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Scalable Ir‑Doped NiFe_(2)O_(4)/TiO_(2) Heterojunction Anode for Decentralized Saline Wastewater Treatment and H_(2) Production

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Nano-Micro Letters 2025年第3期17卷 1-18页

作者： Sukhwa Hong Jiseon Kim Jaebeom Park Sunmi Im Michael R.Hoffmann Kangwoo Cho Division of Environmental Science and Engineering Pohang University of Science and Technology(POSTECH)Pohang 790−784Korea Linde Laboratory California Institute of TechnologyPasadenaCA 91125USA Institute for Convergence Research and Education in Advanced Technology(I‑CREATE) Yonsei University International CampusIncheon 21983Republic of Korea

Wastewater electrolysis cells(WECs)for decentralized wastewater treatment/reuse coupled with H_(2) production can reduce the carbon footprint associated with transportation of water,waste,and energy *** study reports Ir-doped NiFe_(2)O_(4)(NFI,~5 at%Ir)spinel layer with TiO_(2) overlayer(NFI/TiO_(2)),as a scalable heterojunction anode for direct electrolysis of wastewater with circumneutral pH in a single-compartment *** dilute(0.1 M)NaCl solutions,the NFI/TiO_(2) marks superior activity and selectivity for chlorine evolution reaction,outperforming the benchmark IrO_(2).Robust operation in near-neutral pH was *** including operando X-ray absorption spectroscopy unveiled crucial roles of TiO_(2) which serves both as the primary site for Cl−chemisorption and a protective layer for NFI as an ohmic *** electrolysis of NH4+-laden synthetic wastewater demonstrated that NFI/TiO_(2)not only achieves quasi-stoichiometric NH_(4)^(+)-to-N_(2)conversion,but also enhances H_(2)generation efficiency with minimal competing reactions such as reduction of dissolved oxygen and reactive *** scaled-up WEC with NFI/TiO_(2)was demonstrated for electrolysis of toilet wastewater.

关键词： Wastewater electrolysis cell Ir-doped NiFe_(2)O_(4) Reactive chlorine species Decentralized H_(2)production On-site wastewater treatment

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Enhanced removal of high-As(Ⅲ)from Cl(-Ⅰ)-diluted SO_(4)(-Ⅱ)-rich wastewater at pH 2.3 via mixed tooeleite and(Cl(-Ⅰ)-free)ferric arsenite hydroxychloride formation

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Journal of environmental sciences 2023年第2期124卷 31-41页

作者： Zidan Yuan Guoqing Zhang Xing Wu Xu Ma Jinru Lin Shaofeng Wang Yongfeng Jia Key Laboratory of Pollution Ecology and Environmental Engineering Institute of Applied EcologyChinese Academy of SciencesShenyang 110016China Key Laboratory for Yellow River and Huai River Water Environmental and Pollution Control Ministry of EducationHenan Key Laboratory for Environmental Pollution ControlSchool of EnvironmentHenan Normal UniversityHenan 453007China Key Laboratory of Industrial Ecology and Environmental Engineering(Ministry of Education China)School of Environmental Science and TechnologyDalian University of TechnologyDalian 116024China

An advanced cost-saving method of removal of high-As(Ⅲ)from SO_(4)(-Ⅱ)-rich metallurgical wastewater has been developed by diluting the SO_(4)(-Ⅱ)content with As(Ⅲ)-Cl(-Ⅰ)-rich metallurgical wastewater and then by the direct precipitation of As(Ⅲ)with Fe(Ⅲ)at pH ***(Ⅲ)removal at various SO_(4)(-Ⅱ)/Cl(-Ⅰ)molar ratios and temperatures was *** results showed that 65.2–98.2%of As(Ⅲ)immobilization into solids occurred at the SO_(4)(-Ⅱ)/Cl(-I)molar ratios of 1:1–32 and 15–60℃in 3 days,which were far higher than those in aqueous sole SO4(-Ⅱ)or Cl(-Ⅰ)media at the equimolar SO_(4)(-Ⅱ)or Cl(-Ⅰ)and the same ***_(4)(-Ⅱ)/Cl(-Ⅰ)molar ratio of 1:4 and 25℃were optimal conditions to reach the As removal *** aqueous SO4(-Ⅱ)and Cl(-Ⅰ)played a synergetic role in the main tooeleite formation together with(Cl(-Ⅰ)-free)ferric arsenite hydroxychloride(FAHC)involving the substitution of AsO_(3)^(3−)for Cl(-Ⅰ)for enhanced As *** competitive complexation among FeH_(2)AsO_(3)^(2+),FeSO_(4)^(+)and FeCl^(2+)complexes was the main mechanism for the maximum As(Ⅲ)precipitation at the SO4(-Ⅱ)/Cl(-I)molar ratio of 1:*** As(Ⅲ)immobilization at high temperature with increased Fe(Ⅲ)hydrolysis was due to the formation of As(Ⅲ)-bearing ferrihydrite with the relatively high Fe/As molar ratio at acidic pH.

