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Gel-derived NiO–MoS 2 for the scalable fabrication of bifunctional screen-printed electrodes for overall water splitting

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International Journal of Hydrogen Energy 2025年 139卷 247-256页

作者： Zhoveta Yhobu Muralikrishna Sreeramareddygari Chatuporn Phanthong Srinivasa Budagumpi Doddahalli H. Nagaraju Wachira Chaiworn Mithran Somasundrum Patsamon Rijiravanich Surawut Chuangchote Werasak Surareungchai Sensor Technology Laboratory Pilot Plant Development and Training Institute King Mongkut's University of Technology Thonburi Bangkhuntien-chaitalay Road Thakam Bangkok 10150 Thailand Centre for Nano and Material Sciences JAIN (Deemed–to–be University) Jain Global Campus Kanakapura Bangalore 562 112 Karnataka India Industrial Sensor Technology Research Team Biochemical Engineering and System Biology Research Group National Center for Genetic Engineering and Biotechnology National Science and Technology Development Agency at KMUTT (Bangkhuntien Campus) Bangkok 10150 Thailand Department of Chemistry School of Applied Sciences REVA University Kattigenahalli Yelahanka Bangalore 560 064 Karnataka India Department of Tool and Materials Engineering Faculty of Engineering King Mongkut's University of Technology Thonburi (KMUTT) 126 Prachauthit Rd. Bangmod Thungkru Bangkok 10140 Thailand Research Center for Advanced Materials for Energy and Environmental Technology (MEET) King Mongkut's University of Technology Thonburi (KMUTT) 126 Prachauthit Rd. Bangmod Thungkru Bangkok 10140 Thailand Nanoscience & Nanotechnology Graduate Programme Faculty of Science King Mongkut's University of Technology Thonburi Bangkhuntien-chaitalay Road Thakam Bangkok 10150 Thailand

The fabrication of flexible, free-standing electrodes is crucial for advancing renewable energy technologies, particularly in energy conversion and storage. Traditional electrode fabrication methods often involve complex procedures, high material wastage, and limited scalability, whereas screen printing offers a cost-effective, reproducible, and scalable approach for producing high-performance electrodes with uniform coatings. This study introduces a versatile screen-printing strategy for fabricating flexible carbon cloth (CC) electrodes using NiO–MoS 2 ink derived from a solvothermal method. The resulting screen-printed CC electrodes function as efficient bifunctional catalysts for the hydrogen evolution reaction (HER), oxygen evolution reaction (OER), and overall water splitting in alkaline media. The NiO–MoS 2 screen-printed CC electrode exhibits excellent electrocatalytic performance, achieving an OER overpotential ( η 10 ) of 382 mV vs RHE with a Tafel slope of 75 mV/dec and HER overpotential ( η 10 ) of −159 mV vs RHE and Tafel slope of 116 mV/dec. To further demonstrate its bifunctionality, the NiO–MoS 2 screen-printed CC electrode was assembled into a water-splitting electrolyzer, requiring a cell voltage of 1.79 V to reach a current density of 10 mA/cm 2 and exhibiting outstanding operational durability. The robustness and structural integrity of the developed electrode is confirmed by the post-stability analysis, highlighting the potential of the methodology reported in this work for the scalable fabrication of high-performance electrodes for water splitting applications.

关键词： Screen printing

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Expression quantitative trait loci(eQTL):from population genetics to precision medicine

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Journal of Genetics and Genomics 2025年第4期52卷 449-459页

