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Semiempirical equations of state of H_(2)O/CO_(2) binary mixtures in graphite nanoslits

Science China(Physics,Mechanics & Astronomy) 2023年第8期66卷 83-92页

作者： Haoxuan Li Bin Zhao Chengzhen Sun Bofeng Bai State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong UniversityXi'an 710049China

The existence of confining walls limits the prediction accuracy of nanoconfined fluids using macroscopic equations of state(EOSs);moreover,appropriate EOSs for multicomponent mixture fluids in nanoconfined spaces are ***,we derive the EOS of multicomponent mixture fluids confined in nanospaces at high temperatures and pressures,mainly considering the nanoconfinement effect and the competitive adsorption effect between different ***,the EOSs are validated through comparison with the molecular dynamics-simulated Pv T data of CO_(2)/H_(2)O mixtures in graphite *** consider the above effects,we derive two EOSs via two modeling methods:EOS I is obtained through modification of the actual component occupation volume in the Peng-Robinson equation of state(PR EOS)by fitting the binary component interaction coefficient and the number of adsorbed molecules according to a selectivity coefficient,while EOS II is obtained by considering the decreased pressure of the fluids in PR EOS by adding an attractive term between components and *** the simulation results as a benchmark,the two EOSs exhibited good prediction accuracies under low CO_(2) concentrations,and generally,EOS II was more accurate than EOS *** study fills the gap in the EOSs of nanoconfined mixture fluids,and the obtained equations can help to further describe the thermodynamic properties of confined mixture fluids.

关键词： confined fluid mixtures equation of state nanoconfined spaces molecular dynamics simulation

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A numerical investigation on heat transfer characteristics of a particle cluster in fluid with variable properties

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Particuology 2024年第11期94卷 327-344页

作者： Xiaoyu Li Huibo Wang Bowei Zhang Hui Jin State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong UniversityXi'an710049China

This work investigates the heat transfer characteristics of particle clusters under the effects of the complex properties of supercritical water(SCW).It analyzes the heat transfer characteristics of sub-particles and the average heat transfer characteristics of particle *** results reveal a phenomenon of shifting positions of high specific heat *** led to variations in the dimensionless heat transfer coefficient ***,the results indicate that as the heat transfer process strengthens,the effects of variations in property distribution on heat transfer tends to *** on this conclusion,the effects of variations in property distribution on heat transfer are categorized into Stable Effects Region and Non-Stable Effects *** utilizing the principles of fluid flow-heat transfer coupling and similarity,a heat transfer prediction model for particle clusters in SCW is established.

关键词： Heat transfer Supercritical water Particle cluster Modeling

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Development of a fan-stirred constant volume combustion chamber and turbulence measurement with PIV

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Frontiers in Energy 2022年第6期16卷 973-987页

作者： Haoran ZHAO Jinhua WANG Xiao CAI Zhijian BIAN Hongchao DAI Zuohua HUANG State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049China

A fan-stirred combustion chamber is developed for spherically expanding flames,with P and T up to 10 bar and 473 K,*** characteristics are estimated using particle image velocimetry(PIV)at different initial pressures(P=0.5-5 bar),fan frequencies(ω=0-2000 r/min),and impeller diameters(D=100 and 114 mm).The flame propagation of methanol/air is investigated at different turbulence intensities(u′=0-1.77 m/s)and equivalence ratios(f=0.7-1.5).The results show that u′is independent of P and proportional toω,which can be up to 3.5 m/s at 2000 r/min.L_(T)is independent of P and performs a power regression withω*** turbulent field is homogeneous and isotropic in the central region of the chamber while the inertial subrange of spatial energy spectrum is more collapsed to-5/3 law at a high Re_(T).Compared to laminar expanding flames,the morphology of turbulent expanding flames is wrinkled and the wrinkles will be finer with the growth of turbulence intensity,consistent with the decline of the Taylor scale and the Kolmogorov *** determined S_(L)in the present study is in good agreement with that of previous *** S_(L)and S_(T)of methanol/air have a non-monotonic trend with f while peak S_(T)is shifted to the richer side compared to S_(L).This indicates that the newly built turbulent combustion chamber is reliable for further experimental study.

关键词： fan-stirred combustion chamber turbulence characteristics particle image velocimetry(PIV) methanol turbulent expanding flames

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Numerical Investigation on the Heat Transfer Characteristics of Supercritical Water in a Non-Uniformly Heated Tube for a Supercritical CFB Boiler

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Journal of Thermal Science 2023年第5期32卷 1807-1818页

作者： DU Xiaocheng SONG Yuanyuan XIANG Yuxuan ZHOU Yanjun WANG Aoyu YANG Dong State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong UniversityXi'an 710049China

In this paper,a numerical model was built by ANSYS FLUENT to investigate the heat transfer performances of supercritical water in a circumferential non-uniformly heated vertical *** Shear Stress Transport(SST)k-ωmodel was adopted for describing *** operating parameters are chosen according to a 660 MW ultra-supercritical CFB *** heat transfer performances under different operating parameters,such as boiler load,flow direction and heat flux distribution are *** temperature and heat flux on inner wall varies along the circumference and show symmetric *** overall heat transfer performances at each cross section are better than the local heat transfer performance of midpoint of heating *** direction has a great influence on heat transfer performance;it changes the radial distribution of axial velocity and then affects the turbulence ***,upward flow condition shows a better heat transfer *** heat flux improves both the overall and local heat transfer *** the heat flux area is not conducive to the overall heat transfer,but does not affect the local heat transfer at the midpoint of heating ***,a new correlation is fitted based on the simulated results of supercritical water heat transfer with circumferential non-uniform heat flux distributions.

