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Chemical vapor deposition synthesis of intrinsic van der Waals ferroelectric SbSI nanowires

Nano Research 2024年第11期17卷 9756-9763页

作者： Longyi Fu Yang Zhao Dapeng Li Weikang Dong Ping Wang Jijian Liu Denan Kong Lin Jia Yang Yang Meiling Wang Shoujun Zheng Yao Zhou Jiadong Zhou Centre for Quantum Physics Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement (MOE) School of Physics Beijing Institute of Technology Beijing 100081 China School of Instrumentation and Optoelectronic Engineering Beihang University Beijing 100081 China College of Materials Science and Engineering Taiyuan University of Technology Taiyuan 030024 China Advanced Research Institute of Multidisciplinary Science and School of Chemistry and Chemical Engineering Beijing Institute of Technology Beijing 100081 China

Intrinsic ferroelectric materials play a critical role in the development of high-density integrated device. Despite some two-dimensional (2D) ferroelectrics have been reported, the research on one-dimensional (1D) intrinsic ferroelectric materials remains relatively scare since 1D atomic structures limit their van der Waals (vdW) epitaxy growth. Here, we report the synthesis of 1D intrinsic vdW ferroelectric SbSI nanowires via a confined-space chemical vapor deposition. By precisely controlling the partial vapor pressure of I2 and reaction temperature, we can effectively manipulate kinetics and thermodynamics processes, and thus obtain high quality of SbSI nanowires, which is determined by Raman spectroscopy and high-resolution scanning transmission electron microscopy characterizations. The ferroelectricity in SbSI is confirmed by piezo-response force microscopy measurements and the ferroelectric transition temperature of 300 K is demonstrated by second harmonic generation. Moreover, the in-plane polarization switching can be maintained in the thin SbSI nanowires with a thickness of 20 nm. Our prepared 1D vdW ferroelectric SbSI nanowires not only enrich the vdW ferroelectric systems, but also open a new possibility for high-power energy storage nanodevices.

关键词： SbSI chemical vapor deposition one-dimensional(1D) ferroelectricity second harmonic generation thermodynamic and kinetics

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Enhanced N_(2)electroreduction activity of single-atom catalysts:Modulating the linear scaling relationship by coordination engineering and dual-site strategies

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Nano Research 2025年第3期18卷 696-709页

作者： Renyi Li Caimu Wang Jiao Zhang Wei Guo Centre for Quantum Physics Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement(MOE)School of PhysicsBeijing Institute of TechnologyBeijing 100081China Frontiers Science Center for High Energy Material(MOE) Beijing Institute of TechnologyBeijing 100081China

The volcano plot is widely used to elucidate the activity trends among different catalysts,thereby effectively screening and guiding catalyst ***,the inherent linear scaling relationship(LSR)constrains the breakthrough in the activity of catalysts,and the understanding of the activity limit in volcano plot is still *** this work,by employing first-principles calculations and microkinetic modeling,we proposed coordination engineering(CE)and dual-site(DS)strategies to surpass the Sabatier’s limitation of WS_(2)-supported TM(TM@WS_(2))single-atom catalysts(SACs)for electrocatalytic nitrogen reduction reaction(eNRR).We found that the LSR betweenΔG(^(*)N_(2)→^(*)N_(2)H)andΔG(^(*)NH_(2)→^(*)NH_(3))was optimized to be closer to the ideal space of eNRR activity after modulating TM@WS_(2)SACs by these two design *** combining the reaction selectivity trend plot,we picked out N-Os@WS_(2),C-Ir@WS_(2),Fe_(2)@WS_(2),and Ru_(2)@WS_(2)as optimal eNRR catalysts with low limiting potential(UL),and N-Os@WS_(2)SAC(UL:-0.28 V)outperforms the best eNRR catalyst among TM@WS_(2)*** constructing explicit solvent models,we conducted a detailed study on the reaction kinetics of proton transfer over these four *** propose that the activity enhancement in TM@WS_(2)SACs for eNRR can be attributed to the ligand effect and geometric effect brought about by CE and DS strategies,improving the donation-backdonation process of electron transfer between N_(2)and the active *** designed catalyst has certain resistance to demetallization and agglomeration under simulated solvent *** work provides a feasible design strategy for the activity enhancement of SACs and brings a new perspective to deeply understanding the volcano plot in heterogeneous catalysis.

