Urban rail transit (URT) is vulnerable to natural disasters and social emergencies including fire, storm and epidemic (such as COVID-19), and real-time origin-destination (OD) flow prediction provides URT operators wi...
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The recycling of CO_(2)through electrochemical processes offers a promising solution for alleviating the greenhouse effect;however,the activation of CO_(2)and desorption of^(*)CO in electrocatalytic CO_(2)reduction(EC...
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The recycling of CO_(2)through electrochemical processes offers a promising solution for alleviating the greenhouse effect;however,the activation of CO_(2)and desorption of^(*)CO in electrocatalytic CO_(2)reduction(ECR)frequently encounter high energy barriers and competitive hydrogen evolution reactions(HERs),which are urgent problems that need to be *** this study,a catalyst(P100-Fe-N/C)with homogeneous P-tuned FeN_(2)binuclear sites(N_(2)PFe-FePN_(2))was successfully synthesised,demonstrating satisfactory performance in the ECR to CO.P100-Fe-N/C attains a peak FECOof 98.01%and a normalized TOF of 664.7 h-1at-0.7 VRHE,surpassing the performance of the Fe binuclear catalyst without P and singleatoms *** the MEA cell,a FECOexceeding 90%can still be *** functional theory analysis indicates that the asymmetric coordination configuration induced by the incorporation of P facilitates a reduction in the system's *** modulation of P results in the d-band centre of the catalyst being positioned closer to the Fermi level,which facilitates the interaction of the catalyst with CO_(2),allowing more electrons to be injected into the CO_(2)molecule at the Fe binuclear sites and inhibiting the *** P-tuned FeN_(2)binuclear sites effectively lower the^(*)CO desorption barrier.
Studying the characteristics of complex nonlinear systems and designing control strategies necessitates the development of computationally efficient methods. In particular, compressor systems will benefit from accurat...
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The work is devoted to the numerical complete solution of the optimal control problem. The complete solution means the solution of the optimal control problem together with the solution of the control synthesis proble...
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The effect of Zr on the microstructure and mechanical properties of 304 stainless steel joints brazed with Ag-Cu fillers was *** incorporation of Zr had little effect on the solid-liquid phase line of the fillers,and ...
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The effect of Zr on the microstructure and mechanical properties of 304 stainless steel joints brazed with Ag-Cu fillers was *** incorporation of Zr had little effect on the solid-liquid phase line of the fillers,and the melting temperature range of the fillers was narrowed,which enhanced their fluidity and *** presence of Zr in the form of heterogeneous particles augmented the nucleation rate during solidification,transforming the intermittently distributed gray-black coarse dendrites into cellular *** structural transformation led to fragmentation and refinement of the *** dissolution of Zr into Ag and Cu promoted the transformation of low-angle grain boundaries to high-angle grain boundaries(HAGBs),hindering crack *** element in the brazing seam led to grain refinement and increased density of grain *** grain refinement could disperse the stress,and HAGBs could resist the dislocation movement,improving the joint *** results display that when Zr content was 0.75 wt.%,the maximum strength was 221.1 *** fracture occurred primarily at the brazing seam,exhibiting a ductile fracture.
Formaldehyde(HCHO)is a common indoor pollutant that is detrimental to human *** efficient removal has become an urgent demand to reduce the public health *** this work,Ag-MnO_(x)-based catalysts were prepared and acti...
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Formaldehyde(HCHO)is a common indoor pollutant that is detrimental to human *** efficient removal has become an urgent demand to reduce the public health *** this work,Ag-MnO_(x)-based catalysts were prepared and activated under different atmosphere(i.e.,air,hydrogen(H_(2))and carbon monoxide(CO))for efficient oxidation of *** catalyst activated with CO(Ag/Mn-CO)displayed the highest activity among the tested samples with 90% conversion at 100℃ under a gas space velocity of 75,000 mL/(g_(cat)·hr).Complementary characterizations demonstrate that CO reduction treatment resulted in synergically regulated content of surface oxygen on support to adsorb/activate HCHO and size of Ag particle to dissociate oxygen to oxidize the adsorbed *** contrast,other catalysts lack for either abundant surface oxygen species or metallic silver with the appropriate particle size,so that the integrate activity is limited by one specific reaction *** study contributes to elucidating the mechanisms regulating the oxidation activity of Ag-based catalysts.
