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SSRN 2024年

作者： He, Shenggong Huang, Shimin Liu, Xinzhou Zeng, Xianggang Chen, Hedong Zhao, Lingzhi Noor, Hadia Hou, Xianhua Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials School of Physics South China Normal University Guangzhou510006 China Guangdong Engineering Technology Research Center of Efficient Green Energy and Environment Protection Materials School of Electronics and Information Engineering South China Normal University Foshan528225 China Centre of Excellence in Solid State Physics Faculty of Science University of the Punjab Lahore54590 Pakistan SCNU Qingyuan Institute of Science and Technology Innovation Co. Ltd. Qingyuan511517 China

For all-solid-state lithium-ion batteries (ASSLIBs), silicon (Si) stands out as an appealing anodes material due to its high energy density and improved safety compared to lithium metal. However, the substantial volume changes during cycling result in poor solid-state physical contact and electrolyte-electrode interface issues, leading to unsatisfactory electrochemical performance. In this study, we employed in-situ polymerization to construct an integrated Si anodes/self-healing polymer electrolyte for ASSLIBs. The polymer chain reorganization stems from numerous dynamic bonds in the constructed self-healing dynamic supermolecular elastomer electrolyte (SHDSE) molecular structure. Notably, SHDSE also serves as a Si anodes binder with enhanced adhesive capability. As a result, the well-structured Li|SHDSE|Si-SHDSE cell generates subtle electrolyte-electrode interface contacts at the molecular level, which can offer a continuous and stable Li+ transport pathway, reduce Si particle displacement, and mitigate electrode volume expansion. This further enhances cyclic stability (> 500 cycles with 68.1% capacity retention and > 99.8% Coulombic efficiency). More practically, the 2.0 Ah wave-shaped Si||LiCoO2 soft-pack battery with in-situ cured SHDSE exhibits strongly stabilized electrochemical performance (1.68 Ah after 700 cycles, 86.2% capacity retention) in spite of a high operating temperatures up to 100°C and in various bending tests. This represents a groundbreaking report in flexible solid-state soft-pack batteries containing Si anodes. © 2024, The Authors. All rights reserved.

关键词： solid-state Batteries

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Photon avalanche-driven multicolor emission: yttrium vanadate upconversion phosphors for optical thermometry, forensics, and healing light applications

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Chemical engineering Journal 2025年 516卷

作者： Pavitra, Eluri Antony, Lintymol Park, Jin Young Hwang, Seung Kyu Lee, Jeong-Hwan Chandra, Gogineni Rajesh Basaveswara Rao, M.V. Raju, Ganji Seeta Rama Han, Young-Kyu Huh, Yun Suk NanoBio High-Tech Materials Research Center Department of Biological Sciences and Bioengineering Inha University Incheon22212 Korea Republic of 3D Convergence Center Inha University Incheon22212 Korea Republic of Department of Energy and Materials Engineering Dongguk University-Seoul Seoul04620 Korea Republic of Department of Electrical Electronics and Software Engineering Pukyong National University Yongdang Campus Busan48547 Korea Republic of Department of Materials Science and Engineering Inha University Incheon22212 Korea Republic of Program in Semiconductor Convergence Inha University Incheon22212 Korea Republic of Department of Computer Science and Engineering Vignan's Lara Institute of Technology & Science Andhra Pradesh Guntur India Department of Chemistry Krishna University Andhra Pradesh Machillipatnam521001 India

