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Charge and spin degrees of freedom in A-site ordered YCu3Co4O12 and CaCu3Co4O12

Physical Review B 2021年第11期103卷 115149-115149页

作者： Yi-Ying Chin Zhiwei Hu Yuichi Shimakawa Junye Yang Youwen Long A. Tanaka Liu Hao Tjeng Hong-Ji Lin Chien-Te Chen Department of Physics National Chung Cheng University Chiayi 62102 Taiwan Max Planck Institute for Chemical Physics of Solids Nöthnitzer Strasse 40 01187 Dresden Germany Institute for Chemical Research Kyoto University Kyoto 611-0011 Japan Beijing National Laboratory for Condensed Matter Physics Institute of Physics Chinese Academy of Sciences Beijing 100190 China Songshan Lake Materials Laboratory Dongguan Guangdong 523808 China Quantum Matter Program Graduate School of Advanced Science and Engineering Hiroshima University Higashi-hiroshima 739-8530 Japan National Synchrotron Radiation Research Center (NSRRC) 101 Hsin-Ann Road Hsinchu 30076 Taiwan

Using soft x-ray absorption spectroscopy we were able to determine unambiguously the charge and spin states of the transition metal ions in stoichiometric YCu3Co4O12 and CaCu3Co4O12. The trivalent and low-spin nature of both the Cu and Co ions in YCu3Co4O12 makes this correlated system to be effectively a nonmagnetic band semiconductor. The substitution of Y by Ca produces formally tetravalent Co ions but the doped holes are primarily on the oxygen ligands. Concerning the spin degrees of freedom, the trivalent Co ions in YCu3Co4O12 remain low spin upon the Y-Ca substitution, very much unlike the La1−xSrxCoO3 system. The tetravalent Co ions in CaCu3Co4O12 are interestingly also in the low-spin state, which then explains the good electrical conductivity of CaCu3Co4O12 since charge exchange between neighboring Co3+ and Co4+ ions will not be hampered by the spin-blockade mechanism that otherwise would be in effect if the Co4+ and Co3+ spin quantum numbers were to differ by more than one-half. We infer that the stability of the Co low-spin state is related to the very short Co-O bond lengths.

关键词： Electrical conductivity Oxides Strongly correlated systems X-ray absorption spectroscopy

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Correction to: N‑doped carbon nanospheres as selective fluorescent probes for mercury detection in contaminated aqueous media: chemistry, fluorescence probing, cell line patterning, and liver tissue interaction

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Environmental science and pollution research international 2025年第20期32卷 2025 May 6页

作者： Soheil Sojdeh Ali Banitalebi Dehkordi Alireza Badiei Ali Zarrabi Pooyan Makvandi Milad Ashrafizadeh Mohammad Reza Saeb Eder C Lima Mohammad Rabiee Mohsen Asadnia Thomas J Webster Navid Rabiee School of Chemistry College of Science University of Tehran P.O. Box Tehran 14155‑6455 Iran. Department of Biomedical Engineering Faculty of Engineering and Natural Sciences Istinye University Istanbul Turkey. Centre for Materials Interfaces Istituto Italiano Di Tecnologia 56025 Pisa Italy. Sabanci University Orta Mahalle Üniversite Caddesi No. 27 Orhanlı Tuzla 34956 Istanbul Turkey. Department of Polymer Technology Gdańsk University of Technology G. Narutowicza 11/12 80‑233 Gdańsk Poland. Institute of Chemistry Federal University of Rio Grande Do Sul (UFRGS) Av. Bento Goncalves 9500 Postal Box 15003 Porto Alegre ZIP 91501‑970 Brazil. profederlima@***. Biomaterials Group Department of Biomedical Engineering Amirkabir University of Technology Tehran Iran. School of Engineering Macquarie University New South Wales Sydney 2109 Australia. School of Health Sciences and Biomedical Engineering Hebei University of Technology Tijian 300130 China. School of Engineering Saveetha University Chennai 602105 India. Interdisciplinary Laboratory for Advanced Materials (LIMAV) Materials Science and Engineering Graduate Program Federal University of Piaui Teresina 64049‑550 Brazil. Centre for Molecular Medicine and Innovative Therapeutics Murdoch University Perth 6150 Australia.

