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Study of thermophysical properties of binary mixtures of N-phenyl ethanolammonium based protic ionic liquids with water and ethanol solvents

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Journal of Ionic Liquids 2022年第1期2卷

作者： Chennuri, Bharath Kumar Losetty, Venkatramana Sreenivasulu, K. Gardas, Ramesh L. Sivakumar, K. A.P. Tirupati517502 India Department of Chemistry VelTech Rangarajan Dr. Sagunthala R&D Institute of Science and Technology Avadi Chennai600062 India Department of Chemistry State Key Laboratory of Multiphase Flow in Power Engineering Xian Jiaotong University Xian710049 China Department of Chemistry Indian Institute of Technology Madras Chennai600036 India

This work reveals that the physicochemical properties such as density, ρ and speed of sound, u for the binary mixtures of N-phenylethanolammonium formate ([NPEA][For]) and N-phenylethanolammonium acetate ([NPEA][Ace] with water and ethanol solvents were experimentally measured for the temperature ranges from 293.15 K to 318.15 K at atmosphere pressure. The apparent molar volume, VΦ and apparent molar isentropic compressibility, κs,Φ were estimated from the experimental data. Redlich-Mayer type empirical equation was applied to calculate the limiting apparent molar properties at infinite dilution (Vω∞ and k∞) and corresponding empirical parameters (Sv, Bv, Sk and Bk). The type of interaction either IL-solvent or IL-IL or solvent-solvent occurring in solution were determined from the data of empirical parameters. Furthermore, the temperature dependent apparent molar volume at infinite dilution, V∞ was used to calculate the apparent molar expansibility at infinite dilution, E∞. Moreover, these E∞ values of the studied binary solutions were found to be positive. The making and breaking structure ability of both PILs were analyzed at all experimental conditions. © 2021 The Authors

关键词： Dilution

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A Coupled Bioheat Transfer Model for Customized Whole-Eye Modeling in Retinal Laser Surgery

SSRN

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SSRN 2022年

作者： Zhao, P.H. Li, K. Zhang, H. Li, Dong Chen, B. Zheng, Y.P. Li, W.P. Wang, G.X. Fan, L.H. Yao, L. State Key Laboratory of Multiphase Flow in Power Engineering Xi 'an Jiaotong University Shaanxi Xi'An710049 China Department of Ophthalmology The Second Affiliated Hospital of Xi 'an Jiaotong University Shaanxi Xi'An710004 China The First Affiliated Hospital of Xi'an Joao Tong University Shaanxi Xi'An710061 China Department of Mechanical Engineering The University of Akron Akron United States

The photo-thermal effects of laser on tissue is widely used in ophthalmology to treat retinal diseases. By adjusting the pulse duration from nano to tens of seconds, the multi-scale retinal lesion from micro to millimeter size can be thermally targeted. Large scale difference among the target lesions brought extra challenge for retinal laser surgery modeling. In this study, we developed a coupled whole eye model for retinal laser surgery. In the model, Penens bioheat transfer equation was adapted for the whole eye temperature modeling. Simultaneously, we treat the fundus as a multi-layered porous medium made of a tissue matrix buried with highly-absorbing chromophores (melanin or blood). Two-temperature equations, one for the chromophore and the other for the surrounding tissue, will be developed based on the local thermal non-equilibrium theory of porous media. The Pennes model and the two-temperature model was coupled together to calculated the thermal responses of eye during several laser retinal surgery process with pulse duration from nano to tens of seconds. The simulation results proved our model is capable of modeling laser retinal surgery process in different time scale. Furthermore, the present coupled model was applied in a real fundus anatomy from a patient with diabetic retinopathy to illustrate its feasibility in customized laser protocol planning. © 2022, The Authors. All rights reserved.