The exploration of photon upconversion has led to the development of multifunctional lanthanide-based materials, particularly through the mechanism of photon avalanche, marking a transformative advancement in material science. In this study, yttrium vanadate upconversion nanocrystalline phosphors (UCNCPs) activated by Ho3+/Er3+/Tm3+/Yb3+ ions are reported. These UCNCPs demonstrate a remarkable ability in the photon avalanche, offering highly intense and tunable emissions across the visible spectrum at room temperature under low excitation power of 980 nm laser. The average number of photons involved in the UC process at threshold pump power, highlighting the intricate interplay of cross-relaxation and energy transfer loops in avalanche mechanism. Notably, these UCNCPs have shown exceptional temperature sensing capabilities, where non-thermally coupled levels of the Ho3+ and Tm3+ ions provide higher relative sensitivity and accuracy than thermally coupled levels of Er3+ ions. The versatility of these UCNCPs is further established by their application in solid-state lighting, where they can produce vibrant red, green, blue, and warm-white light, and in security, serving as multi-level anti-counterfeiting inks that respond to 980 nm laser illumination. These developments not only pave the way for more energy-efficient lighting solutions but also offer new avenues for enhancing the security of valuable items. The temperature sensing capabilities of these phosphors add another layer of functionality, making them ideal for high-tech applications ranging from medical diagnostics to environmental monitoring. © 2025 Elsevier B.V.

关键词： Phosphors

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Electrolyte Design for Robust Gradient solid-Electrolyte Interfaces to Enable High-Performance Silicon Anodes for Pouch Batteries

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SSRN 2024年

作者： He, Shenggong Huang, Shimin Liu, Xinzhou Zeng, Xianggang Chen, Hedong Zhao, Lingzhi Noor, Hadia Xianhua, Hou Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials School of Physics South China Normal University Guangzhou510006 China Guangdong Engineering Technology Research Center of Efficient Green Energy and Environment Protection Materials School of Electronics and Information Engineering South China Normal University Foshan528225 China Centre of Excellence in Solid State Physics Faculty of Science University of the Punjab Lahore54590 Pakistan SCNU Qingyuan Institute of Science and Technology Innovation Co. Ltd. Qingyuan511517 China

Silicon (Si) anodes has emerged as an ideal anode for the next generation of lithium-ion batteries owing to its high specific capacity. Nevertheless, Si particles undergo large volume expansion during cycling, inducing the continuous fragmentation/re-formation of the solid-electrolyte interphase (SEI) layer, which leads to rapid capacity decay and low Coulombic efficiency in EC-based carbonate electrolytes. Herein, a weakly solvating electrolyte with boric acid tris(hexafluoroisopropyl) Ester (BTHE), 2,2,2-trifluoroethyl methyl carbonate (FDEC), and fluoroethylene carbonate (FEC) is developed to build a stable SEI. BTHE is introduced as a functional solvent, which is induce anion and fluorinated solvent to form a gradient rigid–soft coupling SEI layer. In contrast to other anion-derived interfaces, weakly solvating electrolyte has been proven to construct a highly robust and stable –CF3-rich-organic outer layer and LiF-rich inner layer SEI on the Si anodes, resulting in approximately 99.9% ultra-high Coulombic efficiency and ultra-high areal capacity (~8.1 mAh cm-2). Beyond proof of concept, a 2.68 Ah Si||LiNi0.8Mn0.1Co0.1O2 pouch cell has an impressive 84.3% capacity retention after 1000 cycles and could work normally at temperatures ranging from −30 °C to 100 °C based on this electrolyte, representing a pioneering report in pouch cells incorporating Si anodes. © 2024, The Authors. All rights reserved.

关键词： Lithium-ion batteries

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Ultrathin, Lightweight, and Flexible CNT Buckypaper Enhanced Using MXenes for Electromagnetic Interference Shielding

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Nano-Micro Letters 2021年第4期13卷 208-220页

作者： Rongliang Yang Xuchun Gui Li Yao Qingmei Hu Leilei Yang Hao Zhang Yongtao Yao Hui Mei Zikang Tang State Key Laboratory of Optoelectronic Materials and Technologies School of Electronics and Information TechnologySun Yat-Sen UniversityGuangzhou 510275People’s Republic of China Science and Technology on Thermostructural Composite Materials Laboratory School of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072ShaanxiPeople’s Republic of China Instrumental Analysis and Research Center(IARC) Sun Yat-Sen UniversityGuangzhou 510275People’s Republic of China National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of TechnologyHarbin 150080People’s Republic of China Institute of Applied Physics and Materials Engineering University of MacaoTaipa 999078MacaoPeople’s Republic of China