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Chiral Phonons with Giant Magnetic Moments in a Topological Crystalline Insulator

arXiv

引用

arXiv 2022年

作者： Hernandez, Felix G.G. Baydin, Andrey Chaudhary, Swati Tay, Fuyang Katayama, Ikufumi Takeda, Jun Nojiri, Hiroyuki Okazaki, Anderson K. Rappl, Paulo H.O. Abramof, Eduardo Rodriguez-Vega, Martin Fiete, Gregory A. Kono, Junichiro Instituto de Física Universidade de São Paulo SP São Paulo05508-090 Brazil Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Physics The University of Texas at Austin AustinTX78712 United States Department of Physics Northeastern University BostonMA02115 United States Department of Physics Massachusetts Institute of Technology CambridgeMA02139 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Physics Graduate School of Engineering Science Yokohama National University Yokohama240-8501 Japan Institute for Materials Research Tohoku University Sendai980-8577 Japan Instituto Nacional de Pesquisas Espaciais SP São José dos Campos12201-970 Brazil Department of Physics and Astronomy Rice University HoustonTX77005 United States Department of Material Science and NanoEngineering Rice University HoustonTX77005 United States

We have studied the magnetic response of transverse optical phonons in Pb1−xSnxTe films. Polarization-dependent terahertz magnetospectroscopy measurements revealed Zeeman splittings and diamagnetic shifts, demonstrating that these phonon modes become chiral in magnetic fields. Films in the topological crystalline insulator phase (x > 0.32) exhibited magnetic moment values that are larger than those for topologically trivial films (x Copyright © 2022, The Authors. All rights reserved.

关键词： Phonons

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Correction to: SARS-CoV-2 removal with a polyurethane foam composite

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Environmental science and pollution research international 2023年第8期30卷 22033页

作者： Guilherme Pereira Schoeler Thays França Afonso Carolina Faccio Demarco Victor Dos Santos Barboza Tito Roberto Sant'anna Cadaval Andrei Valerão Igansi Marcos Alexandre Gelesky Janice Luehring Giongo Rodrigo de Almeida Vaucher Rafael de Avila Delucis Robson Andreazza Postgraduate Program in Environmental Sciences Center for Engineering Federal University of Pelotas R. Benjamin Constant 989 Pelotas RS CEP 96010-020 Brazil. Postgraduate Program in Materials Science and Engineering Federal University of Pelotas R. Gomes Carneiro 01 Pelotas RS CEP 96010-610 Brazil. Graduate Program in Biochemistry and Bioprospecting Research Laboratory in Biochemical and Molecular Biology of Microorganisms (LaPeBBiOM) Federal University of Pelotas RS Av. Eliseu Maciel Campus Universitário s/n Capão Do Leão CEP 96160-000 Brazil. School of Chemistry and Food Federal University of Rio Grande Av. Itália Km 8 s/n Rio Grande RS CEP 96203-000 Brazil. Postgraduate Program in Environmental Sciences Center for Engineering Federal University of Pelotas R. Benjamin Constant 989 Pelotas RS CEP 96010-020 Brazil. robsonandreazza@yahoo.com.br. Postgraduate Program in Materials Science and Engineering Federal University of Pelotas R. Gomes Carneiro 01 Pelotas RS CEP 96010-610 Brazil. robsonandreazza@yahoo.com.br.

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The bulk van der Waals layered magnet CrSBr is a quasi-1D material

