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Three-dimensional magnetization reconstruction from electron optical phase images with physical constraints

science China(physics,Mechanics & Astronomy) 2024年第11期67卷 122-132页

作者： Boyao Lyu Shihua Zhao Yibo Zhang Weiwei Wang Fengshan Zheng Rafal E.Dunin-Borkowski Jiadong Zang Haifeng Du Anhui Province Key Laboratory of Low-Energy Quantum Materials and Devices High Magnetic Field LaboratoryHefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China Science Island Branch Graduate School of University of Science and Technology of ChinaHefei 230026China Department of Physics and Astronomy University of New HampshireDurham 03824USA Department of Physics The City College of New YorkNew York 10031USA Physics Program Graduate Center of the City University of New YorkNew York 10016USA Department of Chemistry University of New HampshireDurham 03824USA Institutes of Physical Science and Information Technology Anhui UniversityHefei 230601China Spin-X Institute Center for Electron MicroscopySchool of Physics and OptoelectronicsState Key Laboratory of Luminescent Materials and DevicesGuangdong-Hong Kong-Macao Joint Laboratory of Optoelectronic and Magnetic Functional MaterialsSouth China University of TechnologyGuangzhou 511442China Ernst Ruska-Centre for Microscopy and Spectroscopy with Electrons Forschungszentrum JülichJülich 52425Germany

The ability to characterize three-dimensional(3D)magnetization distributions in nanoscale magnetic materials and devices is essential to fully understand their static and dynamic magnetic *** contrast techniques in the transmission electron microscope(TEM),such as electron holography and electron ptychography,can be used to record two-dimensional(2D)projections of the in-plane magnetic induction of 3D nanoscale *** the 3D magnetic induction can in principle be reconstructed from one or more tilt series of such 2D projections,conventional tomographic reconstruction algorithms do not recover the 3D magnetization within a sample ***,we use simulations to describe the basis of an improved model-based algorithm for the tomographic reconstruction of a 3D magnetization distribution from one or more tilt series of electron optical phase images recorded in the *** algorithm allows a wide range of physical constraints,including a priori information about the sample geometry and magnetic parameters,to be *** also makes use of minimization of the micromagnetic energy in the loss *** demonstrate the reconstruction of the 3D magnetization of a localized magnetic soliton—a hopfion ring—and discuss the influence of noise,choice of magnetic constants,maximum tilt angle and number of tilt axes on the *** algorithm can in principle be adapted for other magnetic contrast imaging techniques in the TEM,as well as for other magnetic characterization techniques,such as those based on X-rays or neutrons.

关键词： three-dimensional magnetization vector field tomography differentiable programming electron holography micromagnetism

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Effect of rare earth Nd^(3+)doping contents on physical,structural,and magnetic properties of Co-Ni spinel ferrite nanoparticles

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Journal of Rare Earths 2023年第11期41卷 1746-1753,I0004页

作者： Junjiao Li Muhammad Yousaf Qaisar Hayat Muhammad Akbar Asma Noor MAK Yousaf Shah Fenghua Qi Yuzheng Lu Department of Electronic and Engineering Nanjing Vocational Institute of Mechatronic TechnologyNanjing211306China Energy Storage Joint Research Centre School of Energy and EnvironmentSoutheast UniversityNanjing210096China Shenzhen Key Laboratory of Laser Engineering Guangdong Provincial Key Laboratory of Micro/Nano Optomechatronics EngineeringCollege of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen518060China Hubei Collaborative Innovation Centre for Advanced Organic Chemical Materials Faculty of Physics and Electronic ScienceHubei UniversityWuhan430062China College of Electronic and Engineering Nanjing Xiaozhuang UniversityNanjing211171China

