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Molecular template derived ultrathin N-doped carbon layer on cobalt selenide nanobelts for durable and rapid sodium storage

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Nano Research 2024年第9期17卷 8145-8154页

作者： Chuanliang Wei Baojuan Xi Kangdong Tian Xinlu Zhang Quanyan Man Keyan Bao Wutao Mao Jinkui Feng Shenglin Xiong Key Laboratory of the Colloid and Interface Chemistry Ministry of EducationSchool of Chemistry and Chemical EngineeringSchool of Materials Science and EngineeringShandong UniversityJinan 250100China Resource Environment and Clean Energy Laboratory School of Chemical and Environmental EngineeringJiangsu University of TechnologyChangzhou 213001China

Sodium-ion batteries(SIBs)are an attractive battery system because of similar characteristics to lithium-ion batteries(LIBs)and large Na element ***,exploring stable,high-capacity and high-rate anode materials for SIBs is still challenging ***,diethylenetriamine(DETA)molecular template derived ultrathin N-doped carbon(NC)layer decorated CoSe_(2)nanobelts(CoSe_(2)/NC)are prepared by solvothermal reaction followed by calcination *** CoSe_(2)/NC exhibits large potential as an anode for *** and theoretical calculations reveal that the in situ formed conductive ultrathin NC layer can not only relieve the volume change of CoSe_(2)but also accelerate electron and ion *** addition,the nanobelt structure of CoSe_(2)/NC with abundant exposed active sites can obviously accelerate the electrochemical *** the synergistic effect of special nanobelt structure and NC layer,the rate as well as cycling performances of CoSe_(2)/NC are obviously improved.A superior capacity retention of 94.8%is achieved at 2 A·g^(-1)after 2000 *** using Na3V2(PO4)3 cathodes,the pouch full batteries can work steadily at 0.5 C,verifying the application ***_(2)/NC anodes also exhibit impressive performances in LIBs and potassium-ion batteries(PIBs).

关键词： CoSe2 nanobelts ultrathin N-doped carbon layer sodium-ion batteries anode high rate

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Effect of CeO_(2) Nanoparticles on the Spread of Antibiotic Resistance in a Reclaimed Water-Soil-Radish System-Shenzhen City,Guangdong Province,China,April 2023

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China CDC weekly 2023年第46期5卷 1029-1037,I0005-I0007页

作者： Kaiqiang Yu Bixi Zhao Yuxi Yan Qing Yang Liming Chen Yu Xia School of Environmental Science and Engineering College of EngineeringSouthern University of Science and TechnologyShenzhen CityGuangdong ProvinceChina School of Resource Environment and Life ScienceNingxia Normal UniversityGuyuan CityGansu ProvinceChina State Environmental Protection Key Laboratory of Integrated Surface Water-Groundwater Pollution Control School of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen CityGuangdong ProvinceChina Guangdong Provincial Key Laboratory of Soil and Groundwater Pollution Control School of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen CityGuangdong ProvinceChina

ABSTRACT Introduction:The use of reclaimed water(RW)for irrigation in agricultural practices raises concerns regarding the dissemination of antibiotic resistance genes(ARGs)from soils to edible *** effectiveness of na... 详细信息

关键词： Antibiotic Guangdong claimed

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Enhanced nitrate removal from groundwater using a conductive spacer in flow-electrode capacitive deionization

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Chinese Chemical Letters 2024年第8期35卷 379-382页

作者： Hongjie Guo Qiang Wei Yangyang Wu Wei Qiu Hongliang Li Changyong Zhang College of Mining Engineering Taiyuan University of TechnologyTaiyuan 030024China CAS Key Laboratory of Urban Pollutant Conversion Department of Environmental Science and EngineeringUniversity of Science and Technology of ChinaHefei 230026China CAS Key Laboratory of Mechanical Behavior and Design of Materials Department of Modern MechanicsUniversity of Science and Technology of ChinaHefei 230026China