关键词： linear scaling relationship volcano plot single-atom catalysts density functional theory(DFT) electrochemical nitrogen reduction

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Bound state noise-like pulses generation from composite filtering effects

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optoelectronics Letters 2025年第3期21卷 142-148页

作者： CHANG Qingyu ZHANG Caishi College of Physics&Optoelectronic Engineering Jinan UniversityGuangzhou510632China Guangdong-Hong Kong-Macao Joint Laboratory for Intelligent Micro-Nano Optoelectronic Technology School of Physics and Optoelectronic EngineeringMacao University of Science and TechnologyMacao999078China School of Innovation Engineering Macao University of Science and TechnologyMacao999078China

This paper demonstrated the generation of multi-wavelength bound state noise-like pulse(BNLP)in a dispersion-managed composite-filtered fiber laser consisting of nonlinear polarization rotation(NPR)and *** the case of BNLP,the generation is caused by the interaction between two noise-like pulses(NLPs)induced by the comb-filtering effect,and bound state level can be artificially controlled in the *** work provides a new method for generating low-coherence pulses and establishes a research idea for the study of the comb-filtering effects.

关键词： comb filtering effect nonlinear polarization composite filtering dispersion managed fiber laser bound state level low coherence pulses artificially controlled nonlinear polarization rotation

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Novel transmission property of zero-index metamaterial waveguide doped with gain and lossy defects

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Chinese physics B 2023年第10期32卷 531-536页

作者：朱琼干柴立臣路海 Department of Science Taiyuan Institute of TechnologyTaiyuan 030008China Engineering Laboratory for Optoelectronic Technology and Advanced Manufacturing School of PhysicsHenan Normal UniversityXinxiang 453007China

Taking inspiration from quantum parity–time(PT) symmetries that have gained immense popularity in the emerging fields of non-Hermitian optics and photonics, the interest of exploring more generalized gain-loss interactions is never seen down. In this paper we theoretically present new fantastic properties through a zero-index metamaterial(ZIM) waveguide loaded gain and loss defects. For the case of epsilon-and-mu-near-zero(EMNZ) based ZIM medium, electromagnetic(EM)waves are cumulative and the system behaves as an amplifier when the loss cavity coefficient is greater than the gain cavity coefficient. Conversely, when loss is less than gain, EM waves are dissipated and the system behaves as an ***, our investigation is extended to non-Hermitian scenarios characterized by tailored distributions of gain and loss in the epsilon-near-zero(ENZ) host medium. The transport effect in ZIM waveguide is amplified in one mode, while it is dissipative in the other mode, which breaks the common sense and its physic is analyzed by magnetic flux. That is which cavity has the smaller loss/gain coefficient, the larger its magnetic flux, which cavity dominates. This paper is of significant importance in the manipulation of electromagnetic waves and light amplification as well as the enhancement of matter interactions.

关键词： zero-index metamaterial non-Hermitian gain-loss interaction magnetic flux

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Spectra-assisted laser focusing in quantitative analysis of laser-induced breakdown spectroscopy for copper alloys

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Plasma science and technology 2023年第4期25卷 204-209页

作者：李守杰郑荣儿出口祥啓叶旺全田野郭金家李颖卢渊 College of Physics and Optoelectronic Engineering Ocean University of ChinaQingdao 266100People’s Republic of China Graduate School of Advanced Technology and Science Tokushima UniversityTokushima 770-8501Japan

Laser-induced breakdown spectroscopy(LIBS)is a capable technique for elementary analysis,while LIBS quantitation is still under *** quantitation,precise laser focusing plays an important role because it ensures the distance between the laser and *** the present work,we employed spectral intensity as a direct way to assist laser focusing in LIBS quantitation for copper *** is found that both the air emission and the copper line could be used to determine the position of the sample surface by referencing the intensity ***,the fine quantitation was only realized at the position where the air emission(e.g.O(I)777.4 nm)reached intensity maximum,and also in this way,a repeatable quantitation was successfully achieved even after 120 *** results suggested that the LIBS quantitation was highly dependent on the focusing position of the laser,and spectra-assisted focusing could be a simple way to find the identical condition for different samples’*** the future,this method might be applicable in field measurements for LIBS analysis of solids.