关键词： High-As(III) Sulfate Chlorine ion Removal Complex

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Mechanistic insight into the biofilm formation and process performance of a passive aeration ditch(PAD)for decentralized wastewater treatment

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Frontiers of environmental science & engineering 2022年第7期16卷 35-46页

作者： Jibin Li Jinxing Ma Li Sun Xin Liu Huaiyu Liao Di He Key Laboratory for City Cluster Environmental Safety and Green Development of the Ministry of Education Institute of Environmental and Ecological EngineeringGuangdong University of TechnologyGuangzhou510006China Southern Marine Science and Engineering Guangdong Laboratory(Guangzhou) Guangzhou511458China School of Environmental Science and Engineering Southern University of Science and TechnologyShenzhen518055China

Decentralized wastewater containing elevated salinity is an emerging threat to the local environment and sanitation in remote coastal *** the cost and treatment efficiencies,we propose a passive aeration ditch(PAD)using non-woven polyester fabric as a feasible bubbleless aerator and biofilm carrier for wastewater *** has been first given to PAD’s efficacy in treating saline decentralized wastewater,and then to the impact of chemical oxygen demand-to-nitrogen(C/N)ratio and salinity on biofilm formation.A multispecies model incorporating the salinity effect has been developed to depict the system performance and predict the microbial *** showed that the PAD system had great capacity for pollutants *** biofilm thickness increased at a higher C/N ratio because of the boost of aerobic heterotrophs and denitrifying bacteria,which consequently improved the COD and total nitrogen ***,this led to the deterioration of ammonia ***,while a higher salinity benefited the biofilm growth,the contaminant removal efficiencies decreased because the salinity inhibited the activity of aerobic heterotrophs and reduced the abundance of nitrifying bacteria inside the *** on the model simulation,feed water with salinity below 2%and C/N ratio in a range of 1 to 3 forms a biofilm that can reach relatively high organic matter and ammonia *** findings not only show the feasibility of PAD in treatment of saline decentralized wastewater,but also offer a systematic strategy to predict and optimize the process performance.

关键词： Decentralized wastewater Passive aeration ditch Biofilm formation C/N ratio Salinity Model simulation

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Developing modified k–εturbulence models for neutral atmospheric boundary layer flow simulation using OpenFOAM

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Building Simulation 2024年第12期17卷 2281-2295页

作者： Yuanbo Wang Jiqin Li Wei Liu Jiankai Dong Jing Liu School of Architecture Harbin Institute of TechnologyKey Laboratory of Cold Region Urban and Rural Human Settlement Environment Science and TechnologyMinistry of Industry and Information TechnologyHarbin 150090China Tianjin Key Laboratory of Indoor Air Environmental Quality Control School of Environmental Science and EngineeringTianjin University92 Weijin RoadTianjin 300072China Division of Sustainable Buildings Department of Civil and Architectural EngineeringKTH Royal Institute of TechnologyBrinellvägen 2310044 StockholmSweden