作者： Zhi Qi Wong Lian Deng Alvin Cengnata Thuhairah Abdul Rahman Aletza Mohd Ismail Renee Lay Hong Lim Shuhua Xu Boon-Peng Hoh Faculty of Applied Sciences UCSI UniversityKuala Lumpur 56000Malaysia State Key Laboratory of Genetic Engineering Center for Evolutionary BiologyCollaborative Innovation Center for Genetics and DevelopmentSchool of Life SciencesFudan UniversityShanghai 200433China Clinical Pathology Diagnostic Centre Research Laboratory Faculty of MedicineUniversiti Teknologi MARA47000Malaysia Key Laboratory of Computational Biology Shanghai Institute of Nutrition and HealthUniversity of Chinese Academy of SciencesChinese Academy of SciencesShanghai 200031China Department of Liver Surgery and Transplantation Liver Cancer Institute Zhongshan HospitalFudan UniversityShanghai 200433China Ministry of Education Key Laboratory of Contemporary Anthropology School of Life SciencesHuman Phenome InstituteFudan UniversityShanghai 200433China School of Life Science and Technology ShanghaiTech UniversityShanghai 201210China Jiangsu Key Laboratory of Phylogenomics and Comparative Genomics School of Life SciencesJiangsu Normal UniversityXuzhouJiangsu 221008China Henan Institute of Medical and Pharmaceutical Sciences Zhengzhou UniversityZhengzhouHenan 450001China Center for Excellence in Animal Evolution and Genetics Chinese Academy of SciencesKunmingYunnan 650223China Division of Applied Biomedical Sciences and Biotechnology School of Health SciencesIMU UniversityKuala Lumpur 57000Malaysia

Evidence has shown that differential transcriptomic profiles among human populations from diverse ancestries,supporting the role of genetic architecture in regulating gene expression alongside environmental *** variants that regulate gene expression,known as expression quantitative trait loci(eQTL),are primarily shaped by human migration history and evolutionary forces,likewise,regulation of gene expression in principle could have been influenced by these ***,a comprehensive understanding of how human evolution impacts eQTL offers important insights into how phenotypic diversity is *** studies,however,suggest that eQTL is enriched in genes that are selectively *** eQTL is minimally affected by selective pressures remains an open question and requires comprehensive *** addition,such studies are primarily dominated by the major populations of European ancestry,leaving many marginalized populations *** observations indicate there exists a fundamental knowledge gap in the role of genomics variation on phenotypic diversity,which potentially hinders precision *** article aims to revisit the abundance of eQTL across diverse populations and provide an overview of their impact from the population and evolutionary genetics perspective,subsequently discuss their influence on phenomics,as well as challenges and opportunities in the applications to precision medicine.

关键词： eQTL Transcriptomics Genomics Phenomics Population genetics Precisionmedicine

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Prediction of methylene blue dye sorption to sulfonated date palm kernel biochar using statistical regression and machine learning methods and DFT studies

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Journal of Molecular Liquids 2025年 429卷

作者： Aigbe, Uyiosa Osagie Ukhurebor, Kingsley Eghonghon Onyancha, Robert Birundu Osibote, Adelaja Otolorin Hassaan, Mohamed A. ElKatory, Marwa R. Nemr, Ahmed El Center for Space Research North-West University Private Bag X6001 Potchefstroom2531 South Africa National Institute of Theoretical and Computational Science Johannesburg2000 South Africa School of Chemistry & Physics University of KwaZulu-Natal Pietermaritzburg Campus Private Bag X01 Scottsville3209 South Africa Department of Physics Faculty of Science Edo State University Uzairue Edo State Nigeria School of Physics and Earth Science Faculty of Applied Science and Technology Technical University of Kenya Nairobi Kenya College of Graduate Studies School of Interdisciplinary Research and Graduate Studies Muckleneuk Campus University of South Africa Pretoria0003 South Africa Department of Mathematics and Physics Cape Peninsula University of Technology Cape Town South Africa Kayet Bey Alexandria Elanfoushy Egypt Advanced Technology and New Materials Research Institute SRTA-City New Borg El-Arab City 21934 Alexandria Egypt

In this study, methylene blue (MB) dye adsorption to synthesised sulfonated date palm kernel biochar (SDPKB) was predicted and optimized using statistical-based regression approach (response surface methodology (RSM), machine-learning algorithms (artificial-neural-network (ANN), and adaptive-neuro-fuzzy-inference-system (ANFIS) models), and quantum chemistry calculations performed using density function theory (DFT) to link the electrical properties of the MB dye with the experimental findings. The percentage (%) of MB dye removed using SDPKB was found to be proportional to the biosorbent dosage and interaction time and inversely proportional to the solution pH and initial concentrations based on different used models results. It was observed that these models were accurate and comparable for the prediction of the removal of MB with coefficient of regression (R2) values of 0.9174, 0.9742, and 0.9999, mean square error (MSE) values of 181.71, 94.50, and 0.00000049, and root MSE (RMSE) values of 13.48, 9.72, and 0.0007 for the RSM, ANN, and ANFIS, respectively. The ANFIS model was found to be more effective in the prediction of MB sorption to SDPKB than the other models (ANFIS > ANN > RSM), and it was highly applicable in the sorption process. This study has revealed that the SDPKB can serve as a better biosorbent for MB adsorption. Therefore, this study will serve as a first reference point data that will be of great assistance in industrial effluent management as well as decision-making on the adoption of statistical and machine learning models for adsorption study. © 2025 Elsevier B.V.

