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Nanodiamond reinforced self-healing and transparent poly(urethane-urea)protective coating for scratch resistance

International Journal of Smart and Nano Materials 2024年第1期15卷 75-94页

作者： Zhuochao Wang Wenxin Cao Chunqiang Sun Dongchao Ji Kunlong Zhao Gang Gao Xingchun Xu Yingqi Liu Tianyu Zhang Jiaqi Zhu Jiecai Han National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of TechnologyHarbinChina School of future technology Harbin institute of TechnologyHarbinChina Key Laboratory of Micro-systems and Micro-structures Manufacturing Ministry of EducationHarbinChina

With increasing demand for scratch-resistant flexible electro-nics,the development of transparent coatings with good scratch resistance and self-healing properties has emerged as a key research *** this study,a high-strength self-healing poly(urethane-urea)(PUU)-based nanocomposite coating was prepared by introducing functionalized nanodiamond(ND)into a PUU matrix via solution *** PUU matrix had hard-segment repeating units and was constructed using iso-phorone diamine and isophorone *** ND particles were modifed using a silane coupling agent,3-aminopropyl-triethoxysilane,to obtain well-dispersed KH-ND ***-ND promoted microphase separation in the PU matrix,inducing the formation of dense and homogeneous hard domains that dissipated stress,prevented further crack devel-opment,and improved the mechanical properties and scratch resistance of the *** addition,the coating exhibited excellent self-healing ***-transform infrared spectroscopy,scanning electron microscopy,and atomic force microscopy were used to characterize the self-healing and hardening mechanisms of the *** environmentally friendly PUU/KH-ND coating is easy to prepare and has broad application prospects in transparent and anti-scratch coatings for flexible electronics,automobiles,and home appliances.

关键词： Nanocomposite coatings self-healing scratch resistance transparent poly(urethane-urea)

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Temperature-Dependent Thermal Conductivity and Absorption Coefficient Identification of Quartz Window up to 1100 K

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Journal of Thermal science 2023年第1期32卷 44-58页

作者： SHI Yu CHEN Xue SUN Chuang XIA Xin-Lin School of Energy Science and Engineering Harbin Institute of Technology(HIT)Harbin 150001China

The temperature-dependent absorption coefficient and thermal conductivity of a quartz window are obtained through experimental tests at a wide range of temperatures.A Fourier transform infrared spectrometer with a heated cavity is used for performing the transmittance *** spectral absorption coefficient of the quartz window is inverted by the transmittance information at different temperatures using a genetic ***,a quartz window-graphite plate-quartz window multilayer structure is designed,and the transient response of the structure subjected to high-temperature heating is recorded by a self-designed *** with the above absorption coefficient,a non-gray radiative-conductive heat transfer model is built for the multilayer structure,and the intrinsic thermal conductivity of the quartz window is ***,the effects of the temperature-dependent absorption coefficient and spectral selective features of the medium on the heat transfer characteristics are *** results show that the absorption coefficient gradually increases with *** intrinsic thermal conductivity of the quartz window varies from 1.35 to 2.52 W/(m·K)as the temperature rises,while the effective thermal conductivity is higher than the intrinsic thermal conductivity due to thermal radiation,specifically 26.4%higher at 1100 *** addition,it is found that the influence of the temperature-dependent absorption coefficient on temperature of unheated side shows a trend of first increasing and then *** the absorption coefficient varies greatly with wavelength,a non-gray radiative-conductive heat transfer model should be built for the semitransparent materials.

关键词： semitransparent material quartz window non-gray body absorption coefficient thermal conductivity

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Overhead-free Noise-tolerant Federated Learning: A New Baseline

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Machine Intelligence Research 2024年第3期21卷 526-537页

作者： Shiyi Lin Deming Zhai Feilong Zhang Junjun Jiang Xianming Liu Xiangyang Ji Department of Computer Science and Technology Harbin Institute of TechnologyHarbin150000China Department of Automation Tsinghua UniversityBeijing100084China

Federated learning (FL) is a promising decentralized machine learning approach that enables multiple distributed clients to train a model jointly while keeping their data private. However, in real-world scenarios, the supervised training data stored in local clients inevitably suffer from imperfect annotations, resulting in subjective, inconsistent and biased labels. These noisy labels can harm the collaborative aggregation process of FL by inducing inconsistent decision boundaries. Unfortunately, few attempts have been made towards noise-tolerant federated learning, with most of them relying on the strategy of transmitting overhead messages to assist noisy labels detection and correction, which increases the communication burden as well as privacy risks. In this paper, we propose a simple yet effective method for noise-tolerant FL based on the well-established co-training framework. Our method leverages the inherent discrepancy in the learning ability of the local and global models in FL, which can be regarded as two complementary views. By iteratively exchanging samples with their high confident predictions, the two models “teach each other” to suppress the influence of noisy labels. The proposed scheme enjoys the benefit of overhead cost-free and can serve as a robust and efficient baseline for noise-tolerant federated learning. Experimental results demonstrate that our method outperforms existing approaches, highlighting the superiority of our method.