arXiv

引用

arXiv 2022年

作者： Klein, Julian Pingault, Benjamin Florian, Matthias Heißenbüttel, Marie-Christin Steinhoff, Alexander Song, Zhigang Torres, Kierstin Dirnberger, Florian Curtis, Jonathan B. Weile, Mads Penn, Aubrey Deilmann, Thorsten Dana, Rami Bushati, Rezlind Quan, Jiamin Luxa, Jan Sofer, Zdenek Alù, Andrea Menon, Vinod M. Wurstbauer, Ursula Rohlfing, Michael Narang, Prineha Lončar, Marko Ross, Frances M. Department of Materials Science and Engineering Massachusetts Institute of Technology CambridgeMA02139 United States John A. Paulson School of Engineering and Applied Sciences Harvard University CambridgeMA02138 United States QuTech Delft University of Technology Delft2600 GA Netherlands Department of Electrical and Computer Engineering Department of Physics University of Michigan Ann ArborMI48109 United States Institut für Festkörpertheorie Westfälische Wilhelms-Universität Münster Münster48149 Germany Institut für Theoretische Physik Universität Bremen P.O. Box 330 440 Bremen28334 Germany Bremen Center for Computational Materials Science University of Bremen Bremen28359 Germany Department of Physics City College of New York New YorkNY10031 United States College of Letters and Science UCLA Los AngelesCA90095 United States Department of Physics Technical University of Denmark Kgs. LyngbyDK-2800 Denmark MIT.nano Massachusetts Institute of Technology CambridgeMA02139 United States Department of Physics The Graduate Center City University of New York New YorkNY10016 United States Photonics Initiative CUNY Advanced Science Research Center New YorkNY10031 United States Physics Program Graduate Center City University of New York New YorkNY10026 United States Department of Inorganic Chemistry University of Chemistry and Technology Prague Technická 5 Prague 6166 28 Czech Republic Institute of Physics Center for Nanotechnology University of Münster Münster48149 Germany

Correlated quantum phenomena in one-dimensional (1D) systems that exhibit competing electronic and magnetic order are of strong interest for studying fundamental interactions and excitations, such as Tomonaga-Luttinger liquids and topological orders and defects with properties completely different from the quasiparticles expected in their higher-dimensional counterparts. However, clean 1D electronic systems are difficult to realize experimentally, particularly magnetically ordered systems. Here, we show that the van der Waals layered magnetic semiconductor CrSBr behaves like a quasi-1D material embedded in a magnetically ordered environment. The strong 1D electronic character originates from the Cr-S chains and the combination of weak interlayer hybridization and anisotropy in effective mass and dielectric screening with an effective electron mass ratio of meX/meY ∼ 50. This extreme anisotropy experimentally manifests in strong electron-phonon and exciton-phonon interactions, a Peierls-like structural instability and a Fano resonance from a van Hove singularity of similar strength of metallic carbon nanotubes. Moreover, due to the reduced dimensionality and interlayer coupling, CrSBr hosts spectrally narrow (1 meV) excitons of high binding energy and oscillator strength that inherit the 1D character. Overall, CrSBr is best understood as a stack of weakly hybridized monolayers and appears to be an experimentally attractive candidate for the study of exotic exciton and 1D correlated many-body physics in the presence of magnetic order. Copyright © 2022, The Authors. All rights reserved.

关键词： Excitons

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Kramers Nodal Lines and Weyl Fermions in SmAlSi

arXiv

引用

arXiv 2022年

作者： Zhang, Yichen Gao, Yuxiang Gao, Xue-Jian Lei, Shiming Ni, Zhuoliang Oh, Ji Seop Huang, Jianwei Yue, Ziqin Zonno, Marta Gorovikov, Sergey Hashimoto, Makoto Lu, Donghui Denlinger, Jonathan D. Birgeneau, Robert J. Kono, Junichiro Wu, Liang Law, Kam Tuen Morosan, Emilia Yi, Ming Department of Physics and Astronomy Rice University HoustonTX77005 United States Department of Physics Hong Kong University of Science and Technology Clear Water Bay Hong Kong Department of Physics and Astronomy University of Pennsylvania PhiladelphiaPA19104 United States Department of Physics University of California BerkeleyCA94720 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Canadian Light Source Inc. 44 Innovation Boulevard SaskatoonSKS7N 2V3 Canada Stanford Synchrotron Radiation Lightsource SLAC National Accelerator Laboratory 2575 Sand Hill Road Menlo ParkCA94025 United States Advanced Light Source Lawrence Berekeley National Laboratory BerkeleyCA94720 United States Materials Science Division Lawrence Berekeley National Laboratory BerkeleyCA94720 United States Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Department of Materials Science and Nanoengineering Rice University HoustonTX77005 United States

