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An agent-based infrastructure for enterprise integration 1

An agent-based infrastructure for enterprise integration

1st International Symposium on Agent Systems and Applications and 3rd International Symposium on Mobile Agents, ASA/MA 1999

作者： Cost, R. Scott Finin, Tim Labrou, Yannis Luan, Xiaocheng Peng, Yun Soboroff, Ian Mayfield, James Boughannam, Akram Department of Computer Science and Electrical Engineering Laboratory for Advanced Information Technology University of Maryland Baltimore County BaltimoreMD21250 United States Research and Technology Development Center Johns Hopkins University Applied Physics Laboratory LaurelMD20723 United States Advanced Manufacturing Solutions Development IBM Corporation Boca RatonFL33431 United States

ISBN: (纸本)0769503403

Jackal is a Java-based tool for communication using the KQML agent communication language. Some features that make it extremely valuable to agent development are its conversation management facilities, flexible, blackboard style interface and ease of integration. Jackal has been developed in support of an investigation of the use of agents in enterprise-wide integration of planning and execution for manufacturing. This paper describes Jackal at a surface and design level, and demonstrates its use in a multiagent system that supports intelligent integration of enterprise planning and execution.

关键词： Multi agent systems

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Brominated PEAI as Multi-Functional Passivator for High-Efficiency Perovskite Solar Cell

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Energy & Environmental Materials 2023年第3期6卷 50-57页

作者： Minghao Li Junjie Zhou Liguo Tan Yue Liu Siyang Wang Chaofan Jiang Hang Li Xing Zhao Xingyu Gao Wolfgang Tress Liming Ding Chenyi Yi State Key Laboratory of Power System Department of Electrical EngineeringTsinghua UniversityBeijing 100084China Shanghai Synchrotron Radiation Facility(SSRF) Shanghai Advanced Research InstituteChinese Academy of ScienceShanghai 201800China Institute of Computational Physics Zurich University of Applied SciencesWinterthur 8401Switzerland Center of Excellence in Nanoscience(CAS) Key Laboratory of Nanosystem and Hierarchical Fabrication(CAS)National Center for Nanoscience and TechnologyBeijing 100190China

The interfaces of perovskite solar cells(PSCs)are well known to be rich in deep-level carrier traps,which serve as non-radiative recombination centers and limit the open-circuit voltage(Voc)and power conversion efficiency(PCE)of *** chemistry and surface passivators have been researched extensively and mainly focused on the neutralization of uncoordinated lead or anion ***,a novel brominated passivator 2-bromophenethylammonium iodide(2-Br-PEAI)is introduced for a multi-functional passivation effect at the perovskite *** brominated species readily form 2D perovskite on top of the 3D perovskite and multi-interact with the 3D perovskite *** from the halide vacancy filling and anion bonding ability,the Br atoms on the benzene ring can interact with the FA cations via strong hydrogen bonding N-H…Br and interact with the[PbI_(6)]^(4−)inorganic *** interface defects in the PSCs are well passivated,minimizing non-radiative recombination and enhancing device *** a result,a champion PCE of 24.22%was achieved with high V_(oc)and fill *** addition,modified devices also showed enhanced operational stability(retention of>95%initial PCE after 400 h)and humidity resistance(>90%initial PCE maintained after 1500 h under~50%RH).

关键词： brominated PEAI high efficiency perovskite solar cell surface passivation

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Suppressed concentration quenching and tunable photoluminescence in Eu^(2+)-activated Rb_(3)Y(PO_(4))_(2) phosphors for full-spectrum lighting

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Light(science & Applications) 2024年第11期13卷 2688-2698页

作者： Ming Zhao Yeping Ge Yurong Li Xiaoyan Song Zhiguo Xia Xinping Zhang Institute of Information Photonics Technology School of Physics and Optoelectronic EngineeringBeijing University of TechnologyBeijing 10083China College of Materials Science and Engineering Key Laboratory of Advanced Functional MaterialsEducation Ministry of ChinaBeijing University of TechnologyBeijing 10083China State Key Laboratory of Luminescent Materials and Devices Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied TechniquesGuangdong Engineering Technology Research and Development Center of Special Optical Fiber Materials and DevicesSchool of Physics and OptoelectronicsSouth China University of TechnologyGuangzhou 510641China

