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Building Better Batteries:Solid-State Batteries with Li-Rich Oxide Cathodes

Energy Material Advances 2023年第1期4卷 402-425页

作者： Lifeng Xu Shi Chen Yuefeng Su Jizhuang He Lian Wang Xing Shen Lai Chen Duanyun Cao Yun Lu Meng Wang Liying Bao Ning Li Feng Wu Beijing Key Laboratory of Environmental Science and Engineering School of Material Science and EngineeringBeijing Institute of TechnologyBeijing 100081China Beijing Institute of Technology Chongqing Innovation Center Chongqing 401120China

High-capacity Li-rich oxide materials have received extensive attention due to their unique anion-cation charge compensation ***,the high operating voltage,poor cycling performance,unsafe oxygen evolution,and voltage decay limit their industrial *** emergence and development of solid-state batteries offer a great opportunity to solve these issues by replacing flammable and unstable liquid electrolytes with solid ***,utilization of high-capacity Li-rich oxide cathodes enables to establish high-energy-density solid-state batteries with wide voltage ranges,light weight,and high mechanical *** review summarizes the recent progress of Li-rich oxide materials and solid electrolytes,emphasizing their major advantages,interface challenges,and modification approaches in the development of Li-rich solid-state *** also propose possible characterization strategies for effective interfacial observation and *** is hoped that this review should inspire the rational design and development of better solid-state batteries for application in portable devices,electric vehicles,as well as power grids.

关键词： Solid rational cycling

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Estimation of unfrozen water content of saturated sandstones using nuclear magnetic resonance, mercury intrusion porosimetry, and ultrasonic tests

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Journal of Rock Mechanics and Geotechnical engineering 2024年第9期16卷 3465-3484页

作者： Fei Liu Shibing Huang Gang Liu Shilin Yu School of Resources and Environmental Engineering Wuhan University of Science and TechnologyWuhan430081China Hubei Key Laboratory for Efficient Utilization and Agglomeration of Metallurgic Mineral Resources Wuhan University of Science and TechnologyWuhan430081China

The unfrozenwater content(UWC)is a crucial parameter that affects the strength and thermal properties of rocks in relation to engineering construction and geological disasters in cold *** this study,three different methods were employed to test and estimate the UWC of saturated sandstones,including nuclear magnetic resonance(NMR),mercury intrusion porosimetry(MIP),and ultrasonic *** NMR method enabled the direct measurement of the UWC of sandstones using the free induction decay(FID).The MIP method was used to analyze the pore structures of sandstones,with the UWC subsequently calculated based on pore ice ***,the MIP test constituted an indirect measurement ***,a correlation was established between the P-wave velocity and the UWC of these sandstones based on the mixture theory,which could be employed to estimate the UWC as an empirical *** methods demonstrated that the UWC initially exhibited a rapid decrease from 0C to5C and then generally became constant beyond20***,these test methods had different *** NMR method was used to directly and accurately calculate the UWC in the ***,the cost and complexity of NMR equipment have precluded its use in the *** UWC can be effectively estimated by the MIP test,but the estimation accuracy is influenced by the ice crystallization process and the pore size *** P-wave velocity has been demonstrated to be a straightforward and practical empirical parameter and was utilized to estimate the UWC based on the mixture *** method may be more suitable in the *** methods confirmed the existence of a hysteresis phenomenon in the freezing-thawing *** average hysteresis coefficient was approximately 0.538,thus validating the GibbseThomson *** study not only presents alternative methodologies for estimating the UWC of saturated sandstones but also contribute to our understanding of the freezin

关键词： Unfrozen water content(UWC) Nuclear magnetic resonance(NMR) Mercury intrusion porosimetry(MIP) Pore structures P-wave velocity Sandstone

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Nano silica aerogel-induced formation of an organic/alloy biphasic interfacial layer enables construction of stable high-energy lithium metal batteries

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Green Energy & Environment 2023年第4期8卷 1071-1080页

作者： Chengwei Ma Xinyu Zhang Chengcai Liu Yuanxing Zhang Yuanshen Wang Ling Liu Zhikun Zhao Borong Wu Daobin Mu Beijing Key Laboratory of Environmental Science and Engineering School of Materials Science and EngineeringBeijing Institute of TechnologyBeijing100081China Collaborative Innovation Center of Electric Vehicles in Beijing Beijing100081China

Lithium metal batteries represent promising candidates for high-energy-density batteries, however, many challenges must still be overcome,e.g., interface instability and dendrite growth. In this work, nano silica aerogel was employed to generate a hybrid film with high lithium ion conductivity(0.6 mS cm^(-1)at room temperature) via an in situ crosslinking reaction. TOF-SIMS profile analysis has revealed conversion mechanism of hybrid film to Li–Si alloy/Li F biphasic interface layer, suggesting that the Li–Si alloy and Li F-rich interface layer promoted rapid Li+transport and shielded the Li anodes from corrosive reactions with electrolyte-derived products. When coupled with nickel-cobalt-manganese-based cathodes, the batteries achieve outstanding capacity retention over 1000 cycles at 1 C. Additionally the developed film coated on Li enabled high coulombic efficiency(99.5%) after long-term cycling when coupled with S cathodes. Overall, the results presented herein confirm an effective strategy for the development of high-energy batteries.

