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Graphene binding on black phosphorus enables high on/off ratios and mobility

National science Review 2024年第2期11卷 188-195页

作者： Fanrong Lin Zhonghan Cao Feiping Xiao Jiawei Liu Jiabin Qiao Minmin Xue Zhili Hu Ying Liu Huan Lu Zhuhua Zhang Jens Martin Qingjun Tong Wanlin Guo Yanpeng Liu Key Laboratory for Intelligent Nano Materials and Devices of Ministry of Education State Key Laboratory of Mechanics and Control of Mechanical Structures and Institute for Frontier Science Nanjing University of Aeronautics and Astronautics Centre for Advanced 2D Materials National University of Singapore School of Physics and Electronics Hunan University Centre for Quantum Physics Key Laboratory of Advanced Optoelectronic Quantum Architecture and MeasurementSchool of PhysicsBeijing Institute of Technology Leibniz Institute für Kristallzüchtung

Graphene is one of the most promising candidates for integrated circuits due to its robustness against short-channel effects, inherent high carrier mobility and desired gapless nature for Ohmic contact, but it is difficult to achieve satisfactory on/off ratios even at the expense of its carrier mobility, limiting its device applications. Here, we present a strategy to realize high back-gate switching ratios in a graphene monolayer with well-maintained high mobility by forming a vertical heterostructure with a black phosphorus multi-layer. By local current annealing, strain is introduced within an established area of the graphene, which forms a reflective interface with the rest of the strain-free area and thus generates a robust off-state via local current depletion. Applying a positive back-gate voltage to the heterostructure can keep the black phosphorus insulating, while a negative back-gate voltage changes the black phosphorus to be conductive because of hole accumulation. Then, a parallel channel is activated within the strain-free graphene area by edge-contacted electrodes, thereby largely inheriting the intrinsic carrier mobility of graphene in the on-state. As a result, the device can provide an on/off voltage ratio of >10～3 as well as a mobility of ～8000 cm2V-1s-1at room temperature, meeting the low-power criterion suggested by the International Roadmap for Devices and Systems.

关键词： graphene on/off ratio mobility black phosphorus reflective interface

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Stepwise colloidal lithography toward scalable and various planar chiral metamaterials

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Rare Metals 2024年第2期43卷 723-735页

作者： Xiu Yang Yong Liu Fei-Liang Chen Qian-Qi Lin Rohit Chikkaraddy Shan-Shan Huang Shi-Lin Xian Yi-Dong Hou Jing-Lei Du Liang-Ping Xia Chun-Lei Du School of Electronic Science and Engineering University of Electronic Science and Technology of ChinaChengdu610054China School of Optoelectronic Science and Engineering University of Electronic Science and Technology of ChinaChengdu610054China Zhuhai Multiscale Optoelectronics Technology Co. Ltd.Zhuhai915060China Hybrid Materials for Opto-Electronics Group Department of Molecules and MaterialsMESA+Institute for NanotechnologyMolecules Center and Center for Brain-Inspired Nano SystemsFaculty of Science and TechnologyUniversity of Twente7500 AEEnschedeThe Netherlands School of Physics and Astronomy University of BirminghamBirminghamB152TTUK College of Physics Sichuan UniversityChengdu610065China Key Laboratory of Micro Nano Optoelectronic Devices and Intelligent Perception Systems Yangtze Normal UniversityChongqing408100China

Chiral metamaterials(CMs)composed by artificial chiral resonators have attracted great attentions in the recent decades due to their strong chiroptical resonance and identifiable interaction with chiral materials,facilitating practical applications in chiral biosensing,chiral emission,and display ***,the complex geometry of CMs improves the fabrication difficulty and hinders their scalable fabrication for practical applications,especially in the visible and ultraviolet *** potential strategy is the colloidal lithography that enables parallel fabrication for scalable and various planar ***,we demonstrate a stepwise colloidal lithography technique that uses sequential deposition from multiple CMs and expand their variety and *** geometry and optical chirality of building blocks from single deposition are systematically investigated,and their combination enables a significant extension of the range of chiral patterns by multiple-step *** approach resulted in a myriad of complex designs with different characteristic sizes,compositions,and shapes,which are particularly beneficial for the development of nanophotonic *** addition,we designed a flexible chiral device based on PDMS,which exhibits a good CD value and excellent stability even after multiple inward and outward *** excellent compatibility to various substrates makes the planar CMs more flexible in practical applications in microfluidic biosensing.

