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Dendritic mesoporous silica nanoparticles for enzyme immobilization

Green Chemical engineering 2024年第2期5卷 173-186页

作者： Shuling Zhang Jing Bai Weixi Kong Haolei Song Yunting Liu Guanhua Liu Li Ma Liya Zhou Yanjun Jiang School of Chemical Engineering and Technology Hebei University of TechnologyTianjin300130China College of Food Science and Biology Hebei University of Science&TechnologyShijiazhuang050018China Hebei Yanuo Bioscience Co. Ltd.Shijiazhuang052165China

Dendritic mesoporous silica nanoparticles(DMSNs)are a new class of solid porous materials used for enzyme immobilization support due to their intrinsic characteristics,including their unique open central-radial structures with large pore channels and their excellent *** this review,we review the recent progress in research on enzyme immobilization using DMSNs with different structures,namely,flower-like DMSNs and tree-branch-like *** DMSN synthesis methods are briefly compared,and the distinct characteristics of the two DMSN types and their effects on the catalytic performance of immobilized enzymes are comprehensively *** directions for future research on enzyme immobilization using DMSNs are also proposed.

关键词： Dendritic mesoporous silica nanoparticles Enzyme immobilization Flower-like Tree-branch-like Central-radial structure

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Stabilization controller of An Extended Chained Nonholonomic System With Disturbance:An FAS Approach

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IEEE/CAA Journal of Automatica Sinica 2024年第5期11卷 1262-1273页

作者： Zhongcai Zhang Guangren Duan School of Engineering Qufu Normal UniversityRizhao 276826China Center for Control Science and Technology Southern University of Science and TechnologyShenzhen 518055 Center for Control Theory and Guidance Technology Harbin Institute of TechnologyHarbin 150001China

This study examines the stabilization issue of extended chained nonholonomic systems(ECNSs)with external *** the existing approaches,we transform the considered system into a fully actuated system(FAS)model,simplifying the stabilizing controller *** implement a separate controller design and propose exponential stabilization controller and finite-time stabilization controller under finite-time disturbance observer(FTDO)for the two system *** addition,we discuss the specifics of global stabilization control *** approach demonstrates that two system states exponentially or asymptotically converge to zero under the provided switching stabilization control strategy,while all other system states converge to zero within a finite time.

关键词： design stabilization system

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Numerical investigation of transient gas–solid heat transfer in a packed bed:Impact of intra-particle thermal diffusion

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Particuology 2024年第7期90卷 404-411页

作者： Hanqiao Che Yuanhe Yue Zhaohua Jiang Duan Li School of Mechanical Engineering Guangxi UniversityNanningGuangxi530004China School of Chemical Engineering University of BirminghamBirminghamB152TTUK Hebei Engineering Research Center of Advanced Energy Storage Technology and Equipment School of Energy and Environmental EngineeringHebei University of TechnologyTianjin300401China Hebei Key Laboratory of Thermal Science and Energy Clean Utilization School of Energy and Environmental EngineeringHebei University of TechnologyTianjin300401China School of Mechatronics and Vehicle Engineering Chongqing Jiaotong UniversityChongqing400074China School of Instrumentation and Opto-Electronic Engineering Beihang UniversityBeijing 100191China

The transient heat transfer behaviours in a packed bed have been studied using coupled computational fluid dynamics(CFD)and discrete element method(DEM).Intra-particle thermal diffusion,which is a crucial but rarely explored issue,is considered by introducing a one-dimensional diffusion equation in the DEM *** achieve a sufficiently long physical time of simulations,we further reduce the computational cost by applying periodic boundary condition to a small segment of the packed *** study demonstrates a shifting peak heat flow rate from the bottom to the top of the packed bed during the initial warming *** affirm that the influence of thermal diffusion within a particle is noteworthy only for particles exhibiting a high Biot number(e.g.,Bi=1.2).This insight enriches our understanding of heat transfer mechanisms in packed beds and their practical engineering applications.

