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N and O vacancies regulation over semiconductor heterojunction to synergistically boost photocatalytic hydrogen peroxide production

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Journal of Materials Science & Technology 2024年第29期196卷 237-247页

作者： Chaoqian Ai Bing Luo Chunyang Zhang Yadi Wang Baoyuan Wang Lijing Ma Dengwei Jing International Research Center for Renewable Energy&State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049China School of Chemical Engineering and Technology Xi’an Jiaotong UniversityXi’an 710049China Department of Chemical Engineering School of Water and Environment&Key Laboratory of Subsurface Hydrology and Ecology in Arid AreasMinistry of Education Chang’an UniversityXi’an 710054China

Defect engineering represents a potent strategy for the modification of electronic properties by introducing atomic vacancies in ***,the synergistic enhancement attributable to different types of atomic vacancies within a heterojunction,as well as their underlying mechanisms,remains sparsely ***,the flexible g-C_(3)N_(4)materials with varying nitrogen vacancies were prepared via a facile calcination method under different atmospheric conditions and then composited with CeO_(2)nanocubes to construct Z-scheme *** was observed that CeO_(2)has abundant O vacancies,and the g-C_(3)N_(4)form tertiary nitrogen defects at the center of the heptazine units under an NH3 atmosphere *** resulting enhancement in the interfacial built-in electric field,coupled with the synergistic effect of O and N vacancies within the Z-scheme heterojunction,has been demonstrated to significantly enhance charge transfer *** results in an optimized photoactivity with a H_(2)O_(2)generation rate of 2.01 mmol g^(-1)h^(-1).This work opens an avenue for constructing and optimizing the heterogeneous photocatalysts by defect engineering technology,and provides deep insight to understand the nature of vacancy engineering in designing effective catalysts for solar energy conversion.

关键词： Photocatalysis H_(2)O_(2) production Z-scheme Defect engineering Synergy effect

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Theoretical and experimental analyses of a novel recirculated regenerative rotary desiccant wheel dehumidification system 32

Theoretical and experimental analyses of a novel recirculate...

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32nd International Conference on Efficiency, Cost, Optimization, Simulation and Environmental Impact of Energy Systems, ECOS 2019

作者： Han, Xiaoqu Wu, Wenxiang Zhou, Zhijie Wang, Yu Chong, Daotong Yan, Junjie State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an China China Ship Development and Design Center Wuhan China

ISBN: (纸本)9788361506515

The high humidity environment in the submarine cabins results in high energy consumption of the air conditioning system. Moreover, the removal of the hydrogen contained in the air, which constitutes a threat to crew’s safety, generates a huge amount of heat. It is of particular significance to reduce the humidity of the air efficiently, through recovery of the waste heat in the dehydrogenation process. Therefore, a novel recirculated regenerative desiccant wheel dehumidification system is proposed in the present work for submarine air-conditioning. The dehumidification rate was optimized through an appropriate proportion between inlet and recirculating air flows. Theoretical modeling and experimental study were carried out to explore the optimal dehumidification performance at different working conditions. The influence of process air parameters (including temperature and humidity), regeneration air parameters (including bypass ratio and regeneration air temperature) and rotary desiccant wheel parameters (including rotation speed and air flow ratio) were analyzed. It was found that the dehumidification rate could be effectively improved compared to sea water direct cooling. It increased with increasing regeneration air temperature and temperature drop. There was an optimal bypass ratio for the system, around 55%-70%, to obtain the highest dehumidification rate. The ratio increased with the regeneration air temperature. There existed an optimal rotary speed (approx. 12 r·h-1) and optimal air flow ratio (approx. 70%). Overall, the feasibility of the proposed system was validated and the dehumidification characteristics at various working conditions were demonstrated to prompt its application. © ECOS 2019 - Proceedings of the 32nd International Conference on Efficiency, Cost, Optimization, Simulation and Environmental Impact of Energy Systems. All rights reserved.