关键词： Lithium metal batteries Nano silica aerogel In situ crosslinking Biphasic interface layer Li–Si alloy

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Insights into the mechanism of the deterioration of mainstream partial nitritation/anammox under low residual ammonium

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Journal of environmental sciences 2023年第4期126卷 29-39页

作者： Yandong Yang Yiming Jiang Yanan Long Jiarui Xu Changqing Liu Liang Zhang Yongzhen Peng School of Environmental and Municipal Engineering Qingdao University of TechnologyQingdao 266033China National Engineering Laboratory for Advanced Municipal Wastewater Treatment and Reuse Technology Key Laboratory of Beijing for Water Quality Science and Water Environment Recovery EngineeringBeijing University of TechnologyBeijing 100124China

Residual ammonium is a critical parameter affecting the stability of mainstream partial nitritation/anammox(PN/A), but the underlying mechanism remains unclear. In this study,mainstream PN/A was established and operated with progressively decreasing residual ammonium. PN/A deteriorated as the residual ammonium decreased to below 5 mg/L, and this was paralleled by a significant loss in anammox activity in situ and an increasing nitrite oxidation rate. Further analysis revealed that the low-ammonium condition directly decreased anammox activity in situ via two distinct mechanisms. First, anammox bacteria were located in the inner layer of the granular sludge, and thus were disadvantageous when competing for ammonium with ammonium-oxidizing bacteria(AOB) in the outer layer. Second, the complete ammonia oxidizer(comammox) was enriched at low residual ammonium concentrations because of its high ammonium affinity. Both AOB and comammox presented kinetic advantages over anammox bacteria. At high residual ammonium concentrations,nitrite-oxidizing bacteria(NOB) were effectively suppressed, even when their maximum activity was high due to competition for nitrite with anammox bacteria. At low residual ammonium concentrations, the decrease in anammox activity in situ led to an increase in nitrite availability for nitrite oxidation, facilitating the activation of NOB despite the dissolved oxygen limitation(0.15–0.35 mg/L) for NOB persisting throughout the operation. Therefore, the deterioration of mainstream PN/A at low residual ammonium was primarily triggered by a decline in anammox activity in situ. This study provides novel insights into the optimized design of mainstream PN/As in engineering applications.

关键词： Mainstream partial nitritation/anammox Residual ammonium Granular sludge Comammox

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Fault Diagnosis based on Behavior and State-Awareness Digital Twin of Key Equipment in Power Supply System

Fault Diagnosis based on Behavior and State-Awareness Digita...

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2023 CAA Symposium on Fault Detection, Supervision and Safety for Technical Processes, SAFEPROCESS 2023

作者： Liu, Haifei Zhao, Qin Hao, Jie Tao, Laifa Lu, Chen Beihang University Institute of Reliability Engineering Beijing China Science & Technology on Reliability & Environmental Engineering Laboratory Beijing China Beihang University School of Reliability and Systems Engineering Beijing China AVIC xi'An Flight Automatic Control Research Institute Xi'an China

ISBN: (纸本)9798350337754

With the rapid development of multi-electric and all-electric aircraft, the role of power supply systems in aircraft is becoming increasingly prominent. Traditional fault diagnosis methods have problems such as a single means of sensory modelling and unbalanced fault data. The rapid development of digital twin technology provides an opportunity to overcome these difficulties. However, how to achieve adaptive updating and how to improve the data-and-model-fusion capabilities are also urgent challenges to be solved. To address the lack of existing research, this paper combines time-frequency domain analysis, physical information neural network based on differential-algebraic equation (DAE-PINN) and transient stability analysis of the power supply system based on a digital twin model with dimensions including fault-behavior-twin and (FBT) fault-state-awareness-twin (FSAT). Ultimately, this paper achieves effective digital twin modelling, fault eigenfeature extraction and high accuracy fault diagnosis, reaching fault data balance and complete state characterization and adaptive update of the diagnostic model. © 2023 IEEE.

