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arXiv 2020年

作者： Arlı, Cihan Kocabaş, Tugbey Çakır, Deniz Sevik, Cem Department of Materials Science and Engineering Institute of Graduate Program Eskisehir Technical University Eskiehir TR26555 Turkey Department of Physics and Astrophysics University of North Dakota Grand ForksND58202 United States Department of Mechanical Engineering Faculty of Engineering Eskisehir Technical University Eskiehir TR26555 Turkey

The rational design of two-dimensional piezoelectric materials has recently garnered increasing interest because of harnessing these materials in technological applications, including sensor technology, actuating devices, energy harvesting, and medical applications. Several materials possessing high piezoelectric response have been reported so far, but a high-throughput first-principles approach to estimate the piezoelectric potential of layered materials has not been performed yet. In this respect, we systematically investigated the piezoelectric (e11, d11) and elastic (C11 and C12) properties of 108 thermodynamically stable two-dimensional (2D) semiconductor materials by employing first-principle methods. Our calculations found a notable difference between the relaxed ion coefficients calculated with GGA and LDA functionals, indicating a strong exchange-correlation functional dependence. Nevertheless, both functionals yield the same trends for the elastic constants and piezoelectric coefficients. Our high-throughput approach demonstrates that the materials containing Group-V elements produce notably high piezoelectric strain constants, d11 > 40 pmV−1, and 42 of considered materials have the e11 coefficient higher than MoS2 insomuch as BrSSb has one of the largest d11 with a value of 503.6 pmV−1. Besides, we established simple empirical models to estimate the d11 coefficients by utilizing the relative ionic motion in the unit cell and the polarizability of the individual elements in the compounds. The proposed models, tested for both exchange-correlation functionals, are successful in estimating the piezoelectric constants of the studied materials with sufficient accuracy. Copyright © 2020, The Authors. All rights reserved.

关键词： Piezoelectricity

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Double affinity ligands modified graphene enabled orientation-controllable cryo-EM sample preparation

Double affinity ligands modified graphene enabled orientatio...

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第七届全国冷冻电子显微学与结构生物学专题研讨会

作者：程航 Liming Zheng Nan Liu Jie Xu Congyuan Huang Ye Lu Hailin Peng Yanan Chen Hong-Wei Wang Ministry of Education Key Laboratory of Protein Sciences Beijing Advanced Innovation Center for Structural BiologySchool of Life SciencesTsinghua University Tsinghua-Peking Joint Center for Life Sciences Tsinghua University Center for Nanochemistry Beijing Science and Engineering Center for NanocarbonsBeijing National Laboratory for Molecular SciencesCollege of Chemistry and Molecular EngineeringPeking University Joint Graduate Program of Peking-Tsinghua-NIBS School of Life SciencesTsinghua University Academy for Advanced Interdisciplinary Studies Peking University School of Materials Science and Engineering Tianjin University Beijing Frontier Research Center for Biological Structures Tsinghua University

With the development of both hardwares and softwares of cryo-electron microscopy (cryo-EM),high- resolution structures of macromolecules have been increasingly ***,the robustness and generality of this technique are severely challenged by the air-water interface and preferred orientation issues during specimen preparation,which practically take plenty of efforts to overcome,especially for those hard *** we reported double-modified graphene (DMG) as the supporting material in cryo-EM sample preparation by covalently modified graphene membrane with two different affinity ligands,

关键词： DMG Double affinity ligands modified graphene enabled orientation-controllable cryo-EM sample preparation

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Alternation of Magnetic Anisotropy Accompanied by Metal-Insulator Transition in Strained Ultrathin Manganite Heterostructures

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Physical Review Applied 2021年第6期15卷 064019-064019页

作者： Masaki Kobayashi Le Duc Anh Masahiro Suzuki Shingo Kaneta-Takada Yukiharu Takeda Shin-ichi Fujimori Goro Shibata Arata Tanaka Masaaki Tanaka Shinobu Ohya Atsushi Fujimori Department of Electrical Engineering and Information Systems The University of Tokyo 7-3-1 Hongo Bunkyo-ku Tokyo 113-8656 Japan Center for Spintronics Research Network The University of Tokyo 7-3-1 Hongo Bunkyo-ku Tokyo 113-8656 Japan Institute of Engineering Innovation Graduate School of Engineering The University of Tokyo 7-3-1 Hongo Bunkyo-ku Tokyo 113-8656 Japan PRESTO JST 4-1-8 Honcho Kawaguchi Saitama 332-0012 Japan Department of Physics The University of Tokyo 7-3-1 Hongo Bunkyo-ku Tokyo 113-0033 Japan Materials Sciences Research Center Japan Atomic Energy Agency Sayo-gun Hyogo 679-5148 Japan Department of Applied Physics Tokyo University of Science Katsushika Tokyo 125-8585 Japan Quantum Matter Program Graduate School of Advanced Science and Engineering Hiroshima University Higashi-Hiroshima 739-8530 Japan Department of Applied Physics Waseda University Okubo Shinjuku Tokyo 169-8555 Japan