关键词： Air conditioning

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Investigation on turbulent characterization of arrayed micro-tube premixed hydrogen flames using an enhanced flamelet library

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Applied Thermal engineering 2025年 275卷

作者： Han, Xiao Yin, Yanxu Wang, Bosen Chang, Yunxin Cai, Xiao Research Institute of Aero-Engine Beihang University Beijing 100191 China National Key Laboratory of Science and Technology on Aero-Engine Aero-thermodynamics Beihang University Beijing 100191 China Collaborative Innovation Center for Advanced Aero-Engine Beihang University Beijing 100191 China Xi'an Jiaotong University State Key Laboratory of Multiphase Flow in Power Engineering Xi'an 710049 China

Lean turbulent premixed hydrogen/air flames exhibit increased flame wrinkling and significantly enhanced flame speeds, posing challenges for stable combustion. In the novel arrayed multi-flame burner, flame instabilities are intensified by flame-flame interactions. This study develops a distributed and efficient numerical framework for the Large Eddy Simulation-Flamelet Generated Manifold (LES-FGM) method, incorporating an improved 1D flamelet library. The framework is applied to investigate flame dynamics in both bluff-body and conical flame systems under varying equivalence ratios (ϕ= 0.4–0.7) and Karlovitz numbers (Ka = 1–100). By accounting for preferential diffusion, thermal-diffusive instability, and heat loss in stretched flames, the framework improves the accuracy of the flamelet library and captures key physical effects. 1D simulations are performed to validate and analyze the influence of differential diffusion on flame characteristics. The impact of transient flame stretching is analyzed in detail, revealing its critical role in stability transitions across varying turbulence intensities. Additionally, this study examines turbulence effects and micromix multi-flame interactions. The flame stretch factor varies from 1.1 to 2.4 in these three cases. At lower equivalence ratios, higher Ka suppresses tip-opening but intensifies small-scale flame wrinkling. Flame pocket detachment becomes more frequent. Vortex interactions play a key role in flame instability. The strain rate of conical flames is 40 % lower than that of bluff-body flames. These findings provide novel insights into flame dynamics in multi-flame burner arrays, which are critical for optimizing combustion performance in gas turbine combustors. © 2025 Elsevier Ltd

关键词： Flame instability Flamelet generated manifold Lean premixed hydrogen Micromix combustion Multi-flame burner array

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Experimental study on loop heat pipe with flat evaporator at different tilt angles

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Hsi-An Chiao Tung Ta Hsueh/Journal of Xi'an Jiaotong University 2013年第5期47卷 38-43页

作者： Long, Yan Wei, Jinjia Lü, Xiao State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China

To realize highly efficient heat dissipation of electronics, a loop heat pipe (LHP) with a flat evaporator was designed to study its operation characteristics at the tilt angles of 0°, 30°, 45°, 60°, 90° with an improved evaporator structure and a well arranged pipes which can reduce heat loss due to back conduction and improve inner flow performance. The results show that the LHP with inclination has a lower power to start up than the horizontal one, and at the same heat load, the operation temperature of the evaporator is much lower and the system is easier to reach a steady state with less temperature oscillations. However, there is slight difference in operating performance for the LHP at different title angles. The thermal resistance decreases with an increase in the heat load and a steady state occurs at last. The thermal resistance is larger for the horizontal case than that for the inclination case at the same heat load. The thermal resistances are very different at different tilt angles at low heat load, but the difference is small at high heat load.

关键词： Thermal load

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Evolution of nanofluid rayleigh-bénard flows between two parallel plates: A mesoscopic modeling study

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Journal of Nanotechnology in engineering and Medicine 2013年第4期4卷 040905页

作者： Lu, Gui Duan, Yuan-Yuan Wang, Xiao-Dong Key Laboratory for Thermal Science and Power Engineering MOE Tsinghua University Beijing 100084 China Institute of Thermal Engineering Beijing Jiaotong University Beijing 100044 China State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources North China Electric Power University Beijing 102206 China Beijing Key Laboratory of Multiphase Flow and Heat Transfer for Low Grade Energy North China Electric Power University Beijing 102206 China

