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Correction: State-of-the-art advancements of atomically thin two-dimensional photocatalysts for energy conversion

Chemical communications (Cambridge, England) 2022年第78期58卷 11017页

作者： Wa Gao Zhengdao Li Qiutong Han Yan Shen Chunhai Jiang Yongcai Zhang Yujie Xiong Jinhua Ye Zhigang Zou Yong Zhou School of Physical Science and Technology Tianjin Polytechnic University Tianjin 300387 P. R. China. ***@***. Nanyang Normal University Chemistry & Pharmaceutical Engineering College Nanyang 473061 Henan P. R. China. nylzd@***. Key Laboratory of Modern Acoustics (MOE) Institute of Acoustics School of Physics National Laboratory of Solid State Microstructures Collaborative Innovation Center of Advanced Microstructures Nanjing University Nanjing Jiangsu 210093 P. R. China. zhouyong1999@***. Xiamen University of Technology Fujan Province Key Lab of Functional Materials and Application Institute of Advanced Energy Materials School of Materials Science and Engineering Xiamen Fujian 361024 P. R. China. chjiang@***. Yangzhou University School of Chemistry & Chemical Engineering Yangzhou 225009 Jiangsu P. R. China. Hefei National Laboratory for Physical Sciences at the Microscale Collaborative Innovation Center of Chemistry for Energy Materials (iChEM) School of Chemistry and Materials Science University of Science and Technology of China Hefei Anhui 230036 P. R. China. Tianjin University TJU-NIMS International Collaboration Laboratory National Institute for Materials Science (NIMS) Photocatalyst Materials Center Quantum Beam Center 1-2-1 Sengen Tsukuba Ibaraki 3050047 Japan. School of Science and Engineering The Chinese University of Hong Kong Shenzhen Guangdong 518172 P. R. China.

Correction for 'State-of-the-art advancements of atomically thin two-dimensional photocatalysts for energy conversion' by Wa Gao , , 2022, , 9594-9613, https://***/10.1039/D2CC02708A.

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Aqueous Electroreduction of Nitric Oxide to Ammonia at Low Concentration via Vacancy Engineered FeOCl

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Angewandte Chemie 2023年第6期136卷

作者： Xiaoxi Guo Pai Wang Prof. Tongwei Wu Zhiqiang Wang Prof. Jiong Li Dr. Kang Liu Prof. Junwei Fu Prof. Min Liu Dr. Jun Wu Prof. Dr. Zhang Lin Prof. Liyuan Chai Prof. Zhenfeng Bian Prof. Hengfeng Li School of Materials Science and Engineering Central South University Changsha 410083 Hunan P. R. China Hunan Joint International Research Center for Carbon Dioxide Resource Utilization State Key Laboratory of Powder Metallurgy School of Physics Central South University Changsha 410083 Hunan P. R. China Institute of Fundamental and Frontier Sciences University of Electronic Science and Technology of China Chengdu 610054 Sichuan P. R. China Key Laboratory for Advanced Materials and Joint International Research Laboratory for Precision Chemistry and Molecular Engineering Centre for Computational Chemistry and Research Institute of Industrial Catalysis School of Chemistry and Molecular Engineering East China University of Science and Technology Shanghai 200237 P. R. China Shanghai Synchrotron Radiation Facility Shanghai Advanced Research Institute Chinese Academy of Sciences Shanghai 201210 P. R. China School of Metallurgy and Environment Central South University Changsha 410083 Hunan P. R. China MOE Key Laboratory of Resource Chemistry and Shanghai Key Laboratory of Rare Earth Functional Materials Shanghai Normal University Shanghai 200234 P. R. China

