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Correction: Additive-mediated intercalation and surface modification of MXenes

Chemical Society reviews 2022年第8期51卷 3314页

作者： Jing Zou Jing Wu Yizhou Wang Fengxia Deng Jizhou Jiang Yizhou Zhang Song Liu Neng Li Han Zhang Jiaguo Yu Tianyou Zhai Husam N Alshareef School of Environmental Ecology and Biological Engineering School of Chemistry and Environmental Engineering Key Laboratory of Green Chemical Engineering Process of Ministry of Education Engineering Research Center of Phosphorus Resources Development and Utilization of Ministry of Education Wuhan Institute of Technology Wuhan Hubei 430205 P. R. China. 027wit@***. Key Laboratory of Rare Mineral Ministry of Natural Resources Geological Experimental Testing Center of Hubei Province Wuhan Hubei 430034 P. R. China. Physical Science and Engineering Division Materials Science & Engineering King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Kingdom of Saudi Arabia. husam.alshareef@kaust.edu.sa. State Key Laboratory of Urban Water Resources and Environment School of Environment Harbin Institute of Technology Harbin 150090 P. R. China. Institute of Advanced Materials and Flexible Electronics (IAMFE) School of Chemistry and Materials Science Nanjing University of Information Science & Technology Nanjing 210044 P. R. China. yizhou.zhang@***. Key Laboratory for Organic Electronics & Information Displays and Institute of Advanced Materials Nanjing University of Posts and Telecommunications Nanjing 210023 P. R. China. Institute of Chemical Biology and Nanomedicine (ICBN) State Key Laboratory of Chemo/Biosensing and Chemometrics College of Chemistry and Chemical Engineering Hunan University Changsha 410082 P. R. China. State Key Laboratory of Advanced Technology for Materials Synthesis and Processing State Key Laboratory of Silicate Materials for Architectures Wuhan University of Technology Wuhan Hubei 430070 P. R. China. Shenzhen Engineering Laboratory of Phosphorene and Optoelectronics and Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province Shenzhen University Shenzhen 518060 P. R. China. State Key Laboratory of Material Processing and Die & Mould Technology School of Materials Science and Engineering H

Correction for 'Additive-mediated intercalation and surface modification of MXenes' by Jing Zou , , 2022, DOI: 10.1039/d0cs01487g.

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MOF Encapsulating N-Heterocyclic Carbene-Ligated Copper Single-Atom Site Catalyst towards Efficient Methane Electrosynthesis

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Angewandte Chemie 2021年第4期134卷

作者： Dr. Shenghua Chen Dr. Wen-Hao Li Dr. Wenjun Jiang Dr. Jiarui Yang Dr. Jiexin Zhu Dr. Liqiang Wang Dr. Honghui Ou Dr. Zechao Zhuang Prof. Mingzhao Chen Dr. Xiaohui Sun Prof. Dingsheng Wang Prof. Yadong Li Department of Chemistry Tsinghua University Beijing 100084 P. R. China Qian Xuesen Laboratory of Space Technology China Academy of Space Technology Beijing 100094 P. R. China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing International School of Materials Science and Engineering Wuhan University of Technology Wuhan 430070 P. R. China Henan Province Industrial Technology Research Institute of Resources and Materials School of Material Science and Engineering Zhengzhou University Zhengzhou Henan 450001 P. R. China Institute of Environmental Research at Greater Bay Area Key Laboratory for Water Quality and Conservation of the Pearl River Delta Ministry of Education Guangzhou Key Laboratory for Clean Energy and Materials Guangzhou University Guangzhou 510006 P. R. China