The developing and developed nanofluid Rayleigh-Bénard flows between two parallel plates was simulated using the mesoscopic thermal lattice-Boltzmann method (LBM). The coupled effects of the thermal conductivity and the dynamic viscosity on the evolution of Rayleigh-Bénard flows were examined using different particle volume fractions (1-4%), while the individual effects of the thermal conductivity and the dynamic viscosity were tested using various particle sizes (11 nm, 20 nm, and 30 nm) and nanoparticle types (Al 2O3, Cu, and CuO2). Two different heating modes were also considered. The results show that Rayleigh-Bénard cell in nanofluids is significantly different from that in pure fluids. The stable convection cells in nanofluids come from the expansion and shedding of an initial vortex pair, while the flow begins suddenly in pure water when the Rayleigh number reaches a critical value. Therefore, the average Nusselt number increases gradually for nanofluids but sharply for pure liquids. Uniform fully developed flow cells with fewer but larger vortex pairs are generated with the bottom heating with nanofluids than with pure liquid, with extremely tiny vortexes confined near the top heating plate for top heating. The number of vortex pairs decreases with increasing nanoparticle volume fraction and particle diameter due to the increasing of dynamic viscosity. The average Nusselt number increases with the increasing Rayleigh number, while decreases with the increasing nanoparticle diameters. The nanoparticle types have little effect on the Rayleigh-Bénard flow patterns. The Rayleigh-Bénard flows are more sensitive with the dynamic viscosity than the thermal conductivity of nanofluids. Copyright © 2013 by ASME.

关键词： Nanoparticles

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Effect of ammonium ion on the corrosion behavior of Ni 2 FeCrMo 0.2 high-entropy alloy in simulated haze solution

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Journal of Materials Research and Technology 2025年

作者： Kai Wang Qilong Zhao Yanhui Li Ruidong Li Qipeng Xu State Key Laboratory of Eco-hydraulics in Northwest Arid Region Xi’an University of Technology No.5 Jinhua South Road Xi’an 710048 China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University No.28 Xianning West Road Xi’an 710049 China School of Chemical Engineering Northwest University No.229 Taibai North Road Xi’an 710069 China

Various constituents of PM 2.5 in haze can accelerate metal corrosion, but traditional carbon steel and stainless steel perform poorly in such complex corrosive environments, and thus developing new corrosion-resistant materials are of great importance for mitigating haze-induced corrosion. The corrosion behavior of Ni 2 FeCrMo 0.2 alloy in haze-simulating aqueous solutions containing various constituents of PM 2.5 in haze is investigated. By the coupling analysis of electrochemical experiments, corrosion morphology, and corrosion product film, the influence of NH+ 4 concentration on the corrosion mechanism related to multi-principal metal elements is revealed. The results show that the Ni 2 FeCrMo 0.2 alloy exhibits superior corrosion resistance compared with 2205 duplex stainless steel. As the NH+ 4 concentration increases, the corrosion rate increases initially but then decreases at higher NH+ 4 concentrations, and the corrosion morphology also confirms this changing trend. The corrosion prompt is primarily due to the lower solution pH caused by the hydrolysis reaction of NH+ 4. In contrast, the corrosion inhibition at higher NH+ 4concentration is attributed to the passive film on the alloy surface, which is composed of Cr, Fe, Mo, Ni, and their oxides, with the presence of Mo elements forming a unique structure that improved the density and stability of the film, thereby inhibiting the growth of corrosion pits. The changing trend of corrosion film resistance and corrosion product film thickness agrees well with this change in corrosion rate. This study provides an insightful understanding of the corrosion behavior of multi-principal alloy materials in haze environments, which is crucial for the corrosion protection design of metal equipment materials.

关键词： Haze constituents Corrosion High entropy alloy Passive film

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Single electron loss in the collisions of Ca+ and atomic hydrogen

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中国物理B（英文版） 2010年第9期19卷 344-348页

作者： Liu Hui-Ping Ouyang Xiao-Ping Hu Hua-Si Su Guang-Hui State Key Laboratory of Multiphase Flow in Power Engineering Department of Nuclear Science and TechnologyXi'anjiaotong UniversityXi'an 710049China

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Thermodynamic analysis on a heat-power decoupling system integrated with absorption heat pump

Thermodynamic analysis on a heat-power decoupling system int...