Electroreduction of nitric oxide (NO) to NH 3 (NORR) has gained extensive attention for the sake of low carbon emission and air pollutant treatment. Unfortunately, NORR is greatly hindered by its sluggish kinetics, especially under low concentrations of NO. Herein, we developed a chlorine (Cl) vacancy strategy to overcome this limitation over FeOCl nanosheets (FeOCl-V Cl ). Density functional theory (DFT) calculations revealed that the Cl vacancy resulted in defective Fe with sharp d-states characteristics in FeOCl-V Cl to enhance the absorption and activation of NO. In situ X-ray absorption near-edge structure (XANES) and attenuated total reflection-infrared spectroscopy (ATR-IR) verified the lower average oxidation state of defective Fe to enhance the electron transfer for NO adsorption/activation and facilitate the generation of key NHO and NH x intermediates. As a result, the FeOCl-V Cl exhibited superior NORR activities with the NH 3 Faradaic efficiency up to 91.1 % while maintaining a high NH 3 yield rate of 455.4 μg cm −2 h −1 under 1.0 vol % NO concentration, competitive with those of previously reported literatures under higher NO concentration. Further, the assembled Zn-NO battery utilizing FeOCl-V Cl as cathode delivered a record peak power density of 6.2 mW cm −2 , offering a new route for simultaneous NO removal, NH 3 production, and energy supply.

关键词： Electrocatalytic NO Reduction Reaction (NORR) Low-Concentration NO NH3 Synthesis In Situ Spectroelectrochemical Cl Vacancy

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Hydrogen Evolution Reaction: Nitrogen-Doped Graphene-Encapsulated Nickel–Copper Alloy Nanoflower for Highly Efficient Electrochemical Hydrogen Evolution Reaction (Small 48/2019)

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Small 2019年第48期15卷

作者： Bin Liu Hui-Qing Peng Junye Cheng Kui Zhang Da Chen Dong Shen Shuilin Wu Tianpeng Jiao Xin Kong Qili Gao Shuyu Bu Chun-Sing Lee Wenjun Zhang Center of Super-Diamond and Advanced Films (COSDAF) and Department of Materials Science and Engineering City University of Hong Kong Tat Chee Avenue Kowloon Hong Kong China State Key Laboratory of Chemical Resource Engineering Beijing University of Chemical Technology Beijing 100029 China Department of Chemistry Institute for Advanced Study Institute of Molecular Functional Materials and Division of Biomedical Engineering The Hong Kong University of Science & Technology Clear Water Bay Kowloon Hong Kong China School of Chemistry and Chemical Engineering Anhui University of Technology Ma'anshan Anhui 243032 China Department of Mechanical and Biomedical Engineering City University of Hong Kong Tat Chee Avenue Kowloon Hong Kong China COSDAF and Department of Chemistry City University of Hong Kong Tat Chee Avenue Kowloon Hong Kong China City University of Hong Kong Shenzhen Research Institute Shenzhen 518057 China

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Single-atom Iron Catalyst with Biomimetic Active Center to Accelerate Proton Spillover for Medical-level Electrosynthesis of H2O2Disinfectant

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Angewandte Chemie 2023年第34期135卷

作者： Dr. Yan Li Dr. Junxiang Chen Yaxin Ji Zilin Zhao Wenjun Cui Dr. Xiahan Sang Dr. Yi Cheng Dr. Bin Yang Dr. Zhongjian Li Dr. Qinghua Zhang Prof. Dr. Lecheng Lei Prof. Dr. Zhenhai Wen Prof. Dr. Liming Dai Prof. Dr. Yang Hou Key Laboratory of Biomass Chemical Engineering of Ministry of Education College of Chemical and Biological Engineering Zhejiang University 310027 Hangzhou China Center of Advanced Carbon Materials School of Chemical Engineering University of New South Wales 2052 Sydney NSW Australia CAS Key Laboratory of Design and Assembly of Functional Nanostructures Fujian Provincial Key Laboratory of Nanomaterials Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences 350002 Fuzhou Fujian China Research and Testing Centre of Material School of Materials Science and Engineering Wuhan University of Technology 430070 Wuhan China Zhejiang Hengyi Petrochemical Research Institute Co. Ltd. 311200 Hangzhou China Institute of Zhejiang University—Quzhou 324000 Quzhou China Donghai Laboratory 316021 Zhoushan China