关键词： Chiral metamaterials Colloidal lithography Nanophotonics Metasurfaces Plasmonics Nanofabrications Flexible devices

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Unusual metallic state in superconducting A15-type La4H23

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National science Review 2024年第12期11卷 94-103页

作者： Jianning Guo Dmitrii Semenok Grigoriy Shutov Di Zhou Su Chen Yulong Wang Kexin Zhang Xinyue Wu Sven Luther Toni Helm Xiaoli Huang Tian Cui State Key Laboratory of Superhard Materials College of Physics Jilin University Center for High Pressure Science and Technology Advanced Research (HPSTAR) Department of High-Temperature Superconductivity Skolkovo Institute of Science and Technology Skolkovo Innovation CenterComputational and Data Science and Engineering HochfeldMagnetlabor Dresden(HLD-EMFL) and Würzburg-Dresden Cluster of Excellence Helmholtz-Zentrum Dresden-Rossendorf(HZDR) School of Physical Science and Technology Ningbo University

Hydride superconductors continue to fascinate the communities of condensed matter physics and material scientists because they host the promising near room-temperature superconductivity. Current research has concentrated on the new hydride superconductors with the enhancement of the superconducting transition temperature（Tc）. The multiple extreme conditions（high pressure/temperature and magnetic field） will introduce new insights into hydride superconductors. The study of transport properties under very high magnetic fields facilitates the understanding of superconductivity in conventional hydride *** the present work, we report experimental evidence of an unusual metal state in a newly synthesized cubic A15-type La4H23that exhibits superconductivity with a Tc reaching 105 K at 118 GPa. A large negative magnetoresistance is observed in strong pulsed magnetic fields in the non-superconducting state of this compound below 40 K. Moreover, we construct the full magnetic phase diagram of La4H23up to 68 T at high pressure. The present work reveals anomalous electronic structural properties of A15-La4H23under high magnetic fields, and therefore has great importance with regard to advancing the understanding of quantum transport behaviors in hydride superconductors.

关键词： high-pressure superconductivity hydrides negative magnetoresistance

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Strong anharmonicity-assisted low lattice thermal conductivities and high thermoelectric performance in double-anion Mo_(2)AB_(2)(A=S,Se,Te;B=Cl,Br,I)semiconductors

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Chinese physics B 2023年第10期32卷 600-608页

作者：廖海俊黄乐谢兴董华锋吴福根孙志鹏李京波 School of Materials and Energy Guangdong University of TechnologyGuangzhou 510006China Guangdong Provincial Key Laboratory of Information Photonics Technology Guangdong University of TechnologyGuangzhou 510006China School of Physics and Optoelectronic Engineering Guangdong University of TechnologyGuangzhou 510006China School of Physics and Electronics Hunan Key Laboratory for Super-microstructure and Ultrafast ProcessCentral South UniversityChangsha 410083China College of Optical Science and Engineering Zhejiang UniversityHangzhou 310027China

The thermoelectric properties of layered Mo_(2)AB_(2)(A=S,Se,Te;B=Cl,Br,I)materials are systematically investigated by first-principles *** transverse acoustic modes and direct Mo d–Mo d couplings give rise to strong anharmonicities and low lattice thermal *** double anions with distinctly different electronegativities of Mo_(2)AB_(2)monolayers can reduce the correlation between electron transport and phonon scattering,and further benefit much to their good thermoelectric *** properties of these Mo_(2)AB_(2)monolayers exhibit obvious anisotropies due to the direction-dependent chemical bondings and transport ***,their thermoelectric properties strongly depend on carrier type(n-type or p-type),carrier concentration and *** is found that n-type Mo_(2)AB_(2)monolayers can be excellent thermoelectric materials with high electric conductivity,σ,and figures of merit,*** the types of A and B anions of Mo_(2)AB_(2)is an effective strategy to optimize their thermoelectric *** results provide rigorous understanding on thermoelectric properties of double-anions compounds and important guidance for achieving high thermoelectric performance in multi-anion compounds.

关键词： thermoelectricity anharmonicity lattice thermal conductivity anisotropy first-principles calculations

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Research on the punch-through phenomenon of separate absorption，charge，and multiplication avalanche photodetectors

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Hongwai Yu Haomibo Xuebao/Journal of Infrared and Millimeter Waves 2025年第3期44卷 327-334页

作者： Li, Chong Ma, Zi-Yi Yang, Shuai Liu, Yue-Wen Wang, Jia-Xuan Liu, Yun-Fei Dong, Yu-Sen Li, Zi-Qian Liu, Dian-Bo Key Laboratory of Optoelectronics Technology of Ministry of Education School of Information Science and Technology Beijing University of Technology Beijing100124 China Institute of Advanced Semiconductor Optoelectronic Technology School of Physics and Optoelectronic Engineering Beijing University of Technology Beijing100124 China