Highly efficient inorganic phosphors are desirable for lighting-emitting diode light sources,and increasing the doping concentration of activators is a common approach for enhancing the photoluminescence quantum yield(PLQY).However,the constraint of concentration quenching poses a great challenge for improving the ***,we propose a fundamental design principle by separating activators and prolonging their distance in Eu^(2+)-activated Rb_(3)Y(PO_(4))_(2)phosphors to inhibit concentration quenching,in which different quenching rates are controlled by the Eu distribution at various crystallographic *** blue-violet-emitting Rb_(3)Y(PO_(4))2:xEu(x=0.1%–15%)phosphors,with the occupation of Rb1,Rb2 and Y sites by Eu^(2+),exhibit rapid luminescence quenching with optimum external PLQY of 10%due to multi-channel energy ***,as the Eu concentration increases above 20%,Eu^(2+)prefer to occupy the Rb1 and Y sites with separated polyhedra and large interionic distances,resulting in green emission with suppressed concentration quenching,achieving an improved external PLQY of 41%.Our study provides a unique design perspective for elevating the efficiency of Eu^(2+)-activated phosphors toward high-performance inorganic luminescent materials for full-spectrum lighting.

关键词： quenching lighting concentration

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Experimental demonstration of generalized quantum fluctuation theorems in the presence of coherence

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science Advances 2025年第22期11卷 eadq6014页

作者： Hui Li Jie Xie Hyukjoon Kwon Yixin Zhao M. S. Kim Lijian Zhang National Laboratory of Solid State Microstructures Key Laboratory of Intelligent Optical Sensing and Manipulation and Collaborative Innovation Center of Advanced Microstructures College of Engineering and Applied Sciences and School of Physics Jiangsu Physical Science Research Center Nanjing University Nanjing 210093 China. School of Computational Sciences Korea Institute for Advanced Study Seoul 02455 Korea. Blackett Laboratory Imperial College London London SW7 2AZ UK. School of Electronics Center for Quantum Information Technology Peking University Beijing 100871 China.

Fluctuation theorems have elevated the second law of thermodynamics to a statistical realm by establishing a connection between time-forward and time-reversal probabilities, providing invaluable insight into nonequilibrium dynamics. While well established in classical systems, their quantum generalization, incorporating coherence and the diversity of quantum noise, remains open. We report the experimental validation of a quantum fluctuation theorem (QFT) in a photonic system, applicable to general quantum processes with nonclassical characteristics, including quasi-probabilistic descriptions of entropy production and multiple time-reversal processes. Our experiment confirms that the ratio between the quasi-probabilities of the time-forward and any multiple time-reversal processes obeys a generalized Crooks QFT. Moreover, coherence induced by a quantum process leads to the imaginary components of quantum entropy production, governing the phase factor in the QFT. These findings underscore the fundamental symmetry between a general quantum process and its time reversal, providing an elementary toolkit to explore noisy quantum information processing.

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Interlayer engineering of lattice dynamics and elastic constants of 2D layered nanomaterials under pressure

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Nature communications 2025年第1期16卷 4901页

