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17th Unified International Technical Conference on Refractories, UNITECR 2022

作者： Borges, O.H. dos Santos, T. Salvini, V.R. Pandolfelli, V.C. Federal University of Sao Carlos Graduate Program in Materials Science and Engineering SP Sao Carlos Brazil FIRE Associate Laboratory SP Sao Carlos Brazil Jordão Borghetti Street 480 SP Sertãozinho14160-050 Brazil

Aiming at reducing the remarkable shrinkage observed when porous ceramics are fired, the in-situ formation of hibonite (also known as CaO·6Al2O3 or CA6) was evaluated in a direct-foamed alumina-based macroporous thermal insulator with the addition of distinct calcium sources and contents. Among the tested compositions, that containing 12.9 wt% of CaCO3 showed promising results as high porosity (~ 80 %), no shrinkage after firing at 1600 ºC for 5 h, suitable mechanical strength, and a 200 ºC-lower strengthening temperature. However, the in-situ formation of CA6 took place just at high temperatures (~ 1600 ºC), implying a high energy consumption. To address this issue, SiO2, ZnO, and TiO2 were evaluated as mineralizing agents. The addition of 2.8 mol% of TiO2 induced CA6 formation at 1300ºC and low thermal conductivity (0.54 Wm-1K-1 at 1200 ºC), without significant changes in the refractoriness. © 2022 Unified International Technical Conference on Refractories, UNITECR 2022 - Proceedings. All rights reserved.

关键词： Titanium dioxide

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Conformity Experiment on Inelastic Scattering Exponent of Electrons in Two Dimensions

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Physical Review Letters 2024年第9期133卷 096302页

作者： Ching-Chen Yeh Pin-Chi Liao Yanfei Yang Wei-Chen Lin Alireza R. Panna Albert F. Rigosi Randolph E. Elmquist Chi-Te Liang Gaithersburg Maryland 20899 USA Department of Physics Graphene Waves Germantown Maryland 20876 USA Taiwan International Graduate Program Department of Engineering and System Science Center for Quantum Science and Engineering (CQSE) Taiwan Consortium of Emergent Crystalline Materials (TCECM) Taipei 106 Taiwan

The quantum Hall (QH) effect is one of the most widely studied physical phenomenon in two dimensions. The plateau-plateau transition within this effect can be comprehensively described by the scaling theory, which encompasses three pivotal exponents: the critical exponent κ, the inelastic scattering exponent p, and the universal exponent γ. Prior studies have focused on measuring κ and estimating γ, assuming a constant p value of 2 across magnetic fields. Here, our work marks a significant advancement by measuring all three exponents within a single graphene device and a conventional two-dimensional electron system. This study uniquely determines p at low magnetic fields (weak localization region and well outside the QH regime) and high magnetic fields (in the vicinity of the QH regime). Employing a comprehensive analytical approach that includes weak localization, plateau-plateau transitions, and variable range hopping, we have directly determined κ, p, and γ. Our findings reveal a distinct variation in p, shifting from 1 in the low magnetic field regime to 2 in the QH regime in graphene.

关键词： Electrical properties Fermions Landau levels Quantum interference effects Quantum phase transitions

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Intelligent micro/nanorobots for improved tumor therapy

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BMEMat(BioMedical engineering materials) 2023年第2期1卷 62-77页

作者： Zhaoli Sun Yanglong Hou Beijing Key Laboratory for Magnetoelectric Materials and Devices(BKL-MMD) School of Materials Science and EngineeringPeking UniversityBeijingChina Peking University-Tsinghua University-National Institute of Biological Sciences Joint Graduate Program School of Life SciencesPeking UniversityBeijingChina

A major bottleneck underlying nanomaterial-based tumor therapy lies in complex biological environment and physiological ***/nanorobots with the features of self-propulsion and controllable navigation have gradually become a research hotspot in the tumor therapeutic community,exhibiting their advantages in efficient cargo loading,controllable cargo delivery,stimulitriggered cargo release,deeper tumor tissue penetration,and enhanced cargo accumulation in tumor *** this review,the self-propulsion and controllable navigation are introduced as two major properties of micro/nanorobots,in which micro/nanorobots are propelled by chemical reactions,physical fields,and biological systems and could be navigated by chemotaxis,remote magnetic guidance,and ***,the recent advances of micro/nanorobots for chemotherapy,immunotherapy,photothermal therapy,photodynamic therapy,chemodynamic therapy,and multimodal tumor therapy would be ***,the perspective and challenges are also *** is expected that this review gives an insight into intelligent micro/nanorobots for improved tumor therapy,aiming for more extensive and in-depth investigations,and final applications in the clinic.