关键词： Failure analysis

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A critical review on thermodynamic mechanisms of membrane fouling in membrane-based water treatment process

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Frontiers of environmental science & engineering 2023年第10期17卷 147-169页

作者： Jiaheng Teng Ying Deng Xiaoni Zhou Wenfa Yang Zhengyi Huang Hanmin Zhang Meijia Zhang Hongjun Lin Key Laboratory of Watershed Earth Surface Processes and Ecological Security College of Geography and Environmental SciencesZhejiang Normal UniversityJinhua 321004China Key Laboratory of Industrial Ecology and Environmental Engineering(Ministry of Education) School of Environmental Science and TechnologyDalian University of TechnologyDalian 116024China

Membrane technology is widely regarded as one of the most promising technologies for wastewater treatment and reclamation in the 21st century. However, membrane fouling significantly limits its applicability and productivity. In recent decades, research on the membrane fouling has been one of the hottest spots in the field of membrane technology. In particular, recent advances in thermodynamics have substantially widened people’s perspectives on the intrinsic mechanisms of membrane fouling. Formulation of fouling mitigation strategies and fabrication of anti-fouling membranes have both benefited substantially from those studies. In the present review, a summary of the recent results on the thermodynamic mechanisms associated with the critical adhesion and filtration processes during membrane fouling is provided. Firstly, the importance of thermodynamics in membrane fouling is comprehensively assessed. Secondly, the quantitative methods and general factors involved in thermodynamic fouling mechanisms are critically reviewed. Based on the aforementioned information, a brief discussion is presented on the potential applications of thermodynamic fouling mechanisms for membrane fouling control. Finally, prospects for further research on thermodynamic mechanisms underlying membrane fouling are presented. Overall, the present review offers comprehensive and in-depth information on the thermodynamic mechanisms associated with complex fouling behaviors, which will further facilitate research and development in membrane technology.

关键词： Membrane fouling Thermodynamic mechanism XDLVO theory Flory-Huggins theory Fouling migration

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Bibliometric analysis and scientific trends on perfluorinated and polyfluoroalkyl substances (PFASs) as an emerging pollutant

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Water-Energy Nexus 2024年第1期7卷 187-199页

作者： Guo, Hongan Xing, Meiyan Sun, Xiaojie Liu, Tao Key Laboratory of Yangtze Water Environment for Ministry of Education College of Environmental Science and Engineering Tongji University Shanghai200092 China Guangxi Key Laboratory of Environmental Pollution Control Theory and Technology Guilin University of Technology Guilin541004 China

The persistence, bioaccumulation, and toxicity of perfluorinated and polyfluoroalkyl substances (PFASs), along with their concentrations in the environment and humans, have attracted global attention. However, so far, there have been seldom reports providing a systematical review in the entire field of PFASs research. Therefore, this study summarizes 14,112 relevant publications (2005–2022) and conducts bibliometric analysis using Vosviewer and CiteSpace. The findings offer insights into global PFASs research trends, assisting scientists in establishing their research directions. Unlike traditional literature reviews, this article presents a new method for data collection and analysis that achieves quantitative visualization of the information from the past 18 years in the field of PFASs. Results show a significant increase in global PFASs publications, with China leading in publication output and the US in international collaborations. Author Kurunthachalam Kanna has the highest publication records. Document co-citation clustering and key line analysis identifies four major research areas and landmarks, while betweenness centrality analysis reveals developmental processes. Citation burst analysis finds that PFASs toxicity and monitoring have been hot areas, suggesting the need for greater attention towards the types and levels of PFASs in various environmental media and the removal processes of PFASs responsible for pollution, which may emerge as future research hotspots. © 2024

关键词： Toxicity

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Software fault localization based on eigenvector centrality in complex network theory 24

Software fault localization based on eigenvector centrality ...

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24th IEEE International Conference on Software Quality, reliability and Security Companion, QRS-C 2024

作者： Wu, Wentao Wang, Shihai Shao, Yuanxun Xie, Wandong School of Reliability and Systems Engineering Beihang University Beijing100191 China Science and Technology on Reliability and Environmental Engineering Laboratory China State Key Laboratory of Software Development Environment China Aerospace Science and Engineering Network Information Development CO. Ltd Beijing China Information Center of China North Industries Group Corporation Beijing China

ISBN: (纸本)9798350365658

Software debugging plays a crucial role in fault localization tasks, and spectrum-based fault localization (SBFL) is a hot topic in software automation debugging research. However, existing SBFL technologies are generally limited by tie within ranks, where a large number of elements share the same suspiciousness, which in turn severely limits the performance of SBFL. To this end, we propose an SBFL model based on eigenvector centrality (FLEC). This algorithm first utilizes the statement coverage information in the program spectrum to construct a statement network, and adopts the correlation between statements as edge weights. Then, FLEC takes statement suspiciousness as node weight. On this basis, the algorithm utilizes the eigenvector centrality to calculate the weighted suspiciousness of each statement while considering both node importance and correlation between nodes. Finally, FLEC conducted experimental validation on 3 datasets of Defects4J, and the results showed an average improvement of 10.7% in ACC@N compared to the optimal baseline. © 2024 IEEE.