Lightweight,flexibility,and low thickness are urgent requirements for next-generation high-performance electromagnetic interference(EMI)shielding materials for catering to the demand for smart and wearable electronic *** several efforts have focused on constructing porous and flexible conductive films or aerogels,few studies have achieved a balance in terms of density,thickness,flexibility,and EMI shielding effectiveness(SE).Herein,an ultrathin,lightweight,and flexible carbon nanotube(CNT)buckypaper enhanced using MXenes(Ti3C2Tx)for high-performance EMI shielding is synthesized through a facile electrophoretic deposition *** obtained Ti3C2Tx@CNT hybrid buckypaper exhibits an outstanding EMI SE of 60.5 dB in the X-band at 100μ*** hybrid buckypaper with an MXene content of 49.4 wt%exhibits an EMI SE of 50.4 dB in the X-band with a thickness of only 15μm,which is 105%higher than that of pristine CNT ***,an average specific SE value of 5.7×10^(4) dB cm^(2) g^(−1) is exhibited in the 5-μm hybrid ***,this assembly process proves promising for the construction of ultrathin,flexible,and high-performance EMI shielding films for application in electronic devices and wireless communications.

关键词： Carbon nanotube MXene Buckypaper Electromagnetic interference shielding

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Enhanced room-temperature Na^(+) ionic conductivity in Na_(4.92)Y_(0.92)Zr_(0.08)Si_(4)O_(12)

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escience 2023年第6期3卷 935-945页

作者： Aikai Yang Kai Yao Mareen Schaller Enkhtsetseg Dashjav Hang Li Shuo Zhao Qiu Zhang Martin Etter Xingchen Shen Huimin Song Qiongqiong Lu Ruijie Ye Igor Moudrakovski Quanquan Pang Sylvio Indris Xingchao Wang Qianli Ma Frank Tietz Jun Chen Olivier Guillon Forschungszentrum Jülich GmbH Institute of Energy and Climate ResearchMaterials Synthesis and Processing(IEK-1)52425 JülichGermany Institute of Mineral Engineering(GHI) RWTH Aachen UniversityForckenbeckstraße 3352074 AachenGermany Institute for Applied Materials-Energy Storage Systems(IAM-ESS) Karlsruhe Institute of Technology(KIT)76344 Eggenstein-LeopoldshafenGermany Renewable Energy Conversion and Storage Center(RECAST) Haihe Laboratory of Sustainable Chemical TransformationsKey Laboratory of Advanced Energy Materials Chemistry(Ministry of Education)College of ChemistryNankai UniversityTianjin 300071China Deutsches Elektronen-Synchrotron(DESY) Notkestrasse 8522607 HamburgGermany Laboratoire de Cristallographie et Sciences des Materiaux(CRISMAT) CNRSENSICAEN14000 CaenFrance Beijing Key Laboratory of Theory and Technology for Advanced Batteries Materials School of Materials Science and EngineeringPeking UniversityBeijing 100871China Institute of Materials Henan Academy of SciencesHenan Key Laboratory of Advanced Conductor MaterialsZhengzhou 450046China Max Planck Institute for Solid State Research Heisenbergstraße 170569 StuttgartGermany State Key Laboratory of Chemistry and Utilization of Carbon Based Energy Resources Key Laboratory of Advanced Functional MaterialsAutonomous RegionInstitute of Applied ChemistryCollege of ChemistryXinjiang UniversityUrumqiXinjiang 830046China Forschungszentrum Jülich GmbH Helmholtz Institute Münster(IEK-12)52425 JülichGermany Jülich Aachen Research Alliance JARA-Energy52425 JülichGermany