Electrosynthesis of H 2 O 2 has great potential for directly converting O 2 into disinfectant, yet it is still a big challenge to develop effective electrocatalysts for medical-level H 2 O 2 production. Herein, we report the design and fabrication of electrocatalysts with biomimetic active centers, consisting of single atomic iron asymmetrically coordinated with both nitrogen and sulfur, dispersed on hierarchically porous carbon (Fe SA -NS/C). The newly-developed Fe SA -NS/C catalyst exhibited a high catalytic activity and selectivity for oxygen reduction to produce H 2 O 2 at a high current of 100 mA cm −2 with a record high H 2 O 2 selectivity of 90 %. An accumulated H 2 O 2 concentration of 5.8 wt.% is obtained for the electrocatalysis process, which is sufficient for medical disinfection. Combined theoretical calculations and experimental characterizations verified the rationally-designed catalytic active center with the atomic Fe site stabilized by three-coordinated nitrogen atoms and one-sulfur atom (Fe-N 3 S-C). It was further found that the replacement of one N atom with S atom in the classical Fe-N 4 -C active center could induce an asymmetric charge distribution over N atoms surrounding the Fe reactive center to accelerate proton spillover for a rapid formation of the OOH* intermediate, thus speeding up the whole reaction kinetics of oxygen reduction for H 2 O 2 electrosynthesis.

关键词： H2O2 Production Medical-Level Disinfectant Fe Single Atom Proton Spillover Promoted Reaction Kinetics

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An Early Stage Researcher's Primer on Systems Medicine Terminology

Network and Systems Medicine

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Network and Systems Medicine 2021年第1期4卷 2-50页

作者： Zanin, Massimiliano Aitya, Nadim A.A. Basilio, José Baumbach, Jan Benis, Arriel Behera, Chandan K. Bucholc, Magda Castiglione, Filippo Chouvarda, Ioanna Comte, Blandine Dao, Tien-Tuan Ding, Xuemei Pujos-Guillot, Estelle Filipovic, Nenad Finn, David P. Glass, David H. Harel, Nissim Iesmantas, Tomas Ivanoska, Ilinka Joshi, Alok Boudjeltia, Karim Zouaoui Kaoui, Badr Kaur, Daman Maguire, Liam P. McClean, Paula L. McCombe, Niamh De Miranda, João Luís Moisescu, Mihnea Alexandru Pappalardo, Francesco Polster, Annikka Prasad, Girijesh Rozman, Damjana Sacala, Ioan Sanchez-Bornot, Jose M. Schmid, Johannes A. Sharp, Trevor Solé-Casals, Jordi Spiwok, Vojtěch Spyrou, George M. Stalidzans, Egils Stres, Blaa Sustersic, Tijana Symeonidis, Ioannis Tieri, Paolo Todd, Stephen Van Steen, Kristel Veneva, Milena Wang, Da-Hui Wang, Haiying Wang, Hui Watterson, Steven Wong-Lin, Kongfatt Yang, Su Zou, Xin Schmidt, Harald H.H.W. Centro de Tecnología Biomédica Universidad Politécnica de Madrid Madrid Spain Intelligent Systems Research Centre School of Computing Engineering and Intelligent Systems Ulster University Ulster United Kingdom Center for Physiology and Pharmacology Institute of Vascular Biology and Thrombosis Research Medical University of Vienna Vienna Austria TUM School of Life Sciences Weihenstephan Technical University of Munich Freising Germany Holon Israel CNR National Research Council IAC Institute for Applied Computing Rome Italy Lab of Computing Medical Informatics and Biomedical Imaging Technologies School of Medicine Aristotle University of Thessaloniki Thessaloniki Greece Université Clermont Auvergne INRAE UNH Plateforme d'Exploration du Métabolisme MetaboHUB Clermont Clermont-Ferrand France Université de Technologie de Compiègne Compiègne France Labex MS2T Control of Technological Systems-of-Systems CNRS and Université de Technologie de Compiègne Compiègne France Faculty of Engineering University of Kragujevac Kragujevac Serbia Kragujevac Serbia Steinbeis Advanced Risk Technologies Institute Doo Kragujevac Kragujevac Serbia Pharmacology and Therapeutics School of Medicine Galway Neuroscience Centre National University of Ireland Galway Ireland School of Computing Ulster University Ulster United Kingdom Holon Israel Department of Mathematics and Natural Sciences Kaunas University of Technology Kaunas Lithuania Faculty of Computer Science and Engineering Ss. Cyril and Methodius University Skopje Macedonia Medicine Faculty Université Libre de Bruxelles CHU de Charleroi Charleroi Belgium Northern Ireland Centre for Stratified Medicine Biomedical Sciences Research Institute Ulster University Ulster United Kingdom Escola Superior de Tecnologia e Gestão Instituto Politécnico de Portalegre Portalegre Portugal Instituto Superior Técnico Universidade de Lisboa Lisboa Portugal Faculty of Automatic Control and Computers University Politehnica of B

