Biophysics Unit Indian Institute of Science Bangalore India Austrian Academy of Sciences Institute of Biophysics and X-ray Structure Research Graz Austria Faculty of Biology University of Konstanz Germany Institute of Medical Biochemistry University of Graz Austria Howard Huges Medical Institute Department of Chemistry & Biochemistry University of California La Jolla USA Department of Chemistry & Biochemistry University of California San Diego La Jolla USA Molecular Biophysics Unit India Department of Microbiology &Cell Biology Indian Institute of Science Bangalore India Macromolecular Structure Laboratory NCI - Frederick Cancer Research and Development Center ABL - Basic Research Program Frederick USA Department of Crystallography and Biophysics University of Madras Chennai Biochemistry Department Indian Institute of Science Bangalore India Condensed Matter Physics Division B.A.R.C. Trombay Mumbai Condensed Matter Physics Division Bhabha Atomic Research Centre Trombay Mumbai IMCB The University of Tokyo Tokyo Japan Mitsubishi Chemical Corporation Yokohama Research Center Yokohama Japan Faculty of Pharmaceutical Sciences Chiba University Chiba Japan Department of Biophysics All India Institute of Medical Sciences New Delhi India Department of Biophysics All India Institute of Medical sciences New Delhi India Institüt Physiologische Chemie Hamburg Germany Biophysics Department Bose Institute Calcutta India Slovak Academy of Sciences Institute of Molecular Biology Bratislava Slovakia Indian Institute of Science Bioinformatics Centre Bangalore Departments of Chemistry and Biochemistry Biological Macromolecular Structure Center USA Bulgarian Academy of Sciences Institute of Organic Chemistry Sofia Bulgaria Chinese Academy of Sciences Institute of Biophysics Beijing China Novartis Pharma AG Preclinical Research Basel Switzerland Department of Chemical Sciences Tata Institute of Fundamental Research Mumbai India Solid State Physics Div

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SYNTHETIC FUEL CONSIDERATIONS FOR NAVAL SHIPBOARD USE

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NAVAL ENGINEERS JOURNAL 1982年第2期94卷 286-295页

作者： FAIRBANKS, JW KENYON, CW Capt. John W. Fairbanks USNR:received his M.S. degree from the University of Santa Clara and his B.S. degrees from Stanford University and the Maine Maritime Academy. He taught at the Texas A&M University and the University of Maryland and from 1954 until 1957 served in the U.S. Navy in the Pacific. Subsequently he was a Research Engineer with Hiller Aircraft where he worked on the annular ejector and designed the High-Speed Bearing and Shaft Test Stand for XC-142A and later at Philco Ford worked on advanced space power systems. At NASA-Goddard in 1967 as a Power System Engineer he was employed on several space craft including the Orbiting Astronomical Observatory. From 1971 until 1977 he was employed by the Naval Ship Engineering Center (NAVSEC) as a Program Engineer for FT9 Marine Gas Turbine Development and the Ceramic Demonstrator Gas Turbine and also as Coordinator of Gas Turbine Material Development. In addition he organized the first two Gas Turbine Materials on Marine Environment Conferences and the U.S. participation in the U.S. Navy/Royal Navy Conference. Currently he is a Program Manager in Applied Heat Engine High Temperature Materials and Instrumentation at the Department of Energy (DOE) where he also served as Chairman Engineering Materials Coordinating Committee for DOE. A Naval Reserve Captain and Chairman of the ASME Washington Chapter he also is the former President of the Washington Chapter of the Maine Maritime Academy Alumni former Vice-President of the Stephen Decatur Chapter Naval Reserve Association and the outstanding 1975 Maine Maritime Academy Alumni. Capt. Fairbanks has authored over forty-five technical papers and in both 1974 and 1975 was the winner of the ASE Niedermair Award. Mr. Clarence W. Kenyon:graduated from the State University of New York Maritime College in 1960 and sailed on a Third Assistant Engineer's license with Isbrandtsen Steamship Company before accepting an engineering position with the Long Beach Naval Shipyard in 1961. In addition to his responsibilit

Synthetic fuels are assessed with respect to their potential use aboard Navy ships. The status of petroleum resources and the development of fuels from shale, coal, and biomass is summarized. A scenario of the projected availability of these fuels is presented which shows the sensitivity to funding and schedule. Diesel engine and gas turbine combustor tests with small quantities of coal derived and shale derived fuels are described and these tests results are evaluated for shipboard applications. Special shipboard modifications are discussed such as the replacement of rubber base seals, gaskets, and hoses with viton and teflon, and the use of stainless steel piping because of the fuel characteristics. Considerations for dual fuel systems using Diesel Fuel Marine for starting, stopping, and maneuvering are included based upon early test results. Consideration is given to the use of these fuels in the shipboard environment since they require special handling and adoption of personnel safety measures.

