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Hierarchical hollow microspheres assembled from carbon nanosheets integrated with molybdenum carbide nanoparticles for boosting microwave absorption properties

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Nano Research 2025年第1期18卷 10-20页

作者： Zongsheng Chen Yahui Wang Yi Liu Zhigang Li Xiangyin Lv Liping Liu Yajing Chang Jiaming Shi Xiao Zhang State Key Laboratory of Pulsed Power Laser Technology School of Electronic EngineeringNational University of Defense TechnologyHefei 230037China Anhui Provincial Laboratory of Advanced Laser Technology School of Electronic EngineeringNational University of Defense TechnologyHefei 230037China Centre for Environmental and Energy Nanomaterials Anhui Key Laboratory of Nanomaterials and NanotechnologyCAS Centre for Excellence in NanoscienceInstitute of Solid State PhysicsHefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China

Hierarchical hollow structure has demonstrated potential for enhancing electromagnetic(EM)attenuation and improving impedance matching,garnering significant attention for ***,we have successfully implemented compositional and structural engineering to fabricate hollow Mo2C/C microspheres with controllable composition by coupling interaction between dopamine hydrochloride and ammonium *** the synergistic effect of composition and hollow structure,the strongest reflection loss intensity and broadest effective absorption of the optimized sample reach-70.2 dB and 6.2 GHz,*** formation of hollow heterogeneous structures not only favors impedance matching feature,but also generates considerable contribution to EM attenuation ***,radar cross-section simulation data indicate that hollow Mo2C/C microspheres with compositional optimization and heterogeneous structures have broad prospects for practical applications.

关键词： electromagnetic absorption Mo2C/C microwave absorption hollow structure

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The degradation of perovskite precursor

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Journal of Semiconductors 2023年第10期44卷 3-6页

作者： Mengjia Li Lixiu Zhang Cong Chen Jiangzhao Chen Liming Ding State Key Laboratory of Reliability and Intelligence of Electrical Equipment School of Materials Science and EngineeringHebei University of TechnologyTianjin 300401China Key Laboratory of Optoelectronic Technology&Systems(MoE) College of Optoelectronic EngineeringChongqing UniversityChongqing 400044China Center for Excellence in Nanoscience(CAS) Key Laboratory of Nanosystem and Hierarchical Fabrication(CAS)National Center for Nanoscience and TechnologyBeijing 100190China Macao Institute of Materials Science and Engineering(MIMSE) Macao University of Science and TechnologyMacao 999078China

Perovskite solar cells(PSCs)are taking a leading position in thin-film optoelectronic devices due to their excellent optical,physical and electrical properties[1-4].Nevertheless,the stability issue of metal halide perovskite precursor solution severely retards the future industrialization of PSCs[5-7].In stoichiometry,slight solution composition change will induce severe degradation of device performance.

关键词： perovskite halide film

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Efficient and selective recovery of Gd(Ⅲ)via polyethyleneimine modification of lanthanum-based metal-organic frameworks

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Journal of Rare Earths 2024年第1期42卷 210-219,I0007页

作者： Wenhao Li Lijinhong Huang Bin Xiao Xiaoguang Duan Haike Li Lang Li Wanfu Huang Ganzhou Key Laboratory of Basin Pollution Simulation and Control Jiangxi University of Science and TechnologyGanzhou341000China Innovation Center for Water Quality Security Technology at Ganjiang River Basin Jiangxi University of Science and TechnologyGanzhou341000China Faculty of Science and Engineering WA School of Mines:MineralsEnergy and Chemical EngineeringCurtin UniversityWAAustralia School of Architecture and Design Jiangxi University of Science and TechnologyGanzhou341000China School of Resources and Architectural Engineering Gannan University of Science and TechnologyGanzhou341000China School of Chemical Engineering and Advanced Materials The University of AdelaideAdelaideSA5005Australia School of Resource and Environmental Engineering Jiangxi University of Science and TechnologyGanzhou341000China