关键词： Adversarial machine learning

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Symmetry-Based Phenomenological Model for Magnon Transport in a Multiferroic

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Physical Review Letters 2025年第1期134卷 016703-016703页

作者： Isaac A. Harris Sajid Husain Peter Meisenheimer Maya Ramesh Hyeon Woo Park Lucas Caretta Darrell G. Schlom Zhi Yao Lane W. Martin Department of Physics University of California Berkeley California USA Materials Science Division Lawrence Berkeley National Laboratory Berkeley California USA Department of Materials Science and Engineering University of California Berkeley California USA Department of Materials Science and Engineering Cornell University Ithaca New York USA Department of Physics Korea Advanced Institute of Science and Technology Daejon Korea School of Engineering Brown University Providence Rhode Island USA Kavli Institute at Cornell for Nanoscale Science Ithaca New York 14853 USA Leibniz-Institut für Kristallzüchtung Max-Born-Straße 2 12489 Berlin Germany Applied Mathematics and Computational Research Division Lawrence Berkeley National Laboratory Berkeley California 94720 USA Department of Materials Science and NanoEngineering Rice University Houston Texas USA Department of Physics and Astronomy Rice University Houston Texas USA Department of Chemistry Rice University Houston Texas USA Rice Advanced Materials Institute Rice University Houston Texas USA

Magnons—carriers of spin information—can be controlled by electric fields in the multiferroic BiFeO3 (BFO), a milestone that brings magnons closer to application in future devices. The origin of magnon-spin currents in BFO, however, is not fully understood due to BFO’s complicated magnetic texture. In this Letter, we present a phenomenological model to elucidate the existence of magnon spin currents in generalized multiferroics by examining the symmetries inherent to their magnetic and polar structures. This model is grounded in experimental data obtained from BFO and its derivatives, which informs the symmetry operations and resultant magnon behavior. By doing so, we address the issue of symmetry-allowed, switchable magnon spin transport in multiferroics, thereby establishing a critical framework for comprehending magnon transport within complex magnetic textures.

关键词： Electric fields

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Thermal analysis of ternary hybrid nanofluid flow in convergent/divergent channel using Box-Behnken design of response surface methodology

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Results in Physics 2025年 74.0卷

作者： Mahariq, Ibrahim Mohana, C.M. Kumar, B. Rushi Mohamed, Kezzar SARI, Mohamed Rafik El-Wahed Khalifa, Hamiden Abd Nagarathnam, Sunitha University College Korea University Seoul 02481 South Korea Najjad Zeenni Faculty of Engineering Al Quds University Jerusalem Palestine Department of Medical Research China Medical University Hospital China Medical University Taichung Taiwan Applied Science Research Center Applied Science Private University Amman Jordan GUST Engineering and Applied Innovation Research Center (GEAR) Gulf University for Science and Technology Mishref Kuwait Department of Mathematics School of Advanced Sciences Vellore Institute of Technology Tamil Nadu Vellore India Materials and Energy Engineering Laboratory (LMGE) Technology Department Faculty of Technology 20 Aout 1955 University of Skikda PO Box 26 Skikda 21000 Algeria Mechanics of Materials and Plant Maintenance Research Laboratory (LR3MI) Mechanical Engineering Department Faculty of Engineering Badji Mokhtar University of Annaba (UBMA) PO Box 12 Annaba 23052 Algeria Department of Operations and Management Research Faculty of Graduate Studies for Statistical Research Cairo University Giza 12613 Egypt Centre for Research in Computational and Applied Mechanics University of Cape Town Rondebosch 7701 South Africa