关键词： intelligent motion micro/nanorobots tumor therapy

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A comparative study of the structural and optoelectronic properties of Al- and Ga-doped ZnO films deposited by atmospheric pressure plasma jet

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Journal of Alloys and Compounds 2025年 1031卷

作者： Chou, Chih-Yun Chiu, Po-Han Chao, Yin-Chun Yen, Hung-Wei Juang, Jia-Yang Program in Nanoengineering and Nanoscience Graduate School of Advanced Technology National Taiwan University Taipei106319 Taiwan Department of Materials Science and Engineering National Taiwan University Taipei106319 Taiwan Department of Mechanical Engineering National Taiwan University Taipei106319 Taiwan

The high cost of gallium has driven interest in aluminum-doped zinc oxide (AZO) as a cost-effective alternative to gallium-doped zinc oxide (GZO). While prior studies have primarily focused on sputtering methods to compare AZO and GZO, research on non-sputtering techniques remains limited. Our previous works demonstrated favorable optoelectronic properties in GZO films deposited via atmospheric pressure plasma jet (APPJ);however, APPJ-deposited AZO has yet to be explored. In this study, we compare AZO and GZO thin films fabricated by APPJ under ambient conditions. We find that the deposition rate of AZO is approximately twice that of GZO under the same processing parameters, due to differences in droplet size from the ultrasonic generator. By adjusting precursor delivery and working distance (the nozzle-to-substrate gap), we can tune film thickness, morphology, and optoelectronic properties, showcasing APPJ's versatility over sputtering. Despite similar precursor concentrations and film thickness, AZO films exhibit lower carrier concentration (∼1 ×1020 cm–3) and mobility (∼7.5 cm2/Vs) than GZO (∼8 ×1020 cm–3 and ∼15 cm²/Vs), attributed to reduced aluminum incorporation (∼0.4 at% vs. ∼2.2 at% in GZO). Reducing the working distance from 2 mm to 1.5 mm improves both films’ structural integrity and optoelectronic performance (figure of merit increases by 140 % for GZO and 100 % for AZO). However, AZO remains inferior to GZO, highlighting the need for further optimization. © 2025 Elsevier B.V.

关键词： Transparent conducting oxides

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Nonsaturated large magnetoresistance and transport dynamics in a n-doped cryogenic WSe2 field-effect device

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Physical Review B 2025年第12期111卷 125307-125307页

作者： Wei-Chen Lin Ching-Chen Yeh Jia-Zhu Zou Nhat Anh Nguyen Phan Inayat Uddin Hai Yen Le Thi Kenji Watanabe Takashi Taniguchi Gil-Ho Kim Department of Engineering and System Science National Tsing Hua University Hsinchu 300 Taiwan Taiwan International Graduate Program Academia Sinica Taipei 115 Taiwan Department of Physics National Taiwan University Taipei 106 Taiwan Department of Electrical and Computer Engineering Sungkyunkwan University (SKKU) Suwon 164 Republic of Korea Sungkyunkwan Advanced Institute of Nano Technology (SAINT) Sungkyunkwan University (SKKU) Suwon 16419 Republic of Korea Research Center for Electronic and Optical Materials National Institute for Materials Science 1-1 Namiki Tsukuba 305-0044 Japan Research Center for Materials Nanoarchitectonics National Institute for Materials Science 1-1 Namiki Tsukuba 305-0044 Japan

Interest in the two-dimensional (2D) semiconducting transition metal dichalcogenides (TMDs) continues to intensify, driven by their suitable band gaps to supplant silicon as next-generation semiconductor materials. Among various TMDs, tungsten diselenide (WSe2) is renowned for its superior electrical properties in carrier density and mobility under ambient conditions. Despite its notable attributes, the behavior of monolayer WSe2 in the electron-doped regime under cryogenic conditions remains largely uncharted, particularly concerning its magnetotransport properties. In this study, we reveal the transport mechanisms of monolayer WSe2 from high temperatures down to the cryogenic regime. As evident by Efros–Shklovskii variable-range hopping (E-S VRH) in the cryogenic regime, strong Coulomb interactions arise between electrons. Above 8 K, an uncommon nonsaturated quadratic large magnetoresistance (MR) can be explained by the wave-function shrinkage model, which is consistent with the E-S VRH transport mechanism. Notably, the nonsaturated quadratic large MR shows a magnitude up to 1740% at 13 T. These findings underscore the potential applications for monolayer WSe2 in cryogenic field-effect devices, magnetic sensors, and memory devices and mark a significant advance in magnetotransport research.

