Most speech translation technologies, which mimic human interpreters, may eventually replace human interpreters. In contrast, our long-term goal is to construct an augmented intelligent system that can support interpr...
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Antiferroelectric PbZrO_(3)(AFE PZO)films have great potential to be used as the energy storage dielectrics due to the unique electric field(E)-induced phase transition ***,the phase transition process always accompan...
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Antiferroelectric PbZrO_(3)(AFE PZO)films have great potential to be used as the energy storage dielectrics due to the unique electric field(E)-induced phase transition ***,the phase transition process always accompanies a polarization(P)hysteresis effect that induces the large energy loss(Wloss)and lowers the breakdown strength(EBDS),leading to the inferior energy storage density(Wrec)as well as low *** this work,the synergistic strategies by doping smaller ions of Li^(+)–Al^(3+)to substitute Pb2+and lowering the annealing temperature(T)from 700 to 550℃are proposed to change the microstructures and tune the polarization characters of PZO films,except to dramatically improve the energy storage *** prepared Pb_((1−x))(Li_(0.5)Al_(0.5))_(x)ZrO_(3)(P_((1−x))(L_(0.5)A_(0.5))_(x)ZO)films exhibit ferroelectric(FE)-like rather than AFE character once the doping content of Li^(+)–Al^(3+)ions reaches 6 mol%,accompanying a significant improvement of W_(rec) of 49.09 J/cm^(3),but the energy storage efficiency(η)is only 47.94%due to the long-correlation of FE ***,the low-temperature annealing is carried out to reduce the crystalline degree and the P loss.P_(0.94)(L_(0.5)A_(0.5))_(0.06)ZO films annealed at 550℃deliver a linear-like polarization behavior rather than FE-like behavior annealed at 700℃,and the lowered remanent polarization(P_(r))as well as improved E_(BDS)(4814 kV/cm)results in the superior Wrec of 58.7 J/cm^(3) and efficiency of 79.16%,simultaneously possessing excellent frequency and temperature stability and good electric fatigue tolerance.
The effect of carbon content on the microstructures and stress rupture properties of a newly developed polycrystalline Ni-based superalloy with high Cr content has been *** was observed that both grain size and the nu...
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The effect of carbon content on the microstructures and stress rupture properties of a newly developed polycrystalline Ni-based superalloy with high Cr content has been *** was observed that both grain size and the number of carbides increased with an increase in carbon *** heat treatment,granular M_(23)C_(6)carbides were dispersed around MC carbides along grain boundaries and inside *** quantity of granular M_(23)C_(6)carbides increased while their sizes *** findings can be verified with the results of thermodynamic calculation and differential scanning calorimetry *** stress rupture times(975℃/225 MPa)increased from 13.3 to 25.5 h with the carbon content increased from 0.1 to 0.2 wt.%.The improvement can be attributed to two primary ***,grain boundary is typically weak region during deformation process and the grain size increased as carbon content increased in the ***,carbides act as hindrances to impede dislocation movement,leading to dislocation *** carbon content rose,the quantity of carbides in interdendritic regions and grain boundaries increased,providing a certain degree of strengthening effect and resulting in a longer stress rupture time.
The challenge in Isolated Sign Language Recognition (ISLR) research is to effectively eliminate transition frame redundancy and to integrate disparate features. To solve these two problems, We proposed an ISLR approac...
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CuBi2O4(CBO) photocathodes hold significant promise for efficient photoelectrochemical(PEC) water splitting due to their favorable band gap and theoretical onset ***,their practical application is hindered by poor...
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CuBi2O4(CBO) photocathodes hold significant promise for efficient photoelectrochemical(PEC) water splitting due to their favorable band gap and theoretical onset ***,their practical application is hindered by poor charge separation ***,we introduce a characteristic in-situ solution Fe-doping strategy that markedly improves photoelectrochemical performance of CBO,doubling the photocurrent density and achieving an unprecedented 190 mV anodic shift in the onset *** integrating with an electrochemical oxidation post-treatment,a record incident photon-to-current efficiency(IPCE) exceeding 40% at 0.6 V *** under visible light illumination is *** versatility of the doping strategy is demonstrated across CBO photocathodes synthesized by different methods with various morphologies,grain sizes,and *** studies reveal that the gradient distribution of Fe3+ions generates an internal electric field that facilitates efficient charge separation and increases acceptor *** strong Fe-O bonding also enhances structural stability against photoinduced ***,our investigation uncovers the non-temperature-dependent nature of CBO photocurrent,indicating that PEC performance enhancement primarily depends on reducing carrier recombination rather than improving bulk *** work lays the groundwork for future advancements in water splitting performance of CBO photocathodes,offering a complementary strategy to conventional methods for enhancing charge separation efficiency.