A fundamental understanding of the interfacial magnetic properties in ferromagnetic heterostructures is essential for utilizing ferromagnetic materials for spintronic device applications. Here, we investigate the interfacial magnetic and electronic structures of epitaxial single-crystalline LaAlO3(LAO)/La0.6Sr0.4MnO3(LSMO)/Nb:SrTiO3(Nb:STO) heterostructures with varying LSMO layer thicknesses, in which the magnetic anisotropy strongly changes with the LSMO thickness due to the delicate balance between strains originating from both the Nb:STO and LAO layers, using x-ray magnetic circular dichroism and photoemission spectroscopy. We successfully detect the clear change of the magnetic behavior of the Mn ions concomitant with the thickness-dependent metal-insulator transition. Our results suggest that the double-exchange interaction induces ferromagnetism in the metallic LSMO film under tensile strain caused by the STO substrate, while the superexchange interaction determines the magnetic behavior in the insulating LSMO film under compressive strain originating from the top LAO layer. The change in strain, depending on LSMO layer thickness, is confirmed by scanning transmission electron microscopy. Based on those findings, the formation of a magnetic dead layer near the LAO/LSMO interface is attributed to competition between the superexchange interaction via Mn 3d3z2−r2 orbitals under compressive strain and the double-exchange interaction via the 3dx2−y2 orbitals. These findings provide key aspects of ferromagnetic oxide heterostructures for the development of spintronic device applications.

关键词： Electronic structure Ferromagnetism Magnetic anisotropy Metal-insulator transition Spintronics Transition metal oxides Photoemission spectroscopy X-ray magnetic circular dichroism

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Photonic analog of bilayer graphene

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Physical Review B 2021年第21期103卷 214311-214311页

作者： Mourad Oudich Guangxu Su Yuanchen Deng Wladimir Benalcazar Renwen Huang Nikhil J. R. K. Gerard Minghui Lu Peng Zhan Yun Jing Graduate Program in Acoustics The Pennsylvania State University University Park Pennsylvania 16802 USA Université de Lorraine CNRS Institut Jean Lamour F-54000 Nancy France National Laboratory of Solid State Microstructures Collaborative Innovation Center of Advanced Microstructures Nanjing University Nanjing 210093 China School of Physics Nanjing University Nanjing 210093 China Department of Physics The Pennsylvania State University University Park Pennsylvania 16801 USA Department of Mechanical and Aerospace Engineering North Carolina State University Raleigh North Carolina 27695 USA Department of Materials Science and Engineering Nanjing University Nanjing Jiangsu 210093 China

Drawing inspiration from bilayer graphene, this paper introduces its photonic analog comprising two stacked graphenelike photonic crystals that are coupled in the near field through spoof surface plasmons. Beyond the twist degree of freedom that can radically alter the band structure of the bilayer photonic graphene, the photonic dispersion can be also tailored via the interlayer coupling which exhibits an exponential dependence on the distance between the two photonic crystals. We theoretically, numerically, and experimentally characterize the band structures of AA- and AB-stacked bilayer photonic graphene, as well as for twisted bilayer photonic graphene with even and odd sublattice exchange symmetries. Furthermore, we numerically predict the existence of magic angles in bilayer photonic graphene, which are associated with ultraflat bands resulting from interlayer hybridization. Finally, we demonstrate that the bilayer photonic graphene at a particular twist angle satisfying even sublattice exchange symmetry is a high-order photonic topological insulator. The proposed bilayer photonic graphene could constitute a useful platform for identifying new quantum materials and inspiring next-generation photonic devices with new degrees of freedom and emerging functionality.