In this paper，the punch-through phenomenon was studied，based on a fabricated separate absorption，charge，and multiplication avalanche photodetector（SACM APD）. The spectral response，capacitance characteristics，and I-V characteristics at different operating temperatures of the APD were measured and analyzed. Meanwhile，the device performance before and after the punch-through phenomenon were compared，and the model of the electric field region formed by external voltage was analyzed，based on the measurement results and the simulated electric field and energy band distributions by SILVACO. When the ion implantation energy of the charge layer was 580 KeV，the simulated device had a punch-through voltage of -30V and a capacitance reduction of one-third before punch-through. Then，a Si SACM APD was prepared based on CMOS process. The punch-through voltage of the device was -30V and the capacitance was reduced to 1/3@1MHz before punch-through，which exactly matched the simulation results. Moreover，the photocurrent after punch-through increases to 2. 18 times of the before value at 808 nm. The peak responsivity increases from 0. 171 A/W@590 nm to 0. 377 A/W@820 nm. © 2025 Chinese Optical Society. All rights reserved.

关键词： Capacitance

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Progress and prospects of graphene-based materials in lithium batteries

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Rare Metals 2024年第5期43卷 1886-1905页

作者： Shen Lai Tao Huang Pei Liu Hong-Bin Wang Shi-Chun Yang Xin-Hua Liu Kai Yang Qian-Ling Zhang Jian-Hong Liu Jiang-Tao Hu Graphene Composite Research Center College of Chemistry and Environmental EngineeringShenzhen UniversityShenzhen 518060China College of Physics and Optoelectronic Engineering Shenzhen UniversityShenzhen 518060China Shenzhen Eigen-Equation Graphene Technology Co.Ltd Shenzhen518060China School of Transportation Science and Engineering Beihang UniversityBeijing 100191China Department of Electrical and Electronic Engineering Advanced Technology InstituteUniversity of SurreyGuildfordSurrey GU27XHUK

Reasonable design and applications of graphene-based materials are supposed to be promising ways to tackle many fundamental problems emerging in lithium batteries,including suppression of electrode/electrolyte side reactions,stabilization of electrode architecture,and improvement of conductive ***,extensive fundamental research on this aspect has been performed so ***,when it comes to large-scale industrial applications,the utilization of graphene-based materials progresses at a very slow ***,there presents a severe technological decoupling between academic research and industrial application,and there is an urgent need to link ***,in order to address current issues of graphene-based materials used in lithium batteries,we present their latest advancements with stateof-the-art *** applications of graphenebased materials in practical lithium batteries are highlighted and predicted to bridge the gap between the academic progress and industrial manufacture,thereby paving the way for accelerating the development of graphenebased material as well as lithium battery industry.

关键词： Lithium batteries Graphene-based materials Academic research Industrial application Development direction

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Design of NV color center fluorescence signal acquisition circuit based on FPGA architecture

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optoelectronics Letters 2024年第12期20卷 721-727页

作者： ZENG Sen YANG Shuqiang LIU Jingyan ZHAO Chuang SHANG Zhengguo HE Xianming Key Laboratory of Optoelectronic Technology and Systems Ministry of Education of ChinaChongqing UniversityChongqing 400044China College of Physics and Electronics Information Luoyang Normal UniversityLuoyang 471934China School of Electrical Engineering Chongqing University of Science and TechnologyChongqing 401331China

Nitrogen-vacancy(NV)quantum defects in diamond are sensitive detectors of magnetic *** rapid development of NV-center magnetic sensor has higher requirements for high-speed and high-precision data acquisition,weak signal detection and ***,the existing sensing technologies based on diamond NV centers rely on bulky and expensive instruments,which must be replaced by a more compact *** we combine NV quantum sensing technology with integrated circuit technology to create a compact and easy-to-operate platform,which includes microwave source module,transistor-transistor logic(TTL)modulation module,digital lock-in amplifier(DLIA)module,*** order to confirm the reliability of the experimental platform,we not only tested the performance of each individual module,but also carried out optical detection magnetic resonance(ODMR)*** this platform,we can obtain a magnetic sensitivity of 465 nT/Hz^(1/2).This experimental platform with convenient operation and low noise has the potential to become an independent magnetic measuring instrument.