Flow-electrode capacitive deionization(FCDI)represents a promising approach for ion separation from aqueous ***,the optimization of spacer,particularly for nitrate-contaminated groundwa-ter systems,has often been *** research comprehensively investigates the influence of using a conductive(carbon cloth,CC)spacer on nitrate removal performance within FCDI system,comparing it to a non-conductive(nylon net,NN)*** both CC and NN FCDI systems,it is unsurprisingly that nitrate removal efficiency improved notably with the increasing current density and hydraulic retention time(HRT).Interestingly,the specific energy consumption(SEC)for nitrate removal did not show obvious fluctuations when the current density and HRT varied in both *** the auspiciously optimized process parameters,CC-FCDI attained a 20%superior nitrate removal efficiency relative to NN-FCDI,ac-companied by a notably diminished SEC for CC-FCDI,registering at a mere 28%of *** great improvement can be primarily attributed to the decrement in FCDI internal resistance after using con-ductive spacer,which further confirmed by electrochemical tests such as linear sweep voltammetry(LSV)and electrochemical impedance spectroscopy(EIS).Upon prolonged continuous nitrate removal at the optimized conditions,the CC-FCDI system achieved a consistent 90%nitrate removal efficiency with a low SEC of 2.7-7.8 kWh/kg NO_(3)-N,underscoring its steady ***,this study highlights the pivotal importance of careful spacer design and optimization in realizing energy-efficient groundwater treatment via FCDI.

关键词： Flow-electrode capacitive deionization Carbon cloth Nitrate Underground water Ions transport

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Achieving high ductility and low in-plane anisotropy in magnesium alloy through a novel texture design strategy

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Journal of Magnesium and Alloys 2024年第7期12卷 2863-2873页

作者： Shi Liu Cheng Wang Hong Ning Zhao-Yuan Meng Kai Guan Hui-Yuan Wang State Key Laboratory of Automotive Simulation and Control Jilin UniversityPR China Key Laboratory of Automobile Materials of Ministry of Education&School of Materials Science and Engineering Nanling CampusJilin UniversityNo.5988 Renmin StreetChangchun130025 PR China State Key Laboratory of Reliability and Intelligence of Electrical Equipment School of Material Science and EngineeringHebei University of TechnologyTianjin300130 PR China

Texture regulation is a prominent method to modify the mechanical properties and anisotropy of magnesium *** this work,the Mg-1Al-0.3Ca-0.5Mn-0.2Gd(wt.%)alloy sheet with TD-tilted and circular texture was fabricated by unidirectional rolling(UR)and multidirectional rolling(MR)method,*** generating a strong in-plane mechanical anisotropy in conventional TD-tilted texture,the novel circular texture sample possessed a weak in-plane yield *** can be rationalized by the similar proportion of soft grains with favorable orientation for basalslip and{10.12}tensile twinning during the uniaxial tension of circular-texture sample along different ***,compared with the TD-tilted texture,the circular texture improved the elongation to failure both along the rolling direction(RD)and transverse direction(TD).By quasi-in-situ EBSD-assisted slip trace analysis,higher activation of basal slip was observed in the circular-texture sample during RD tension,contributing to its excellent *** loading along the TD,the TD-tilted texture promoted the activation of{10.12}tensile twins significantly,thus providing nucleation sites for cracks and deteriorating the *** research may shed new insights into the development of formable and ductile Mg alloy sheets by texture modification.

关键词： Magnesium alloy TD-tilted texture Circular texture In-plane yield anisotropy Ductility

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Fault Diagnosis for Aircraft Aileron Actuator Based on Graph Regularization Network

Fault Diagnosis for Aircraft Aileron Actuator Based on Graph...