关键词： Monolayers

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An ultra thin,bright,and sensitive interactive tactile display based on organic mechanoluminescence for dual-mode handwriting identification

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InfoMat 2024年第6期6卷 76-87页

作者： Tingting Hou Wenlang Li Haoyu Wang Yuantian Zheng Chaojie Chen Haoran Zhang Kai Chen Huilin Xie Xin Li Shaoshuai He Siwei Zhang Dengfeng Peng Cheng Yang Jacky W.Y.Lam Ben Zhong Tang Yunlong Zi Department of Mechanical and Automation Engineering The Chinese University of Hong KongHong Kongthe People's Republic of China Department of Chemistry Hong Kong Branch of Chinese National Engineering Research Center for Tissue Restoration and Reconstruction and Institute for Advanced StudyThe Hong Kong University of Science and TechnologyHong Kongthe People's Republic of China Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province College of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhenthe People's Republic of China Thrust of Sustainable Energy and Environment The Hong Kong University of Science and Technology(Guangzhou)Guangzhouthe People's Republic of China The Hong Kong University of Science and Technology Interdisciplinary Program Office Hong Kong SARthe People's Republic of China Institute of Materials Research Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhenthe People's Republic of China School of Science and Engineering Shenzhen Institute of Aggregate Science and TechnologyThe Chinese University of Hong KongShenzhenthe People's Republic of China HKUST Shenzhen-Hong Kong Collaborative Innovation Research Institute Shenzhenthe People's Republic of China Guangzhou HKUST Fok Ying Tung Research Institute Guangzhouthe People's Republic of China

Visible light-based human–machine interactive media is capable of transmitting electrical readouts to machines and providing intuitive feedback to users ***,many inorganic mechanoluminescent(ML)materials-based interactive media,typically ZnS-loaded phosphors(ZLPs),have been successfully ***,organic ML materials-based solutions were rarely exploited despite their huge merits of strong structural modification,abundant luminescence property,low cost,easy preparation,and so ***,we propose a novel interactive tactile display(ITD)based on organic ML materials(Cz-A6-dye)and triboelectric nanogenerator,with ultra-brightness(130%enhancement)and ultra-low threshold pressure(57%reduction)as compared to *** proposed ITD achieves the conversion of weak mechanical stimuli into visible light and electrical signals simultaneously,without extra power ***,the relationship between the luminous performance of organic ML materials and mechanical force is quantified,benefiting from the uniform ML layer *** by convolutional neural networks,the high-accuracy recognition(97.1%)for handwriting and identity of users is realized at the same ***,the ITD has great potential for intelligent wearable electronics and classified military applications.

关键词： interactive media organic mechanoluminescence triboelectric nanogenerators

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Synthesis of Nanostructured Sphere-Like Copper Oxide by Microwave Spray Pyrolysis

SSRN

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SSRN 2023年

作者： Cancellieri, Igor C. Perdomo, Claudia P.F. Muche, Dereck Ferreira N. Cordeiro, Marco A.L. Gunnewiek, Rodolfo Foster Klein Graduate Program in Materials Science and Engineering Federal University of São Carlos rod. Washington Luis s/n São Carlos13565-905 Brazil

CuO/Cu2O microspheres were synthesized via rapid microwave-assisted spray pyrolysis within only 20 minutes, requiring no additional treatment. The microspheres, with an average size of 577 ± 192 nm, consist of nanostructured primary particles (crystallites) measuring 17.9 ± 2.8 nm. X-ray diffraction analysis confirmed the presence of well-crystallized phases, revealing significant lattice distortion in Cu2O. The material exhibited a bandgap of 1.28 eV, rendering it suitable for applications in photoelectrochemistry and photocatalysis. © 2023, The Authors. All rights reserved.

关键词： Copper oxides

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Techno-economic and life-cycle assessment of electrochemical captured CO2 conversion process in monoethanolamine

Techno-economic and life-cycle assessment of electrochemical...