Background: Systems Medicine is a novel approach to medicine, that is, an interdisciplinary field that considers the human body as a system, composed of multiple parts and of complex relationships at multiple levels, and further integrated into an environment. Exploring Systems Medicine implies understanding and combining concepts coming from diametral different fields, including medicine, biology, statistics, modeling and simulation, and data science. Such heterogeneity leads to semantic issues, which may slow down implementation and fruitful interaction between these highly diverse fields. Methods: In this review, we collect and explain more than100 terms related to Systems Medicine. These include both modeling and data science terms and basic systems medicine terms, along with some synthetic definitions, examples of applications, and lists of relevant references. Results: This glossary aims at being a first aid kit for the Systems Medicine researcher facing an unfamiliar term, where he/she can get a first understanding of them, and, more importantly, examples and references for digging into the topic. © Massimiliano Zanin et al., 2021;Published by Mary Ann Liebert, Inc. 2021.

关键词： Semantics

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Damage sensing and mechanical characteristics of CFRP strengthened steel plate

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AIP Conference Proceedings 2017年第1期1892卷

作者： Genki Mieda Daiki Nakano Yuya Fuji Hitoshi Nakamura Yosuke Mizuno Kentaro Nakamura Takahiro Matsui Yutaka Ochi Yukihiro Matsumoto 1Department of Architecture and Civil Engineering Toyohashi University of Technology Hibarigaoka 1-1 Tempaku-cho Toyohashi-shi Japan 2Department of Architecture and Civil Engineering Toyohashi University of Technology Hibarigaoka 1-1 Tempaku-cho Toyohashi-shi Japan 3Department of Architecture and Civil Engineering Toyohashi University of Technology Hibarigaoka 1-1 Tempaku-cho Toyohashi-shi Japan 4Department of Civil and Environmental Engineering Tokyo Metropolitan University Minami-Osawa 1-1 Hachioji-shi Japan 5Laboratory for Future Interdisciplinary Research of Science and Technology Tokyo Institute of Technology 4259 Nagatsuta-cho Midori-ku Yokohama-shi Japan 6Laboratory for Future Interdisciplinary Research of Science and Technology Tokyo Institute of Technology 4259 Nagatsuta-cho Midori-ku Yokohama-shi Japan 7First Advanced Composites Technical Department Toray Industries Inc Ohe-cho 9-1 Minatoku Nagoya-shi Japan 8Advanced Composite Center Toray Industries Inc Oe-cho 9-1 Minatoku Nagoya-shi Japan 9Department of Architecture and Civil Engineering Toyohashi University of Technology Hibarigaoka 1-1 Tempaku-cho Toyohashi-shi Japan

In recent years, a large number of structures that were built during the period of high economic growth in Japan is beginning to show signs of aging. For example, the structural performance of steel structures has degraded due to corrosion. One measure that has been proposed and studied to address this issue is the adhesive bonding method, which can be used to repair and reinforce these structures. However, this method produces brittle fracture in the adhesive layer and is difficult to maintain after bonding. To solve the problem faced by this method, a clarification of the mechanical properties inside the adhesive is necessary. Then this background, a fiber Bragg grating (FBG) sensor has been used in this study. This sensor can be embedded within the building material that needs repairing and reinforcing because an FBG sensor is extremely small. Eventually based on this, a three-point bending test of a carbon fiber reinforced plastic (CFRP) strengthened steel plate that was embedded with an FBG sensor was conducted. This paper demonstrates that an FBG sensor is effectively applicable for sensing when damage occurs.