Developing cost-effective and reliable solid-state sodium batteries with superior performance is crucial for stationary energy storage.A key component in facilitating their application is a solid-state electrolyte with high conductivity and ***,we employed aliovalent cation substitution to enhance ionic conductivity while preserving the crystal *** substitution of Y^(3+)with Zr^(4+)in Na_(5)YSi_(4)O_(12) introduced Naþion vacancies,resulting in high bulk and total conductivities of up to 6.5 and 3.3 mS cm^(-1),respectively,at room temperature with the composition Na_(4.92)Y_(0.92)Zr_(0.08)Si_(4)O_(12)(NYZS).NYZS shows exceptional electrochemical stability(up to 10 V ***þ/Na),favorable interfacial compatibility with Na,and an excellent critical current density of 2.4 mA cm^(-2).The enhanced conductivity of Naþions in NYZS was elucidated using solid-state nuclear magnetic resonance techniques and theoretical simulations,revealing two migration routes facilitated by the synergistic effect of increased Naþion vacancies and improved chemical environment due to Zr^(4+)*** extends the list of suitable solid-state electrolytes and enables the facile synthesis of stable,low-cost Naþion silicate electrolytes.

关键词： solid-state electrolytes Sodium superionic conductors Na_(4.92)Y_(0.92)Zr_(0.08)Si_(4)O_(12) High conductivity Ultra-wide electrochemical window

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Continuous water-water hydrogen bonding network across the rim of carbon nanotubes facilitating water transport for desalination

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Nano research 2021年第7期14卷 2171-2178页

作者： Yaqi Hou Miao Wang Xinyu Chen Xu Hou State Key Laboratory of Physical Chemistry of Solid Surfaces College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005China College of Materials Xiamen UniversityXiamen 361005China Research Institute for Biomimetics and Soft Matter Fujian Provincial Key Laboratory for Soft Functional Materials ResearchJiujiang Research InstituteCollege of Physical Science and TechnologyXiamen UniversityXiamen 361005China Collaborative Innovation Center of Chemistry for Energy Materials Xiamen UniversityXiamen 361005China Tan Kah Kee Innovation Laboratory Xiamen 361102China CAS Key Laboratory of Bio-inspired Materials and Interfacial Sciences Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijing 100190China

The development of membranes featuring carbon nanotubes(CNTs)have provided possibilities of next-generation solar desalination *** solar desalination,the microstructures and interactions between the filter membrane and seawater play a crucial role in desalination *** the mechanisms of water evaporation and ion rejection in confined pores or channels is necessary to optimize the desalting ***,using non-equilibrium molecular dynamics simulations,we found that continuous water-water hydrogen bonding network across the rims of CNTs is the key factor in facilitating water transport through *** the continuous hydrogen bonding network,the water flux is two times of that without the continuous hydrogen bonding *** CNT arrays,each CNT transports water molecules and rejects salt ions *** on these observations,using CNT arrays consisted with densely packed thin CNTs is the most advisable strategy for evaporation desalination,possessing high transport flux as well as maintaining high salt rejection.

关键词： carbon nanotubes hydrogen bonding network facilitated water transport salt rejection desalination

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Mitigating Fast Thermal Instability by Engineered Laser Sweep in AIN Soliton Microcomb Generation

Mitigating Fast Thermal Instability by Engineered Laser Swee...

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Asia Communications and Photonics Conference and Exhibition (ACP)

作者： Zihao Wang Kewei Liu Shunyu Yao Yanan Guo Jianchang Yan Junxi Wang Changxi Yang Chengying Bao Department of Precision Instruments State Key Laboratory of Precision Measurement Technology and Instruments Tsinghua University Beijing China Center for Materials Science and Optoelectronics Engineering University of the Chinese Academy of Sciences Beijing China Research and Development Center for Solid State Lighting Institute of Semiconductors Chinese Academy of Sciences Beijing China

Transient thermal instability represents a significant challenge in generating soliton microcombs. Fast laser sweep can be an efficient method to mitigate thermal instability, but it would require ultrahigh laser sweep rate for crystalline microresonators with fast thermal relaxation. Here, we engineer the laser sweep waveform to generate AIN-on-sapphire soliton microcombs with an intermediate sweep speed $(< 30\text{GHz}/\mu \mathrm{s})$ . Two laser sweep methods with a backward + forward tuning or a two-step backward tuning added after the fast forward laser sweep are demonstrated to stabilize solitons.