Convergent/divergent channels represent a critical advancement in thermal management systems, offering enhanced heat transfer capabilities through geometrically optimized flow paths. This study investigates the thermal and hydrodynamic characteristics of UO₂-ZnO-Fe₃O₄/EG-water ternary hybrid nanofluid in rotating convergent/divergent channels with magnetohydrodynamic and radiation effects, a critical area for enhancing heat transfer efficiency in modern thermal management systems. Employing the Runge-Kutta-Fehlberg method coupled with a Box-Behnken design approach, we analyzed how key parameters affect flow behavior and heat transfer performance. The numerical simulations reveal that increasing the nanoparticle volume fraction from 0.01 to 0.06 enhances the Nusselt number by 27.3 %, while an increase in the magnetic parameter reduces the friction coefficient by 41.2 %. The Reynolds number demonstrates a strong positive correlation with the Nusselt number (R² = 0.978). Maximum heat transfer (Nu = 33.4859) achieved at: α = 1°, Re = 40, φ = 3 %, Ha = 50, Rd = 1, Kn = 0.04, De = 0.5, Ro = 50, ε = 0, λ = 0.5 whereas a minimum flow resistance (Cf = -2.60454) occurred at: α = -3°, Re = 60, φ = 6 %, Ha = 25, Rd = 1, Kn = 0, De = 0.5, Ro = 50, ε = 0.2, λ = 0.5. For the convergent channel configuration (α = -3°), the friction coefficient was 28.3 % higher than in the divergent channel (α = 5°) under identical flow conditions. This work advances the field beyond previous studies by comprehensively analyzing the synergistic effects of rotation, magnetohydrodynamic, radiation, and channel geometry on the performance of ternary hybrid nanofluids, providing crucial insights for designing more efficient thermal systems in electronics cooling, heat exchangers, and industrial processing applications. © 2025 The Authors

关键词： Box-Behnken Design Convergent/Divergent Channels Heat Transfer Enhancement Non-linear Solar Radiation Ternary Hybrid Nanofluids Variable thermal conductivity

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Correction: Modeling of concrete-filled PVC tube columns confined with CFRP strips under uniaxial eccentric compression: machine learning and finite element approaches

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Journal of Big Data 2025年第1期12卷 1-2页

作者： Wang, Yan Elmeligy, Mohamed A. Isleem, Haytham F. Hamed, Asmaa Y. Qader, Diyar N. Sharaf, Mohamed Jangir, Pradeep Arpita Tejani, Ghanshyam G. School of Mechanical and Electrical Engineering Guilin University of Electronic Technology Guilin China Advanced Manufacturing Institute King Saud University Riyadh Saudi Arabia Jadara University Research Center Jadara University Irbid Jordan Department of Computer Science University of York York UK Construction and Building Department The Higher Institute of Engineering and Technology Luxor Luxor Egypt Civil Engineering Department University of Kirkuk Kirkuk Iraq Industrial Engineering Department College of Engineering King Saud University Riyadh Saudi Arabia University Centre for Research and Development Chandigarh University Gharuan Mohali India Hourani Center for Applied Scientific Research Al-Ahliyya Amman University Amman Jordan Department of CSE Graphic Era Hill University Dehradun India Graphic Era Deemed Department of CSE To Be University Dehradun India Department of Biosciences Saveetha School of Engineering Saveetha Institute of Medical and Technical Sciences Chennai India Department of Industrial Engineering and Management Yuan Ze University Taoyuan Taiwan Applied Science Research Center Applied Science Private University Amman Jordan

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Phase-field simulations of the effect of temperature and interface for zirconiumδ-hydrides

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Chinese Physics B 2024年第4期33卷 701-710页

作者：陈子航盛杰刘瑜施小明黄厚兵许可王越超武帅孙博刘海风宋海峰 School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081China Advanced Research Institute of Multidisciplinary Science Beijing Institute of TechnologyBeijing 100081China Laboratory of Computational Physics Institute of Applied Physics and Computational MathematicsBeijing 100088China Department of Physics University of Science and Technology BeijingBeijing 100083China