Rare earth(RE)low doping has a significant influence on the structural,morphological,and magnetic properties of spinel ferrite ***,rare earth neodymium(Nd)oxide was fully doped into spinel ferrite with a composition of Co_(0.80)Ni_(0.20)Nd_xFe_(2-x)O_4(x=0.0,0.05,0.10,and 0.15)using the sol-gel auto combustion *** analysis of the synthesized samples with low doping of Nd using X-ray diffraction(XRD)and Rietveld refinements reveals a pure single-phase cubic structure,while the second phase appears with increasing content of Nd^(3+)at x=0.10 and *** electron microscopy(SEM)and high-resolution transmission electron microscopy(HR-TEM)show well-shaped spherical grains within the nanometer range of the pure Co_(0.80)Ni_(0.20)Fe_(2)O_(4) sample,while larger grains with the presence of agglomeration are observed with doping of Nd^(3+)into the spinel ferrite *** magnetic parameters,i.e.,saturation magnetization M_s,remanence and magnetic moments exhibit decreasing trend with Nd^(3+)doping and M_s values are in 65.69 to 53.34 emu/g *** coercivity of the Nd-doped Co-Ni spinel ferrite sample was calculated to be 1037.76 to~827.24 *** work demonstrates remarkable improvements in the structural and magnetic characteristics of Nddoped Co-Ni spinel ferrite nanoparticles for multiple versatile applications.

关键词： Co-Ni spinel ferrites Rare earth Nd^(3+)doping Structural analysis Magnetic evaluations

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多带笼目超导体CsV_(3)Sb_(5)衍生体系的可调磁通涡旋束缚态

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science Bulletin 2024年第7期69卷 885-892页

作者：黄子豪韩相和赵振刘锦锦李鹏飞谭恒心王秩伟姚裕贵杨海涛颜丙海蒋坤胡江平汪自强陈辉高鸿钧 Beijing National Center for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China School of Physical Sciences University of Chinese Academy of SciencesBeijing 100190China Centre for Quantum Physics Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement(MOE)School of PhysicsBeijing Institute of TechnologyBeijing 100081China Beijing Key Lab of Nanophotonics and Ultrafine Optoelectronic Systems Beijing Institute of TechnologyBeijing 100081China Department of Condensed Matter Physics Weizmann Institute of ScienceRehovot 7610001Israel Hefei National Laboratory Hefei 230088China Department of Physics Boston CollegeChestnut Hill MA 02467USA

Vortices and bound states offer an effective means of comprehending the electronic properties of ***,surface-dependent vortex core states have been observed in the newly discovered kagome superconductors CsV_(3)Sb_(5).Although the spatial distribution of the sharp zero energy conductance peak appears similar to Majorana bound states arising from the superconducting Dirac surface states,its origin remains *** this study,we present observations of tunable vortex bound states(VBSs)in two chemically-doped kagome superconductors Cs(V_(1-x)Tr_(x))_(3)Sb_(5)(Tr=Ta or Ti),using low-temperature scanning tunneling microscopy/*** CsV_(3)Sb_(5)-derived kagome superconductors exhibit full-gap-pairing superconductivity accompanied by the absence of long-range charge orders,in contrast to pristine CsV_(3)Sb_(5).Zero-energy conductance maps demonstrate a field-driven continuous reorientation transition of the vortex lattice,suggesting multiband *** Ta-doped CsV_(3)Sb_(5)displays the conventional cross-shaped spatial evolution of Caroli-de Gennes-Matricon bound states,while the Tidoped CsV_(3)Sb_(5)exhibits a sharp,non-split zero-bias conductance peak(ZBCP)that persists over a long distance across the *** spatial evolution of the non-split ZBCP is robust against surface effects and external magnetic field but is related to the doping *** study reveals the tunable VBSs in multiband chemically-doped CsV_(3)Sb_(5)system and offers fresh insights into previously reported Y-shaped ZBCP in a non-quantum-limit condition at the surface of kagome superconductor.

关键词： Kagome superconductor Chemical doping Vortex lattice transition Vortex bound states Majorana bound states

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Effective CO_(2)activation of enriched oxygen vacancies for photothermal CO_(2)methanation

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Journal of Materials science & technology 2024年第22期189卷 203-210页