关键词： Photonic crystals Plasmonics Surface plasmons

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Spectral evidence for unidirectional charge density wave in detwinned BaNi2As2

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Physical Review B 2023年第8期108卷 L081104-L081104页

作者： Yucheng Guo Mason Klemm Ji Seop Oh Yaofeng Xie Bing-Hua Lei Luca Moreschini Cheng Chen Ziqin Yue Sergey Gorovikov Tor Pedersen Matteo Michiardi Sergey Zhdanovich Andrea Damascelli Jonathan Denlinger Makoto Hashimoto Donghui Lu Chris Jozwiak Aaron Bostwick Eli Rotenberg Sung-Kwan Mo Rob G. Moore Junichiro Kono Robert J. Birgeneau David J. Singh Pengcheng Dai Ming Yi Department of Physics and Astronomy Rice University Houston Texas 77005 USA Advanced Light Source Lawrence Berkeley National Laboratory Berkeley California 94720 USA Department of Physics University of California Berkeley California 94720 USA Department of Physics and Astronomy University of Missouri Columbia Missouri 65211 USA Materials Science Division Lawrence Berkeley National Laboratory Berkeley California 94720 USA Department of Physics University of Oxford Oxford OX1 3PU United Kingdom Applied Physics Graduate Program Smalley-Curl Institute Rice University Houston Texas 77005 USA Canadian Light Source Inc. 44 Innovation Boulevard Saskatoon SK S7N 2V3 Canada Department of Physics and Astronomy University of British Columbia Vancouver British Columbia V6T 1Z1 Canada Quantum Matter Institute University of British Columbia Vancouver British Columbia V6T 1Z4 Canada Max Planck Institute for Chemical Physics of Solids Nöthnitzer Straße 40 01187 Dresden Germany Stanford Synchrotron Radiation Lightsource SLAC National Accelerator Laboratory Menlo Park California 94025 USA Materials Science and Technology Division Oak Ridge National Laboratory Oak Ridge Tennessee 37831 USA Department of Electrical and Computer Engineering Rice University Houston Texas 77005 USA Smalley-Curl Institute Rice University Houston Texas 77005 USA Department of Materials Science and NanoEngineering Rice University Houston Texas 77005 USA Department of Chemistry University of Missouri Columbia Missouri 65211 USA

In the iron-based superconductors, unconventional superconductivity emerges in proximity to intertwined electronic orders consisting of an electronic nematic order and a spin density wave (SDW). Recently, BaNi2As2, like its well-known iron-based analog BaFe2As2, has been discovered to host a symmetry-breaking structural transition but coupled to a unidirectional charge density wave (CDW) instead of SDW, providing a novel platform to study intertwined orders. Here, through a systematic angle-resolved photoemission spectroscopy study combined with a detwinning B1g uniaxial strain, we identify distinct spectral evidence of band evolution due to the structural transition as well as CDW-induced band folding. In contrast to the nematicity and spin density wave in BaFe2As2, the structural and CDW order parameters in BaNi2As2 are observed to be strongly coupled and do not separate in the presence of uniaxial strain. Furthermore, no nematic band splitting is resolved above the structural transition. Our measurements point to a likely lattice origin of the CDW order in BaNi2As2.

关键词： Charge density waves Nematic phase transition Iron-based superconductors Angle-resolved photoemission spectroscopy

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Electron Transfer Enhanced by a Minimal Energetic Driving Force at the Organic-Semiconductor Interface

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Angewandte Chemie 2024年第37期136卷

作者： Hiroto Iwasaki Keisuke Fujimoto Koki Banno Qing-jun Shui Yutaka Majima Masaki Takahashi Seiichiro Izawa Laboratory for Materials and Structures Tokyo Institute of Technology 4259 Nagatsuta-cho Midori-ku Yokohama Kanagawa 226-8503 Japan Applied Chemistry Program Graduate School of Advanced Science and Engineering Hiroshima University 1-4-1 Kagamiyama Higashi-Hiroshima Hiroshima 739-8527 Japan Department of Applied Chemistry Faculty of Engineering Shizuoka University 3-5-1 Johoku Chuo-ku Hamamatsu Shizuoka 432-8561 Japan Precursory Research for Embryonic Science and Technology (PRESTO) Japan Science and Technology Agency (JST) 4-1-8 Honcho Kawaguchi Saitama 332-0012 Japan

The energetic driving force for electron transfer must be minimized to realize efficient optoelectronic devices including organic light-emitting diodes (OLEDs) and organic photovoltaics (OPVs). Exploring the dynamics of a charge-transfer (CT) state at an interface leads to a comprehension of the relationship between energetics, electron-transfer efficiency, and device performance. Here, we investigate the electron transfer from the CT state to the triplet excited state (T 1 ) in upconversion OLEDs with 45 material combinations. By analyzing the CT emission and the singlet excited-state emission from triplet–triplet annihilation via the dark T 1 , their energetics and electron-transfer efficiencies are extracted. We demonstrate that the CT→T 1 electron transfer is enhanced by the stronger CT interaction and a minimal energetic driving force (<0.1 eV), which is explained using the Marcus theory with a small reorganization energy of <0.1 eV. Through our analysis, a novel donor–acceptor combination for the OLED is developed and shows an efficient blue emission with an extremely low turn-on voltage of 1.57 V. This work provides a solution to control interfacial CT states for efficient optoelectronic devices without energy loss.