Kramers nodal lines (KNLs) have recently been proposed theoretically as a special type of Weyl line degeneracy connecting time-reversal invariant momenta. KNLs are robust to spin orbit coupling and are inherent to all non-centrosymmetric achiral crystal structures, leading to unusual spin, magneto-electric, and optical properties. However, their existence in in real quantum materials has not been experimentally established. Here we gather the experimental evidence pointing at the presence of KNLs in SmAlSi, a non-centrosymmetric metal that develops incommensurate spin density wave order at low temperature. Using angle-resolved photoemission spectroscopy, density functional theory calculations, and magneto-transport methods, we provide evidence suggesting the presence of KNLs, together with observing Weyl fermions under the broken inversion symmetry in the paramagnetic phase of SmAlSi. We discuss the nesting possibilities regarding the emergent magnetic orders in SmAlSi. Our results provide a solid basis of experimental observations for exploring correlated topology in SmAlSi. © 2022, CC BY-NC-SA.

关键词： Temperature

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The Ni isotopic composition of Ryugu reveals a common accretion region for carbonaceous chondrites

arXiv

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arXiv 2024年

作者： Spitzer, Fridolin Kleine, Thorsten Burkhardt, Christoph Hopp, Timo Yokoyama, Tetsuya Abe, Yoshinari Aléon, Jérôme OD. Alexander, Conel M. Amari, Sachiko Amelin, Yuri Bajo, Ken-Ichi Bizzarro, Martin Bouvier, Audrey Carlson, Richard W. Chaussidon, Marc Choi, Byeon-Gak Dauphas, Nicolas Davis, Andrew M. Rocco, Tommaso Di Fujiya, Wataru Fukai, Ryota Gautam, Ikshu Haba, Makiko K. Hibiya, Yuki Hidaka, Hiroshi Homma, Hisashi Hoppe, Peter Huss, Gary R. Ichida, Kiyohiro Iizuka, Tsuyoshi Ireland, Trevor R. Ishikawa, Akira Itoh, Shoichi Kawasaki, Noriyuki Kita, Noriko T. Kitajima, Kouki Komatani, Shintaro Krot, Alexander N. Liu, Ming-Chang Masuda, Yuki Morita, Mayu Moynier, Fréderic Motomura, Kazuko Nakai, Izumi Nagashima, Kazuhide Nguyen, Ann Nittler, Larry Onose, Morihiko Pack, Andreas Park, Changkun Piani, Laurette Qin, Liping Russell, Sara S. Sakamoto, Naoya Schönbächler, Maria Tafla, Lauren Tang, Haolan Terada, Kentaro Terada, Yasuko Usui, Tomohiro Wada, Sohei Wadhwa, Meenakshi Walker, Richard J. Yamashita, Katsuyuki Yin, Qing-Zhu Yoneda, Shigekazu Young, Edward D. Yui, Hiroharu Zhang, Ai-Cheng Nakamura, Tomoki Naraoka, Hiroshi Noguchi, Takaaki Okazaki, Ryuji Sakamoto, Kanako Yabuta, Hikaru Abe, Masanao Miyazaki, Akiko Nakato, Aiko Nishimura, Masahiro Okada, Tatsuaki Yada, Toru Yogata, Kasumi Nakazawa, Satoru Saiki, Takanao Tanaka, Satoshi Terui, Fuyuto Tsuda, Yuichi Watanabe, Sei-Ichiro Yoshikawa, Makoto Tachibana, Shogo Yurimoto, Hisayoshi Max Planck Institute for Solar System Research Justus-von-Liebig-Weg 3 Göttingen37077 Germany Department of Earth and Planetary Sciences Tokyo Institute of Technology Tokyo152-8551 Japan Graduate School of Engineering Materials Science and Engineering Tokyo Denki University Tokyo120-8551 Japan Institut de Minéralogie de Physique des Matériaux et de Cosmochimie Sorbonne Université Museum National d'Histoire Naturelle CNRS UMR 7590 IRD Paris75005 France Earth and Planets Laboratory Carnegie Institution for Science WashingtonDC20015 United States McDonnell Center for the Space Sciences and Physics Department Washington University 35 St. LouisMO63130 United States Geochemical Research Center The University of Tokyo Tokyo113-0033 Japan Guangzhou Institute of Geochemistry Chinese Academy of Sciences GD Guangzhou510640 China Departement of Natural History Sciences Hokkaido University Sapporo001-0021 Japan Centre for Star and Planet Formation Globe Institute University of Copenhagen Copenhagen1350 Denmark Bayerisches Geoinstitut Universität Bayreuth Bayreuth95447 Germany Université Paris Cité Institut de Physique du Globe de Paris CNRS Paris75005 France Department of Earth Science Education Seoul National University Seoul08826 Korea Republic of Department of the Geophysical Sciences Enrico Fermi Institute The University of Chicago 5734 South Ellis Avenue Chicago60637 United States Faculty of Geosciences and Geography University of Göttingen GöttingenD-37077 Germany Faculty of Science Ibaraki University Mito310-8512 Japan ISAS/JSEC JAXA Sagamihara252-5210 Japan Research Center for Advanced Science and Technology The University of Tokyo Tokyo153-8904 Japan Research Institute for Marine Resources Utilization Japan Agency for Marine-Earth Science and Technology Kanagawa237-0061 Japan Departement of Earth and Planetary Sciences Nagoya University Nagoya464-8601 Japan Osaka Application Laboratory SBUWDX Rigaku Corporation Osaka569-1