Each joint of a hydraulic-driven legged robot adopts a highly integrated hydraulic drive unit(HDU),which features a high power-weight ***,most HDUs are throttling-valve-controlled cylinder systems,which exhibit high e...
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Each joint of a hydraulic-driven legged robot adopts a highly integrated hydraulic drive unit(HDU),which features a high power-weight ***,most HDUs are throttling-valve-controlled cylinder systems,which exhibit high energy *** contrast,pump control systems offer a high ***,their response ability is *** fully utilize the advantages of pump and valve control systems,in this study,a new type of pump-valve compound drive system(PCDS)is designed,which can not only effectively reduce the energy loss,but can also ensure the response speed and response accuracy of the HDUs in robot joints to satisfy the performance requirements of ***,considering the force control requirements of energy conservation,high precision,and fast response of the robot joint HDU,a nonlinear mathematical model of the PCDS force control system is first *** addition,pressure-flow nonlinearity,friction nonlinearity,load complexity and variability,and other factors affecting the system are considered,and a novel force control method based on quantitative feedback theory(QFT)and a disturbance torque observer(DTO)is designed,which is denoted as QFT-DTOC *** method improves the control accuracy and robustness of the force control system,reduces the effect of the disturbance torque on the control performance of the servo motor,and improves the overall force control performance of the ***,experimental verification is performed using the PCDS performance test *** experimental results and quantitative data show that the QFT-DTOC proposed herein can significantly improve the force control performance of the *** relevant force control method can be used as a bottom-control method for the hydraulic servo system to provide a foundation for implementing the top-level trajectory planning of the robot.
Traffic flow prediction is a vital part of an intelligent traffic management system. The critical challenge of the traffic flow prediction task is to fully use observable historical information to extract the hidden s...
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Photocatalytic synthesis of hydrogen peroxide has gradually become a promising method for in-situ pro-duction of hydrogen peroxide,which relies on sustainable solar ***,the commonly used photocatalyst,i.e.,carbon nitr...
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Photocatalytic synthesis of hydrogen peroxide has gradually become a promising method for in-situ pro-duction of hydrogen peroxide,which relies on sustainable solar ***,the commonly used photocatalyst,i.e.,carbon nitride(CN),still suffers from the drawbacks of narrow light absorption range and fast charge ***,we report a facile method to introduce nitrogen defects into carbon nitride together with sodium *** adjusting the ratio of sodium dicyandiamide,the band gap of carbon nitride can be controlled,while the carrier separation and transfer ability of carbon nitride is *** modified CN with sodium doping and nitrogen defect(SD-CN)demonstrates outstanding H_(2)O_(2)pro-duction performance(H_(2)O_(2)yield rate of 297.2μmol L^(−1)h^(−1))under visible light irradiation,which is approximately 9.8 times higher than that of pristine *** work deepens the understanding of the coordinated effect of structural defect and element doping of carbon nitride on the photocatalytic H_(2)O_(2)production performance,and provides new insight into the design of photocatalytic system for efficient production of H_(2)O_(2).
In solving many-objective optimization problems(MaO Ps),existing nondominated sorting-based multi-objective evolutionary algorithms suffer from the fast loss of selection *** candidate solutions become nondominated du...
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In solving many-objective optimization problems(MaO Ps),existing nondominated sorting-based multi-objective evolutionary algorithms suffer from the fast loss of selection *** candidate solutions become nondominated during the evolutionary process,thus leading to the failure of producing offspring toward Pareto-optimal front with *** we find a more effective way to select nondominated solutions and resolve this issue?To answer this critical question,this work proposes to evolve solutions through line complex rather than solution points in Euclidean ***,Plücker coordinates are used to project solution points to line complex composed of position vectors and momentum *** position vectors of the solution points,momentum vectors are used to extend the comparability of nondominated solutions and enhance selection ***,a new distance function designed for high-dimensional space is proposed to replace Euclidean distance as a more effective distancebased *** on them,a novel many-objective evolutionary algorithm(MaOEA)is proposed by integrating a line complex-based environmental selection strategy into the NSGAⅢ*** proposed algorithm is compared with the state of the art on widely used benchmark problems with up to 15 *** results demonstrate its superior competitiveness in solving MaOPs.
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