The exploitation of highly efficient carbon dioxide reduction (CO 2 RR) electrocatalyst for methane (CH 4 ) electrosynthesis has attracted great attention for the intermittent renewable electricity storage but remains challenging. Here, N-heterocyclic carbene (NHC)-ligated copper single atom site (Cu SAS) embedded in metal–organic framework is reported (2Bn-Cu@UiO-67), which can achieve an outstanding Faradaic efficiency (FE) of 81 % for the CO 2 reduction to CH 4 at −1.5 V vs. RHE with a current density of 420 mA cm −2 . The CH 4 FE of our catalyst remains above 70 % within a wide potential range and achieves an unprecedented turnover frequency (TOF) of 16.3 s −1 . The σ donation of NHC enriches the surface electron density of Cu SAS and promotes the preferential adsorption of CHO* intermediates. The porosity of the catalyst facilitates the diffusion of CO 2 to 2Bn-Cu, significantly increasing the availability of each catalytic center.

关键词： CH4 electrosynthesis CO2RR Cu single-atom site catalyst n-heterocyclic carbene

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Preface to Special Issue on the International Symposium on Environmental Catalysis (ISEC 2016)

Preface to Special Issue on the International Symposium on E...

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作者： Li, Jinlin Yu, Jiaguo Key Laboratory of Catalysis and Materials Science of the State Ethnic Affairs Commission and Ministry of Education South-Central University for Nationalities China State Key Laboratory of Advanced Technology for Material Synthesis and Processing Wuhan University of Technology China

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Effects of Intrinsic Pentagon Defects on Electrochemical Reactivity of Carbon Nanomaterials

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Angewandte Chemie 2019年第12期131卷

作者： Jiawei Zhu Yupeng Huang Wencen Mei Chenyang Zhao Chengtian Zhang Jian Zhang Ibrahim Saana Amiinu Shichun Mu State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan 430070 P. R. China State Key Laboratory of Material Processing and Die & Mould Technology School of Materials Science and Engineering Huazhong University of Science and Technology Wuhan 430074 P. R. China

Theoretical calculations reveal that intrinsic pentagons in the basal plane can contribute to the local electronic redistribution and the contraction of band gap, making the carbon matrix possess superior binding affinity and electrochemical reactivity. To experimentally verify this, a pentagon‐defect‐rich carbon nanomaterial was constructed by means of in situ etching of fullerene molecules (C 60 ). The electrochemical tests show that, relative to hexagons, such a carbon‐based material with abundant intrinsic pentagon defects makes much greater contribution to the electrocatalytic oxygen reduction activity and electric double layer capacitance. It shows a four‐electron‐reaction mechanism similar to commercial Pt/C and other transition‐metal‐based catalysts, and a higher specific capacitance than many reported metal‐free carbon materials. These results show the influence of intrinsic pentagon defects for developing carbon‐based nanomaterials toward energy conversion and storage devices.

关键词： Kohlenstoffmaterialien Pentagondefekte Sauerstoffreduktion Superkondensatoren Zink-Luft-Batterien

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Hierarchically porous materials:synthesis strategies and emerging applications

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Frontiers of Chemical Science and Engineering 2016年第3期10卷 301-347页

作者： Minghui Sun Chen Chen Lihua Chen Baolian Su State Key Laboratory of Advanced Technology for Material Synthesis and Processing Wuhan University of Technology Laboratory of Inorganic Materials Chemistry

Great interests have arisen over the last decade in the development of hierarchically porous *** hierarchical structure enables materials to have maximum structural functions owing to enhanced accessibility and mass transport properties,leading to improved performances in various *** porous materials are in high demand for applications in catalysis,adsorption,separation,energy and *** the present review,recent advances in synthesis routes to hierarchically porous materials are reviewed together with their catalytic contributions.