With the development of the economy and the increasing demand for environmental protection,the efficient and selective recovery of Gd(Ⅲ)from actual wastewater is of critical *** this work,lanthanum-based metal-organic framework(LaBDC)materials were prepared by a hydrothermal method,and then polyethyleneimine(PEI)and LaBDC were combined by an impregnation method to form a novel LaBDC@xPEI *** prepared materials were characterized using Fourier transfo rm infrared spectroscopy(FTIR),X-ray diffraction(XRD),scanning electron microscopy(SEM),energy dispersive X-ray spectroscopy(EDX),B runauer-Emmett-Teller(BET),thermogravimetric analysis(TGA)and X-ray photoelectron spectroscopy(XPS).Experiments show that LaBDC@50%PEI has the highest adsorption capacity(181.77 mg/g)among lanthanum-based MOFs with different PEI loadings at pH=5.5,which is about 5.1 times that of bare *** adsorption isotherm analysis shows that LaBDC@50%PEI follows the Langmuir *** addition,the adsorption kinetics of LaBDC@50%PEI follows a pseudo-second-order kinetic model,indicating that the adsorption process is chemical *** is worth noting that LaBDC@50%PEI maintains good adsorption performance and stability after three recycling tests,and exhibits excellent selectivity in cation interference ***,the LaBDC@50%PEI composites possess good stability and hold great promises in rapid recovery of Gd(Ⅲ)from practical aqueous environments.

关键词： Wet-impregnation method Polyethylene imine Metaleorganic frameworks Lanthanum Recovery of Gd(Ⅲ) Rare earths

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Plasmonic Ag nanoparticles decorated MIL-101(Fe) for enhanced photocatalytic degradation of bisphenol A with peroxymonosulfate under visible-light irradiation

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Chinese Chemical Letters 2024年第1期35卷 418-423页

作者： Yan Gong Yu Ding Qi Tang Fei Lian Chun Bai Ruiyi Xie Haijiao Xie Xu Zhao School of Energy and Environmental Engineering Hebei University of TechnologyTianjin 300401China Hangzhou Yanqu Information Technology Co. Ltd.Hangzhou 310003China Key Laboratory of Drinking Water Science and Technology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Collapse

Photocatalytic activation of peroxymonosulfate (PMS) has garnered a lot of interest in the field of wastewater treatment. Herein, a plasmonic Ag nanoparticles decorated MIL-101(Fe) hybrid was synthesized through a photodeposition process. Upon light irradiation, the Ag/MIL-101(Fe) exhibit reinforced photocatalytic activities for elimination of bisphenol A (BPA) with PMS. The optimized 2.0% Ag/MIL-101(Fe) composite presented the highest photocatalytic activity with kinetic constant k of 0.102 min-1, which was about 10-fold of the pristine MIL-101(Fe). Loading of plasmonic Ag into MIL-101(Fe) boosts photoinduced carrier separation and accelerates PMS activation to generate strong oxidative radicals. Photoelectrochemical tests and multiple spectroscopic studies confirmed the promoted charge carrier separation and transfer capability of Ag/MIL-101(Fe). Combining the results of radical trapping experiments and electron spin resonance (ESR), the formed SO4·-, ·OH, ·O2- and 1O2 had a significant role in the photocatalytic process. According to intermediate study, the degradation pathway was studied, and the possible mechanism was proposed.