关键词： center centers fir

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Theoretical investigation on optical properties of Möbius carbon nanobelts in one-and two-photon absorption

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Frontiers of physics 2023年第3期18卷 131-137页

作者： Zhiqiang Yang Yichuan Chen Jing Li Chen Lu Junfang Zhao Mengtao Sun School of Mathematics and Physics Beijing Advanced Innovation Center for Materials Genome EngineeringUniversity of Science and Technology BeijingBeijing 100083China Orient Scientific Software(Beijing)Technology Ltd BeijingChina Key Laboratory of Photochemical Conversion and Optoelectronic Materials Technology Institution Physical and ChemistryChinese Academy of SciencesBeijing 100190China College of Science Liaoning Petrochemical UniversityFushun 113001China

The first successful synthesis of fully fused and fully conjugated Möbius carbon nanobelts(CNBs)has attracted considerable ***,theoretical calculations based on suchπ-conjugated Möbius CNB are still ***,we theoretically investigated molecular spectroscopy of Möbius CNBs without and with n-butoxy groups via visualization *** results show that the presence of n-butoxy groups can significantly affect Möbius CNBs’optical performance,changing electron-hole coherence and enhancing two-photon absorption *** work provides a deeper understanding of photophysical mechanisms of Möbius CNBs in one-and two-photon absorption and reveals possible applications on optoelectronic devices.

关键词： optical properties Möbius carbon nanobelts photon spectroscopy

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Local probing of the non-uniform distribution of ferrielectric and antiferroelectric phases

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Nano Research 2023年第2期16卷 3021-3027页

作者： Huimin Qiao Fangping Zhuo Zhen Liu Jinxing Wang Jeongdae Seo Chenxi Wang Jinho Kang Bin Yang Yunseok Kim School of Advanced Materials and Engineering Sungkyunkwan University(SKKU)Suwon 16419Republic of Korea Research Center for Advanced Materials Technology Sungkyunkwan University(SKKU)Suwon 16419Republic of Korea Department of Materials and Earth Sciences Technical University of DarmstadtDarmstadt 64287Germany Department of Physics College of ScienceNortheast Forestry UniversityHarbin 150040China Department of Physics Korea Advanced Institute of Science and Technology(KAIST)Daejeon 34141Republic of Korea School of Instrumentation Science and Engineering Harbin Institute of TechnologyHarbin 150080China

Piezoresponse force microscopy(PFM)is an indispensable tool in the investigation of local electromechanical responses and polarization *** acquired data provide spatial information on the local disparity of polarization switching and electromechanical responses,making this technique advantageous over macroscopic *** its widespread application in ferroelectrics,it has rarely been used to investigate the ferrielectric(FiE)behaviors in antiferroelectric(AFE)***,the PFM was utilized to study the local electromechanical behavior and distribution of FiE,and the AFE phases of PbZrO_(3)thin-film were studied,where only the FiE behavior is observable using a macroscopic *** FiE region resembles a ferroelectric material at low voltages but exhibits a unique on-field amplitude response at high *** contrast,the AFE region only yields an observable response at high ***-field simulations reveal the coexistence of AFE and FiE states as well as the phase-transition processes that underpin our experimental *** work illustrates the usefulness of PFM as an analytical tool to characterize AFE/FiE materials and their phase-coexistence behavior,thereby providing insights to guide property modification and potential applications.

关键词： scanning probe microscopy ferrielectrics antiferroelectrics local electromechanical response

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In situ photoelectric biosensing based on ultranarrowband near-infrared plasmonic hot electron photodetection

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advanced Photonics 2024年第2期6卷 81-89页

作者： Xianghong Nan Wenduo Lai Jie Peng Haiquan Wang Bojun Chen Huifan He Zekang Mo Zikun Xia Ning Tan Zhong Liu Long Wen Dan Gao Qin Chen Jinan University College of Physics&Optoelectronic EngineeringInstitute of NanophotonicsGuangdong Provincial Key Laboratory of Nanophotonic ManipulationGuangzhouChina Tsinghua University Shenzhen International Graduate SchoolState Key Laboratory of Chemical OncogenomicsShenzhenChina Jinan University College of Life Science and TechnologyGuangzhouChina

Narrowband photodetection is an important measurement technique for material analysis and sensing,for example,nondispersive infrared sensing *** photoactive material engineering and nanophotonic filtering schemes have been explored to realize wavelength-selective photodetection,while most devices have a responsive bandwidth larger than 2%of the operating wavelength,limiting sensing ***-infrared photodetection with a bandwidth of less than 0.2%of the operating wavelength was demonstrated experimentally in Au/Si Schottky nanojunctions.A minimum linewidth of photoelectric response down to 2.6 nm was obtained at a wavelength of 1550 nm by carefully tailing the absorptive and radiative loss in the *** functions were achieved on chip with the corrugated Au film,including narrowband resonance,light harvesting for sensing and photodetection,and electrodes for hot electron *** from such a unity integration with in situ photoelectric conversion of the optical sensing signal and the ultranarrowband resonance,self-contained on-chip biosensing via simple intensity interrogation was demonstrated with a limit of detection down to 0.0047%in concentration for glucose solution and 150 ng∕m L for rabbit *** potential of this technique is expected for the applications in on-site sensing,spectroscopy,spectral imaging,etc.

关键词： plasmonics hot electron sensor photodetector spectroscopy

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