Accurate turbulence modeling is essential for simulation studies of urban *** this study,the comprehensive atmospheric boundary layer(ABL)model involving a variable model coefficient and an additional turbulent dissipation source term was implemented using the open-source software *** with consistent inlet wind profiles and rough wall functions of different turbulence variables based on the aerodynamic roughness,the model maintained the horizontal homogeneity ***,a hybrid approach was introduced to consider buildings immersed in ABL flows,enabling automatic transformation of the turbulence model between the region around the buildings and the free flow region away from any ***,the effects of applying different model forms to the airflow field around buildings were evaluated in detail through three-dimensional building cases representing six urban prototypes based on three wind tunnel *** findings indicated that all modified k–εmodels perform well in reproducing the flow data of the CEDVAL and Architectural Institute of Japan(AIJ)experiments consisting of a single building,an array of buildings,and an isolated high-rise ***,the modified k–εmodel with an additional correction term performed poorly in the database of Niigata Institute of technology and the case of complex terrain and urban building configurations,because the correction term inhibited the generation of turbulent kinetic *** addition,from the comparison between the experimental data of all cases,the model with the original formulation of the coefficient performed the best in terms of prediction *** root mean square errors of the normalized velocity were 0.1250,0.0879,0.1145,0.1350,and 0.1492 in different cases,which proved the reliability of this turbulence model.

关键词： urban airflow computational fluid dynamics(CFD) atmospheric boundary layer OpenFOAM turbulence model

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Honeycomb-like biochar framework coupled with Fe_(3)O_(4)/FeS nanoparticles as efficient heterogeneous Fenton catalyst for phenol degradation

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Journal of environmental sciences 2024年第2期136卷 390-399页

作者： Aihua Cheng Yi He Xiaohe Liu Chi He Department of Environmental Engineering College of Geology and EnvironmentXi’an University of Science and TechnologyXi’an 710054China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power EngineeringXi’an Jiaotong UniversityXi’an 710049China National Engineering Laboratory for VOCs Pollution Control Material and Technology University of Chinese Academy of SciencesBeijing 101408China

Achieving an efficient and stable heterogeneous Fenton reaction over a wide pH range is of great significance for wastewater ***,a pollen-derived biochar catalyst with a unique honeycomb-like structure,coupled with the dispersion of magnetic Fe_(3)O_(4)/FeS(Fe/S)nanoparticles,was synthesized by simple impregnation precursor,followed by *** prepared Fe/S-biochar catalyst demonstrated outstanding phenol degradation efficiency across a wide pH range,with 98%of which eliminated even under neutral conditions(pH 7.0).The high catalytic activity was due to the multilevel porous structure of pollenderived biochar provided enough active sites and allowed for better electron transfer,then increases oxidation ability to promote the ***,the acid microenvironment formed by SO_(4)^(2-)group from Fe/S composite extended the pH range for Fenton reaction,and S^(2-)facilitated the conversion of≡Fe^(3+)to≡Fe^(2+),resulting in remarkable degradation ***,biochar can effectively promote cycling stability by limiting Fe *** work may provide a general strategy for designing 3D framework biochar-based Fe/S catalysts with excellent performance for heterogeneous Fenton reactions.

关键词： Biomass Biochar Fenton reaction Fe_(3)O_(4)/FeS(Fe/S) Phenol degradation

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In-situ construction of abundant active centers on hierarchically porous carbon electrode toward high-performance phosphate electrosorption: Synergistic effect of electric field and capture sites

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Green Energy & Environment 2024年第1期9卷 126-137页

作者： Peng Zhang Fukuan Li Mingming He Silu Huo Xueli Zhang Benqiang Cen Dezhi Fang Kexun Li Hao Wang College of Environmental Science and Engineering Nankai UniversityTianjin300350China MOE Key Laboratory of Pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Remediation and Pollution ControlTianjin Key Laboratory of Environmental Technology for Complex Trans-Media PollutionNankai UniversityTianjin300350China State Key Laboratory of Simulation and Regulation of Water Cycles in River Basins China Institute of Water Resources and Hydropower ResearchBeijing100038China

Phosphate removal is crucial for eutrophication control and water quality ***-assisted adsorption,an eco-friendly elec-trosorption process,exhibited a promising potential for wastewater ***,there are few works focused on phosphate electro-sorption,and reported electrodes cannot attach satisfactory removal capacities and ***,electro-assisted adsorption of phosphate via in-situ construction of La active centers on hierarchically porous carbon(LaPC)has been originally *** resulted LaPC composite not only possessed a hierarchically porous structure with uniformly dispersed La active sites,but also provided good conductivity for interfacial electron *** LaPC electrode achieved an ultrahigh phosphate electrosorption capability of 462.01 mg g^(-1) at 1 V,outperforming most existing *** superior phosphate removal performance originates from abundant active centers formed by the coupling of electricﬁeld and capture ***,the stability and selectivity toward phosphate capture were maintained well even under comprehensive ***,a series of kinetics and isotherms models were employed to validate the electrosorption *** work demonstrates a deep understanding and promotes a new level of phosphate electrosorption.