关键词： Photocatalysis MOF Peroxymonosulfate Plasmonic Ag BPA

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Investigating the effect of volatility on the hygroscopicities of acetate nanoparticle aerosols by surface plasmon resonance microscopy

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Journal of environmental sciences 2024年第4期138卷 167-178页

作者： Bo Yang Zhibo Xie Jianguo Liu Huaqiao Gui Jiaoshi Zhang Xiuli Wei Zetao Fan Douguo Zhang Key Laboratory of Environmental Optics and Technology Anhui Institute of Optics and Fine MechanicsHefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China University of Science and Technology of China Hefei 230026China CAS Center for Excellence in Regional Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China Advanced Laser Technology Laboratory of Anhui Province Department of Optics and Optical EngineeringUniversity of Science and Technology of ChinaHefei 230026China

Under high relative humidity(RH)conditions,the release of volatile components(such as acetate)has a significant impact on the aerosol *** this work,one surface plasmon resonance microscopy(SPRM)measurement system was introduced to determine the hygroscopic growth factors(GFs)of three acetate aerosols separately or mixed with glucose at different *** Ca(CH_(3)COO)_(2) or Mg(CH_(3)COO)_(2) aerosols,the hygroscopic growth trend of each time was lower than that of the previous time in three cyclic humidification from 70% RH to 90% RH,which may be due to the volatility of acetic acid leading to the formation of insoluble hydroxide(Ca(OH)_(2) or Mg(OH)_(2))under high RH *** the third calculated GF(using the Zdanovskii-Stokes-Robinson method)for Ca(CH_(3)COO)_(2) or Mg(CH_(3)COO)_(2) in bicomponent aerosols with 1:1 mass ratio were 3.20% or 5.33% lower than that of the first calculated GF at 90% *** calculated results also showed that the hygroscopicity change of bicomponent aerosol was negatively correlated with glucose content,especially when the mass ratio of Mg(CH_(3)COO)_(2) to glucose was 1:2,the GF at 90% RH only decreased by4.67% after three cyclic *** coupled plasma atomic emission spectrum(ICP-AES)based measurements also indicated that the changes of Mg^(2+)concentration in bicomponent was lower than that of the *** results of this study reveal thatduring the efflorescence transitions of atmospheric nanoparticles,the organic acids diffusion rate may be inhibited by the coating effect of neutral organic components,and the particles aging cycle will be prolonged.

关键词： Hygroscopic growth Volatility Acetate aerosols Nanoparticle aerosol Surface plasmon resonance

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Photodegradation of hydroxyfluorenes in ice and water: A comparison of kinetics, effects of water constituents, and phototransformation by-products

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Journal of environmental sciences 2023年第2期124卷 139-145页

作者： Linke Ge Shengkai Cao Crispin Halsall Junfeng Niu Dongxiao Bai Guangkai He Peng Zhang Hongrui Ma School of Environmental Science and Engineering Shaanxi University of Science&TechnologyXi’an 710021China Lancaster Environment Centre Lancaster UniversityLancaster LA14YQUK State Environmental Protection Key Laboratory of Coastal Ecosystem National Marine Environmental Monitoring CenterDalian 116023China

The photochemical behavior of organic pollutants in ice is poorly studied in comparison to aqueous *** we report a detailed comparison of ice and aqueous photodegradation of two representative OH-PAHs,2-hydroxyfluorene(2-OHFL)and 9-hydroxyfluorene(9-OHFL),which are newly recognized contaminants in the wider environment including colder ***,their photodegradation kinetics were clearly influenced by whether they reside in ice or *** the same simulated solar irradiation(λ>290 nm),OHFLs photodegraded faster in ice than in equivalent aqueous solutions and this was attributed to the specific concentration effect caused by ***,the presence of dissolved constituents in ice also influenced photodegradation with 2-OHFL phototransforming the fastest in‘seawater’ice(k=(11.4±1.0)×10^(−2) min^(−1))followed by‘pure-water’ice((8.7±0.4)×10^(−2) min^(−1))and‘freshwater’ice((8.0±0.7)×10^(−2) min^(−1)).The presence of dissolved constituents(specifically Cl^(−),NO_(3)^(−),Fe(Ⅲ)and humic acid)influences the phototransformation kinetics,either enhancing or suppressing phototransformation,but this is based on the quantity of the constituent present in the matrixes,the specific OHFL isomer and the matrix type(e.g.,ice or aqueous solution).Careful derivation of key photointermediates was undertaken in both ice and water samples using tandem mass *** phototransformation exhibited fewer by-products and‘simpler’pathways giving rise to a range of hydroxylated fluorenes and hydroxylated fluorenones in *** results are of importance when considering the fate of PAHs and OH-PAHs in cold regions and their persistence in sunlit ice.