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Synergistic Interface Layer Optimization and Surface Passivation with Fluorocarbon Molecules toward Efficient and Stable Inverted Planar Perovskite Solar Cells

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research 2021年第1期2021卷 1225-1235页

作者： Long Zhou Jie Su Zhenhua Lin Xing Guo Jing Ma Tao Li Jincheng Zhang Jingjing Chang Yue Hao State Key Discipline Laboratory of Wide Band Gap Semiconductor Technology Shaanxi Joint Key Laboratory of GrapheneSchool of MicroelectronicsXidian University2 South Taibai RoadXi’an 710071China Centre for Spintronics and Quantum System State Key Laboratory for Mechanical Behavior of MaterialsSchool of Materials Science and EngineeringXi’an Jiaotong UniversityXi’anShaanxi 710049China Advanced Interdisciplinary Research Center for Flexible Electronics Xidian University2 South Taibai RoadXi’an 710071China

Large-size organic halide passivation has been considered an efficient approach to enhance the perovskite solar cell(PSC)efficiency and ***,a facile posttreatment strategy was demonstrated,wherein trifluoromethyl-phenethylamine hydrobromide(CF_(3)-PEABr)is firstly used to passivate the perovskite film *** CF_(3)-PEABr surface posttreatment could coordinate with halide dangling bonds that exist at the perovskite crystal ***,the surface treatment with CF_(3)-PEABr could efficiently passivate the defects in the perovskite film and suppress the nonradiative carrier *** a result,a high efficiency of 21.3%is obtained,and an increment of 80 mV in V_(oc)(a large V_(oc)of 1.15 V,with a 0.42 V voltage deficit)occurs,compared to the control *** relieve the hydrophobic nature properties of the-CF_(3)functional group and the dewetting problem of PCBM layer deposition,a surfactant Triton X-100 is used to modify the PCBM ***,the devices with CF_(3)-PEABr posttreatment exhibit better operational,thermal(85℃),and long storage stabilities without any encapsulation.

关键词： surface stability perovskite

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Applications of nanogenerators for biomedical engineering and healthcare systems

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InfoMat 2022年第2期4卷 53-109页

作者： Wanli Wang Jinbo Pang Jie Su Fujiang Li Qiang Li Xiaoxiong Wang Jingang Wang Bergoi Ibarlucea Xiaoyan Liu Yufen Li Weijia Zhou Kai Wang Qingfang Han Lei Liu Ruohan Zang Mark HRümmeli Yang Li Hong Liu Han Hu Gianaurelio Cuniberti College of Electrical Engineering Qingdao UniversityQingdaoChina Collaborative Innovation Center of Technology and Equipment for Biological Diagnosis and Therapy in Universities of Shandong Institute for Advanced Interdisciplinary Research(iAIR)University of JinanJinanChina College of Electronic Information Qingdao UniversityQingdaoChina Department of Pediatric Surgery The Affiliated Hospital of Qingdao UniversityQingdaoChina College of Physics Qingdao UniversityQingdaoChina Institute for Materials Science and Max Bergmann Center of Biomaterials Technische Universität DresdenDresdenGermany Center for Advancing Electronics Dresden Technische Universität DresdenDresdenGermany College of Biological Science and Technology University of JinanJinanChina School of Chemistry and Chemical Engineering University of JinanShandongJinanChina College of Energy Soochow Institute for Energy and Materials InnovationsSoochow UniversitySuzhouChina Key Laboratory of Advanced Carbon Materials and Wearable Energy Technologies of Jiangsu Province Soochow UniversitySuzhouChina Centre of Polymer and Carbon Materials Polish Academy of SciencesZabrzePoland Institute for Complex Materials IFW DresdenDresdenGermany Institute of Environmental Technology VŠB-Technical University of OstravaOstravaCzech Republic School of Information Science and Engineering University of JinanJinanChina Shandong Provincial Key Laboratory of Network Based Intelligent Computing University of JinanJinanChina State Key Laboratory of Crystal Materials Center of Bio&Micro/Nano Functional MaterialsShandong UniversityJinanChina College of Chemical Engineering China University of Petroleum(East China)QingdaoChina Dresden Center for Computational Materials Science Technische Universität DresdenDresdenGermany The Dresden Center for Intelligent Materials(DCIM) Technische Universität DresdenDresdenGermany