关键词： electron transfer Marcus theory organic optoelectronic devices organic light-emitting diodes organic photovoltaics

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Localized growth drives spongy mesophyll morphogenesis

arXiv

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arXiv 2022年

作者： Treado, John D. Roddy, Adam B. Théroux-Rancourt, Guillaume Zhang, Liyong Ambrose, Chris Brodersen, Craig Shattuck, Mark D. O’Hern, Corey S. Department of Mechanical Engineering & Materials Science Integrated Graduate Program in Physical and Engineering Biology Yale University New HavenCT06520 United States Institute of Environment Department of Biological Sciences Florida International University MiamiFL33199 United States University of Natural Resources and Life Sciences Vienna Department of Integrative Biology and Biodiversity Research Institute of Botany Vienna1180 Austria Department of Biology College of Arts and Science University of Saskatchewan SaskatoonS7N 5E2 Canada School of the Environment Yale University New HavenCT06520 United States Department of Physics Benjamin Levich Institute City College of New York New YorkNY10031 United States Department of Physics Department of Applied Physics Yale University New HavenCT06520 United States

The spongy mesophyll is a complex, porous tissue found in plant leaves that enables carbon capture and provides mechanical stability. Unlike many other biological tissues, which remain confluent throughout development, the spongy mesophyll must develop from an initially confluent tissue into a tortuous network of cells with a large proportion of intercellular airspace. How the airspace in the spongy mesophyll develops while the cells remain mechanically stable remains unknown. Here, we used computer simulations of deformable particles to develop a purely mechanical model for the development of the spongy mesophyll tissue. By stipulating that (1) cell perimeter grows only near voids, (2) cells both form and break adhesive bonds, and (3) the tissue pressure remains constant, the computational model was able to recapitulate the developmental trajectory of the microstructure of the spongy mesophyll observed in Arabidopsis thaliana leaves. Robust generation of pore space in the spongy mesophyll requires a balance of cell growth, adhesion, stiffness and tissue pressure to ensure cell networks remain both porous yet mechanically robust. The success of this mechanical model of tissue growth and porosity evolution suggests that simple physical principles can coordinate and drive the development of complex plant tissues like the spongy mesophyll. © 2022, CC BY.

关键词： Tissue

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Plasma-Derived Nanoclusters for Site-Specific Multimodality Photo/Magnetic Thrombus Theranostics

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Advanced Healthcare materials 2023年第28期12卷 e2301504页

作者： Liu, Chia-Hung Liu, Ming-Che Jheng, Pei-Ru Yu, Jiashing Fan, Yu-Jui Liang, Jia-Wei Hsiao, Yu-Cheng Chiang, Chih-Wei Bolouki, Nima Lee, Jyh-Wei Hsieh, Jang-Hsing Mansel, Bradley W Chen, Yan-Ting Nguyen, Hieu Trung Chuang, Er-Yuan Department of Urology School of Medicine College of Medicine Taipei Medical University 250 Wu-Hsing Street Taipei11031 Taiwan TMU Research Center of Urology and Kidney Taipei Medical University 250 Wu-Hsing Street Taipei11031 Taiwan Department of Urology Shuang Ho Hospital Taipei Medical University 291 Zhongzheng Road Zhonghe District New Taipei City23561 Taiwan Clinical Research Center Taipei Medical University Hospital Taipei11031 Taiwan School of Dental Technology College of Oral Medicine Taipei Medical University Taipei11031 Taiwan Graduate Institute of Biomedical Materials and Tissue Engineering International Ph.D. Program in Biomedical Engineering Graduate Institute of Biomedical Optomechatronics School of Biomedical Engineering Research Center of Biomedical Device Innovation Entrepreneurship Education Center College of Interdisciplinary Studies Taipei Medical University Taipei11031 Taiwan Department of Chemical Engineering College of Engineering National Taiwan University Taipei106 Taiwan Department of Orthopedics Taipei Medical University Taipei11031 Taiwan Department of Orthopedics Taipei Medical University Hospital Taipei11031 Taiwan Department of Physical Electronics Faculty of Science Masaryk University Brno60177 Czech Republic Department of Materials Engineering Ming Chi University of Technology New Taipei City24301 Taiwan Center for Plasma and Thin Film Technologies Ming Chi University of Technology New Taipei City24301 Taiwan National Synchrotron Radiation Research Center Hsinchu Science Park Hsinchu30076 Taiwan Department of Orthopedics and Trauma Faculty of Medicine University of Medicine and Pharmacy at Ho Chi Minh City Ho Chi Minh City700000 Viet Nam Cell Physiology and Molecular Image Research Center Taipei Medical University Wan Fang Hospital Taipei11696 Taiwan Precision Medicine and Translational Cancer Research Center Taipei Medical University Hospital Taipei11031 Taiwan