关键词： Federated learning noise-label learning privacy-preserving machine learning edge intelligence distributed machine learning

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Performance of the Multilayer Film for Infrared Stealth based on VO_(2) Thermochromism

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Journal of Thermal science 2024年第4期33卷 1312-1324页

作者： LI Yaru WANG Fuqiang ZHANG Aoyu FU Zhichang SU Ronghua GAO Tengfei WANG Zhen GUO Jicheng ORDOS Institute of Technology Ordos017000China School of Energy Science and Engineering Harbin Institute of TechnologyHarbin150001China School of New Energy Harbin Institute of Technology at WeihaiWeihai264209China Defense Engineering Institute AMSPLABeijing100850China

With the development of detection and identification technology,infrared stealth is of great value to realize anti-reconnaissance detection of military *** present,infrared stealth materials generally have deficiency,such as complex structure,inconvenient radiation regulation and cumbersome preparation steps,which greatly limit the practical application of infrared stealth *** view of the above deficiency of infrared stealth materials,we proposed a kind of multilayer film for infrared stealth using VO2thermochromism based on the temperature response mechanism of tuna to adjust its color,and through the intelligent reversible radiation regulation mechanism to meet the infrared stealth requirements of tanks in different actual *** results show that when the temperature increases from 300 K to 373 K,the peak emissivity of the film decreases from 94%to 20%in the 8-14μm band after structural optimization,which can realize the infrared stealth of the high temperature target in the 8-14μm *** average emissivity of the multilayer film for infrared stealth at3-5μm and 8-14μm band can be reduced to 34%and 27%at 373 K,and the peak emissivity at 5-8μm band can reach 65%,realizing dual-band infrared stealth in the 3-5μm and 8-14μm bands and heat dissipation in the 5-8μm *** multilayer film for infrared stealth based on VO2thermochromism designed by the authors can meet the characteristics of simple film structure,convenient radiation regulation and simple preparation.

关键词： vanadium dioxide multilayer film infrared stealth thermal management

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The iron-based biochar activating chlorite(ClO_(2)^(−))driven by mechanochemical ultrasonic:piecewise kinetics,biomimetic catalytic-mechanism,and novel advanced redox process

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Frontiers of Environmental science & Engineering 2025年第2期19卷 151-168页

作者： Qihui Xu Qianhui Yang Yuming Xie Lin Hu Zhenghao Fei Hong You School of Chemical and Environmental Engineering Yancheng Teachers UniversityYancheng 224007China State Key Laboratory of Urban Water Resources and Environment Harbin Institute of TechnologyHarbin 150090China School of Marine Science and Technology Harbin Institute of Technology at WeihaiWeihai 264209China

Chlorite(ClO_(2)^(−)or COI)is used to establish the advanced reduction and oxidation process(AROP).The iron/biochar-based particles(iron-based hydrothermal carbon with hinge-like structure,FebHCs,20 mg/L)can be utilized to activate COI(2 mmol/L)to present selective oxidation in removing triphenylmethane derivatives(15 min,90%).The protonation(H+at~102μmol/L level)played a huge role(k-2nd=0.136c-H+−0.014(R^(2)-adj=0.986),and rapp=−0.0876/c-H++1.017(R^(2)-adj=0.996))to boost the generation of the active species(e.g.,high-valent iron oxidizing species(HVI=O)and chlorine dioxide(ClO_(2))).The protonation-coupled electron transfer promoted Fe-substances in Feb/HCs activating COI(the calculated kobs ranging from 0.066−0.285 min^(−1)).The form of ClO_(2) mainly attributed to proton-coupled electron transfer(1e/1H+).The HVI=O was generated from the electron transfer within the coordination ***,carbon particles in FebHCs serve as the bridge for electron *** above roles contribute to the fracture and formation of coordination-induced bonds between Lx-FeII/III and ClO_(2)^(−)at phase interface to form *** ultrasonic(US)cavitation enhanced the mass transfer of active species in bulk solution,and the HVI=O and ClO_(2) attack unsaturated central carbon atoms of triphenylmethane derivatives to initiate selective ***,the scale-up experiment with continuous flow(k values of approximately 0.2 min^(−1),COD removal efficiency of approximately 80%)and the reactor with COMSOL simulation have also proved the applicability of the *** study offers a novel AROP and new insights into correspondingly heterogeneous interface activation mechanisms.