关键词： hierarchically porous materials synthesis application

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Lithium/Sodium-Ion Batteries: In Situ, Atomic-Resolution Observation of Lithiation and Sodiation of WS2Nanoflakes: Implications for Lithium-Ion and Sodium-Ion Batteries (Small 24/2021)

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Small 2021年第24期17卷

作者： Yaobin Xu Ke Wang Zhenpeng Yao Joohoon Kang David Lam Dan Yang Wei Ai Chris Wolverton Mark C. Hersam Ying Huang Wei Huang Vinayak P. Dravid Jinsong Wu Department of Materials Science and Engineering Northwestern University Evanston IL 60208 USA NUANCE Center Northwestern University Evanston IL 60208 USA Frontiers Science Center for Flexible Electronics (FSCFE) Institute of Flexible Electronics (IFE) Northwestern Polytechnical University (NPU) 127 West Youyi Road Xi'an 710072 China Department of Chemistry and Chemical Biology Harvard University 12 Oxford Street Cambridge MA 02138 USA Department of Chemistry and Computer Science University of Toronto Toronto Ontario Canada School of Advanced Materials Science and Engineering Sungkyunkwan University (SKKU) Suwon 16419 Republic of Korea MOE Key Laboratory of Material Physics and Chemistry Under Extraordinary Conditions School of Chemistry and Chemical Engineering Northwestern Polytechnical University Xi'an 710072 China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Nanostructure Research Centre Wuhan University of Technology 122 Luoshi Road Wuhan Hubei 430070 China

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医用增材制造——从前沿技术到产品研发

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Engineering 2020年第11期6卷 31-41页

作者：邱贵兴丁文江田伟秦岭赵宇张联盟吕坚陈代杰袁广银吴成铁卢秉恒杜如虚陈继明 Mo Elbestawi 顾忠伟李涤尘孙伟赵远锦赫捷金大地刘斌张凯李鉴墨 Kam W.Leong 赵德伟郝定均敖英芳邓旭亮杨惠林徐少克陈英奇李龙樊建平聂国辉陈芸曾晖陈玮赖毓霄 Department of Orthopedics Peking Union Medical College Hospital Chinese Academy of Medical Science & Peking Union Medical College National Engineering Research Center of Light Alloys Net Forming & State Key Laboratory of Metal Matrix Composite Shanghai Jiao Tong University National Engineering Research Center of Mg Materials and Applications and School of Materials Science & Engineering Shanghai Jiao Tong University Department of Spine Surgery Beijing Jishuitan Hospital Center for Translational Medicine Research and Development Institute of Biomedical and Health Engineering Shenzhen Institute of Advanced Technology Chinese Academy of Sciences Guangdong Engineering Laboratory of Biomaterials Additive Manufacturing State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Center for Advanced Structural Materials City University of Hong Kong Shenzhen Research Institute Hong Kong Branch of National Precious Metals Material Engineering Research Center Department of Material Science and Engineering City University of Hong Kong Department of Mechanical Engineering City University of Hong Kong School of Pharmacy Shanghai Jiao Tong University China State Institute of Pharmaceutical Industry Shanghai Institute of Pharmaceutical Industry State Key Laboratory of High-Performance Ceramics and Superfine Microstructure Shanghai Institute of Ceramics Chinese Academy of Sciences Center of Materials Science and Optoelectronics Engineering University of the Chinese Academy of Sciences Micro- and Nano-Technology Research Center State Key Laboratory for Manufacturing Systems Engineering Xi’an Jiaotong University Shien-Ming Wu School of Intelligent Engineering Guangzhou International Campus South China University of Technology Beijing Engineering Research Center of 3D Printing for Digital Medical Health Beijing University of Technology Beijing Engineering Research Center of Laser Technology Beijing University of Technology Key Laboratory of Trans-Scale Las

1.医用增材制造原料的研发和挑战医用增材制造的原料与其他多个领域使用的原料具有广泛通用性,这是构成三维(3D)打印领域的重要基础。这些领域的增材制造在材料类型、粉体特性、成型性和黏弹性等方面面临着相同的问题和挑战。例如,航空...

