Copper nanoparticles (Cu) anchored lithium niobate (LiNbO3) nanostructures were prepared by a simple hydrothermal technique. The fine and sparse Cu nanoparticles were homogeneously dispersed over the surface of LiNbO3...
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The evolution process of magnetic domains in response to external fields is crucial for the modern understanding and application of *** this study,we investigated the domain rotation in stripe domain films of varying ...
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The evolution process of magnetic domains in response to external fields is crucial for the modern understanding and application of *** this study,we investigated the domain rotation in stripe domain films of varying thicknesses by examining their response to microwave excitation in four different *** resonance spectra indicate that the rotation field of stripe domain film under an applied magnetic field approaches the field where the resonance mode of sample *** saturation field of the stripe domain film corresponds to the field where the resonance mode disappears when measured in the stripe direction parallel to the microwave magnetic *** results are reproducible and consistent with micromagnetic simulations,providing additional approaches and techniques for comprehending the microscopic mechanisms of magnetic domains and characterizing their rotation.
We present the coherent enhancement of the frequency comb via high-order harmonic generation (HHG) in a train of infrared laser pulses combined with terahertz (THz) laser fields. The HHG spectra are obtained by solvin...
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We present the coherent enhancement of the frequency comb via high-order harmonic generation (HHG) in a train of infrared laser pulses combined with terahertz (THz) laser fields. The HHG spectra are obtained by solving the three-dimensional time-dependent Schrödinger equation by means of the time-dependent generalized pseudospectral method. We find that the structure of the frequency comb via HHG becomes much smoother and more regular, and the yield of the comb is increased by nearly two orders of magnitude. By analyzing the phase coherence of HHG spectra, we demonstrate that the THz laser fields are responsible for the optimization of the structure and yield of the frequency comb since the constructive phase coherence of the HHG spectra is modulated by the THz field. The physical origin of the constructive phase coherence is thanks to the uniform ionization efficiency induced by the THz laser field for each laser pulse, which greatly improves the synchronization of the harmonic emission. Our finding provides a promising method for the enhancement of the frequency comb via HHG.
This review provides a critical analysis of the global water and sanitation crisis, as well as how community-based approaches have led to innovative water management solutions. Regions of sub-Saharan Africa, south Asi...
The excessive energy demand of the conventional Haber–Bosch process for ammonia (NH3) generation, coupled with the disruptive effects of nitrate (NO3−) pollution on the global nitrogen cycle, has made the electrocata...
The excessive energy demand of the conventional Haber–Bosch process for ammonia (NH3) generation, coupled with the disruptive effects of nitrate (NO3−) pollution on the global nitrogen cycle, has made the electrocatalytic nitrate reduction reaction (NO3−RR) an essential exit strategy for sustainable NH3 synthesis. However, the intricate multi-step proton and electron transfer process posed a great challenge in achieving high-efficiency electrocatalysts. In this study, we report a selective and highly active NO3−RR electrocatalyst featuring molecular M–Nx sites derived from the immobilization of Fe ions within N-doped graphene quantum dots (NGQDs). We demonstrated that the formation of molecular Fe–Nx coordination activated the NO3−RR of NGQDs-Fe, despite the initial inactivity of NGQDs. In situ Raman analysis revealed that those Fe–Nx sites served as favourable adsorption sites for *NO3. Such catalyst achieved an FE of 93% and a yield rate of 15.41 mmol h−1 cm−2 for NH3 at −0.8 V (vs. RHE) in an alkaline medium. These findings revealed the preferential sequential 2e− and 6e− transfer pathways over the direct 8e− pathway in the NO3−RR, which provides new mechanistic insights into the nitrate reduction reaction.
The inspection of products and assessment of quality is connected with high costs and time effort in many industrial domains. This also applies to the forestry industry. Utilizing state-of-the-art deep learning models...
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Atomic layer deposited Al2O3 films are incorporated into miniature light emitting diodes (mini-LEDs) as an internal moisture barrier layer. The experimental results show that the water vapor transmission rate reaches ...
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The amplitude and phase of a photoionization channel provide deep insights into the nature of ionization dynamics. Here, we propose a novel experimental approach to retrieve these parameters from the photoelectron mom...
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The amplitude and phase of a photoionization channel provide deep insights into the nature of ionization dynamics. Here, we propose a novel experimental approach to retrieve these parameters from the photoelectron momentum distribution (PMD), where a 400 nm femtosecond laser is used to ionize polarized Rb atoms prepared in the 5p state. The magnetic quantum numbers of polarized atoms are well controlled by breaking down the symmetry of the cooling laser in a magneto-optical trap reaction microscope. From the tilt angle of the PMD and the interference structure of εs and εd ionization channels, we are able to extract their relative amplitude and phase shift, in good agreement with ab initio calculations. This exhibits a benchmark one-photon single ionization study of the hydrogen-like atom, providing a complete measurement with full characterizations of intermediate and final state wave functions.
Complex correlated states emerging from many-body interactions between quasiparticles (electrons, excitons and phonons) are at the core of condensed matter physics and material science. In low-dimensional materials, q...
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Complex correlated states emerging from many-body interactions between quasiparticles (electrons, excitons and phonons) are at the core of condensed matter physics and material science. In low-dimensional materials, quantum confinement affects the electronic, and subsequently, optical properties for these correlated states. Here, by combining photoluminescence, optical reflection measurements and ab initio theoretical calculations, we demonstrate an unconventional excitonic state and its bound phonon sideband in layered silicon diphosphide (SiP2), where the bound electron–hole pair is composed of electrons confined within one-dimensional phosphorus–phosphorus chains and holes extended in two-dimensional SiP2 layers. The excitonic state and emergent phonon sideband show linear dichroism and large energy redshifts with increasing temperature. Our ab initio many-body calculations confirm that the observed phonon sideband results from the correlated interaction between excitons and optical phonons. With these results, we propose layered SiP2 as a platform for the study of excitonic physics and many-particle effects.
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