作者： Guoshuai Du Lili Zhao Shuchang Li Jing Huang Susu Fang Wuxiao Han Jiayin Li Yubing Du Jiaxin Ming Tiansong Zhang Jun Zhang Jun Kang Xiaoyan Li Weigao Xu Yabin Chen Advanced Research Institute of Multidisciplinary Sciences (ARIMS) Beijing Institute of Technology Beijing China. School of Aerospace Engineering Beijing Institute of Technology Beijing China. State Key Laboratory of Coordination Chemistry Key Laboratory of Mesoscopic Chemistry of MOE School of Chemistry and Chemical Engineering Nanjing University Nanjing China. Mechano-X Institute Applied Mechanics Laboratory Department of Engineering Mechanics Tsinghua University Beijing China. Beijing Computational Science Research Center Beijing China. School of Chemistry and Chemical Engineering Beijing Institute of Technology Beijing China. Institute of Semiconductors Chinese Academy of Sciences Beijing China. Beijing Computational Science Research Center Beijing China. jkang@***. Mechano-X Institute Applied Mechanics Laboratory Department of Engineering Mechanics Tsinghua University Beijing China. xiaoyanlithu@***. State Key Laboratory of Coordination Chemistry Key Laboratory of Mesoscopic Chemistry of MOE School of Chemistry and Chemical Engineering Nanjing University Nanjing China. xuwg@***. Advanced Research Institute of Multidisciplinary Sciences (ARIMS) Beijing Institute of Technology Beijing China. chyb0422@***. School of Aerospace Engineering Beijing Institute of Technology Beijing China. chyb0422@***. BIT Chongqing Institute of Microelectronics and Microsystems Chongqing China. chyb0422@***.

Interlayer coupling in two-dimensional (2D) layered nanomaterials can provide us strategies to evoke their superior properties, such as the layer-dependent phonon vibration, the formation of moiré excitons and related nontrivial topology. However, to accurately quantify interlayer potential and further measure elastic properties of 2D materials remain challenging, despite significant efforts. Herein, the layer-dependent lattice dynamics and elastic constants of 2D nanomaterials have been systematically investigated via pressure-engineering strategy based on ultralow frequency Raman spectroscopy. The shear and layer-breathing modes Raman shifts of 2H-MoS with various thicknesses are analyzed by the monoatomic chain model (MCM). Intriguingly, it is found that the layer-dependent dω/dP of shear (S) and breathing (LB) modes display the opposite trends, quantitatively consistent with MCM analysis, our molecular dynamics simulations and density functional theory calculations. The diatomic chain model is combined with Raman data to analyze the intralayer and interlayer shear force constants and their pressure coefficients, revealing a strong dependence on the number of layers. These results can be generalized to other van der Waals systems, and may shed light on the potential applications of 2D materials in nanomechanics and nanoelectronics.

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Novel Z-Scheme ZnIn_(2)S_(4)-based photocatalysts for solar-driven environmental and energy applications: Progress and perspectives

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Journal of Materials science & technology 2021年第28期87卷 234-257页

作者： Yogesh Kumar Rohit Kumar Pankaj Raizada Aftab Aslam Parwaz Khan Quyet Van Le Pardeep Singh Van-Huy Nguyen School of Advanced Chemical Sciences Shoolini UniversitySolanHP173229India Department of Chemistry Government Degree CollegeSolanHP173212India Chemistry Department Faculty of ScienceKing Abdulaziz UniversityP.O.Box 80203Jeddah21589Saudi Arabia Institute of Research and Development Duy Tan UniversityDa Nang550000Vietnam Department for Management of Science and Technology Development Ton Duc Thang UniversityHo Chi Minh CityVietnam Faculty of Applied Sciences Ton Duc Thang UniversityHo Chi Minh CityVietnam

Benefiting from strong redox ability,improved charge transport,and enhanced charge separation,Zscheme heterostructures of ZnIn_(2)S_(4) based photocatalysts have received considerable interest to tackle energy needs and environmental *** present review highlights the properties of ZnIn_(2)S_(4),which make it a promising photocatalyst,and a suitable combination with oxidation photocatalyst to form Zscheme,leading to improve their photocatalytic properties *** the central part of this review,various types of Z-scheme heterojunction developed recently based on ZnIn_(2)S_(4) and their application in pollutant degradation,water splitting,CO_(2) reduction,and toxic metals *** analytical techniques to detect or trap the active radical and study the charge separation and lifetime of charge carriers in these Z-schemes are *** review offers its readers a broad optical window for the structural architecture of ZnIn_(2)S_(4)-based Z-schemes,photocatalytic activity,stability,and their technological ***,we discuss the challenges and opportunities for further development on Z-Scheme ZnIn_(2)S_(4)-based photocatalysts toward energy and environmental applications based on the recent progress.