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2019 Canadian Society for Civil engineering Annual Conference, CSCE 2019

作者： Wang, Liyuan Liu, Ming Fu, Yue Liu, Jiping Yan, Junjie MOE Key Laboratory of Thermal Fluid Science Engineering School of Energy and Power Engineering Xi'an Jiaotong University Xi'an Shaanxi China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University Xi'an Shaanxi China

ISBN: (纸本)9780791883747

Because of the continuous expanding of the district heating, the heating load of combined heat and power(CHP) plants increases year by year. The minimum power load of CHP plant increases with the heating load due to the heat-power coupling mechanism. Therefore, heat-power decoupling is necessary to improve the operation flexibility for CHP units. Integrating the absorption heat pump(AHP) is an effective method to realize the heat-power decoupling. In this study, a 330MW CHP unit model and AHP model have been developed and validated. The performance of the heat-power decoupling and energy saving performance has been investigated by comparing the thermodynamic performance indicators. Results show that, the proposed system can increase the maximum heating load and decrease the power generation when the primary network return temperature is decreased. When the heating steam extraction is kept constant, with the increase of the primary network return water temperature, the heat generation efficiency and the standard coal consumption rate of heating increases, the coal consumption rate of power generation and the heating efficiency decreases. And the primary network return water temperature increases from 40 °C to 70 °C, the coal consumption rate of power generation decreases by 4.3 g/kWh, and the coal consumption rate of heating increases by 0.67 kg/GJ. Copyright © 2020 ASME.

关键词： Water temperature

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Ultrafine polycrystalline titania nanofibers for superior sodium storage

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Journal of Energy Chemistry 2019年第11期28卷 153-161页

作者： Zhidan Diao Daming Zhao Chunxiao Lv Hongli Liu Dongjiang Yang Shaohua Shen International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049ShaanxiChina School of Environmental Science and Engineering Collaborative Innovation Centerfor Marine Biomass FibersMaterials and Textiles of Shandong ProvinceQingdao UniversityQingdao 266071ShandongChina

Sodium ion batteries have a huge potential for large-scale energy storage for the low cost and abundance of sodium resources. In this work, a novel structure of ultrafine polycrystalline TiO2 nanofibers is prepared on nickel foam/carbon cloth by a simple vapor deposition method. The as-prepared TiO2 nanofibers show excellent performance when used as anodes for sodium-ion batteries. Specifically, the TiO2 nanofibers@nickel foam electrode delivers a high reversible capacity of 263.2 m Ahg^-1 at 0.2 C and maintains a considerable capacity of 144.2 m Ahg^-1 at 10 C. The TiO2 nanofibers@carbon cloth electrode also shows excellent high-rate capability, sustaining a capacity of 148 m Ahg^-1 after 20 0 0 cycles at 10 C. It is believed that the novel nanofibrous structure increases the contact area with the electrolyte and greatly shortens the sodium ion diffusion distance, and meanwhile, the polycrystalline nature of nanofibers exposes more intercalation sites for sodium storage. Furthermore, the density functional theory calculations exhibit strong ionic interactions between the exposed TiO2(101) facets and sodium ions, leading to a preferable sodiation/desodiation process. The unique structural features endow the TiO2 nanofibers electrodes great advantages in rapid sodium storage with an outstanding high-rate capability.

关键词： Polycrystalline titania Nanofibers Sodium storage High-rate capability

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Pressure drops and model modification for two-phase flow in porous beds with coarse particles 25

Pressure drops and model modification for two-phase flow in ...

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2017 25th International Conference on Nuclear engineering, ICONE 2017

作者： Li, Xumao Zou Liangxing Wang, Liubo Kong Huasheng State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xianning West Road 28# Xi'an city710049 China

ISBN: (纸本)9780791857823

Motivated by reducing the uncertainties in coolability analysis of a debris bed, this paper proposed a modified model for the pressure drops of two phase flow through packed beds with coarse particles based on the experimental studies. The experiments are carried out on the test facility of DEBECO-LT (DEbris BEd COolability-Low Temperature), which was designed to investigate single / two-phase flow in porous beds. The coarse particles are packed in the cylindrical test section with the inner diameter of 120 mm and the height of 600 mm. Through single-phase flow tests in homogeneous beds, the reliability of the whole experimental system is ensured. Then two-phase flow tests are performed to investigate the flow characteristics, to provide basic data for verifying and modifying the existing models. The results show that, the interfacial drag in beds with coarse particles will result in a decreasing tendency in the pressure drop curves along with the fluid velocity, and the the effect of interfacial drag should be considered in the debris coolability analysis models for beds with coarse particles. Compared with the existing models, the new model shows relatively satisfactory forecasting ability, and the predictions have favorable agreement with existing experimental data under various conditions. This modified model could be applied to calculate the pressure drops of twophase flow in coarse-particle beds. © Copyright 2017 ASME.

关键词： Pressure drop

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