关键词： Ice photochemistry Hydroxyfluorene Photodegradation Kinetics Water constituents Intermediates

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Belief reliability modeling and analysis for planetary reducer considering multi-source uncertainties and wear

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Journal of Systems engineering and Electronics 2021年第5期32卷 1246-1262页

作者： LI Yun JIANG Kaige ZENG Ting CHEN Wenbin LI Xiaoyang LI Deyong ZHANG Zhiqiang Beijing Spacecraft Manufacturing Co. LtdChina Academy of Space TechnologyBeijing 100094China School of Reliability and Systems Engineering Beihang UniversityBeijing 100191China Science and Technology on Reliability and Environmental Engineering Laboratory Beijing 100191China

The planetary reducer is a common type of transmission mechanism,which can provide high transmission accuracy and has been widely used,and it is usually required with high reliability of transmission characteristics in *** the manufacturing and usage stages of planetary reducers,uncertainties are ubiquitous and wear is inevitable,which affect the transmission characteristics and the reliability of planetary *** this paper,belief reliability modeling and analysis considering multi-uncertainties and wear are proposed for planetary ***,based on the functional principle and the influence of wear,the performance margin degradation model is established using the hysteresis error as the key performance parameter,where the degradation is mainly caused by the accumulated *** that,multi-source uncertainties are analyzed and quantified separately,including manufacturing errors,uncertainties in operational and environmental conditions,and uncertainties in performance ***,the belief reliability model is established based on the performance margin degradation model.A case study of a planetary reducer is applied and the reliability sensitivity analysis is implemented to show the practicability of the proposed *** results show that the proposed method can provide some suggestions to the design and manufacturing phases of the planetary reducer.

关键词： belief reliability planetary reducer performance margin wear multi-source uncertainty

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Exploring the mechanism of a novel cationic surfactant in bastnaesite flotation via the integration of DFT calculations,in-situ AFM and electrochemistry

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International Journal of Mining science and technology 2024年第10期34卷 1475-1484页

作者： Chang Liu Longhua Xu Jiushuai Deng Zhiguo Han Yi Li Jiahui Wu Jia Tian Donghui Wang Kai Xue Jinmei Fang School of Chemical&Environmental Engineering China University of Mining&Technology(Beijing)Beijing 100083China Key Laboratory of Solid Waste Treatment and Resource Recycle Ministry of Education Southwest University of Science and TechnologyMianyang 621010China State Key Laboratory of Mineral Processing Beijing 100160China

Effectively separating bastnaesite from calcium-bearing gangue minerals(particularly calcite)presents a formidable challenge,making the development of efficient collectors *** achieve this,we have designed and synthesized a novel,highly efficient,water-soluble cationic collector,N-dodecylisopropanolamine(NDIA),for use in the bastnaesite-calcite flotation *** functional theory(DFT)calculations identified the amine nitrogen atom in NDIA as the site most susceptible to electrophilic attack and electron *** introducing an OH group into the traditional collector dodecylamine(DDA)structure,NDIA provided additional adsorption sites,enabling synergistic adsorption on the surface of bastnaesite,thereby significantly enhancing both the floatability and selectivity of these *** recovery of bastnaesite was 76.02%,while the calcite was 1.26%.The NDIA markedly affected the zeta potential of bastnaesite,while its impact on calcite was relatively *** Fourier-transform infrared spectroscopy(FTIR)and X-ray photoelectron spectroscopy(XPS)results elucidated that the―NH―and―OH groups in NDIA anchored onto the bastnaesite surface through robust electrostatic and hydrogen bonding interactions,thereby enhancing bastnaesite's affinity for ***,in situ atomic force microscopy(AFM)provided conclusive evidence of NDIA aggregation on the bastnaesite surface,improving contact angle and hydrophobicity,and significantly boosting the flotation recovery of bastnaesite.