作者： Peipei Du Guoqiang Deng Zhonghua Li Junchuan Sun Lu Wang Yongqiang Yang Jun Wang Yaguang Li Xiaoming Xu Yuanming Zhang Wangxi Liu Gang Liu Zhigang Zou Zhaosheng Li Collaborative Innovation Center of Advanced Microstructures National Laboratory of Solid State MicrostructuresCollege of Engineering and Applied SciencesNanjing UniversityNanjing 210093China Jiangsu Key Laboratory of Nano Technology Nanjing UniversityNanjing 210093China Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China School of Science and Engineering The Chinese University of Hong KongShenzhen 518172China Research Center for Solar Driven Carbon Neutrality Engineering Research Center of Zero-carbon Energy Buildings and Measurement TechniquesMinistry of EducationThe College of Physics Science and TechnologyInstitute of Life Science and Green DevelopmentHebei UniversityBaoding 071002China

Oxygen vacancies have been widely concerned with the facilitation effects of CO_(2)activation for CO_(2)***,little attention has been paid to the generation of active intermediate species induced by enriched oxygen ***,we discovered that CeNiO_(3−δ)catalyst enriched oxygen vacancies can efficiently activate CO_(2)and realize high activity for photothermal CO_(2)*** situ diffuse reflectance infrared Fourier transform spectroscopy(DRIFTS)proved that oxygen vacancies are beneficial to the formation of reactive intermediate species of polydentate carbonate over CeNiO_(3−δ),which is crucial for efficient CO_(2)*** results revealed mechanistic insights into how effective CO_(2)activation induced by oxygen vacancies can be manipulated by adjusting the adsorption intermediate species.

关键词： Oxygen vacancies CO_(2)activation Active intermediate species Photo-thermal CO_(2)methanation CeNiO_(3)

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Real-time and modelled performance assessment and validation studies of PV modules operating in varied climatic zones

Energy and Built Environment

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Energy and Built Environment 2025年第4期6卷 585-595页

作者： Singh, Yogesh Kumar Dubey, Santosh Rajput, Pramod Singh, K.Y. Pandey, Kailash Gurugram122003 India J. S. University Mainpuri Road Shikohabad Uttar Pradesh Firozabad283135 India Indian Institute of Technology Delhi New Delhi110016 India Department of Physics Applied Science Cluster School of Advanced Engineering UPES Dehradun248007 India College Uttar Pradesh Mathura281001 India

With the increasing adoption of solar energy as a sustainable power source, it is crucial to evaluate the performance of photovoltaic (PV) modules under diverse environmental conditions to ensure optimal energy production and system efficiency. Present work gives a comprehensive overview of performance assessment and validation studies conducted on different PV module technologies such as multi-crystalline silicon (mc-Si), cadmium telluride (CdTe), copper indium gallium selenide (CIGS), amorphous silicon (a-Si), heterojunction with intrinsic thin layer (HIT) and interdigitated back contact (IBC) operating under varied climatic conditions at different locations in India. To ensure accuracy and reliability, rigorous data collection and analysis methodologies were employed. The performance assessment has been computed through simulation using PVSOL software. Moreover, the performance ratio (PR) of all the PV module technologies was found to vary from 0.76 to 1.04. The present work validates the efficacy of the software as we have compared the computed results with real-time data obtained for all the PV modules, which were installed at NISE (National Institute of Solar Energy), Gurugram India. The performance ratio of all the PV module technologies has been evaluated through both the PVSOL and using real time data. The results show that the mean percentage change in PR values has been estimated approximately to be 2% in CdTe, CIGS, and a-Si modules technologies and 3% in mc-Si, HIT and IBC module technologies. © 2023

关键词： Amorphous silicon

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Textured Asymmetric Membrane Electrode Assemblies of Piezoelectric Phosphorene and Ti_(3)C_(2)T_(x)MXene Heterostructures for Enhanced Electrochemical Stability and Kinetics in LIBs

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Nano-Micro Letters 2024年第4期16卷 394-414页