关键词： Packed bed Intra-particle heat transfer CFD–DEM

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Hierarchical controller Synthesis Under Linear Temporal Logic Specifications Using Dynamic Quantization

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IEEE/CAA Journal of Automatica Sinica 2024年第10期11卷 2082-2098页

作者： Wei Ren Zhuo-Rui Pan Weiguo Xia Xi-Ming Sun the Key Laboratory of Intelligent Control and Optimization for Industrial Equipment of Ministry of Education Dalian University of Technology the School of Control Science and Engineering Dalian University of TechnologyDalian 116024China

Linear temporal logic(LTL)is an intuitive and expressive language to specify complex control tasks,and how to design an efficient control strategy for LTL specification is still a *** this paper,we implement the dynamic quantization technique to propose a novel hierarchical control strategy for nonlinear control systems under LTL *** on the regions of interest involved in the LTL formula,an accepting path is derived first to provide a high-level solution for the controller synthesis ***,we develop a dynamic quantization based approach to verify the realization of the accepting *** realization verification results in the necessity of the controller design and a sequence of quantization regions for the controller ***,the techniques of dynamic quantization and abstraction-based control are combined together to establish the local-to-global control *** abstraction construction and controller design are local and dynamic,thereby resulting in the potential reduction of the computational *** each quantization region can be considered locally and individually,the proposed hierarchical mechanism is more efficient and can solve much larger problems than many existing ***,the proposed control strategy is illustrated via two examples from the path planning and tracking problems of mobile robots.

关键词： Abstraction-based control design dynamic quantization formal methods linear temporal logic(LTL)

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Amorphous high-entropy phosphoxides for efficient overall alkaline water/seawater splitting

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Journal of Materials science & technology 2024年第6期173卷 1-10页

作者： Han-Ming Zhang Lihao Zuo Yuhang Gao Junxia Guo Caizhen Zhu Jian Xu Jinfeng Sun School of Materials Science and Engineering Hebei University of Science and TechnologyShijiazhuangHebei 050018China Hebei Key Laboratory of Flexible Functional Materials ShijiazhuangHebei 0500180China Institute of Low-dimensional Materials Genome Initiative College of Chemistry and Environmental EngineeringShenzhen UniversityShenzhenGuangdong 518060China

Designing and synthesizing cost-effective bifunctional catalysts for overall alkaline water/seawater splitting is still a huge challenge for hydrogen ***,Co/Ni/Fe/Mn based-amorphous high-entropy phosphoxide self-standing electrode(CNFMPO)is synthesized by the facile and fast electrodeposition *** exhibits excellent bifunctional electrocatalytic performances on alkaline water/seawater *** hydrogen evolution reaction(HER)and oxygen evolution reaction(OER)overpotentials of CNFMPO in alkaline water/seawater are as low as 43/73 and 252/282 mV to reach a current density of 10 mA cm^(-2),***,two-electrode electrolyzers with CNFMPO||CNFMPO successfully achieve the current density of 10 mA cm^(-2) at low voltages of 1.54 and 1.56 V for overall alkaline water/seawater splitting,*** exhibits satisfactory long-term stability on overall alkaline water/seawater splitting for the surface reconstruction into active metal hydroxide/(oxy)hydroxide,phosphite,and ***,no hypochlorite is detected during seawater electrolysis for the beneficial chlorite oxidation inhibition of the reconstructed phosphite and *** excellent catalytic performances of CNFMPO are due to the unique amorphous structure,multi-component synergistic effect,beneficial electronic structure modulation,and surface reconstruction during the catalytic reaction ***,CNFMPO has shown potential promotion to the development of the water/seawater splitting industry as a promising substituent for noble-metal *** work provides new insights into the design of efficient bifunctional catalysts for overall water/seawater splitting.

关键词： Amorphous high-entropy phosphoxides Water/seawater splitting Synergistic effect Surface reconstruction Electronic structure modulation Inhibition of chloride oxidation reaction

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In situ regulating intimately connected heterostructure by decomposition of solid solution oxides toward high-efficient water oxidation

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Rare Metals 2024年第4期43卷 1557-1569页