The dream of human beings for long living has stimulated the rapid development of biomedical and healthcare ***,conventional biomedical and healthcare devices have shortcomings such as short service life,large equipment size,and high potential safety ***,the power supply for conventional implantable device remains predominantly *** emerging nanogenerators,which harvest micro/nanomechanical energy and thermal energy from human beings and convert into electrical energy,provide an ideal solution for self-powering of biomedical *** combination of nanogenerators and biomedicine has been accelerating the development of self-powered biomedical *** article first introduces the operating principle of nanogenerators and then reviews the progress of nanogenerators in biomedical applications,including power supply,smart sensing,and effective ***,the microbial disinfection and biodegradation performances of nanogenerators have been ***,the protection devices have been discussed such as face mask with air filtering function together with real-time monitoring of human health from the respiration and heat ***,the nanogenerator devices have been categorized by the types of mechanical energy from human beings,such as the body movement,tissue and organ activities,energy from chemical reactions,and gravitational potential ***,the challenges and future opportunities in the applications of nanogenerators are delivered in the conclusive remarks.

关键词： biomedical engineering healthcare implantable devices nanogenerators self-powered devices sensors

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Near-Infrared Response Organic Synaptic Transistor for Dynamic Trace Extraction

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Journal of Physical Chemistry Letters 2024年第34期15卷 8845-8852页

作者： Luan, Wanhong Zhao, Zherui Li, Hang Zhai, Yongbiao Lv, Ziyu Zhou, Kui Xue, Shuangmei Zhang, Meng Yan, Yan Cao, Yan Ding, Guanglong Han, Su-Ting Kuo, Chi-Ching Zhou, Ye Institute for Advanced Study Shenzhen University Shenzhen518060 China College of Electronics and Information Engineering Shenzhen University Shenzhen518060 China The Construction Quality Supervision and Inspection Station of Zhuhai Zhuhai519000 China State Key Laboratory of Radio Frequency Heterogeneous Integration Shenzhen University Shenzhen518060 China South China Advanced Institute for Soft Matter Science and Technology School of Emergent Soft Matter South China University of Technology Guangzhou510640 China Department of Applied Biology and Chemical Technology The Hong Kong Polytechnic University Hung Hom Hong Kong999077 Hong Kong Institute of Organic and Polymeric Materials National Taipei University of Technology Taipei10608 Taiwan Advanced Research Center for Green Materials Science and Technology National Taiwan University Taipei10617 Taiwan

The development of neuromorphic hardware capable of detecting and recognizing moving targets through an in-sensor computing strategy is considered to be an important component of the construction of edge computing systems with distributed computation. In addition to responsiveness to visible light, the implementation of neuromorphic hardware should also demonstrate the ability to sense and process nonvisible light, which is essential for tracking target object trajectories in specialized environments. In this work, we fabricated an organic synaptic transistor with a near-infrared (NIR) response by incorporating doped LaF3: Yb/Ho upconversion quantum dots (UCQDs) into the channel of a Poly3-hexylthiophene (P3HT)-based organic field effect transistor (FET), serving as charge trapping and infrared sensing sites. The obtained synaptic transistor not only replicates common synaptic behaviors when exposed to NIR illumination but also demonstrates potential applications for the dynamic trajectory recognition of animals in the dark. Compared to other monitoring technologies, P3HT transistors doped with LaF3: Yb/Ho UCQDs exhibit distinct advantages, including a NIR response, high-efficiency computing, and sensitivity, which provide an experimental foundation and a design reference for the development of next-generation intelligent dynamic image recognition systems. © 2024 American Chemical Society.

关键词： Organic field effect transistors

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