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2022 AIChE Annual Meeting

作者： Lee, Suhyun Choi, Woong Kim, Jae Hyung Hwang, Yun Jeong Na, Jonggeol Ewha Womans University School of Chemical Engineering and Materials Science Korea Republic of Ewha Womans University Graduate program in System Health Science and Engineering Korea Republic of Clean Energy Research Center Korea Institute of Science and Technology Korea Republic of Seoul National University School of Chemistry Korea Republic of Korea Republic of Ewha Womans University Dept. of Chemical Engineering & Material science Advanced Manufacturing Systems Laboratory Korea Republic of

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Solidification, A-Al Morphologies, Tensile Properties and Plc of Low-Sc Modified Al-Mg Alloys

SSRN

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SSRN 2023年

作者： Nunes, Anderson Thadeu Lisboa de Gouveia, Guilherme Spinelli, José Eduardo Federal University of São Carlos Graduate Program in Materials Science and Engineering SP São Carlos13565905 Brazil Department of Materials Engineering Federal University of São Carlos – UFSCar SP São Carlos13565905 Brazil

Al alloys are very attractive in engineering applications that require a combination of low density and mechanical strength, such as in aeronautical and aerospace industry devices. Therefore, the search for alloys with higher specific strength is justified from environmental and economic points of view. This work aims to study the influence of cooling rates on the phase morphology and tensile properties of ternary Al-Mg-Sc alloys, whose composition covers the spectrum of low-Sc Al-Mg-Sc alloys. The ternary Al-3, -5, and -10wt.% Mg-0.1wt.% Sc alloys were processed by transient directional solidification. This process induces a wide range of cooling rates which causes the formation of a microstructural variety along the longitudinal cooling direction and, consequently, different tensile properties. Several characterization methods were employed, including: thermal analysis, x-ray diffraction (XRD) structural analysis, SEM-EDS, optical microscopy, CALPHAD, tensile tests, and fractography. Two major findings should be noted after fully characterizing the microstructures, the formed phases, and the tensile properties. Solidification evolution revealed that more Mg added resulted in higher solidification rates due to higher fluidity with more Mg. Furthermore, cell growth was mapped in the three alloy compositions while competing with dendrites. Second, although the Al-10 wt.% Mg-Sc alloy had more Mg in solid solution and slightly higher Portevin–Le Chatelier (PLC) severity, the Al-5 wt.% Mg-Sc alloy showed superior tensile strength due to the predominance of cells and thinner primary dendrites trunks forming its microstructure. © 2023, The Authors. All rights reserved.

关键词： Aluminum alloys

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Thermal-Protective and Oxygen-Resistant Nanocoating Using Silica-Nanocomposites for Laser Thinning of Polymorphic Molybdenum Ditellurides

SSRN

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SSRN 2023年

作者： Heo, Soyoung Kim, Seulbi Lee, Seung Yeon Yang, Heejun Park, Ji Hun Cho, Suyeon Division of Chemical Engineering and Materials Science Graduate Program in System Health Science and Engineering Ewha Womans University Seoul03760 Korea Republic of Department of Science Education Ewha Womans University Seoul03760 Korea Republic of Daejeon34141 Korea Republic of

Laser irradiation has been investigated as a method of fabricating atomically-thin crystals from layered two-dimensional (2D) materials with precise thickness control. However, during laser irradiation, inevitable structural changes can occur in the 2D materials due to the high thermal energy, altering their physical and chemical properties and introducing disorder, which has hindered the study and use of the intrinsic properties of atomically-thin materials. In this study, we report a laser thinning method using a new coating material, a layered silica-based nanocomposite (SNC), that preserves the pristine crystal structure of a polymorphic 2D material, MoTe2, down to an atomically thin geometry. The nano-porous coating of layered silica-based nanocomposite (SNC) was robust against thermal heating and behaved as a good thermal-protective and oxygen-resistant material in the laser thinning process. Therefore, the SNC-coated MoTe2 flakes were successfully thinned down to atomically-thin geometry, while preserving their 2H structure. Accordingly, our SNC coating of 2D materials is a promising way to engineer the phase and geometry of polymorphic 2D materials, enabling versatile applications in various optoelectronic, spintronic, and electronic devices. © 2023, The Authors. All rights reserved.

关键词： Coatings

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