关键词： Program debugging

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Enhancing anoxic denitrification of low C/N ratio wastewater with novel ZVI composite carriers

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Journal of environmental sciences 2022年第2期34卷 180-191页

作者： Yanping Shi Tao Liu Hongtao Yu Xie Quan Key Laboratory of Industrial Ecology and Environmental Engineering(Ministry of Education) School of Environmental Science and TechnologyDalian University of TechnologyDalian 116024China

External organic carbon sources are needed to provide electron donors for the denitrification of wastewater with a low COD/NO_(3)^(-)-N(C/N)ratio,increasing the treatment *** economic strategy is to enhance the bioactivity and/or biodiversity of denitrifiers to efficiently utilize organic substances in *** this study,novel zero-valent iron(ZVI)composite carriers were prepared and implemented in a suspended carrier biofilm reactor to enhance the bioactivity and/or biodiversity of *** the influent C/N ratio of 4(COD was 179.5±5.0 mg/L and TN was 44.2±0.8 mg/L),COD and TN removal efficiencies were 85.1%and 66.4%,respectively,in the reactors filled with 3 wt%ZVI composite *** contrast,COD and TN removal efficiencies were 70.4%and 55.3%,respectively,in the reactor filled with conventional high-density polyethylene(HDPE)biofilm *** biofilm formation on the 3 wt%ZVI composite carriers was optimized due to its higher roughness(surface square roughness increased from 76.0 nm to 93.8 nm)and favorable hydrophilicity(water contact angle dropped to 72.5°±1.4°from 94.3°±3.2°)compared with the HDPE biofilm *** addition,heterotrophic denitrifiers,Thauera and Dechloromonas,were enriched,whereas autotrophic denitrifiers,Raoultella and Thiobacillus,exhibited high relative abundance in the biofilm of ZVI composite *** coexistence of heterotrophic denitrifiers and autotrophic denitrifiers on the surface of ZVI composite carriers provided mixotrophic metabolism of denitrification(including heterotrophic and iron-based autotrophic),thereby ensuring effective denitrification for wastewater with a low C/N ratio without external organic carbon source addition.

关键词： ZVI Biofilm carrier Low C/N ratio Integrated floating fixed-film and activated sludge(IFFAS) Denitrification

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Optimized reinforcement of granite residual soil using a cement and alkaline solution: A coupling effect

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Journal of Rock Mechanics and Geotechnical engineering 2025年第1期17卷 509-523页

作者： Bingxiang Yuan Jingkang Liang Baifa Zhang Weijie Chen Xianlun Huang Qingyu Huang Yun Li Peng Yuan School of Civil and Transportation Engineering Guangdong University of TechnologyGuangzhou510006China School of Environmental Science and Engineering Guangdong University of TechnologyGuangzhou510006China Shenzhen Key Laboratory of Natural Gas Hydrates Academy for Advanced Interdisciplinary StudiesSouthern University of Science and TechnologyShenzhen518055China

Granite residual soil (GRS) is a type of weathering soil that can decompose upon contact with water, potentially causing geological hazards. In this study, cement, an alkaline solution, and glass fiber were used to reinforce GRS. The effects of cement content and SiO_(2)/Na2O ratio of the alkaline solution on the static and dynamic strengths of GRS were discussed. Microscopically, the reinforcement mechanism and coupling effect were examined using X-ray diffraction (XRD), micro-computed tomography (micro-CT), and scanning electron microscopy (SEM). The results indicated that the addition of 2% cement and an alkaline solution with an SiO_(2)/Na2O ratio of 0.5 led to the densest matrix, lowest porosity, and highest static compressive strength, which was 4994 kPa with a dynamic impact resistance of 75.4 kN after adding glass fiber. The compressive strength and dynamic impact resistance were a result of the coupling effect of cement hydration, a pozzolanic reaction of clay minerals in the GRS, and the alkali activation of clay minerals. Excessive cement addition or an excessively high SiO_(2)/Na2O ratio in the alkaline solution can have negative effects, such as the destruction of C-(A)-S-H gels by the alkaline solution and hindering the production of N-A-S-H gels. This can result in damage to the matrix of reinforced GRS, leading to a decrease in both static and dynamic strengths. This study suggests that further research is required to gain a more precise understanding of the effects of this mixture in terms of reducing our carbon footprint and optimizing its properties. The findings indicate that cement and alkaline solution are appropriate for GRS and that the reinforced GRS can be used for high-strength foundation and embankment construction. The study provides an analysis of strategies for mitigating and managing GRS slope failures, as well as enhancing roadbed performance.

关键词： Granite residue soil(GRS) Reinforcement Coupling effect Alkali activation Mechanical properties

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