关键词： LIBS laser focusing spectra assistance quantitative analysis copper alloys

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Anti-aging performance improvement and enhanced combustion efficiency of boron via the coating of PDA

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Defence technology（防务技术） 2024年第3期33卷 399-410页

作者： Shuai Ma Qinghai Shu Mengyang Zhang Hongyu Huang Yansong Shi Xijuan Lv Shuai Zhao School of Materials Science and Engineering Beijing Institute of TechnologyBeijing100081China Key Lab of Advanced Optoelectronic Quantum Architecture and Measurement(MOE) Beijing Key Lab of Nanophotonics&Ultrafine Optoelectronic SystemsSchool of PhysicsBeijing Institute of TechnologyBeijing100081China Tangshan Research Institute of Beijing Institute of Technology Tangshan063000HebeiChina

Boron is an ambitious fuel in energetic materials since its high heat release values,but its application is prohibited by low combustion efficiency and oxidization during *** polydopamine(PDA)was introduced into boron particles,investigating the impact of PDA content on the energetic behavior of *** results indicated that the PDA coating formed a fishing net structure on the surface of boron *** heat release results showed that the combustion calorific value of B@PDA was higher than that of the raw ***,the actual combustion heat of boron powder in B@10%PDA increased by 38.08%.Meanwhile,the DSC peak temperature decreased by 100.65℃under similar oxidation rate compared to raw ***,the B@PDA@AP and B@AP composites were prepared,and their combustion properties were *** was demonstrated that B@10%PDA@AP exhibited superior performance in terms of peak pressure and burning time,*** peak pressure is 12.43 kPa more than B@AP and burning time is 2.22 times higher than B@***,the coating of PDA effectively inhibits the oxidization of boron during storage and enhances the energetic behavior of boron and corresponding composites.

关键词： Boron particles Polydopamine Anti-aging performance improvement Heat release

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Color-conversion displays:current status and future outlook

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Light(science & Applications) 2024年第12期13卷 2941-2961页

作者： Guijun Li Man-Chun Tseng Yu Chen Fion Sze-Yan Yeung Hangyu He Yuechu Cheng Junhu Cai Enguo Chen Hoi-Sing Kwok Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province College of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen 518060China State Key Laboratory of Advanced Displays and Optoelectronics Technologies Department of Electronic and Computer EngineeringThe Hong Kong University of Science and TechnologyHong KongChina National and Local United Engineering Laboratory of Flat Panel Display Technology College of Physics and Information EngineeringFuzhou UniversityCollege of Physics and Information Engineering 350108FuzhouChina Fujian Science&Technology Innovation Laboratory for Optoelectronic Information of China Fuzhou 350108China

The growing focus on enhancing color quality in liquid crystal displays(LCDs)and organic light-emitting diodes(OLEDs)has spurred significant advancements in color-conversion ***,color conversion is also important for the development and commercialization of *** article provides a comprehensive review of different types of color conversion methods as well as different types of color conversion *** summarize the current status of patterning process,and discuss key strategies to enhance display ***,we speculate on the future prospects and roles that color conversion will play in ultra-high-definition micro-and projection displays.

关键词： materials projection outlook

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Single crystal growth and characterization of 166-type magnetic kagome metals

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Chinese physics B 2024年第9期33卷 145-150页

作者： Huangyu Wu Jinjin Liu Yongkai Li Peng Zhu Liu Yang Fuhong Chen Deng Hu Zhiwei Wang Centre for Quantum Physics Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement(MOE)School of PhysicsBeijing Institute of TechnologyBeijing 100081China Beijing Key Laboratory of Nanophotonics and Ultrafine Optoelectronic Systems Beijing Institute of TechnologyBeijing 100081China Beijing Institute of Technology Zhuhai 519000China Material Science Center Yangtze Delta Region Academy of Beijing Institute of TechnologyJiaxing 314011China

Kagome magnets were predicted to be a good platform to investigate correlated topology band structure,Chern quantum phase,and geometrical frustration due to their unique lattice *** we reported single crystal growth of 166-type kagome magnetic materials,including HfMn_(6)Sn_(6),ZrMn_(6)Sn_(6),GdMn_(6)Sn_(6)and GdV_(6)Sn_(6),by using the flux method with Sn as the *** them,HfMn_(6)Sn_(6)and ZrMn_(6)Sn_(6)single crystals were grown for the first time.X-ray diffraction measurements reveal that all four samples crystallize in HfFe6Ge6-type hexagonal structure with space group P6/*** samples show metallic behavior from temperature dependence of resistivity measurements,and the dominant carrier is hole,except for GdV6Sn6 which is electron *** samples have magnetic order with different transition temperatures,HfMn_(6)Sn_(6),ZrMn_(6)Sn_(6)and GdV_(6)Sn_(6)are antiferromagnetic with TN of 541 K,466 K and 4 K respectively,while GdMn_(6)Sn_(6)is ferrimagnetic with the critical temperature of about 470 *** study will enrich the research platform of magnetic kagome materials and help explore the novel quantum phenomena in these interesting *** dataset of specific crystal structure parameters for HfMn_(6)Sn_(6)are available in science Data Bank,with the link.