1.医用增材制造原料的研发和挑战医用增材制造的原料与其他多个领域使用的原料具有广泛通用性,这是构成三维(3D)打印领域的重要基础。这些领域的增材制造在材料类型、粉体特性、成型性和黏弹性等方面面临着相同的问题和挑战。例如,航空领域采用了多种金属材料,而生物医学领域会使用金属、聚合物和无机材料。在生物医学领域,

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1D carbon [email protected] 2 core-shell nanocomposites with enhanced photocatalytic activity toward CO 2 reduction

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Journal of Alloys and Compounds 2018年 746卷 168-176页

作者： Jinfeng Zhang Junwei Fu Shifu Chen Jiali Lv Kai Dai State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan Hubei 430070 PR China College of Physics and Electronic Information Huaibei Normal University Huaibei Anhui 235000 PR China College of Chemistry and Material Science Huaibei Normal University Huaibei Anhui 235000 PR China Hefei National Laboratory for Physical Sciences at the Microscale University of Science and Technology of China Hefei 230026 PR China

More and more serious energy crisis and greenhouse effect force people to find the appropriate solutions. Photocatalytic reduction of CO 2 into hydrocarbon fuels is one of the most potential strategies. In this paper, novel one-dimensional (1D) carbon [email protected] 2 core-shell nanocomposites have been prepared via electrospun synthesis of carbon nanofibers core followed by in situ growth of TiO 2 shell, which exhibit a 2.3-fold higher photocatalytic activity than the pure TiO 2 . The increase of catalytic performance attributed to higher specific surface areas of carbon [email protected] 2 core-shell nanocomposites for providing more surface-active sites. Moreover, the black carbon nanofibers promote light absorption, and the light energy can be converted into heat energy that can speed up the diffusion of reactants and products. Most importantly, the carbon nanofibers with good electrical conductivity can speed up the separation of the photo-induced electron and hole pairs in photocatalyst. This work provides a good synthesis of 1D core-shell heterostructure, and proves that the carbon nanofibers can be an ideal cocatalyst for enhancing photocatalytic CO 2 reduction performance of TiO 2 .

关键词： Composite materials Chemical synthesis X-ray diffraction CO 2 Photocatalytic reduction

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Fast Welding of Chromium Carbide and Nickel Alloy by Spark Plasma Sintering

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Journal of Wuhan University of technology(materials Science) 2016年第4期31卷 835-837页

作者：刘国玺 LI Kezhi LENG Xiaoxuan 张金咏 ZHANG Fan School of Materials Science Northwestern Polytechinical University Xi'an 710072 China Ningbo Branch of Ordnance Science Institute of China Yantai 264003 China China State Key Laboratory of Advanced Technology for Material Synthesis and Processing Wuhan University of Technology Wuhan 430070 China

Spark plasma sintering（SPS） was used to weld the ceramics,eg,Cr3C2 and metal,Ni in this *** is found that the SPS can weld the Cr3C2 and Ni plates at lower temperatures and shorter holding time comparing with that of hot-pressing（HP）.The binding strength was 113 MPa when the temperature was 1000 ℃ by SPS,compared with 10 MPa by HP at the same *** remarkably enhances the atom diffusion in *** analysis at different welding temperatures and holding times of SPS or HP shows that the local temperature gradient,different from the past effects of by-passing current,is the dominative mechanism of the SPS welding.

关键词： Sintering welding Welding holding ceramics sintering welded pressing remarkably heating

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Preface to Special Issue on the International Symposium on Environmental Catalysis(ISEC 2016)

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Chinese Journal of Catalysis 2017年第2期38卷 191-191页

作者：李金林余家国 Key Laboratory of Catalysis and Materials Science of the State Ethnic Affairs Commission and Ministry of Education South-Central University for Nationalities State Key Laboratory of Advanced Technology for Material Synthesis and Processing Wuhan University of Technology

With a growing awareness of pollution and increasing demands for environmental protection, a great deal of effort is being put into the development of catalysts with improved activity for the abatement of pollutants, ... 详细信息

关键词： awareness emitted thank helping symposium speakers invitation acceptance reviewers editorial

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