Hydrogen energy,whether in generation plants or utilization facilities,plays a decisive role in the mission to achieve net-zero greenhouse gas emissions,all to minimize *** growing demand for clean energy carrier stea...
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Hydrogen energy,whether in generation plants or utilization facilities,plays a decisive role in the mission to achieve net-zero greenhouse gas emissions,all to minimize *** growing demand for clean energy carrier steadily accelerates the development of hydrogen production processes,and therein proton exchange membrane(PEM)water electrolysis is deemed a promising long-term strategy for hydrogen preparation and *** review retrospects recent developments and applications of bipolar plates(BPs)as key components in PEM fuel cells and water *** main content includes multifaceted challenges in the R&D or fabrication of BPs and potential future trends have also been *** details cover the BPs matrix(metallic materials and carbon composites)and the surface coating types(metal and compound coatings,carbon-based coatings,and polymer coatings),as well as the influence of flow field design for mass ***-term development and feasible researches of BPs are *** in the following aspects:(1)Structural and functional integration of components,such as material fabrication and flow field geometry optimization using 3D printing technology;(2)Introduction of environment-friendly renewable energy for hydrogen production;(3)Research on hydrogen energy reversible systems;(4)Composition optimization of surface coatings based on computational materials science and(5)systematic design expected to evolve into the next generation of BPs.
Flexible photodetectors have garnered significant attention by virtue of their potential applications in environmental monitoring,wearable healthcare,imaging sensing,and portable optical *** stand out as particularly ...
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Flexible photodetectors have garnered significant attention by virtue of their potential applications in environmental monitoring,wearable healthcare,imaging sensing,and portable optical *** stand out as particularly promising materials for photodetectors,offering exceptional optoelectronic properties,tunable band gaps,low-temperature solution processing,and notable mechanical *** this review,we explore the latest progress in flexible perovskite photodetectors,emphasizing the strategies developed for photoactive materials and device structures to enhance optoelectronic performance and ***,we discuss typical applications of these devices and offer insights into future directions and potential applications.
Currently, 3D Lidar is widely used in indoor SLAM tasks due to its stable and reliable measurement performance. However, it suffers from significant positioning and mapping errors in indoor degraded environments, maki...
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As an important computer vision task that can be used in many areas, facial expression recognition (FER) has been widely studied which much progress has been obtained especially when deep learning (DL) approaches have...
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Exploration of efficient and stable photocatalysts to mimic natural leaves for the conversion of atmospheric CO_(2)into hydrocarbons utilizing solar light is very important but remains a major ***,we report the design...
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Exploration of efficient and stable photocatalysts to mimic natural leaves for the conversion of atmospheric CO_(2)into hydrocarbons utilizing solar light is very important but remains a major ***,we report the design of four novel metal-salen-incorporated conjugated microporous polymers as robust artificial leaves for photoreduction of atmospheric CO_(2)with gaseous *** to the rich nitrogen and oxygen moieties in the polymeric frameworks,they show a maximum CO_(2)adsorption capacity of 46.1 cm3 g^(−1)and adsorption selectivity for CO_(2)/N_(2)of up to 82 at 273 *** air atmosphere and simulated solar light(100mWcm^(−2)),TEPT-Zn shows an excellent CO yield of 304.96μmol h^(−1)g^(−1)with a selectivity of approximately 100%,which represents one of the best results in terms of organic photocatalysts for gas-phase CO_(2)photoreduction so ***,only small degradation in the CO yield is observed even after 120-h continuous *** importantly,a good CO yield of 152.52μmol g^(−1)was achieved by directly exposing the photocatalytic reaction of TEPT-Zn in an outdoor environment for 3 h(25-28℃,52.3±7.9mWcm^(−2)).This work provides an avenue for the continued development of advanced polymers toward gas-phase photoconversion of CO_(2)from air.
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