关键词： supercritical CFB boiler circumferential non-uniform heat flux numerical simulation heat transfer correlation

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Optimization of cold-end system of thermal power plants based on entropy generation minimization

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Frontiers in Energy 2022年第6期16卷 956-972页

作者： Yue FU Yongliang ZHAO Ming LIU Jinshi WANG Junjie YAN State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049China

Cold-end systems are heat sinks of thermal power cycles,which have an essential effect on the overall performance of thermal power *** enhance the efficiency of thermal power plants,multi-pressure condensers have been applied in some large-capacity thermal power ***,little attention has been paid to the optimization of the cold-end system with multi-pressure condensers which have multiple parameters to be ***,the design optimization methods of coldend systems with single-and multi-pressure condensers are developed based on the entropy generation rate,and the genetic algorithm(GA)is used to optimize multiple *** parameters,including heat transfer area of multi-pressure condensers,steam distribution in condensers,and cooling water mass flow rate,are optimized while considering detailed entropy generation rate of the cold-end *** results show that the entropy generation rate of the multi-pressure cold-end system is less than that of the single-pressure cold-end system when the total condenser area is ***,the economic performance can be improved with the adoption of the multi-pressure cold-end *** compared with the single-pressure cold-end system,the excess revenues gained by using dual-and quadruplepressure cold-end systems are 575 and 580 k$/a,respectively.

关键词： cold-end system entropy generation minimization optimization economic analysis genetic algorithm(GA)

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Large Eddy Simulation Study on the Turbulence and Flame Characteristics under Analogical Integral Scale and Turbulence Intensity of Turbulent Premixed Flames

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Journal of Thermal Science 2023年第1期32卷 488-501页

作者： WEI Xutao WANG Jinhua ZHANG Meng HUANG Zuohua State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong UniversityXi'an 710049China

Bunsen burner is a typical geometry for investigating the turbulence-flame *** most experimental studies,only turbulence intensity u′and integral scale l0 are used to characterize the turbulent flow field,regardless of the perforation geometry of perforated ***,since the geometry influences the developing process and vortex broken,the plate geometry has to be considered when discussing the flame-turbulence *** order to investigate conditions at the same l0 and u′using different geometries,large eddy simulation of CH_(4)/air flames with dynamic TF combustion model was *** model validation shows good agreement between Large Eddy Simulation(LES)and experimental *** the non-reacting flows,the Vortex Stretching of circular-perforated plate condition is always larger than that of slot-perforated plate condition,which comes from the stresses in the flow fields to stretch the vorticity *** reacting flows,at the root of the flame,the Vortex Stretching plays a major role,and the total vorticity here of circular-perforated plate condition is still larger(53.8%and 300%larger than that of the slot-perforated plate at x/D=0 and x/D=2.5,respectively).More small-scale vortex in circular-perforated plate condition can affect and wrinkle the flame front to increase the Probability Density Function(PDF)at large *** 3D curvature distributions of both cases bias to negative *** negative trend of curvatures at the instant flame front results from the Dilatation ***,the value of the Vortex Stretching and the Dilatation at the flame front of circular-perforated plate condition is obviously larger.

关键词： large eddy simulation integral scale turbulence intensity vorticity flame curvature

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Assisting effect of Al_(2)O_(3) on MnO_(x) for NO catalytic oxidation

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Green Energy & Environment 2021年第6期6卷 903-909页

作者： Denghui Wang Hui Li Qi Yao Shien Hui Yanqing Niu State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power EngineeringXi'an Jiaotong UniversityXi'an710049China

Various Mn-based catalysts for NO oxidation were prepared using MnO_(x)as active compound,while Ti O_(2)and Al_(2)O_(3)were adopted as catalyst *** performance of the catalysts was tested to study the effect of support on Mn-based catalyst *** of the catalysts followed as Mn_(0.4)/Al>Mn_(0.2)/Al>Mn_(0.4)/Ti>Mn_(0.2)/Ti>MnO_(x)>Al_(2)O_(3)on the whole,indicating the synergism of MnO_(x)and Al_(2)O_(3)for NO catalytic *** were analyzed according to characterization *** oxygen on catalyst rather than lattice oxygen was detected as the active oxidizer for NO *** catalyst support,Al_(2)O_(3)provided more sites to carry surface adsorbed oxygen than TiO_(2),resulting in the presence of more active oxygen on Mn O_(x)/Al_(2)O_(3)than on MnO_(x)/TiO_(2).Moreover,MnO_(x)/Al_(2)O_(3)possessed high surface area and pore volume,which greatly benefited the adsorption of NO on catalyst and further favored the oxidation of NO by active *** these advantages helped Mn_(0.4)/Al exhibited the best catalytic efficiency.