作者： Yihui Li Juan Xie Ruofei Wang Shugang Min Zewen Xu Yangjian Ding Pengcheng Su Xingmin Zhang Liyu Wei Jing‑Feng Li Zhaoqiang Chu Jingyu Sun Cheng Huang Volta and DiPole Materials Labs College of EnergySoochow Institute for Energy and Materials InnovationS(SIEMIS)Key Laboratory of Advanced Carbon Materials and Wearable Energy Technologies of Jiangsu ProvinceKey Laboratory of Core Technology of High Specific Energy Battery and Key Materials for Petroleum and Chemical IndustrySoochow UniversitySuzhou 215006People’s Republic of China School of Materials Science and Engineering Jiangsu UniversityZhenjiang 212013People’s Republic of China College of Underwater Acoustic Engineering Harbin Engineering UniversityHarbin 150001People’s Republic of China Shanghai Synchrotron Radiation Facility Shanghai Advanced Research InstituteShanghai Institute of Applied PhysicsChinese Academy of SciencesShanghai 201204People’s Republic of China State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084People’s Republic of China High Density Materials Technology Center for Flexible Hybrid Electronics Suzhou Institute of Electronic Functional Materials TechnologySuzhou Industrial Technology Research InstituteSuzhou 215151People’s Republic of China Institute of Advanced Materials and Institute of Membrane Science and Technology Jiangsu National Synergistic Innovation Center for Advanced MaterialsSuzhou Laboratory and Nanjing Tech UniversityNanjing 211816People’s Republic of China

Black phosphorus with a superior theoretical capacity(2596 mAh g^(-1))and high conductivity is regarded as one of the powerful candidates for lithium-ion battery(LIB)anode materials,whereas the severe volume expansion and sluggish kinetics still impede its applications in *** contrast,the exfoliated two-dimensional phosphorene owns negligible volume variation,and its intrinsic piezoelectricity is considered to be beneficial to the Li-ion transfer kinetics,while its positive influence has not been discussed ***,a phosphorene/MXene heterostructure-textured nanopiezocomposite is proposed with even phosphorene distribution and enhanced piezo-electrochemical coupling as an applicable free-standing asymmetric membrane electrode beyond the skin effect for enhanced Li-ion *** experimental and simulation analysis reveals that the embedded phosphorene nanosheets not only provide abundant active sites for Li-ions,but also endow the nanocomposite with favorable piezoelectricity,thus promoting the Li-ion transfer kinetics by generating the piezoelectric field serving as an extra *** waltzing with the MXene framework,the optimized electrode exhibits enhanced kinetics and stability,achieving stable cycling performances for 1,000 cycles at 2 A g^(-1),and delivering a high reversible capacity of 524 m Ah g^(-1)at-20℃,indicating the positive influence of the structural merits of self-assembled nanopiezocomposites on promoting stability and kinetics.

关键词： Phosphorene Nanopiezocomposite Piezo-electrochemical coupling Membrane electrode assembly Lithium-ion storage

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General synthesis of 2D rare-earth oxide single crystals with tailorable facets

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National science Review 2022年第5期9卷 22-29页

作者： Linyang Li Fangyun Lu Wenqi Xiong Yu Ding Yangyi Lu Yao Xiao Xin Tong Yao Wang Shuangfeng Jia Jianbo Wang Rafael G.Mendes Mark H.Rümmeli Shengjun Yuan Mengqi Zeng Lei Fu College of Chemistry and Molecular Sciences Wuhan University Key Laboratory of Artificial Micro-and Nano-Structures of Ministry of Education and School of Physics and Technology Wuhan University The Institute for Advanced Studies Wuhan University College of Physics Optoelectronics and Energy and Collaborative Innovation Center of Suzhou Nano Science and TechnologySoochow University Institute for Complex Materials IFW Dresden Centre of Polymer and Carbon Materials Polish Academy of Sciences Institute of Environmental Technology VSB-Technical University of Ostrava

Two-dimensional(2D) rare-earth oxides(REOs) are a large family of materials with various intriguing applications and precise facet control is essential for investigating new properties in the 2D ***,a bottleneck remains with regard to obtaining their 2D single crystals with specific facets because of the intrinsic non-layered structure and disparate thermodynamic stability of different ***,for the first time,we achieve the synthesis of a wide variety of high-quality 2D REO single crystals with tailorable facets via designing a hard-soft-acid-base couple for controlling the 2D nucleation of the predetermined facets and adjusting the growth mode and direction of ***,the facet-related magnetic properties of 2D REO single crystals were *** approach provides a foundation for further exploring other facet-dependent properties and various applications of 2D REO,as well as inspiration for the precise growth of other non-layered 2D materials.

