Currently, 3D Lidar is widely used in indoor SLAM tasks due to its stable and reliable measurement performance. However, it suffers from significant positioning and mapping errors in indoor degraded environments, maki...
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Hydrogen energy,whether in generation plants or utilization facilities,plays a decisive role in the mission to achieve net-zero greenhouse gas emissions,all to minimize *** growing demand for clean energy carrier stea...
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Hydrogen energy,whether in generation plants or utilization facilities,plays a decisive role in the mission to achieve net-zero greenhouse gas emissions,all to minimize *** growing demand for clean energy carrier steadily accelerates the development of hydrogen production processes,and therein proton exchange membrane(PEM)water electrolysis is deemed a promising long-term strategy for hydrogen preparation and *** review retrospects recent developments and applications of bipolar plates(BPs)as key components in PEM fuel cells and water *** main content includes multifaceted challenges in the R&D or fabrication of BPs and potential future trends have also been *** details cover the BPs matrix(metallic materials and carbon composites)and the surface coating types(metal and compound coatings,carbon-based coatings,and polymer coatings),as well as the influence of flow field design for mass ***-term development and feasible researches of BPs are *** in the following aspects:(1)Structural and functional integration of components,such as material fabrication and flow field geometry optimization using 3D printing technology;(2)Introduction of environment-friendly renewable energy for hydrogen production;(3)Research on hydrogen energy reversible systems;(4)Composition optimization of surface coatings based on computational materials science and(5)systematic design expected to evolve into the next generation of BPs.
CuBi2O4(CBO) photocathodes hold significant promise for efficient photoelectrochemical(PEC) water splitting due to their favorable band gap and theoretical onset ***,their practical application is hindered by poor...
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CuBi2O4(CBO) photocathodes hold significant promise for efficient photoelectrochemical(PEC) water splitting due to their favorable band gap and theoretical onset ***,their practical application is hindered by poor charge separation ***,we introduce a characteristic in-situ solution Fe-doping strategy that markedly improves photoelectrochemical performance of CBO,doubling the photocurrent density and achieving an unprecedented 190 mV anodic shift in the onset *** integrating with an electrochemical oxidation post-treatment,a record incident photon-to-current efficiency(IPCE) exceeding 40% at 0.6 V *** under visible light illumination is *** versatility of the doping strategy is demonstrated across CBO photocathodes synthesized by different methods with various morphologies,grain sizes,and *** studies reveal that the gradient distribution of Fe3+ions generates an internal electric field that facilitates efficient charge separation and increases acceptor *** strong Fe-O bonding also enhances structural stability against photoinduced ***,our investigation uncovers the non-temperature-dependent nature of CBO photocurrent,indicating that PEC performance enhancement primarily depends on reducing carrier recombination rather than improving bulk *** work lays the groundwork for future advancements in water splitting performance of CBO photocathodes,offering a complementary strategy to conventional methods for enhancing charge separation efficiency.
Flexible photodetectors have garnered significant attention by virtue of their potential applications in environmental monitoring,wearable healthcare,imaging sensing,and portable optical *** stand out as particularly ...
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Flexible photodetectors have garnered significant attention by virtue of their potential applications in environmental monitoring,wearable healthcare,imaging sensing,and portable optical *** stand out as particularly promising materials for photodetectors,offering exceptional optoelectronic properties,tunable band gaps,low-temperature solution processing,and notable mechanical *** this review,we explore the latest progress in flexible perovskite photodetectors,emphasizing the strategies developed for photoactive materials and device structures to enhance optoelectronic performance and ***,we discuss typical applications of these devices and offer insights into future directions and potential applications.
As an important computer vision task that can be used in many areas, facial expression recognition (FER) has been widely studied which much progress has been obtained especially when deep learning (DL) approaches have...
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Bacterial wound infections are a growing challenge in healthcare,posing severe risks like systemic infection,organ failure,and sepsis,with projections predicting over 10 million deaths annually by *** hydrogels,with a...