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International Conference on Guidance, Navigation and Control, ICGNC 2022

作者： Cheng, Yujie Wu, Ruipeng Song, Dengwei School of Reliability and Systems Engineering Beihang University Beijing100191 China School of Instrumentation and Optoelectronic Engineering Beihang University Beijing100191 China Science and Technology on Reliability and Environmental Engineering Laboratory Beijing100191 China Institute of Reliability Engineering Beihang University Beijing100191 China

ISBN: (纸本)9789811966125

During the operation of aircraft aileron actuators, a large number of monitoring samples will be accumulated. However, most of the monitoring samples are without labels since the lack of effective data management and data analysis. Most traditional fault diagnosis methods simply use sample parameters to analyze the health condition of aircraft aileron actuators. These methods ignore the relationship between sample parameters and fail to effectively use the fault information in unlabeled samples, which results in low accuracy of fault diagnosis under label missing conditions. Graph regularization network can exploit the relationship between sample parameters to improve the fault diagnosis accuracy and performance under label missing conditions. In this paper, a fault diagnosis method based on graph regularization network is proposed. First, for the monitoring samples, a sample association graph is constructed based on the K-nearest neighbor method. Second, for the nodes in the graph with labeled samples, subgraphs are extracted and generated, each containing one labeled node and K unlabeled nodes. Then, a fault diagnosis model based on graph regularization network is constructed by using subgraphs, and the relationship between sample parameters is used to constrain the optimization, forcing the fault diagnosis model to be trained toward a fixed direction. Finally, a simulation dataset is generated by injecting different faults to an aileron actuator simulation model established using Simulink and AMESim software, and some of the fault labels are removed for case validation of the proposed fault diagnosis method. The results show that the proposed fault diagnosis method based on graph regularization network can effectively use the relationship between sample parameters and improve the performance of fault diagnosis under label missing conditions compared with typical supervised learning methods. © 2023, The Author(s), under exclusive license to Springer Nature Singapo

关键词： Failure analysis

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Dynamic coupling of ferrihydrite transformation and associated arsenic desorption/redistribution mediated by sulfate-reducing bacteria

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Journal of environmental sciences 2024年第1期135卷 39-50页

作者： Wenjing Zhou Huiyan Zhu Shiwen Hu Bowei Zhang Kun Gao Zhi Dang Chongxuan Liu State Environmental Protection Key Laboratory of Integrated Surface Water-Groundwater Pollution Control School of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen 518055China The Key Lab of Pollution Control and Ecosystem Restoration in Industry Clusters Ministry of EducationSouth China University of TechnologyGuangzhou 510006China

Sulfate-reducing bacteria play an important role in the geochemistry of iron(oxyhydr)oxide and arsenic(As)in natural environments;however,the associated reaction processes are yet to be fully *** this study,batch experiments coupled with geochemical,spectroscopic,microscopic,and thermodynamic analyses were conducted to investigate the dynamic coupling of ferrihydrite transformation and the associated As desorption/redistribution mediated by Desulfovibrio vulgaris(***).The results indicated that *** could induce ferrihydrite transformation via S^(2-)-driven and direct reduction *** the absence of SO_(4)^(2-),*** directly reduced ferrihydrite,and As desorption and re-sorption occurred simultaneously during the partial transformation of ferrihydrite to *** increase in SO_(4)^(2-)loading promoted the S^(2-)-driven reduction of ferrihydrite and accelerated the subsequent mineralogical *** the low and medium SO_(4)^(2-)treatments,ferrihydrite was completely transformed to a mixture of magnetite and mackinawite,which increased the fraction of As in the residual phase and stabilized *** the high SO_(4)^(2-)treatment,although the replacement of ferrihydrite by only mackinawite also increased the fraction of As in the residual phase,22.1%of the total As was released into the solution due to the poor adsorption affinity of As to mackinawite and the conversion of As^(5+)to As^(3+).The mechanisms of ferrihydrite reduction,mineralogy transformation,and As mobilization and redistribution mediated by sulfate-reducing bacteria are closely related to the surrounding SO_(4)^(2-)*** results advance our understanding of the biogeochemical behavior of Fe,S,and As,and are helpful for the risk assessment and remediation of As contamination.