关键词： Ophthalmology

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Beam dynamics induced by the quantum metric of exceptional rings

arXiv

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arXiv 2024年

作者： Zhang, Zhaoyang Septembre, Ismaël Liu, Zhenzhi Kokhanchik, Pavel Liang, Shun Liu, Fu Li, Changbiao Wang, Hongxing Liu, Maochang Zhang, Yanpeng Xiao, Min Malpuech, Guillaume Solnyshkov, Dmitry Key Laboratory for Physical Electronics and Devices The Ministry of Education Shaanxi Key Lab of Information Photonic Technique School of Electronic Science and Engineering Faculty of Electronics and Information Xi’an Jiaotong University Xi’an710049 China Institut Pascal PHOTON-N2 Université Clermont Auvergne CNRS Clermont INP Clermont-FerrandF-63000 France Naturwissenschaftlich-Technische Fakultät Universität Siegen Walter-Flex-Straße 3 Siegen57068 Germany International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Department of Physics University of Arkansas FayettevilleAR72701 United States Paris75231 France

Topological physics has broadened its scope from the study of topological insulating phases to include nodal phases containing band structure singularities. The geometry of the corresponding quantum states is described by the quantum metric which provides a theoretical framework for explaining phenomena that conventional approaches fail to address. The field has become even broader by encompassing non-Hermitian singularities: in addition to Dirac, Weyl nodes, or nodal lines, it is now common to encounter exceptional points, exceptional or Weyl rings, and even Weyl spheres. They give access to fascinating effects that cannot be reached within the Hermitian picture. However, the quantum geometry of non-Hermitian singularities is not a straightforward extension of the Hermitian one, remaining far less understood. Here, we study experimentally and theoretically the dynamics of wave packets at exceptional rings stemming from Dirac points in a photonic honeycomb lattice. First, we demonstrate a transition between conical diffraction and non-Hermitian broadening in real space. Next, we predict and demonstrate a new non-Hermitian effect in the reciprocal space, induced by the non-orthogonality of the eigenstates. We call it transverse non-Hermitian drift, and its description requires biorthogonal quantum metric. The non-Hermitian drift can be used for applications in beam steering. Copyright © 2024, The Authors. All rights reserved.

关键词： Topology

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Characterizing the catalyst fluidization with field synergy to improve the amine absorption for CO2 capture

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Chinese Journal of Chemical engineering 2019年第7期27卷 1608-1617页

作者： Yunsong Yu Chen Zhang Zaoxiao Zhang Geoff Wang School of Chemical Engineering and Technology Xi’an Jiaotong UniversityXi’an 710049China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049China School of Chemical Engineering The University of QueenslandSt LuciaQLD 4072Australia

There are great interests to capture the CO2 to control the greenhouse gas *** absorption of CO2 is being taken as an effective way to capture CO2 in ***,the amine absorption of CO2 is cost-ineffective due to great energy consumption and solution *** order to reduce the capture cost,catalyst fluidization is proposed here to intensify the mass transfer and heat *** fluidization with field synergy and DFT model is developed by incorporating the effects of catalyst reaction kinetics,drag force and multi-field into the mass transfer,heat transfer,fluid flow and catalyst *** with an improved distributor are performed well to validate the *** reaction kinetics is determined by the DFT simulation and *** mass transfer coefficient in the fluidized reactor is identified as 17%higher than the conventional packed *** the field synergy of catalyst fluidization,the energy consumption for CO2 desorption is reduced by 9%.Stepwise operation and inclination reactor are used to improve catalyst fluidization process.

关键词： CO2 capture Catalyst fluidization Mass transfer DFT Energy consumption Field synergy

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Multi-Objective optimization of oil–gas cyclone separators considering liquid storage in the tank bottom

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Separation and Purification Technology 2025年 374卷

作者： Wang, Lingzi Du, Wei Liu, Ruiyi Feng, Jianmei Peng, Xueyuan Cao, Feng School of Energy and Power Engineering Xi'an Jiaotong University Shaanxi Xi'an710049 China The First Gas Plant of PetroChina Changqing Oilfield Company Shaanxi Jingbian718500 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China

As an efficient separation device, the gas–liquid cyclone separator has been widely used in oil injection compressor systems. It can effectively reduce the oil content in the high-pressure airflow, directly affecting the fuel consumption, operating efficiency, and exhaust quality parameters of compressors, making it crucial to enhance the separator's performance. Given the critical role of geometric configuration in determining cyclone separator efficiency, this study comprehensively considers several influencing factors including the structure parameters. Taguchi method and analysis of variance (ANOVA) were used to quantify the contribution of three factors to the performance percentage of the separator, and the dual-objective optimization of the efficiency and pressure drop of the separator was carried out with the grey correlation analysis method. In the simulation calculation, this paper employs the DPM-to-VOF method coupled with the Euler wall film (EWF) to simulate the oil droplet particle separation process, featuring model transformation capabilities under specified conditions. The investigation culminates in the development of a parametric-performance prediction model and establishes optimal operational parameters for cyclone separators: the inlet velocity (vin) should be set at 24.49 m/s, the height of the inner cylinder of the separator tank (Ht) should be 1.2 times the diameter, and the buffer height between the inner cylinder and the liquid surface (Hm) should be 0.9 times the diameter. © 2025

