The existence of alkali metals in fl ue gases originating from stationary sources can result in catalyst deactivation in the low-temperature selective catalytic reduction(SCR)of nitrogen oxides(NO_(x)).It is widely ac...
详细信息
The existence of alkali metals in fl ue gases originating from stationary sources can result in catalyst deactivation in the low-temperature selective catalytic reduction(SCR)of nitrogen oxides(NO_(x)).It is widely accepted that alkali metal poisoning causes damage to the acidic sites of ***,in this study,a series of CoMn catalysts doped with heteropolyacids(HPAs)were prepared using the coprecipitation *** these,CoMnHPMo exhibited superior catalytic performance for SCR and over 95%NO_(x) conversion at 150-300.Moreover,it exhibited excellent catalytic activity and stability after alkali poisoning,demonstrating outstanding alkali metal *** characterization indicated that HPMo increased the specifi c surface area of the catalyst,which provided abundant adsorption sites for NO_(x) and NH_(3).Comparing catalysts before and after poisoning,CoMnHPMo enhanced its alkali metal resistance by sacrifi cing Brønsted acid sites to protect its Lewis acid *** situ DRIFTS was used to study the reaction pathways of the *** results showed that CoMnHPMo maintained high NH_(3) adsorption capacity after K poisoning and then reacted rapidly with NO intermediates to ensure that the active sites were not ***,SCR performance was ensured even after alkali metal *** sum-mary,this research proposed a simple method for the design of an alkali-resistant NH_(3)-SCR catalyst with high activity at low temperatures.
Traumatic wounds are the prevalent scenarios encountered in battleground and emergency rooms. The rapid and effective hemostasis is imperative for life saving in these scenarios, for which the development of high-effi...
详细信息
Traumatic wounds are the prevalent scenarios encountered in battleground and emergency rooms. The rapid and effective hemostasis is imperative for life saving in these scenarios, for which the development of high-efficiency and biocompatible hemostatic materials is essential. Due to its excellent hemostatic property and biocompatibility,collagen has emerged as an ideal component of hemostatic materials. Furthermore, the properties of collagen-based hemostatic materials could be improved by the integration of other biomacromolecules, such as alginate, cellulose derivatives, and chitosan derivatives. Therefore, more and more novel hemostatic materials with exceptional hemostatic properties have been developed. This review aims to overview recent progress of collagen-based hemostatic materials. Firstly, the hemostatic mechanism of collagen was introduced. Secondly, various forms of collagen-based hemostatic materials, such as hydrogels, sponges, and powders, were highlighted. Thirdly, composite hemostatic materials of collagen and other biomacromolecules were overviewed. Finally, the outlook of collagen-based hemostatic materials was discussed.
Cable accessory insulation system is inevitably affected by its interface states causing insulation failure. Insulating oils are often applied in the interface with a certain pressure to improve its performance, but t...
详细信息
A thorough analysis of the framework structure of the YOLO algorithm is conducted, and based on the YOLOv5 algorithm, rapid detection and classification of extracted features are implemented. Addressing the issue of m...
详细信息
Coal washing and sorting plays a vital role for coal production. Reasonable scheduling of washing and sorting equipment, crushers and various coal silos in the coal washing and sorting process can effectively increase...
详细信息
This paper investigates the event-triggered H∞ filtering problem for interval type-2 fuzzy networked control systems with data loss. The goal of this paper is to design an event-triggered fuzzy filter with adjustable...
详细信息
With the extensive penetration of distributed renewable energy and self-interested prosumers,the emerging power market tends to enable user autonomy by bottom-up control and distributed *** paper is devoted to solving...
详细信息
With the extensive penetration of distributed renewable energy and self-interested prosumers,the emerging power market tends to enable user autonomy by bottom-up control and distributed *** paper is devoted to solving the specific problems of distributed energy management and autonomous bidding and peer-to-peer(P2P)energy sharing among prosumers.A novel cloud-edge-based We-Market is presented,where the prosumers,as edge nodes with independent control,balance the electricity cost and thermal comfort by formulating a dynamic household energy management system(HEMS).Meanwhile,the autonomous bidding is initiated by prosumers via the modified Stone-Geary utility *** the cloud center,a distributed convergence bidding(CB)algorithm based on consistency criterion is developed,which promotes faster and fairer bidding through the interactive iteration with the edge ***,the proposed scheme is built on top of the commercial cloud platform with sufficiently secure and scalable computing *** results show the effectiveness and practicability of the proposed We-Market,which achieves 15%cost reduction with shorter running *** analysis indicates better scalability,which is more suitable for largerscale We-Market implementation.