The isotopic compositions of samples returned from Cb-type asteroid Ryugu and Ivuna-type (CI) chondrites are distinct from other carbonaceous chondrites, which has led to the suggestion that Ryugu/CI chondrites formed in a different region of the accretion disk, possibly around the orbits of Uranus and Neptune. We show that, like for Fe, Ryugu and CI chondrites also have indistinguishable Ni isotope anomalies, which differ from those of other carbonaceous chondrites. We propose that this unique Fe and Ni isotopic composition reflects different accretion efficiencies of small FeNi metal grains among the carbonaceous chondrite parent bodies. The CI chondrites incorporated these grains more efficiently, possibly because they formed at the end of the disk’s lifetime, when planetesimal formation was also triggered by photoevaporation of the disk. Isotopic variations among carbonaceous chondrites may thus reflect fractionation of distinct dust components from a common reservoir, implying CI chondrites/Ryugu may have formed in the same region of the accretion disk as other carbonaceous chondrites. © 2024, CC BY.

关键词： Nickel

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A Photo- and Thermo-Driven Azoarene-Based Circularly Polarized Luminescence Molecular Switch in a Liquid Crystal Host

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Angewandte Chemie 2023年第48期135卷

作者： Wenxin Kang Yuqi Tang Xianyu Meng Siyang Lin Xinfang Zhang Prof. Jinbao Guo Prof. Quan Li Key Laboratory of Carbon Fibers and Functional Polymers Ministry of Education and College of Materials Science and Engineering Beijing University of Chemical Technology Beijing 100029 China Contribution: Investigation (lead) Writing - original draft (equal) Writing - review & editing (supporting) Institute of Advanced Materials and School of Chemistry and Chemical Engineering Southeast University Nanjing 211189 China Contribution: Investigation (supporting) Writing - original draft (supporting) Writing - review & editing (supporting) Materials Science Graduate Program Kent State University Kent OH 44242 USA Contribution: Conceptualization (equal) Funding acquisition (equal) Investigation (supporting) Project administration (lead) Writing - original draft (lead) Writing - review & editing (equal) Contribution: Conceptualization (equal) Funding acquisition (equal) Investigation (supporting) Supervision (lead) Writing - original draft (supporting) Writing - review & editing (equal)