关键词： Cyclone separators

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Kinetics of oxygen bubble growth in water decomposition

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Wuli Xuebao/Acta Physica Sinica 2025年第10期74卷

作者： Nie, Tengfei Xu, Qiang Luo, Xinyi Hong, Aoyue Cao, Zeshui Guo, Liejin State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China

In order to enhance the efficiency of large-scale water decomposition, it is important to understand the oxygen bubble evolution on the electrode surface. In this work, a numerical model for the growth of oxygen bubbles on the electrode surface is proposed based on the dissolved oxygen flux at the bubble boundary, and the mechanisms of the reaction area and current during the bubble growth are investigated. The results show that the bubble diameters calculated from the oxygen flux at the bubble boundary are in good agreement with the diameters of the bubbles growing in the control phase of the chemical reaction. As the reaction region increases, the transition time from the diffusion-controlled stage to the chemical reaction-controlled stage becomes longer during the bubble growth. The concentration maximum value on the microelectrode surface is significantly higher than that on the large electrode surface, which leads to a steeper concentration gradient between the microelectrode surface and the bubble surface. As the current increases, the bubble growth rate increases and the time coefficient decreases faster. The bubble diameter at a current of 0.06 mA accords well with the bubble diameter at a current of 0.1 mA in the photoelectrochemical water splitting experiments. This is because the scattering of light by the growing bubbles leads to a decrease in the current density at the bottom of the bubble.(Figure Presented) © 2025 Chinese Physical Society.

关键词： Pyrolysis

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Corrigendum to “Numerical simulation of an externally heated fixed bed reactor for coal pyrolysis based on porous media” [Chem. Eng. Res. Des. 211 (2024) 137–151]

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Chemical engineering Research and Design 2025年 218卷 454-454页

作者： Haoyue Li Yuanpei Luo Fei Dai Jun Sui Hongguang Jin Laboratory of Distributed Energy Systems and Renewable Energy Institute of Engineering Thermophysics Chinese Academy of Sciences Beijing 100190 China University of Chinese Academy of Sciences Beijing 100049 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China

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Non-Hermitian delocalization in a 2D photonic quasicrystal

arXiv

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arXiv 2023年

作者： Zhang, Zhaoyang Liang, Shun Septembre, Ismaël Yu, Jiawei Huang, Yongping Liu, Maochang Zhang, Yanpeng Xiao, Min Malpuech, Guillaume Solnyshkov, Dmitry Key Laboratory for Physical Electronics and Devices The Ministry of Education Shaanxi Key Lab of Information Photonic Technique School of Electronic Science and Engineering Faculty of Electronics and Information Xi’an Jiaotong University Xi’an710049 China Institut Pascal PHOTON-N2 Université Clermont Auvergne CNRS Clermont INP Clermont-FerrandF-63000 France International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Department of Physics University of Arkansas FayettevilleAR72701 United States National Laboratory of Solid State Microstructures School of Physics Nanjing University Nanjing210093 China Paris75231 France

Quasicrystals show long-range order, but lack translational symmetry. So far, theoretical and experimental studies suggest that both Hermitian and non-Hermitian quasicrystals show localized eigenstates. This localization is due to the fractal structure of the spectrum in the Hermitian case and to the transition to diffusive bands via exceptional points in the non-Hermitian case. Here, we present an experimental study of a dodecagonal (12-fold) photonic quasicrystal based on electromagnetically-induced transparency in a Rb vapor cell. The transition to a quasicrystal is obtained by superposing two honeycomb lattices at 30◦ with a continuous tuning of their amplitudes. Non-Hermiticity is controlled independently. We study the spatial expansion of a probe wavepacket. In the Hermitian case, the wavepacket expansion is suppressed when the amplitude of the second lattice is increased (quasicrystal localization). We find a new regime, where increasing the non-Hermitian potential in the quasicrystal enhances spatial expansion, with the C12 symmetry becoming visible in the wavepacket structure. This real-space expansion is due to a k-space localization on specific quasicrystal modes. Our results show that the non-Hermitian quasicrystal behavior is richer than previously thought. The localization properties of the quasicrystals can be used for beam tailoring in photonics, but are also important in other fields. Copyright © 2023, The Authors. All rights reserved.