关键词： Electro-assisted adsorption Electrosorption Phosphate removal Active centers MOF-derived carbon

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A Wind Gearbox Fault Detection Method Based on a Lightweight Attention Network 15

A Wind Gearbox Fault Detection Method Based on a Lightweight...

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15th IEEE Global reliability and Prognostics and Health Management Conference, PHM-Beijing 2024

作者： Xie, Keqiang Chen, Liping School of Mechanical Science and Engineering Huazhong University of Science and Technology Wuhan China China Electronic Product Reliability and Environmental Testing Research Institute Guangzhou China

ISBN: (纸本)9798350354010

It is of great importance to realize effective fault diagnosis of wind turbines gearbox in modern industrial systems. This paper proposes a fault diagnosis method that based on a lightweight attention network. This method uses a lightweight convolutional neural network MobileNetV3_L based on the Transformer to improve the new network RepViT network for wind gearbox fault diagnosis. The diagnosis process includes short-time Fourier transform processing of the laboratory artificial wind gearbox fault data set, and establishing a fault classification and recognition model based on a lightweight convolutional neural network. Finally, the model is used to perform fault diagnosis on a real wind gearbox dataset to verify its performance. Experimental research is conducted on the University of Macau gearbox dataset to validate the proposed method. The results demonstrate that the method exhibits superior stability and accuracy than other methods. © 2024 IEEE.

关键词： Wind turbines

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Mesoscale modeling on the influence of surfactants on seepage law during water injection in coal

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Particuology 2025年第1期96卷 1-13页

作者： Yanan Miao Haoran Li Mingzhu Zhu Chaojie Zhao Tengwen Zhang Hussein Mohammed Ahmed Kaid College of Safety and Environmental Engineering Shandong University of Science and TechnologyQingdao266590China State Key Laboratory of Mining Disaster Prevention and Control Co-Founded By Shandong Province and the Ministry of Science and Technology Shandong University of Science and TechnologyQingdao266590China Sinopec Research Institute of Safety Engineering Co. Ltd.Qingdao266000China State Key Laboratory of Safety and Control for Chemicals SINOPEC Research Institute of Safety Engineering Co.Ltd.Qingdao266000China College of Mechanical and Electronic Engineering Shandong University of Science and TechnologyQingdao266590China

To investigate the mesoscopic influence of surfactants on seepage law during water injection in coal seam, this paper innovatively establishes a fluid transport lattice Boltzmann (LBM) model by incorporating the seepage resistance generated from the porous media and external forces, which embodies the impact of wettability degree resulted from cocamidopropyl betaine (CAB), sodium dodecyl sulfate (SDS), and coconutt diethanol amide (CDEA) reagents at a 0.1% concentration. The main conclusions derived from this investigation are as follows: Firstly, as the lattice number in the X direction increases, the average seepage velocities in coal samples treated by deionized water, 0.1% CAB, 0.1% SDS, and 0.1% CDEA reagents (Nos. 1, 2, 3, and 4) exhibit three distinct stages: rapid decline, slow decline, and steady decline;in comparison to raw coal sample, modified coal samples demonstrate decreases of 20.84%, 33.91%, and 61.70%, respectively. Secondly, the critical values of displacement pressure difference exist during the phenomenon that modified reagents spread out in the entire flow channel, which are 3.5, 3.5, and 5.2 MPa, respectively, for coal samples Nos. 2, 3, and 4;this signifies that surpassing these critical values help prevent issues such as blank belts within the wetting range and insufficient dust control. Finally, at a displacement pressure difference of 0.01 (lattice unit), the average velocity ratios for samples (Nos. 2, 3, and 4) are 0.78, 0.56, and 0.37 (lattice unit), respectively;notably, the water flow velocities in modified coal samples are lower compared to that in raw coal sample, indicating that the addition of surfactants impede the seepage process of water injection in coal seam. Moreover, when the displacement pressure difference reaches 0.03 (lattice unit), the velocity ratio of CDEA-modified coal sample exceeds 100%;this means that when the displacement pressure difference surpasses 15.6 MPa, the water injection effect of CDEA-modified coal sa