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Bacterial wound infections are a growing challenge in healthcare,posing severe risks like systemic infection,organ failure,and sepsis,with projections predicting over 10 million deaths annually by *** hydrogels,with adaptable extracellular matrix-like features,are emerging as promising solutions for treating infectious ***,the antibacterial properties of most of these hydrogels are largely attributed to extrinsic agents,and their mechanisms of action remain poorly *** we introduce for the first time,modified imidazolidinyl urea(IU)as the polymeric backbone for developing tissue-like antibacterial ***-designed hydrogels behave tissue-like mechanical features,outstanding antifreeze behavior,and rapid self-healing *** dynamics(MD)simulation and density functional theory(DFT)calculation were employed to well-understand the extent of H-bonding and metal-ligand coordination to finetune hydrogels’*** vitro studies suggest good biocompatibility of hydrogels against mouse fibroblasts&human skin,lung,and red blood cells,with potential wound healing ***,the hydrogels exhibit good 3D printability and remarkable antibacterial activity,attributed to concentration dependent ROS genera-tion,oxidative stress induction,and subsequent disruption of bacterial *** top of that,in vitro biofilm studies confirmed that developed hydrogels are effective in preventing biofilm ***,these tissue-mimetic hydrogels present a promising and effective platform for accelerating wound healing while simulta-neously controlling bacterial infections,offering hope for the future of wound care.
Exploration of efficient and stable photocatalysts to mimic natural leaves for the conversion of atmospheric CO_(2)into hydrocarbons utilizing solar light is very important but remains a major ***,we report the design...
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Exploration of efficient and stable photocatalysts to mimic natural leaves for the conversion of atmospheric CO_(2)into hydrocarbons utilizing solar light is very important but remains a major ***,we report the design of four novel metal-salen-incorporated conjugated microporous polymers as robust artificial leaves for photoreduction of atmospheric CO_(2)with gaseous *** to the rich nitrogen and oxygen moieties in the polymeric frameworks,they show a maximum CO_(2)adsorption capacity of 46.1 cm3 g^(−1)and adsorption selectivity for CO_(2)/N_(2)of up to 82 at 273 *** air atmosphere and simulated solar light(100mWcm^(−2)),TEPT-Zn shows an excellent CO yield of 304.96μmol h^(−1)g^(−1)with a selectivity of approximately 100%,which represents one of the best results in terms of organic photocatalysts for gas-phase CO_(2)photoreduction so ***,only small degradation in the CO yield is observed even after 120-h continuous *** importantly,a good CO yield of 152.52μmol g^(−1)was achieved by directly exposing the photocatalytic reaction of TEPT-Zn in an outdoor environment for 3 h(25-28℃,52.3±7.9mWcm^(−2)).This work provides an avenue for the continued development of advanced polymers toward gas-phase photoconversion of CO_(2)from air.
Layered materials with unique structures and symmetries have attracted tremendous interest for constructing 2-dimensional(2D)*** weak interlayer interaction renders them to be readily isolated into various ultrathin n...
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Layered materials with unique structures and symmetries have attracted tremendous interest for constructing 2-dimensional(2D)*** weak interlayer interaction renders them to be readily isolated into various ultrathin nanosheets with exotic properties and diverse *** order to enrich the library of 2D materials,extensive progress has been made in the field of ternary layered ***,many brand-new materials are derived,which greatly extend the members of 2D *** this review,we emphasize the recent progress made in synthesis and exploration of ternary layered *** first classify them in terms of stoichiometric ratio and summarize their difference in interlayer interaction,which is of great importance to produce corresponding 2D *** compositional and structural characteristics of resultant 2D ternary materials are then discussed so as to realize desired structures and *** a new family of 2D materials,we overview the layer-dependent properties and related applications in the fields of electronics,optoelectronics,and energy storage and *** review finally provides a perspective for this rapidly developing field.
作者:
Ramasamy, G.Kamalakkannan, S.Vels Institute of Science
Technology & Advanced Studies Department of Computer Science School of Computing Sciences Pallavaram Chennai India Vels Institute of Science
Technology & Advanced Studies Department of Information Technology School of Computing Sciences Pallavaram Chennai India
Container-based virtualisation has become a cornerstone of Cloud Computing (CC) due to its lightweight and scalable properties when compared to traditional virtual machines. However, it is still difficult to optimisin...
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With the rapid development of computer techniques,atomistic modeling is playing an increasingly important role in understanding the structure-activity relationship of *** dynamics (MD) is a computational simulation ap...
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With the rapid development of computer techniques,atomistic modeling is playing an increasingly important role in understanding the structure-activity relationship of *** dynamics (MD) is a computational simulation approach to predicting the structural evolution of an atomic system over time,widely used to understand physical and chemical phenomena including phase transition,diffusion,crystallization,and reaction [1].
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