关键词： ZnIn_(2)S_(4) Z-scheme photocatalyst Charge transfer mechanism Pollutant degradation Environmental remediation

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Work roll cooling system design optimisation in presence of uncertainty 19

Work roll cooling system design optimisation in presence of ...

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19th CIRP Design Conference: Competitive Design

作者： Azene, Y.T. Roy, R. Farrugia, D. Onisa, C. Mehnen, J. Trautmann, H. School of Applied Science Cranfield University Cranfield Bedfordshire MK43 0AL United Kingdom Corus Research Development and Technology Swindon Technology Centre S60 3AR United Kingdom Department of Computational Statistics TU Dortmund University Germany

ISBN: (纸本)9780955743641

The paper presents a framework to optimise the design of work roll based on the cooling performance. The framework develops Meta models from a set of Finite Element Analysis (FEA) of the roll cooling. A design of experiment technique is used to identify the FEA runs. The research also identifies sources of uncertainties in the design process. A robust evolutionary multi-objective algorithm is applied to the design optimisation I order to identify a set of good solutions in the presence of uncertainties both in the decision and objective spaces. © Cranfield University 2009.

关键词： Multiobjective optimization

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Enhanced energy coupling for indirect-drive fast-ignition fusion targets (vol 17, pg 435, 2020)

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NATURE PHYSICS 2020年第7期16卷 815-815页

作者： Zhang, F. Cai, H. B. Zhou, W. M. Dai, Z. S. Shan, L. Q. Xu, H. Chen, J. B. Ge, F. J. Tang, Q. Zhang, W. S. Wei, L. Liu, D. X. Gu, J. F. Du, H. B. Bi, B. Wu, S. Z. Li, J. Lu, F. Zhang, H. Zhang, B. He, M. Q. Yu, M. H. Yang, Z. H. Wang, W. W. Zhang, H. S. Cui, B. Yang, L. Wu, J. F. Qi, W. Cao, L. H. Li, Z. Liu, H. J. Yang, Y. M. Ren, G. L. Tian, C. Yuan, Z. Q. Zheng, W. D. Cao, L. F. Zhou, C. T. Zou, S. Y. Gu, Y. Q. Du, K. Ding, Y. K. Zhang, B. H. Zhu, S. P. Zhang, W. Y. He, X. T. Science and Technology on Plasma Physics Laboratory Laser Fusion Research Center CAEP Mianyang China (GRID:grid.249079.1) (ISNI:0000 0004 0369 4132) Institute of Applied Physics and Computational Mathematics Beijing China (GRID:grid.418809.c) (ISNI:0000 0000 9563 2481) HEDPS Center for Applied Physics and Technology Peking University Beijing China (GRID:grid.11135.37) (ISNI:0000 0001 2256 9319) Institute of Applied Physics and Computational Mathematics Beijing China (GRID:grid.418809.c) (ISNI:0000 0000 9563 2481) National University of Defense Technology College of Computing Science Changsha China (GRID:grid.412110.7) (ISNI:0000 0000 9548 2110) Shenzhen Technology University Center for Advanced Material Diagnostic Technology Shenzhen China (GRID:grid.499351.3) (ISNI:0000 0004 6353 6136) Science and Technology on Plasma Physics Laboratory Laser Fusion Research Center CAEP Mianyang China (GRID:grid.249079.1) (ISNI:0000 0004 0369 4132) Institute of Applied Physics and Computational Mathematics Beijing China (GRID:grid.418809.c) (ISNI:0000 0000 9563 2481) China Academy of Engineering Physics Graduate School Beijing China (GRID:grid.249079.1) (ISNI:0000 0004 0369 4132)

An amendment to this paper has been published and can be accessed via a link at the top of the paper.

关键词： Energy science and technology Laser-produced plasmas

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Vacancy-Type Defects in Thin HfO2 Layers Probed by Monoenergetic Positron Beams 30

Vacancy-Type Defects in Thin HfO2 Layers Probed by Monoenerg...