关键词： Sulfate-reducing bacteria Arsenic Ferrihydrite Transformation Redistribution

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Effectiveness of Precursor Emission Reductions for the Control of Summertime Ozone and PM2.5 in the Beijing–Tianjin–Hebei Region under Different Meteorological Conditions

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Advances in Atmospheric sciences 2025年第4期42卷 653-669页

作者： Jing QIAN Hong LIAO Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and EngineeringNanjing University of Information Science&TechnologyNanjing 210044JiangsuChina

We used observed concentrations of air pollutants,reanalyzed meteorological parameters,and results from the Goddard Earth Observing System Chemical Transport Model to examine the relationships between concentrations of maximum daily 8-h average ozone(MDA8 O_(3)),PM_(2.5)(particulate matter with diameter of 2.5μm or less),and PM_(2.5)components and 2-m temperature(T2)or relative humidity(RH),as well as the effectiveness of precursor emission reductions on the control of O_(3) and PM_(2.5) in Beijing–Tianjin–Hebei(BTH)under different summertime temperature and humidity *** observed(simulated)MDA8 O_(3) and PM_(2.5) concentrations increased as T2 went up,with linear trends of 4.8(3.2)ppb℃^(−1) and 1.9(1.5)μg m^(−3)℃^(−1),*** results showed that the decreases in MDA8 O_(3) from precursor emission reductions were more sensitive to T2 than to *** a larger proportion of volatile organic compound(VOC)emissions at higher T2 was more effective for the control of summertime O_(3) in *** the control of summertime PM_(2.5) in BTH,reducing nitrogen oxides(NOx)combined with a small proportion of VOCs was the best *** magnitude of reduction in PM_(2.5) from reducing precursor emissions was more sensitive to RH than to T2,with the best efficiency at high *** from this study are helpful for formulating effective policies to tackle O_(3) and PM_(2.5) pollution in BTH.

关键词： ozone PM_(2.5) emission reductions meteorological conditions

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In situ observation of the electrochemical behavior of Li–CO_(2)/O_(2)batteries in an environmental transmission electron microscope

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Carbon Energy 2024年第4期6卷 244-255页

作者： Peng Jia Yunna Guo Dongliang Chen Jingming Yao Xuedong Zhang Jianguo Lu Yuqing Qiao Liqiang Zhang Hebei Key Laboratory of Applied Chemistry College of Environmental and Chemical EngineeringYanshan UniversityQinhuangdaoChina State Key Laboratory of Metastable Materials Science and Technology Clean Nano Energy CenterYanshan UniversityQinhuangdaoChina State Key Laboratory of Silicon and Advanced Semiconductor Materials School of Materials Science and EngineeringZhejiang UniversityHangzhouChina Key Laboratory of Low Dimensional Materials and Application Technology of Ministry of Education School of Materials Science and EngineeringXiangtan UniversityXiangtanChina

Li–CO_(2)/O_(2)batteries,a promising energy storage technology,not only provide ultrahigh discharge capacity but also capture CO_(2)and turn it into renewable *** electrochemical reaction pathways'ambiguity,however,creates a hurdle for their practical *** study used copper selenide(CuSe)nanosheets as the air cathode medium in an environmental transmission electron microscope to in situ study Li–CO_(2)/O_(2)(mix CO_(2)as well as O_(2)at a volume ratio of 1:1)and Li–O_(2)batteries as well as Li–CO_(2)*** discharge reactions take place successively in the Li–CO_(2)/O_(2)–CuSe nanobattery:(I)4Li^(+)+O_(2)+4e^(−)→2Li_(2)O;(II)Li_(2)O+CO_(2)→Li_(2)CO_(3).The charge reaction proceeded via(III)2Li_(2)CO_(3)→4Li^(+)+2CO_(2)+O_(2)+4e^(−).However,Li–O_(2)and Li–CO_(2)nanobatteries showed poor cycling stability,suggesting the difficulty in the direct decomposition of the discharge *** fluctuations of the Li–CO_(2)/O_(2)battery's electrochemistry were also shown to depend heavily on O_(2).The CuSe‐based Li–CO_(2)/O_(2)battery showed exceptional electrochemical *** Li^–CO_(2)/O_(2)battery offered a discharge capacity apex of 15,492 mAh g^(−1) and stable cycling 60 times at 100 mA g^(−1).Our research offers crucial insight into the electrochemical behavior of Li–CO_(2)/O_(2),Li–O_(2),and Li–CO_(2)nanobatteries,which may help the creation of high‐performance Li–CO_(2)/O_(2)batteries for energy storage applications.