关键词： Chlorite Iron-based biochar Ultrasonic Chlorine dioxide High-valent iron oxidizing species

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Flow excitation mechanisms of unbalanced impeller forces after pump power-trip of ultra-high head pump-turbines

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science China(Technological sciences) 2024年第5期67卷 1602-1611页

作者： FU XiaoLong LI DeYou LV JingWei YANG Biao WANG HongJie WEI XianZhu School of Energy Science and Engineering Harbin Institute of TechnologyHarbin150001China State Key Laboratory of Hydro-Power Equipment Harbin Institute of Large Electrical MachineryHarbin150040China

To elucidate the dynamic mechanisms of unbalanced impellers in ultra-high head pump-turbines(PTs),this study employed a one-and three-dimensional coupled method to simulate the pump power-trip(PPT)process of an ultra-high head *** investigation revealed two novel pulsation frequency components,denoted as fDVand fINFT,associated with impeller *** pulsation intensities of these components were markedly higher than those of rotor-stator interaction frequency components in ultra-high head ***,the fDVcomponents exhibited pulsations at 1–2 times the rated rotation frequency of the impeller,spanning the entire transition ***,the fINFTcomponents constituted a complex frequency band with various frequency values,primarily occurring near conditions(Q=0,n=0,M=0,and d M/dt=0).These two pulsation frequency components were predominantly linked to the unsteady evolution of dean vortices inside the volute and complex transitions of the flow pattern within the impeller,*** is crucial to note that these unbalanced flow-induced impeller axial forces can elevate the risk of accidents where the rotor is subjected to significant upwind axial *** findings offer valuable insights into mitigating the risk of rotor lifting due to axial forces during PT events in ultra-high head PTs.

关键词： ultra-high head pump-turbine pump power-trip unbalanced impeller forces pressure pulsations flow pattern transitions

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Improvement strategy on thermophysical properties of A_(2)B_(2)O_(7)-type rare earth zirconates for thermal barrier coatings applications:A review

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International Journal of Minerals,Metallurgy and Materials 2024年第5期31卷 1147-1165页

作者： Zijian Peng Yuhao Wang Shuqi Wang Junteng Yao Qingyuan Zhao Enyu Xie Guoliang Chen Zhigang Wang Zhanguo Liu Yaming Wang Jiahu Ouyang School of Materials Science and Engineering Harbin Institute of TechnologyHarbin 150001China School of Materials and Metallurgical Engineering Inner Mongolia University of Science&TechnologyBaotou 014010China

The A_(2)B_(2)O_(7)-type rare earth zirconate compounds have been considered as promising candidates for thermal barrier coating(TBC) materials because of their low sintering rate,improved phase stability,and reduced thermal conductivity in contrast with the currently used yttria-partially stabilized zirconia (YSZ) in high operating temperature *** review summarizes the recent progress on rare earth zirconates for TBCs that insulate high-temperature gas from hot-section components in gas *** on the first principles,molecular dynamics,and new data-driven calculation approaches,doping and high-entropy strategies have now been adopted in advanced TBC materials *** this paper,the solid-state heat transfer mechanism of TBCs is explained from two aspects,including heat conduction over the full operating temperature range and thermal radiation at medium and high *** paper also provides new insights into design considerations of adaptive TBC materials,and the challenges and potential breakthroughs are further highlighted for extreme environmental *** for improving thermophysical performance are proposed in two approaches:defect engineering and material compositing.

关键词： rare earth zirconates thermal barrier coatings defect engineering doping and compositing thermal conductivity thermal expansion

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Image Enhancement via Associated Perturbation Removal and Texture Reconstruction Learning

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IEEE/CAA Journal of Automatica Sinica 2024年第11期11卷 2253-2269页

作者： Kui Jiang Ruoxi Wang Yi Xiao Junjun Jiang Xin Xu Tao Lu IEEE the School of Computer Science and Technology Harbin Institute of Technology Zhengzhou Research Institute Harbin Institute of Technology the School of Artificial Intelligence Jianghan University the School of Geodesy and Geomatics Wuhan University the Hubei Province Key Laboratory of Intelligent Information Processing and Real-Time Industrial System Wuhan University of Science and Technology the School of Computer Science and Engineering and also with the Hubei Province Key Laboratory of Intelligent Robot Wuhan Institute of Technology

Degradation under challenging conditions such as rain, haze, and low light not only diminishes content visibility, but also results in additional degradation side effects, including detail occlusion and color distortion. However, current technologies have barely explored the correlation between perturbation removal and background restoration, consequently struggling to generate high-naturalness content in challenging scenarios. In this paper, we rethink the image enhancement task from the perspective of joint optimization: Perturbation removal and texture reconstruction. To this end, we advise an efficient yet effective image enhancement model, termed the perturbation-guided texture reconstruction network(PerTeRNet). It contains two subnetworks designed for the perturbation elimination and texture reconstruction tasks, respectively. To facilitate texture recovery,we develop a novel perturbation-guided texture enhancement module(PerTEM) to connect these two tasks, where informative background features are extracted from the input with the guidance of predicted perturbation priors. To alleviate the learning burden and computational cost, we suggest performing perturbation removal in a sub-space and exploiting super-resolution to infer high-frequency background details. Our PerTeRNet has demonstrated significant superiority over typical methods in both quantitative and qualitative measures, as evidenced by extensive experimental results on popular image enhancement and joint detection tasks. The source code is available at https://***/kuijiang94/PerTeRNet.