Hydride precipitation in zirconium cladding materials can damage their integrity and *** temperature and material defects have a significant effect on the dynamic growth of *** this study,we have developed a phasefield model based on the assumption of elastic behaviour within a specific temperature range(613 K-653 K).This model allows us to study the influence of temperature and interfacial effects on the morphology,stress,and average growth rate of zirconium *** results suggest that changes in temperature and interfacial energy influence the length-to-thickness ratio and average growth rate of the hydride *** ultimate determinant of hydride orientation is the loss of interfacial coherency,primarily induced by interfacial dislocation defects and quantifiable by the mismatch degree *** escalation in interfacial coherency loss leads to a transition of hydride growth from horizontal to vertical,accompanied by the onset of redirection ***,redirection occurs at a critical mismatch level,denoted as qc,and remains unaffected by variations in temperature and interfacial ***,this redirection leads to an increase in the maximum stress,which may influence the direction of hydride crack *** research highlights the importance of interfacial coherency and provides valuable insights into the morphology and growth kinetics of hydrides in zirconium alloys.

关键词： zirconium hydride phase-field method temperature effect mismatch degree

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Engineering grain boundaries in monolayer molybdenum disulfide for efficient water-ion separation

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science (New York, N.Y.) 2025年第6735期387卷 776-782页

作者： Shen, Jie Aljarb, Areej Cai, Yichen Liu, Xing Min, Jiacheng Wang, Yingge Wang, Qingxiao Zhang, Chenhui Chen, Cailing Hakami, Mariam Fu, Jui-Han Zhang, Hui Li, Guanxing Wang, Xiaoqian Chen, Zhuo Li, Jiaqiang Dong, Xinglong Shih, Kaimin Huang, Kuo-Wei Tung, Vincent Shi, Guosheng Pinnau, Ingo Li, Lain-Jong Han, Yu Physical Sciences and Engineering Division (PSE) King Abdullah University of Science and Technology (KAUST) Thuwal Saudi Arabia School of Materials Science and Engineering Nanyang Technological University 50 Nanyang Avenue Singapore Department of Physics King Abdulaziz University Jeddah Saudi Arabia KAUST Catalysis Center King Abdullah University of Science and Technology (KAUST) Thuwal Saudi Arabia Key Laboratory of Flexible Electronics (KLOFE) and Institute of Advanced Materials (IAM) Nanjing Tech University (NanjingTech) Nanjing China Shanghai Applied Radiation Institute Shanghai Key Laboratory of Atomic Control and Application of Inorganic 2D Supermaterials Shanghai University Shanghai China Department of Mechanical Engineering University of Hong Kong Pok Fu Lam Road Hong Kong China Department of Civil Engineering University of Hong Kong Pok Fu Lam Road Hong Kong China Imaging and Characterization Core Lab King Abdullah University of Science and Technology (KAUST) Thuwal Saudi Arabia Department of Chemical System Engineering School of Engineering University of Tokyo Tokyo Japan Center for Electron Microscopy South China University of Technology Guangzhou China School of Emergent Soft Matter South China University of Technology Guangzhou China Catalyst Center of Excellence (CCoE) Research and Development Center Saudi Aramco Dhahran Saudi Arabia Center for Sustainability and Energy Technologies Chang Gung University Taoyuan Taiwan Key Laboratory of Comprehensive and Highly Efficient Utilization of Salt Lake Resources Qinghai Institute of Salt Lakes Chinese Academy of Sciences Xining Qinghai China University of Chinese Academy of Sciences Wenzhou China

Two-dimensional (2D) materials have long been considered as ideal platforms for developing separation membranes. However, it is difficult to generate uniform subnanometer pores over large areas on 2D materials. We report that the well-defined eight-membered ring (8-MR) pores, typically formed at the boundaries of two antiparallel grains of monolayer molybdenum disulfide (MoS2), can serve as molecular sieves for efficient water-ion separation. The density of grain boundaries and, consequently, the number of 8-MR pores can be tuned by regulating the grain size. Optimized MoS2 membranes outperformed the state-of-the-art membranes in forward osmosis tests by demonstrating both ultrahigh water/sodium chloride selectivity and exceptional water permeance. Creating precise pore structures on atomically thin films through grain boundary engineering presents a promising route for producing membranes suitable for various applications.