关键词： NO catalytic oxidation MnO_(x)/Al_(2)O_(3) NO_(2) Active oxygen

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Characterizations of gas-liquid interface distribution and slug evolution in a vertical pipe

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Petroleum Science 2023年第5期20卷 3157-3171页

作者： Hai-Yang Yu Qiang Xu Ye-Qi Cao Bo Huang Han-Xuan Wang Lie-Jin Guo State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong UniversityXi’an710049ShaanxiChina

Large vertical pipes are key structures connecting subsea wells to offshore ***,existing studies mainly focus on small vertical *** a vertical acrylic pipe with 80 mm inner diameter and 11 m height,a high-speed camera was used to visually research the influences of pipe diameters,liquid properties and inlet effect on air-water co-flow *** flow regime maps of vertical pipes(diameters are in the range of 50e189 mm)were compared and the critical gas velocity of the transition boundary from bubble to slug flow tended to increase with the increase of diameters at D≥80 ***-flux models were established in different flow regimes and liquid properties have a significant effect on drift coefficients of bubble flow and slug flow(void fraction a≤0.4).The influence of inlet turbulent effect on the gas-liquid interface distribution gradually weakened and disappeared from the pipe base to 85D,where the flow was fully *** frequency has a trend of increase first and then decrease with the gas Weber numbers increasing at low liquid superficial velocities(J_(L)≤0.31 m/s).And on the basis of this law,a new slug frequency correlation was *** was found that there was an exponential relationship between the ratio of lengths of Taylor bubble to slug and the void fraction.

关键词： Void fraction flow regime Drift coefficien Slug frequency Taylor bubble length

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Cyclone separation in a supercritical water circulating fluidized bed reactor for coallbiomass gasification： Structural design and numerical analysis

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Particuology 2018年第4期16卷 55-67页

作者： Guoxing Li Youjun Lu State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an Shaanxi 710049 China

A new concept of a supercritical water （SCW） circulating fiuidized bed reactor is proposed to produce hydrogen from coal/biomass gasification. The cyclone is a key component of the reactor system, in this paper, cyclones with a single circular inlet （SCI） or a double circular inlet （DCI） were designed to adapt to the supercritical conditions. We evaluated the separation performance of the two cyclones using numerical simulations. A three-dimensional Reynolds stress model was used to simulate the turbulent flow of the fluid, and a stochastic Lagrangian model was used to simulate the particle motion. The flow fields of both cyclones were three-dimensionally unsteady and similar to those of traditional gas-solid cyclones. Secondary circulation phenomena were discovered and their influence on particle separation was estimated. Analyzing the distribution of the turbulence kinetic energy revealed that the most intensive turbulence existed in the zone near the vortex finder while the flow in the central part was relatively stable. The particle concentration distribution was non-uniform because of centrifugal forces. The distribution area can be divided into three parts according to the motion of the particles. In addition, the separation efficiency of both cyclones increased with the inlet SCaN velocity. Because of its perturbance flow, the DCI separator had higher separation efficiency than the SCI separator under comparable simulations. However, this was at the expense of a higher pressure drop across the cyclone.

关键词： CycloneStructural design Supercritical water-solid flow Separation performance Circulating fluidized bed Computational fluid dynamics

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Numerical simulation of bubble behavior in a quasi-2D fluidized bed using a bubble-based EMMS model

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Particuology 2019年第5期17卷 40-54页

作者： Hao Wang Youjun Lu State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi'an 710049 Shaanxi China

Bubbles formed during chemical processes in fluidized beds govern the bed hydrodynamics and opera-tional efficiency, thereby having a significant impact on their design and scale-up. In this study, a two-fluid model was used to simulate the bubble behavior in a quasi-two-dimensional fluidized bed within the bubble-based energy minimization multiscale (EMMS) approach. We performed experiments to verify the model and proposed a correlation of the heterogeneous index for various parameters to calculate the coefficient of drag for the bubble-based EMMS model. Moreover, the simulation results obtained from the homogeneous drag models and EMMS bubbling model were compared with experimental data and empirical correlations. The simulation results of the EMMS approach showed good agreement with the experimental data in the distribution of the vertical bubble velocity with chord length. Compared with the results from the homogeneous models, the distributions of vertical velocity and diameter of the bubbles predicted by the EMMS-bubbling model were in better agreement with empirical correlations. Moreover, the frequency distributions of bubble properties including bubble diameter, aspect ratio, and shape factor for different gas-inlet velocities were obtained.

关键词： Energy minimization multi-scale approach Heterogeneous index Fluidized bed Bubble

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