Traditional thrombolytic therapeutics for vascular blockage are affected by their limited penetration into thrombi, associated off-target side effects, and low bioavailability, leading to insufficient thrombolytic efficacy. It is hypothesized that these limitations can be overcome by the precisely controlled and targeted delivery of thrombolytic therapeutics. A theranostic platform is developed that is biocompatible, fluorescent, magnetic, and well-characterized, with multiple targeting modes. This multimodal theranostic system can be remotely visualized and magnetically guided toward thrombi, noninvasively irradiated by near-infrared (NIR) phototherapies, and remotely activated by actuated magnets for additional mechanical therapy. Magnetic guidance can also improve the penetration of nanomedicines into thrombi. In a mouse model of thrombosis, the thrombosis residues are reduced by ≈80% and with no risk of side effects or of secondary embolization. This strategy not only enables the progression of thrombolysis but also accelerates the lysis rate, thereby facilitating its prospective use in time-critical thrombolytic treatment. © 2023 Wiley-VCH GmbH.

关键词： Diseases

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Dielectric Modulation of Two-Dimensional Dipolar materials

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Physical Review Letters 2019年第9期123卷 096101-096101页

作者： Ziwei Wang Erik Luijten Graduate Program in Applied Physics Northwestern University Evanston Illinois 60208 USA Departments of Materials Science & Engineering Engineering Sciences & Applied Mathematics and Physics & Astronomy Northwestern University Evanston Illinois 60208 USA

Spontaneous pattern formation plays an important role in a wide variety of natural phenomena and materials systems. A key ingredient for the occurrence of modulated phases is the presence of competing interactions, generally of different physical origins. We demonstrate that in dipolar films, a prototypical system for pattern formation, patterns can be induced by dielectric effects alone. A rich phase diagram arises, where striped and circular morphologies emerge with geometric properties that can be controlled through variation of particle shape and substrate permittivity or permeability. These effects are particularly enhanced by metamaterial substrates.

关键词： Classical statistical mechanics Dielectrics Electric polarization Pattern formation 2-dimensional systems Interfaces Monte Carlo methods

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Magic-angle bilayer phononic graphene

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Physical Review B 2020年第18期102卷 180304(R)-180304(R)页

作者： Yuanchen Deng Mourad Oudich Nikhil JRK Gerard Jun Ji Minghui Lu Yun Jing Graduate Program in Acoustics Penn State University University Park Pennsylvania 16802 USA Université de Lorraine CNRS Institut Jean Lamour F-54000 Nancy France Department of Mechanical and Aerospace Engineering North Carolina State University Raleigh North Carolina 27695 USA National Laboratory of Solid State Microstructures and Department of Materials Science and Engineering Nanjing University Nanjing Jiangsu 210093 China

Thanks to the recent discovery of the magic-angle bilayer graphene, twistronics is quickly becoming a burgeoning field in condensed matter physics. This Rapid Communication expands the realm of twistronics to acoustics by introducing twisted bilayer phononic graphene, which remarkably also harbors the magic angle, evidenced by the associated ultraflat bands. Beyond mimicking quantum-mechanical behaviors of twisted bilayer graphene, we show that their acoustic counterpart offers a considerably more straightforward and robust way to alter the interlayer hopping strength, enabling us to unlock magic angles (>3∘) inaccessible in classical twisted bilayer graphene. This study not only establishes the acoustical analog of twisted (magic-angle) bilayer graphene, providing a test bed more easily accessible to probe the interaction and misalignment between stacked two-dimensional materials, but also points out the direction to a new phononic crystal design paradigm that could benefit applications such as enhanced acoustic emission and sensing.

关键词： Acoustic wave phenomena Mechanical & acoustical properties Phonons Acoustic metamaterials Metamaterials

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