关键词： 2D materials cerium crystal engineering rare earth CVD

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Fully depleted vdW heterojunction based high performance photovoltaic photodetector

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Journal of Materiomics 2023年第6期9卷 1039-1047页

作者： Yonghong Zeng Fanxu Meng Sidi Fan Pengfei Wang Cuiyun Kou Mingyi Sun Haiguo Hu Rui Cao Swelm Wageh Omar A.Al-Hartomy Abul Kalam Bowen Du Wenchao Ding Songrui Wei Zhinan Guo Qiuliang Wang Han Zhang College of Physics and Optoelectronic Engineering Institute of Microscale OptoelectronicsInternational Collaborative Laboratory of 2D Materials for Optoelectronics Science and TechnologyInterdisciplinary Center of High Magnetic Field Physics of Shenzhen UniversityShenzhen UniversityShenzhen518060China Guangzhou Key Laboratory of Sensing Materials and Devices Center for Advanced Analytical ScienceSchool of Chemistry and Chemical EngineeringGuangzhou UniversityGuangzhou510006China Department of Physics Faculty of ScienceKing Abdulaziz UniversityJeddah21589Saudi Arabia Research Center for Advanced Materials Science(RCAMS) Department of ChemistryCollege of ScienceKing Khalid UniversityP.O.Box 9004Abha61413Saudi Arabia Foshan Electrical and Lighting Co. LTD64 North Fenjiang RoadFoshanChina Institute of Electrical Engineering Chinese Academy of SciencesBeijing100190China Center of Characterization and Analysis Jilin Institute of Chemical TechnologyJilin132022China

Van der Waals(vdW)heterojunctions,with their unique electronic and optoelectronic properties,have become promising candidates for photodetector *** the contribution of the depletion region in vdW heterojunction,which would enhance both of the collection efficiency and speed of the photogenerated carriers,presents an effective strategy for achieving high performance vdW heterojunction ***,a fully depleted vdW heterojunction photodetector is built on two-dimensional(2D)semiconductor materials(GaTe and InSe)layered on a pattered bottom electrode in vertical structure,in which the generation and motion of carriers are exclusively achieved in the depletion *** to the intrinsic built-in electric field,the elimination of series resistance and the depletion region confinement of carriers,the as-fabricated photodetector exhibits prominent photovoltaic properties with a high open-circuit voltage of 0.465 V,as well as photoresponse characteristics with outstanding responsivity,detectivity and photoresponse speed of 63.7 A/W,3.88×10^(13)Jones,and 32.7 ms *** overall performance of this fully depleted GaTe/InSe vdW heterojunctions photodetectors are ranking high among the top level of 2D materials based *** indicates the device architecture can provide new opportunities for the fabrication of high-performance photodetectors.

关键词： Two-dimensional material van der waals heterojunction Fully depleted photodetector Photovoltaic

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Epsilon-near-zero phase-matching for second-harmonic generation in semiconductor-based nanowire hyperbolic metamaterial

Epsilon-near-zero phase-matching for second-harmonic generat...

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Metamaterials, Metadevices, and Metasystems 2023

作者： Wicharn, Surawut Buranasiri, Prathan Advanced Photonics Laboratory Department of Physics Faculty of Science Srinakharinwirot University 114 Sukhumvit 23 Watthana Bangkok10110 Thailand Artificial Intelligence Photonics Advanced Research Laboratory Department of Physics School of Science King Mongkut’s Institute of Technology Ladkrabang Chalongkrung Rd. Bangkok10520 Thailand Electronic and Optoelectronic Device Research Unit School of Science King Mongkut’s Institute of Technology Ladkrabang Chalongkrung Rd. Bangkok10520 Thailand