关键词： kagome metal single crystal growth crystal structure physical property

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Interlayer Magnetic Interaction in the CrI_(3)/CrSe_(2) Heterostructure

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Chinese physics Letters 2024年第5期41卷 85-89页

作者：王秋皓倪美燕李淑静郑法伟路洪艳张平 School of Physics and Physical Engineering Qufu Normal UniversityQufu 273165China Center for Quantum Physics Key Laboratory of Advanced Optoelectronic Quantum Architecture and MeasurementSchool of PhysicsBeijing Institute of TechnologyBeijing 100081China Beijing Key Lab of Nanophotonics and Ultrafine Optoelectronic Systems School of PhysicsBeijing Institute of TechnologyBeijing 100081China College of Mathematics and Physics Beijing University of Chemical TechnologyBeijing 100029China Institute of Applied Physics and Computational Mathematics Beijing 100088China

Based on first-principles calculations, we systematically study the stacking energy and interlayer magnetic interaction of the heterobilayer composed of CrI_(3) and CrSe_(2) monolayers. It is found that the stacking order plays a crucial role in the interlayer magnetic coupling. Among all possible stacking structures, the AA-stacking is the most stable heterostructure, exhibiting interlayer antiferromagnetic interactions. Interestingly, the interlayer magnetic interaction can be effectively tuned by biaxial strain. A 4.3% compressive strain would result in a ferromagnetic interlayer interaction in all stacking orders. These results reveal the magnetic properties of CrI_(3)/CrSe_(2) heterostructure, which is expected to be applied to spintronic devices.

关键词： strain stacking interlayer

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Disentangling the electron-lattice dichotomy of the excitonic insulating phase in Ta_(2)Ni(Se_(1-x)S_(x))_(5) with sulfur substitution and potassium deposition

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science China(physics,Mechanics & Astronomy) 2024年第12期67卷 119-126页

作者： Tongrui Li Yang Liu Hongen Zhu Haiping Chen Zhanfeng Liu Zhengming Shang Yuliang Li Hui Tian Yunbo Wu Yuhao Hong Haihua Luo Yi Liu Guobin Zhang Lidong Zhang Yuqiao Guo Changzheng Wu Li Song Shengtao Cui Zhe Sun National Synchrotron Radiation Laboratory University of Science and Technology of ChinaHefei230029China School of Chemistry and Materials Science University of Science and Technology of ChinaHefei230026China School of Mechanics and Optoelectronic Physics Anhui University of Science and TechnologyHuainan232001China CAS Key Laboratory of Strongly-coupled Quantum Matter Physics University of Science and Technology of ChinaHefei230026China Collaborative Innovation Center of Advanced Microstructures Nanjing210093China

Ta_(2)NiSe_(5) is a promising candidate for hosting an excitonic insulator(EI)phase,a novel electronic state driven by electron-hole Coulomb ***,the role of electron-lattice coupling in the formation of the EI phase remains ***,we use angle-resolved photoemission spectroscopy(ARPES)to study the band structure evolution of Ta_(2)Ni(Se_(1-x)S_(x))_(5) with sulfur substitution and potassium deposition,which modulate the band gap and the carrier concentration,*** find that the Ta 5d states originating from the bottom of the conduction band persist at the top of the valence band in the low-temperature monoclinic phase,indicating the importance of exciton condensation in opening the gap in the semi-metallic band *** also observe that the characteristic overlap between the conduction and valence bands can be restored in the monoclinic lattice by mild carrier injection,suggesting that the lattice distortion in the monoclinic phase is not the main factor for producing the insulating gap,but rather the exciton condensation in the electronic system is the dominant driving *** results shed light on the electron-lattice decoupling and the origin of the EI phase in Ta_(2)Ni(Se_(1-x)Sx)_(5).

关键词： excitonic insulator angle-resolved photoemission spectroscopy sulfur substitution potassium deposition

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