关键词： CuSe nanosheets electrochemical reaction in situ environmental transmission electron microscopy Li-CO_(2)battery Li-CO_(2)/O_(2)battery Li-O_(2)battery

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Electrodeposited 3D hierarchical NiFe microflowers assembled from nanosheets robust for the selective electrooxidation of furfuryl alcohol

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Green Energy & Environment 2023年第3期8卷 874-882页

作者： Biying Liu Man Zhang Yaoyu Liu Yuchen Wang Kai Yan Guangdong Provincial Key Laboratory of Environmental Pollution Control and Remediation Technology School of Environmental Science and EngineeringSun Yat-sen University135 Xingang Xi RoadGuangzhou510275China

A robust and green strategy for the selective upgrading of biomass-derived platform chemicals towards highly valuable products is important for the sustainable ***,the efficient electrocatalytic oxidation of biomass-derived furfuryl alcohol(FFA)into furoic acid(FurAc)catalyzed by the electrodeposited non-precious NiFe microflowers was successfully reached under the low temperature and ambient *** 3D hierarchical NiFe microflowers assembled from ultrathin nanosheets were controllably synthesized by the electrodeposition method and uniformly grown on carbon fiber paper(CFP).Electrochemical analysis confirmed that NiFe nanosheets more preferred in the selective oxidation of FFA(FFAOR)than oxygen evolution reaction(OER).The linear sweep voltammetry(LSV)in FFAOR displayed a clear decrease towards lower potential,resulting in 30 mV reduction of overpotential at 20 mA cm^(-2) compared with that of *** optimal catalyst Ni_(1)Fe_(2) nanosheets exhibited the highest selectivity of FurAc(94.0%)and 81.4%conversion of FFA within 3 ***,the influence of various reaction parameters on FFAOR was then explored in *** that,the reaction pathway was investigated and rationally *** outstanding performance for FFAOR can be ascribed to the unique structure of 3D flower-like NiFe nanosheets and oxygen vacancies,resulting in large exposure of active sites,faster electron transfer and enhanced adsorption of *** findings highlight a facile and convenient mean with a promising green future,which is promising for processing of various biomass-derived platform chemicals into value-added products.

关键词： Electrodeposition Microflowers assembled by nanosheets NiOOH Oxygen vacancies Electrochemical oxidation Furfuryl alcohol Furoic acid

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Stretchable artificial vision sensor with retinomorphic transistorreservoir computing

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Nano Research 2025年第3期18卷 486-493页

作者： Tongrui Sun Xu Liu Yutong Xu Xinglei Zhao Pu Guo Junyao Zhang Ziyi Guo Yue Wu Shilei Dai Jia Huang School of Materials Science and Engineering Tongji UniversityShanghai 201804China State Key Laboratory of Petroleum Pollution Control BeijingCNPC Research Institute of Safety and Environmental TechnologyBeijing 102206China

Artificial visual sensors(AVSs)with bio-inspired sensing and neuromorphic signal processing are essential for next-generation intelligent *** optoelectronic devices employed in AVSs operate discretely in terms of sensing,processing,and memorization,and not ideal for applications necessitating shape deformation to achieve wide fields-of-view and deep ***,we present stretchable artificial visual sensors(S-AVS)capable of concurrently sensing and processing optical signals while adapting to shape ***,these S-AVSs use a stretchable transistor structure with a meticulously engineered photosensitive semiconductor layer,comprising an organic semiconductor,thermoplastic elastomer,and cesium lead bromide quantum dots(CsPbBr_(3) QDs).They exhibit synaptic behaviors such as excitatory postsynaptic current(EPSC)and paired-pulse facilitation(PPF)under optical signals,maintaining functionality under 30%strain and repeated *** nonlinear response and fading memory effect support in-sensor reservoir computing,achieving image recognition accuracies of 97.46%and 97.1%at 0%and 30%strain,respectively.

关键词： stretchable electronics artificial vision sensors(AVSs) retinomorphic transistors reservoir computing neuromorphic computing

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