ISBN: (纸本)9781510665064

Hyperbolic metamaterials have been widely used for nonlinear optical applications. Their unique functionality for nonlinear optics enhancement due to the hyperbolic dispersion is induced by a strong shape anisotropy. In this work, we numerically investigated the second-harmonic generation (SHG) in two-dimensional periodic arrays of aluminium gallium arsenide (AlGaAs) nanowires embedded in ordered porous aluminum oxide (Al2O3) or the nanowire hyperbolic metamaterial (NHMM). Under local effective medium approximation, the homogenization of the NHMM was achieved due to deep sub-wavelength size of each nanowire radius. Then this medium was classified as an effective uniaxial medium with anisotropic electric permittivity. The NHMM provided the spectral position of second-harmonic (SH) wavelength, which is determined at the epsilon-near-zero (ENZ) by the optimal design of NHMM structural parameters such as AlGaAs radius or fill fraction. Consequently, a gigantic increment of SHG conversion efficiency was achieved because of dramatic phase-matching at ENZ point. This mechanism is attributed to electric field enhancement of SHG inside the metamaterial. According to numerical results, the NHMM can be applied as nonlinear frequency converters in integrated nanophotonic systems. © 2023 SPIE.

关键词： Harmonic generation

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Enhanced performance of monocrystalline silicon solar cells using sol-gel synthesized zinc stannate anti-reflective coating via electro-spraying technique

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Ceramics International 2025年第8期51卷 10899-10912页

作者： Mostafa, Ayman M. Velu Kaliyannan, Gobinath Gunasekaran, Raja El-Tayeb, Zaynb Rao, Subha Krishna Al-Ahmadi, Ameenah N. Darwish, A.A.A. Younes, Ayman A.O. Elsharkawy, Wafaa B. Palaniappan, Sathish Kumar Department of Physics College of Science Qassim University P.O. Box 6644 Almolaydah Buraydah51452 Saudi Arabia Department of Mechatronics Engineering Kongu Engineering College Perundurai Tamil Nadu Erode638060 India Department of Mechanical Engineering Velalar College of Engineering and Technology Tamil Nadu Erode638012 India Department of Physics Faculty of Science Taibah University Yanbu46423 Saudi Arabia Centre for Nanoscience and Nanotechnology International Research Centre Sathyabama Institute of Science and Technology Tamil Nadu Chennai600119 India Department of Physics College of Sciences Umm Al-Qura University Makkah24382 Saudi Arabia Advanced Materials Research Laboratory Department of Physics Faculty of Science University of Tabuk Tabuk71491 Saudi Arabia Department of Chemistry College of Science University of Bisha Bisha 61922 Saudi Arabia Pysics Department College of Science and Humanities Prince Sattam Bin Abdulaziz University Alkharj11942 Saudi Arabia Natural Composites Research Group Lab Department of Materials and Production Engineering The Sirindhorn International Thai-German Graduate School of Engineering King Mongkut's University of Technology North Bangkok Bangsue Bangkok10800 Thailand

The current situation necessitates advancements in renewable energy to serve as a viable alternative to traditional energy sources. The photovoltaic cells can entirely change the need for fossil fuels since they can transform light energy into electrical energy. The reflection loss in photovoltaic cells is a contributing factor to reduced power conversion efficiency that could be mitigated by using antireflective coatings on the surface of the solar cells. This study examines the deposition of zinc stannate (ZnSnO3) as an efficient antireflective material to improve light capturing capability and it is synthesized by sol-gel method. The electro spraying method was employed to deposit the ZnSnO3 layers on photovoltaic cells. The ZnSnO3 AR material was uniformly distributed on the solar substrate at 2 ml/h for 1 h (Z1), 2 h (Z2), 3 h (Z3) and 4 h (Z4) respectively. The impact of ZnSnO3 ARC on the structural, electrical, absorbance, reflectance characteristics and temperature variation in monocrystalline silicon (m-Si) solar cells was examined. The optical properties were determined by UV–visible spectroscopy technique. At a wavelength (300–800 nm), the ZnSnO3 coated for 3 h (Z3 specimen) exhibited highest absorbance of 92.65 % and the lowest electrical resistivity of 3.69 × 10−3 Ω-cm. When compared with bare and various ZnSnO3 coated cells, Z3 specimen showed a significant impact on solar cell efficiency. In direct solar radiation and stimulated light, the Z3 specimen achieved the maximum power conversion efficiency (PCE) of 21.16 % and 25.11 %. The findings indicated that ZnSnO3 could be a suitable AR coating material for reducing incoming photon reflection. © 2025 Elsevier Ltd and Techna Group S.r.l.

关键词： Antireflection coatings

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