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The recent progress of high-entropy layered double hydroxides and high-entropy amorphous materials for water electrocatalysis

DeCarbon

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DeCarbon 2025年 8卷

作者： Wondimu, Tadele Hunde Yong, Zuo Shah, Akeel A. Leung, Puiki Dessie, Yilkal Abraha, Filimon Hadish Flox, Cristina Liao, Qiang Key Laboratory of Low-grade Energy Utilization Technologies and Systems MOE Chongqing University Chongqing 400030 China Adama Science and Technology University Department of Materials Science and Engineering Center of Excellence Advanced Materials Science and Engineering P.O. Box 1888 Ethiopia Department of Applied Chemistry Adama Science and Technology University Adama Ethiopia Department of Chemistry College of Natural and Computational Sciences Aksum University Aksum 1010 Ethiopia Department of Electrical Energy Storage Iberian Centre for Research in Energy Storage Campus University of Extremadura Avda. de las Letras s/n Cáceres 10004 Spain

High-entropy materials (HEMs), which are typically composed of five or more elements in near-equimolar ratios with concentrations ranging from 5 % to 35 %, have distinct elemental compositions and geometric properties that allow for the development of advanced electrocatalysts for renewable energy conversion systems. The high-entropy effect, crystal dislocations, cocktail effect, and slow diffusion in high-entropy layered double hydroxides (HE-LDHs) and amorphous materials (HE-AMs) have all been shown to boost electrocatalytic water oxidation performance significantly. These materials exhibit remarkable activity and stability in both alkaline and acidic conditions. HE-AMs, in particular, benefit from a variety of defects, including coordinatively unsaturated sites and loosely connected atoms, which are critical to their improved catalytic capabilities. HEMs engineering and precise nanostructure control can address the low intrinsic activity, restricted active sites, and poor conductivity of binary and ternary amorphous and LDH catalysts. This study discusses current advances in HE-LDHs and HE-AMs for water electrolysis, including synthesis methods, structural features, active site identification by DFT calculations, and their applications in water electrocatalysis. The presentation also covers potential problems and future directions for developing these materials in energy conversion device systems. © 2025

关键词： Amorphous high-entropy and renewable energy Electrocatalyst Layered double hydroxides Water oxidation

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Enhanced magnetic and electrical properties of Ba2+ doped BiFeO3 multiferroic materials

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Ceramics International 2025年

作者： Sravani, G.M. Murali, N. Sekhar, B. Chandra Shanmukhi, P.S.V. Chohan, Jasgurpreet Singh Mammo, Tulu Wegayehu Parajuli, D. Batoo, Khalid Mujasam Ijaz, Muhammad Farzik Samatha, K. A. P. Visakhapatnam India Andhra University Visakhapatnam India Faculty of Allied Health Sciences Chettinad Hospital and Research Institute Chettinad Academy of Research and Education Tamil Nadu Kelambakkam603103 India Department of Physics Aditya College of Engineering and Technology Surampalem India University Centre for Research & Development Department of Mechanical Engineering Chandigarh University Gharuan Punjab Mohali India Department of Physics College of Natural and Computational Sciences Aksum University Axum Tigray Ethiopia Research Center for Applied Science and Technology Tribhuvan University Nepal King Abdullah Institute for Nanotechnology King Saud University P.O. Box-2455 Riyadh11451 Saudi Arabia Department of Mechanical Engineering College of Engineering King Saud University P. O. Box-800 Riyadh11421 Saudi Arabia Department of Physics Andhra University A. P. Visakhapatnam India

This study investigates the structural, morphological, magnetic, and electrical properties of sol-gel auto-combusted Bi1-xBaxFeO3 (x = 0.00, 0.05, 0.10, 0.15, 0.20, and 0.25) multiferroics using XRD, FESEM, VSM, and LCR methods. The samples exhibit rhombohedral spinel crystal structures in the R3c space group, confirmed by vibrational spectra of Fe–O bonds at approximately 450–465 cm−1 and 560–582 cm−1. FESEM micrographs reveal that the materials are spherical, tightly packed, and have minimal porosity. Saturation magnetization increases in Ba-doped samples, ranging from 1.45 emu/g to 2.49 emu/g at 20 kOe. The Cole-Cole plots display broader semicircles and increased frequency shifts (10 Hz–1 MHz), indicating enhanced granularity and improved grain boundary characteristics. © 2025 Elsevier Ltd and Techna Group S.r.l.

关键词： Nanocrystals

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