The development of chiral optical active materials with switchable circularly polarized luminescence (CPL) signals remains a challenge. Here an azoarene-based circularly polarized luminescence molecular switch, ( S, R, S )-switch 1 and ( R, R, R )-switch 2 , are designed and prepared with an ( R )-binaphthyl azo group as a chiral photosensitive moiety and two ( S )- or ( R )-binaphthyl fluorescent molecules with opposite or the same handedness as chiral fluorescent moieties. Both switches exhibit reversible trans/cis isomerization when irradiated by 365 nm UV light and 520 nm green light in solvent and liquid crystal (LC) media. In contrast with the control ( R, R, R )-switch 2 , when switch 1 is doped into nematic LCs, polarization inversion and switching-off of the CPL signals are achieved in the resultant helical superstructure upon irradiation with 365 nm UV and 520 nm green light, respectively. Meanwhile, the fluorescence intensity of the system is basically unchanged during this switching process. In particular, these variations of the CPL signals could be recovered after heating, realizing the true sense of CPL reversible switching. Taking advantage of the unique CPL switching, the proof-of-concept for “a dual-optical information encryption system” based on the above CPL active material is demonstrated.

关键词： Chirality Inversion Cholesteric Liquid Crystal Circularly Polarized Luminescence Information Encryption Molecular Switch

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Correction: Characterizing country-specific human and ecosystem health impact and damage cost of agricultural pesticides: the case for Thailand

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The International Journal of Life Cycle Assessment 2022年第12期27卷 1377-1377页

作者： Mankong, Phatchari Fantke, Peter Phenrat, Tanapon Mungkalasiri, Jitti Gheewala, Shabbir H. Prapaspongsa, Trakarn Graduate Program in Environmental and Water Resources Engineering Department of Civil and Environmental Engineering Faculty of Engineering Mahidol University Nakhon Pathom Thailand Quantitative Sustainability Assessment Department of Environmental and Resource Engineering Technical University of Denmark Kongens Lyngby Denmark Department of Civil Engineering Faculty of Engineering Naresuan University Phitsanulok Thailand Technology and Informatics Institute for Sustainability (TIIS) National Metal and Materials Technology Center (MTEC) National Science and Technology Development Agency (NSTDA) Pathum Thani Thailand The Joint Graduate School of Energy and Environment (JGSEE) King Mongkut’s University of Technology Thonburi Bangkok Thailand Centre of Excellence On Energy Technology and Environment Ministry of Higher Education Science Research and Innovation Bangkok Thailand

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Sub-picosecond all-optical switching in a hybrid VO2:silicon waveguide at 1550 nm

arXiv

引用

arXiv 2020年

作者： Hallman, Kent A. Miller, Kevin J. Baydin, Andrey Weiss, Sharon M. Haglund, Richard F. Department of Physics and Astronomy Vanderbilt University NashvilleTN37235 United States Interdisciplinary Graduate Program in Materials Science NashvilleTN37235 United States Department of Electrical Engineering and Computer Science Vanderbilt University NashvilleTN37235 United States AEgis Technologies Group 410 Jan Davis Drive HuntsvilleAL35803 United States Department of Electrical and Computer Engineering Rice University HoustonTX70005 United States

Achieving ultrafast all-optical switching in a silicon waveguide geometry is a key milestone on the way to an integrated platform capable of handling the increasing demands for higher speed and higher capacity for information transfer. Given the weak electro-optic and thermo-optic effects in silicon, there has been intense interest in hybrid structures in which that switching could be accomplished by integrating another material into the waveguide, including the phase-changing material, vanadium dioxide (VO2). It has long been known that the phase transition in VO2 can be triggered by ultrafast laser pulses, and that pump-laser fluence is a critical parameter governing the recovery time of thin films irradiated by femtosecond laser pulses near 800 nm. However, thin-film experiments are not a priori reliable guides to using VO2 for all-optical switching in on-chip silicon photonics because of the large changes in VO2 optical constants in the telecommunications band, the requirement of low insertion loss, and the limits on switching energy permissible in integrated photonic systems. Here we report the first measurements to show that the reversible, ultrafast photo-induced phase transition in VO2 can be harnessed to achieve sub-picosecond switching when small VO2 volumes are integrated in a silicon waveguide as a modulating element. Switching energies above threshold are of order 600 fJ/switch. These results suggest that VO2 can now be pursued as a strong candidate for all-optical switching with sub-picosecond on-off times. Copyright © 2020, The Authors. All rights reserved.

关键词： Optical switches

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