关键词： Novel cationic surfactant DFT calculation Bastnaesite Electrochemistry In-situ AFM

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Stable partial nitrification was achieved for nitrogen removal from municipal wastewater by gel immobilization:A pilot-scale study

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Journal of environmental sciences 2025年第5期151卷 529-539页

作者： Xin Hu Hong Yang Xiaoyue Fang Xuyan Liu Jiawei Wang Xiaotong Wang Yongsheng Bai Bojun Su Key Laboratory of Beijing for Water Quality Science and Water Environmental Recovery Engineering Faculty of ArchitectureCivil and Transportation EngineeringBeijing University of TechnologyBeijing 100124China Beijing General Municipal Engineering Design&Research Institute Co. Ltd.Beijing 100044China Hebei GEO University Shijiazhuang 050031China Hebei Key Laboratory of Water Quality Engineering and Comprehensive Utilization of Water Resources Hebei University of ArchitectureZhangjiakou 075000China School of Environmental Science and Safety Engineering Tianjin University of TechnologyTianjin 300384China Beijing Drainage Group Co.Ltd. Beijing 100022China

As an energy and carbon saving process for nitrogen removal from wastewater,the partial nitrification and denitrification process(PN/D)has been extensively ***,achieving stable PNinmunicipalwastewater has always been *** this study,a gel immobilized PN/D nitrogen removal process(GI-PN/D)was established.A 94 days pilot-scale experiment was conducted using real municipal wastewater with an ammonia concentration of 43.5±5.3mg N/L at a temperature range of 11.3–28.7◦*** nitrogen removal performance and associated pathways,shifts in the microbial community as well as sludge yield were *** results were as follows:the effluent TN and COD were 0.6±0.4mg/L and 31.1±3.8 mg/L respectively,and the NAR exceeding 95%.GI-PN/D achieved deep nitrogen removal ofmunicipalwastewater through stable PN without taking any *** primary pathways for nitrogen removal were identified as denitrification,simultaneous nitrification-denitrification,and aerobic ***-throughput sequencing analysis revealed that the immobilized fillers facilitated the autonomous enrichment of functional bacteria in each reactor,effectively promoting the dominance and stability of the microbial *** addition,GI-PN/D had the characteristic of low sludge yield,with an average sludge yield of 0.029 kg SS/kg *** study provides an effective technical for nitrogen removal from municipal wastewater through PN.

关键词： Gel immobilization Partial nitrification Deep nitrogen removal Autonomous enrichment Sludge yield

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Rational design of metal-metal hydroxide interface for efficient electrocatalytic oxidation of biomass-derived platform molecules

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Chinese Journal of Structural Chemistry 2025年第1期44卷 10-12页

作者： Yuchen Wang Zhenhao Xu Kai Yan Guangdong Provincial Key Laboratory of Environmental Pollution Control and Remediation Technology School of Environmental Science and EngineeringSun Yat-Sen UniversityGuangzhou510275China CAS Key Laboratory of Renewable Energy Guangzhou Institute of Energy ConversionGuangzhou510640China

With the acceleration of global industrialization,the human society has an increasing demand for high-value *** chemicals are mostly derived from non-renewable fossil fuels,causing inevitable energy shortage and accompanied environmental pollution issues during the conversion processes[1].Recently,biomass-derived platform molecules with abundant source,low price,and variable chemical structure have attracted tremendous attention from researchers,and their catalytic oxidation has become a promising route to reduce the dependence of fossil fuels and alleviate the harmful impact of environmental pollution for the production of high-value chemicals[2].

关键词： rational design metal metal hydroxide interface energy shortage electrocatalytic oxidation catalytic oxidation environmental pollution global industrialization biomass derived platform molecules

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