In this paper,a two-step control method is proposed,leveraging the generalized Halanay inequality and existing finite-time stability theorems,to achieve finite-time synchronization for a class of neural networks with ...
In this paper,a two-step control method is proposed,leveraging the generalized Halanay inequality and existing finite-time stability theorems,to achieve finite-time synchronization for a class of neural networks with bounded time-varying *** the first step,the system state is attenuated from V (t0) to γV (t0) using the generalized Halanay inequality,where0<γ 1 is a free *** the second step,by applying existing finite-time stability theorems,the system state further decays from γV (t0) to *** on the above ideas,two novel finite-time stability lemmas for the error system are presented,and the convergence rate as well as the settling time is ***,the value of γ that results in the shortest settling time for the error system is also *** the help of the derived lemmas,several sufficient algebraic criteria are established to achieve finite-time synchronization between the considered delayed neural *** results of this paper not only improve the existing two-step control method but also overcome the limitations of certain one-step finite-time control ***,the validity and practical applicability of the obtained theoretical results are demonstrated through two numerical examples and an image protection experiment.
Though there are numerous intrinsic merits of metal-organic frameworks(MOFs),low charge separation efficiency has imposed heavy restrictions on their photocatalytic ***,in situ porphyrin ligand substitution,as a strat...
详细信息
Though there are numerous intrinsic merits of metal-organic frameworks(MOFs),low charge separation efficiency has imposed heavy restrictions on their photocatalytic ***,in situ porphyrin ligand substitution,as a strategy for improving the charge separation efficiency and increasing the amounts of active sites,has been designed and realized in a Hf-biphenyl dicarboxylic acid(BPDC)***,a size and geometry matched meso-tetra(4-carboxyphenyl)porphyrin(TCPP)ligand was selected and doped into Hf-BPDC MOF by forming coordinating bonds with Hf centers,forming dualligand Hf-BPDC-TCPP *** resultant Hf-BPDC-TCPP MOF showed significantly improved activity and chemical stability in the photocatalytic H_(2)generation(261μmol·g^(-1)·h^(-1))and tetracycline(TC)degradation reactions(95.8%),which was 48 and 1.47 folds higher than that of the Hf-BPDC *** and electrochemical studies revealed that the introduction of porphyrin ligand could generate a stronger internal electric field for boosting the charge separation and transfer,increase the specific surface area for providing more active sites,and narrow the band gap to enhance the visible light *** in situ ligand substitution method provides a promising approach to build a tunable platform for constructing high-performance MOF photocatalysts.
Anaerobic digestion has been defined as a competitive approach to facilitate the recycling of corn ***,few studies have focused on the role of direct interspecies electron transfer(DIET)pathway in the acidification st...
详细信息
Anaerobic digestion has been defined as a competitive approach to facilitate the recycling of corn ***,few studies have focused on the role of direct interspecies electron transfer(DIET)pathway in the acidification stage under the addition of different particle sizes of zero-valent iron(ZVI).In this study,three types of ZVI,namely iron filings,iron powder and nanoscale iron,were investigated,respectively,to enhance its high-value *** in volatile fatty acids(VFAs)and methane(CH4)production associated with the underlyingmechanisms were emphatically *** indicated that the addition of ZVI could increase the concentration of VFAs,with the most outstanding performance observed with the use of nanoscale ***,the conversion of propionic acid to acetic acid was driven by adding ZVI with no between-group differences in acidizing ***,the substrate was more fully utilized when supplied with iron powder compared with other groups in methanogenic phase,thereby displaying the maximumCH4 yield with a value of 263.1 mL/(g total solids(TS)).However,adding nanoscale iron could signally shorten the digestion time(T80),saving 7 days in comparison to the group of iron powder.
暂无评论