作者： Shao-Fei Zhang Xiao-Lu Yin Jin Wang Jian-Li Kang Tian-Tian Li Jin-Feng Sun Yong-Qiang Meng Jian-Jiang Wang Dian-Long Wang Kai-Qiang Qin Hebei Key Laboratory of Flexible Functional Materials/Hebei Key Laboratory of Material Near-Net Forming Technology School of Materials Science and EngineeringHebei University of Science and TechnologyShijiazhuang050018China Key Laboratory of Advanced Ceramics and Machining Technology/Ministry of Education School of Materials Science and EngineeringTianjin UniversityTianjin300072China Electrochemical Engine Center Department of Mechanical EngineeringPennsylvania State UniversityUniversity ParkPA16802USA

Heterogeneous interfaces produced by interdomain interactions on a nanoscale performs a crucial role in boosting the properties of an electrocatalyst toward oxygen evolution reaction(OER)***,a series of dual-phase electrodes with intimately connected heterointerfaces are prepared by in situ decomposing solid solution oxide of Ni_(x)Co_(y)Fe_(100-x-y)O,which grew on Ni foam massively via an ultrafast combustion ***,with high-reaction kinetics caused by the reduction treatment at 450℃,the less electronegative Fe and Co are more oxyphilic than Ni,which facilitated their co-exsolution and formation of CoFe_2O_4/NiO oxide with enriched oxygen *** from the nanoporous framework,heterojunction structure,and oxygen defects,the self-supporting electrodes present rapid charge/mass transmission and provide abundant active sites for *** optimized sample(R-SNCF4.5)shows low overpotentials of 226 and 324 mV at 10 and100 mA·cm^(-2),a small Tafel slope(46.7 mV·dec^(-1)),and excellent *** assembled R-SNCF4.5//Pt/C/NF electrolyzer demonstrates continuous electrolysis over 50 h at a current density of 10 mA·cm^(-2),under 1.51 *** functional theory(DFT)calculations verify that the strong electronic modulation plays a critical part in the CoFe_2O_4/NiO hybrid by lowering the energy barriers for the ratedetermining steps,and Fe sites are the most active OER sites.

关键词： Rapid combustion Decomposition of solid solution oxide Dual-phase heterostructure Oxygen evolution reaction Theoretical calculation

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Model Based Quadriceps Activation Strategy in Squat Training with Exhaustion Method Under Different Loads 8

Model Based Quadriceps Activation Strategy in Squat Training...

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8th International Symposium on Computer science and Intelligent control, ISCSIC 2024

作者： Xie, Cong Guo, Xin Qie, Botao Hebei University of Technology Control Engineering Technology Innovation Center of Hebei Province Hebei University of Technology School of Artificial Intelligence and Data Science Tianjin China

ISBN: (纸本)9798350380286

The aim of this study is to explore the muscle activation strategy of quadriceps muscle training in untrained sedentary people under different resistance training to exhaustion to provide control target for body state-based intelligence exercise equipment. Ten daily sedentary men with no training experience performed three sets of heavy load squats (single leg bench squat) in exhaustion mode (4RM) and one set of lower resistance squats (double leg squat with 10 KG garment) in exhaustion mode (18-26RM) to explore which and when the muscle fibers will be recruited as much as more. EMG signals from the dominant side of the vastus medialis), rectus femoris, and vastus lateralis in both squats were recorded, and the maximum RMS of 500 MS length in each movement was normalized to the maximum voluntary isometric contraction. Reliability analysis of the normalized EMG signal for each muscle between the three groups of heavy-load squats was as follows: Alpha (vastus medialis)= 0.885, Alpha (rectus femoris)=0.903, Alpha (vastus lateralis) = 0.925. Paired samples t-test of the three muscles under different resistance:p (vastus medialis) © 2024 IEEE.

关键词： Exercise equipment

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Impact of asymptomatic infected individuals on epidemic transmission dynamics in multiplex networks with partial coupling

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Chinese Physics B 2024年第10期33卷 80-87页

作者： Xin Hu Jiaxing Chen Chengyi Xia School of Control Science and Engineering Tiangong UniversityTianjin 300387China School of Computer Science and Engineering Tianjin University of TechnologyTianjin 300384China School of Artificial Intelligence Tiangong UniversityTianjin 300387China