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THE FT9 MARINE GAS TURBINE ENGINE development PROGRAM

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Naval Engineers Journal 1975年第6期87卷 79-96页

作者： FAIRBANKS, JOHN W. The author is a graduate of the Maine Maritime Academy Stanford University and the University of Santa Clara. His undergraduate degrees were in Marine and Mechanical Engineering and his Masters Degree Specialization was in Heat-Mass-Momentum Transfer within the Mechanical Engineering Department He has taught Gas Dynamics Thermodynamics and Direct Energy Conversion at Texas A&M and the University of Maryland and has sailed as a licensed Marine Engineer for two and a half years with the American Export Lines currently holding active First Assistant Steam Unlimited and Third Assistant Diesel Unlimited licenses. From 1954 to 1957 he was on active duty in the U.S. Navy serving in the USS Montrose (APA-212) as both Main Propulsion Assistant and Chief Engineer. While employed at Hiller Aircraft Company he was in the Advanced Research Group and worked on the Detached Coanda Effect for VTOL and ground effect machines as well as designing high-speed bearings and high-speed shaft test stands for the SC-142A an experimental tilt wing aircraft program. In 1963 he went to Philco-Ford to design a Brayton Cycle Power System for a solar probe spacecraft and also worked on the Thermal and Power System Design of the IDCSP (DOD's Communication Satellite). At NASA's Goddard Space Center for six years his responsibilities included design fabrication integration test launch and flight operation of solar arrays on two spacecraft and also as Power Systems Engineer for the Orbiting Astronomical Observatory the largest unmanned spacecraft flown. In 1971 he joined NAVSEC where he is currently the Program Engineer on the FT9 Gas Turbine Development Program and Coordinator of the Navy's Materials Programs for advanced gas turbines. Having organized the first two Navy Gas Turbine Materials Conferences he is presently organizing U.S. participation in a joint U.S. Navy Royal Navy Gas Turbine Materials Conference to be held in ‘the United Kingdom in September 1976. Mr. Fairbanks has authored or coauthored 21 technical papers and i

The current Navy philosophy for marine gas turbine engine development is to marinize an existing aircraft turbo jet engine. The FT9 Marine Gas Turbine Engine is a 33,000 horsepower version of the Pratt and Whitney JT9D engine, which powers the 747 aircraft. Marinization of the JT9D basically involves removal of the fan section, addition of a power turbine, structural modification to several components, and material changes to provide corrosion‐resistance in the marine environment. Characteristics and ratings of the individual engine components are discussed as well as the assembled engine. The FT9 design incorporates the modular replacement concept. Modular replacement permits replacement of short‐life components such as the hot‐section without removing the engine from its mounts. The FT9 specification requires development of a condition monitoring system as an integral part of the engine development. Thus, provisions for sensor installations are incorporated in the design. Accelerometers are installed on the internal engine bearing housings to provide improved vibration signals. These accelerometers are mounted on rods such that they are removable without engine disassembly. Extensive borescope provisions are included to provide capability to inspect all hot‐section components without disassembling the engine. The engine life‐limiting component is the hot‐section because of the susceptibility of the blade and vane materials to sulphidation/oxidation at the temperatures encountered with the advanced engines. Sophisticated Made and vane cooling is used to allow high turbine inlet temperatures while keeping blade metal temperatures in a region where sulphidation/oxidation is only moderately active. Coatings are added to blades and vanes to extend engine life. Three FT9 engines will be delivered to the Navy. The target date for provisional Service Approval of FT9 is mid‐1978. FT9 will provide the U.S. Navy with the most advanced marine gas turbine with the highest powe

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