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30th International Symposium on Semiconductor Manufacturing, ISSM 2024

作者： Uedono, Akira Kawakami, Kazuya Kuribara, Tatsunori Hasunuma, Ryu Harashima, Yosuke Shigeta, Yasuteru Ni, Zeyuan Yan, Ruolin Nakamura, Hideo Notake, Akira Moriya, Tsuyoshi Michishio, Koji Ishibashi, Shoji University of Tsukuba Faculty of Pure and Applied Science Ibaraki Tsukuba305-8573 Japan Nara Institute of Science and Technology Graduate School of Science and Technology Nara Ikoma630-0192 Japan Tokyo Electron Technology Solutions Ltd. S-Technology Development Center Yamanashi Nirasaki407-0192 Japan Tokyo Electron Technology Solutions Ltd. Development Department 1 Yamanashi Nirasaki407-0192 Japan Tokyo Electron Ltd. Digital Design Center Hokkaido Sapporo060-0003 Japan Tokyo Electron Technology Solutions Ltd. Software and Data Engineering Division Yamanashi Nirasaki407-0192 Japan National Institute of Advanced Industrial Science and Technology Research Institute for Measurement and Analytical Instrumentation Ibaraki Tsukuba305-8568 Japan National Institute of Advanced Industrial Science and Technology Research Center for Computational Design of Advanced Functional Materials Ibaraki Tsukuba305-8568 Japan

ISBN: (纸本)9798331510589

Behaviors of vacancies during the amorphous-to-crystalline transition of thin HfO2 layers were studied by monoenergetic positron beams. The HfO2 layers with 430 nm thickness were fabricated on TiN/Si templates by atomic layer deposition technique. The major vacancy-type defects in the layers were identified as (i) Hf vacancies (VHf) coupled with oxygen vacancies (VOs) and (ii) vacancy clusters. After annealing at 500°C, the concentration of vacancy clusters increased, which was attributed to the agglomeration of intrinsic open spaces in the amorphous phase upon the phase transition from amorphous to crystalline phases. The phase transition started near the interface between the HfO2 layer and bottom electrodes (TiN). After the crystallization, the concentration of vacancy clusters decreased as the annealing temperature increased. © 2024 IEEE.

关键词： Positron annihilation

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Stable phases of freestanding monolayer TiO2: Emergence of out-of-plane ferroelectricity

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Physical Review B 2024年第16期109卷 165435-165435页

作者： Xiangtian Bu Haitao Liu Yuanchang Li Key Lab of Advanced Optoelectronic Quantum Architecture and Measurement (MOE) and Advanced Research Institute of Multidisciplinary Science Beijing Institute of Technology Beijing 100081 China Institute of Applied Physics and Computational Mathematics Beijing 100088 China National Key Laboratory of Computational Physics Beijing 100088 China

Despite being successfully synthesized [Zhang et al., Nat. Mater. 20, 1073 (2021)], the monolayer structure of stable hexagonal TiO2 is unknown, and it is not even clear whether it can exist in a freestanding form. Through first-principles calculations, we have identified two previously uncharted stable structures, namely, distorted 1×3 1T−TiO2 and 3×3 1T−TiO2, both of which are energetically more favorable than commonly adopted 1H and 1T phases. Here, structural distortions are characterized by the out-of-plane shifts of Ti atoms due to the pseudo-Jahn-Teller interactions, which break one and all two inversion symmetries of 1T configuration. As a consequence, the 1×3 1T remains centrosymmetric, while the 3×3 1T exhibits out-of-plane ferroelectricity. Electronic structure calculations show that both are wide-band-gap semiconductors with band gaps larger than their bulk counterparts. In this paper, we not only deepen the understanding of structural instability in wide-gap semiconductors but also add a member to the rare family of two-dimensional out-of-plane ferroelectrics.

关键词： Crystal structure Ferroelectricity Pseudo Jahn-Teller effect Monolayer films First-principles calculations

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