The theory of network science has attracted great interest of many researchers in the realm of biomathematics and public health,and numerous valuable epidemic models have been *** previous studies,it is common to set up a one-to-one correspondence between the nodes of a multi-layer network,ignoring the more complex situations in *** the present work,we explore this situation by setting up a partially coupled model of a two-layer network and investigating the impact of asymptomatic infected individuals on *** propose a self-discovery mechanism for asymptomatic infected individuals,taking into account situations such as nucleic acid testing in the community and individuals performing self-antigen testing during the *** these factors together,through the microscopic Markov chain approach(MMCA)and extensive Monte Carlo(MC)numerical simulations,we find that the greater the coupling between the networks,the more information dissemination is *** order to control the epidemics,more asymptomatic infected individuals should be made aware of their *** adoption of nucleic acid testing and individual adoption of antigenic self-testing can help to contain epidemic ***,the epidemic threshold of the proposed model is derived,and then miscellaneous factors affecting the epidemic threshold are also *** results are conducive to devising the prevention and control policies of pandemics.

关键词： asymptomatic infected individuals multi-layer networks partial interdependence

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Hybrid tri-memristor hyperchaotic map and application in Wasserstein Generative Adversarial Nets

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science China(Technological sciences) 2024年第6期67卷 1855-1865页

作者： GU Yang BAO Han YU XiHong HUA ZhongYun BAO BoCheng XU Quan School of Microelectronics and Control Engineering Changzhou UniversityChangzhou213159China School of Computer Science and Technology Harbin Institute of TechnologyShenzhen518055China

Inspired by basic circuit connection methods,memristors can also be utilized in the construction of complex discrete chaotic *** investigate the dynamical effects of hybrid memristors,we propose two hybrid tri-memristor hyperchaotic(HTMH)mapping structures based on the hybrid parallel/cascade and cascade/parallel operations,*** the HTMH mapping structure with hybrid parallel/cascade operation as an example,this map possesses a spatial invariant set whose stability is closely related to the initial states of the *** distributions and bifurcation behaviours dependent on the control parameters are explored with numerical ***,the memristor initial offset-boosting mechanism is theoretically demonstrated,and memristor initial offset-boosting behaviours are numerically *** results clarify that the HTMH map can exhibit hyperchaotic behaviours and extreme multistability with homogeneous coexisting infinite *** addition,an FPGA hardware platform is fabricated to implement the HTMH map and generate pseudorandom numbers(PRNs)with high ***,the generated PRNs can be applied in Wasserstein generative adversarial nets(WGANs)to enhance training stability and generation capability.

关键词： memristor hybrid tri-memristor map spatial invariant set hyperchaos extreme multistability generative adversarial nets

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A Memory-Guided Anomaly Detection Model with Contrastive Learning for Multivariate Time Series

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Computers, Materials & Continua 2023年第11期77卷 1893-1910页

作者： Wei Zhang Ping He Ting Li Fan Yang Ying Liu School of Electronic and Information Engineering Hebei University of TechnologyTianjin300401China School of Artificial Intelligence Hebei University of TechnologyTianjin300401China School of Computer Science and Engineering University of Electronic Science and Technology of ChinaChengdu611731China

Some reconstruction-based anomaly detection models in multivariate time series have brought impressive performance advancements but suffer from weak generalization ability and a lack of anomaly *** limitations can result in the misjudgment of models,leading to a degradation in overall detection *** paper proposes a novel transformer-like anomaly detection model adopting a contrastive learning module and a memory block(CLME)to overcome the above *** contrastive learning module tailored for time series data can learn the contextual relationships to generate temporal fine-grained *** memory block can record normal patterns of these representations through the utilization of attention-based addressing and reintegration *** two modules together effectively alleviate the problem of ***,this paper introduces a fusion anomaly detection strategy that comprehensively takes into account the residual and feature *** a strategy can enlarge the discrepancies between normal and abnormal data,which is more conducive to anomaly *** proposed CLME model not only efficiently enhances the generalization performance but also improves the ability of anomaly *** validate the efficacy of the proposed approach,extensive experiments are conducted on well-established benchmark datasets,including SWaT,PSM,WADI,and *** results demonstrate outstanding performance,with F1 scores of 90.58%,94.83%,91.58%,and 91.75%,*** findings affirm the superiority of the CLME model over existing stateof-the-art anomaly detection methodologies in terms of its ability to detect anomalies within complex datasets accurately.

关键词： Anomaly detection multivariate time series contrastive learning memory network

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