关键词： Association learning attention mechanism image enhancement perturbation modeling

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Electronic structure regulation of Fe-doped Ni2P nanocrystals towards durable electrocatalytic oxygen evolution

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Rare Metals 2024年第12期43卷 6405-6415页

作者： Ya Liu Xing Cao Jia-Jia Liu Mei-Sheng Han Gao-Wei Zhang Yu-Bin Zhao Huan-Hui Chen Liang Yu Jun-Rong Zeng Zhi-Kai Cheng Liu-Biao Zhong Li-Juan Song Ye-Jun Qiu Shenzhen Engineering Lab of Flexible Transparent Conductive Films School of Materials Science and EngineeringHarbin Institute of TechnologyShenzhen518055China School of Physics Harbin Institute of TechnologyHarbin150001China Department of Mechanical and Energy Engineering Southern University of Science and TechnologyShenzhen518055China School of Science Harbin Institute of TechnologyShenzhen 518055China Guangdong Provincial Key Laboratory of Semiconductor Optoelectronic Materials and Intelligent Photonic Systems Harbin Institute of TechnologyShenzhen518055China

The inherent electrocatalytic potential of transition metal phosphides(TMPs)for oxygen evolution is influenced by the reduced efficiency of electron transfer resulting from the interaction between electronegative phosphorus atoms and transition ***,we introduce Fe into Ni_(2)P nanocrystals by thermal injection synthesis method,and anchor them on nickel foam(NF)by facile spraying to prepare self-supporting oxygen evolution reaction(OER)***,the optimized electrode of Ni_(2)P-Fe-2/NF demonstrates low overpotentials of 212 mV with 10 mA·cm^(-2)and a 0.9%decay within300 h test of 50 mA·cm^(-2).Notably,when electrode size was expanded to 600 cm^(2)and applied to a larger electrolyzer,its 9 h decay rate at 6 A current was only 1.69%.Characterization results show that Fe doped NiOOH is generated during OER reaction as actual catalyst,Results from density functional theory(DFT)computations suggest that Fe doping shifts NiOOH d-band center to Fermi level,lowering critical *OOH intermediates formation energy barrier during the OER *** findings inform the large-scale industrial application of TMPs as robust electrocatalysts.

关键词： Electronic structure regulation Fe doping Colloidal nanocrystals Ni2P Oxygen evolution reaction

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Content-Aware Dynamic In-loop Filter with Adjustable Complexity for VVC Intra Coding

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IEEE Transactions on Circuits and Systems for Video technology 2025年第6期35卷 6114-6128页

作者： Man, Hengyu Wang, Hao Lu, Riyu Wan, Zhaolin Fan, Xiaopeng Zhao, Debin Harbin Institute of Technology Department of Computer Science and Technology Harbin150001 China City University of Hong Kong Department of Computer Science 999077 Hong Kong

Recently, neural network-based in-loop filters have been rapidly developed, effectively improving the reconstruction quality and compression efficiency in video coding. Existing deep in-loop filters typically employed networks with fixed structures to process all image blocks. However, under various bitrate conditions, compressed image blocks with different textures exhibit varying degradations, which poses a challenge for high-quality and low-complexity filtering. Additionally, different complexity requirements for coding tools in various scenarios limit the versatility of fixed models. To address these problems, a content-aware dynamic in-loop filter (dubbed DILF) with adjustable complexity is proposed in this paper. Specifically, DILF comprises a policy network and a filtering network. For each reconstructed image block, the policy network dynamically generates a filtering network topology based on pixel information and the quantization parameter (QP), guiding the filtering network to skip redundant layers and conduct content-aware image enhancement, thereby improving the filtering performance. In addition, by introducing a user-defined balancing factor into the policy network, the content-aware filtering network topology can be further adjusted according to user's requirements, facilitating adjustable complexity with a single model. We integrate DILF into Versatile Video Coding (VVC) to replace the built-in deblocking filter. Extensive experiments demonstrate the efficiency of DILF in processing image blocks with varying degrees of degradation and its flexibility in controlling complexity. When the balancing factor is set to 2e-5, DILF achieves bitrate savings of 8.07%, 17.97%, and 20.93% on average for YUV components over VVC reference software VTM-11.0 under all-intra configuration. Compared to static networks with fixed structures, DILF demonstrates superior performance and lower computational complexity. © 1991-2012 IEEE.

关键词： Image coding

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