关键词： Quasicrystals

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Remote open-path laser-induced breakdown spectroscopy for the analysis of manganese in steel samples at high temperature

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Plasma Science and Technology 2019年第3期21卷 52-59页

作者： Minchao CUI Yoshihiro DEGUCHI Zhenzhen WANG Seiya TANAKA Min-Gyu JEON Yuki FUJITA Shengdun ZHAO School of Mechanical Engineering Xi'an Jiaotong University Graduate School of Advanced Technology and Science University of Tokushima State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Division of Mechanical Engineering Korea Maritime and Ocean University School of Mechanical Engineering Xi’an Jiaotong University

A remote open-path laser-induced breakdown spectroscopy(LIBS) system was designed and studied in the present work for the purpose of combining the LIBS technique with the steel production line. In this system, the relatively simple configuration and optics were employed to measure the steel samples at a remote distance and a hot sample temperature. The system has obtained a robustness for the deviation of the sample position because of the open-path and alloptical structure. The measurement was carried out at different sample temperatures by placing the samples in a muffle furnace with a window in the front door. The results show that the intensity of the spectral lines increased as the sample temperature increased. The influence of the sample temperature on the quantitative analysis of manganese in the steel samples was investigated by measuring ten standard steel samples at different temperatures. Three samples were selected as the test sample for the simulation measurement. The results show that, at the sample temperature of 500 ℃, the average relative error of prediction is 3.1% and the average relative standard deviation is 7.7%, respectively.

关键词： remote open-path LIBS steel manganese sample temperature quantitative analysis

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CO₂-to-C₂H₅OH photoconversion by an amorphization-activated catalyst

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Chem Catalysis 2025年第5期5卷

作者： Xue, Fei Zhang, Chunyang Liu, Maochang Liu, Feng Yan, Xueli Liu, Shangheng Peng, Huiping Hu, Zhiwei Pao, Chih-Wen Huang, Wei-Hsiang Yang, Ye Huang, Xiaoqing Xu, Yong i-lab of Suzhou Institute of Nano-Tech and Nano-Bionics (SINANO) Chinese Academy of Sciences (CAS) Suzhou 215123 China State Key Laboratory of Physical Chemistry of Solid Surfaces College of Chemistry and Chemical Engineering Xiamen University Xiamen 361005 China International Research Center for Renewable Energy & State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China Max Planck Institute for Chemical Physics of Solids Nothnitzer Strasse 40 Dresden 01187 Germany National Synchrotron Radiation Research Center 101 Hsin-Ann Road Hsinchu 30076 Taiwan Innovation Laboratory for Sciences and Technologies of Energy Materials of Fujian Province (IKKEM) Xiamen 361005 China

CO2 photoconversion into value-added C2 products with high selectivity and efficiency is formidably challenging due to highly energetic and kinetic restriction of C–C coupling. Designing catalysts to overcome those b... 详细信息

CO₂ photoconversion into value-added C₂ products with high selectivity and efficiency is formidably challenging due to highly energetic and kinetic restriction of C–C coupling. Designing catalysts to overcome those barriers is therefore crucial. Here, for the first time, we demonstrate an amorphization strategy to boost photocatalytic CO₂ ethanolization. By integrating amorphous Pd onto Cd_0.9Zn_0.1S nanorods (a-Pd/CZS), an activity of 412.1 μmol g⁻¹ h⁻¹ and a selectivity of 96.5% for CO₂-to-C₂H₅OH photoconversion were achieved without a sacrificial agent with an apparent quantum efficiency (AQE) of 0.87% at 420 nm. The superior performance results from rapid migration of photogenerated electrons to amorphous Pd via interfacial Ohmic junction. In situ characterization and theoretical calculation further reveal that amorphous Pd can optimize CO₂ adsorption/activation and reduce the C–C coupling energy barrier via intensified interaction and stabilization with a ^∗OCCO intermediate, thereby maximizing conversion efficiency and selectivity. This work highlights an efficient photocatalyst for a CO₂-to-C₂ product and inspires high-performance photocatalyst design. © 2025 Elsevier Inc.

关键词： amorphization C2H5OH CO2 photocatalytic conversion SDG7: Affordable and clean energy

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