关键词： Mesoscale seepage Surfactant Lattice Boltzmann method Velocity ratio Critical displacement pressure difference

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Integration of Bio-Enzyme-Treated Super-Wood and AIE-Based Nonwoven Fabric for Efficient Evaporating the Wastewater with High Concentration of Ammonia Nitrogen

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Nano-Micro Letters 2025年第8期17卷 1-16页

作者： Qian Ding Bingqi Jin Yinxia Zheng Huiru Zhao Jun Wang Haoxuan Li Dong Wang Ben Zhong Tang Engineering Research Center of Technical Textiles Ministry of EducationCollege of Materials Science and EngineeringDonghua UniversityShanghai 201620People’s Republic of China State Key Laboratory of Pollution Control and Resources Reuse School of Environmental Science and EngineeringTongji UniversityShanghai 200092People’s Republic of China Nonwoven Technology Laboratory College of Textile Science and EngineeringJiangnan UniversityWuxi 214122People’s Republic of China Centre for AIE Research Shenzhen Key Laboratory of Polymer Science and TechnologyGuangdong Research Center for Interfacial Engineering of Functional MaterialsCollege of Material Science and EngineeringShenzhen UniversityShenzhen 518061People’s Republic of China School of Science and Engineering Shenzhen Institute of Aggregate Science and TechnologyThe Chinese University of Hong KongShenzhen(CUHK-Shenzhen)Shenzhen 518172People’s Republic of China

The treatment of ammonia nitrogen wastewater(ANW)has garnered significant attention due to the ecology,and even biology is under increasing threat from over discharge *** ANW treatment methods often encounter challenges such as complex processes,high costs and secondary *** progress has been made in employing solar-induced evaporators for wastewater ***,there remain notable barriers to transitioning from fundamental research to practical applications,including insufficient evaporation rates and inadequate resistance to ***,we propose a novel evaporator,which comprises a bio-enzyme-treated wood aerogel that serves as water pumping and storage layer,a cost-effective multi-walled carbon nanotubes coated hydrophobic/hydrophilic fibrous nonwoven mat functioning as photothermal evaporation layer,and aggregation-induced emission(AIE)molecules incorporated as anti-biofouling *** resultant bioinspired evaporator demonstrates a high evaporation rate of 12.83 kg m^(−2) h^(−1) when treating simulated ANW containing 30 wt%NH4Cl under 1.0 sun of ***-doped evaporator exhibits remarkable photodynamic antibacterial activity against mildew and bacteria,ensuring outstanding resistance to biofouling over extended periods of wastewater *** enhanced by natural wind under 1.0 sun irradiation,the evaporator achieves an impressive evaporation rate exceeding 20 kg m^(−2) h^(−1) .This advancement represents a promising and viable approach for the effective removal of ammonia nitrogen wastewater.

关键词： Wood aerogel AIE Anti-biofouling Solar-driven interface evaporation Ammonia nitrogen wastewater treatment

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Investigation of Off-state Stress Time-Dependent Dynamic On-resistance of Commercial High Voltage GaN HEMTs 18

Investigation of Off-state Stress Time-Dependent Dynamic On-...

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18th IEEE Conference on Industrial Electronics and Applications, ICIEA 2023

作者： Li, Yao Tang, Hui Zhang, Ke Ni, Yiqiang He, Liang He, Zhiyuan Shi, Yijun Liu, Jun University of South China School of Electrical Engineering Hengyang China Electronic Product Reliability and Environmental Testing Research Institute Science and Technology on Reliability Physics and Application of Electronic Component Laboratory Guangzhou China

ISBN: (纸本)9798350312201

The effects of off-state stress time on dynamic on-resistance are investigated in a commercial 650 V GaN power device. A modified double pulse test (DPT) circuit is used to evaluate the dynamic on-resistance degradation with various stress value and time under hard-switching conditions. Our experimental results reveal partial recovery behaviors of dynamic on-resistance with stress voltage increasing. The dynamic on-resistance degradation gets more severe as stress voltage initially increases. Then the dynamic on-resistance reaches a peak value and begins to decrease as the stress voltage further increases. Furthermore, we find that the turning point of maximum dynamic on-resistance occurs at a lower stress voltage with longer stress time. It indicates that stress time is a very important factor affecting the degree of dynamic on-resistance degradation. © 2023 IEEE.

关键词： III-V semiconductors

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