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Revealing the Origin of Transition-Metal Migration in Layered Sodium-Ion Battery Cathodes: Random Na Extraction and Na-Free Layer Formation

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Angewandte Chemie 2023年第12期135卷

作者： Dr. Shiyong Chu Prof. Duho Kim Gwanghyeon Choi Chunchen Zhang Haoyu Li Prof. Wei Kong Pang Yameng Fan Anita M. D'Angelo Prof. Shaohua Guo Prof. Haoshen Zhou College of Engineering and Applied Sciences Jiangsu Key Laboratory of Artificial Functional Materials National Laboratory of Solid State Microstructures Collaborative Innovation Center of Advanced Microstructures Frontiers Science Center for Critical Earth Material Cycling Nanjing University Nanjing 210023 China Shenzhen Research Institute of Nanjing University Shenzhen 518000 China Department of Mechanical Engineering (Integrated Engineering Program) Kyung Hee University 1732 Deogyeong-daero Giheung-gu Yongin-si Gyeonggi-do 17104 (Republic of Korea Institute for Superconducting & Electronic Materials University of Wollongong Wollongong NSW-2522 Australia Australian Synchrotron Australian Nuclear Science and Technology Organization 800 Blackburn Road Clayton Victoria 3168 Australia

Cation migration often occurs in layered oxide cathodes of lithium-ion batteries due to the similar ion radius of Li and transition metals (TMs). Although Na and TM show a big difference of ion radius, TMs in layered cathodes of sodium-ion batteries (SIBs) can still migrate to Na layer, leading to serious electrochemical degeneration. To elucidate the origin of TM migration in layered SIB cathodes, we choose NaCrO 2 , a typical layered cathode suffering from serious TM migration, as a model material and find that the TM migration is derived from the random desodiation and subsequent formation of Na-free layer at high charge potential. A Ru/Ti co-doping strategy is developed to address the issue, where the doped active Ru is first oxidized to create a selective desodiation and the doped inactive Ti can function as a pillar to avoid complete desodiation in Ru-contained TM layers, leading to the suppression of the Na-free layer formation and subsequent enhanced electrochemical performance.

关键词： Layered Sodium-Ion Battery Cathodes Na-Free Layer Random Na Extraction Selective Na Extraction Transition-Metal Migration

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Correction to: Semiconductor Electrochemistry for Clean Energy Conversion and Storage

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Electrochemical Energy Reviews 2023年第1期6卷 1-1页

作者： Zhu, Bin Fan, Liangdong Mushtaq, Naveed Raza, Rizwan Sajid, Muhammad Wu, Yan Lin, Wenfeng Kim, Jung-Sik Lund, Peter D. Yun, Sining Jiangsu Provincial Key Laboratory of Solar Energy Science and Technology/Energy Storage Joint Research Center School of Energy and Environment Southeast University Nanjing China Shenzhen Key Laboratory of New Lithium-Ion Batteries and Mesoporous Materials College of Chemistry and Environmental Engineering Shenzhen University Shenzhen China Clean Energy Research Lab (CERL) Department of Physics COMSATS University Islamabad Lahore Campus Lahore Pakistan Engineering Research Center of Nano-Geo Materials of Ministry of Education Faculty of Materials Science and Chemistry China University of Geosciences Wuhan China Department of Chemical Engineering School of Aeronautical Automotive Chemical and Materials Engineering Loughborough University Loughborough UK Department of Aeronautical & Automotive Engineering School of Aeronautical Automotive Chemical and Materials Engineering Loughborough University Loughborough UK Department of Engineering Physics/Advanced Energy Systems School of Science Aalto University Aalto Espoo Finland Functional Materials Laboratory (FML) School of Materials Science and Engineering Xi’an University of Architecture and Technology Xi’an China

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A Facile Strategy to Obtain Low-Cost and High-Performance Gold-Based Catalysts from Artificial Electronic Waste by [Zr48Ni6] Nano-Cages in MOFs for CO2Electroreduction to CO

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Angewandte Chemie 2022年第49期134卷

作者： Dr. Zi-Hao Zhu Ze-Long Liang Dr. Zhuo-Hao Jiao Dr. Xiao-Lei Jiang Yao Xie Dr. Hang Xu Prof. Bin Zhao Department of Chemistry Key Laboratory of Advanced Energy Material Chemistry (Ministry of Education) and Collaborative Innovation Center of Chemical Science and Engineering Nankai University Tianjin 300071 China School of Chemistry and Chemical Engineering Jiangxi Provincial Key Laboratory of Functional Molecular Materials Chemistry Jiangxi University of Science and Technology Ganzhou 341000 Jiangxi Province China Contribution: Conceptualization (equal) Investigation (lead) Writing - original draft (lead) Contribution: Investigation (supporting) Contribution: Conceptualization (equal) Funding acquisition (equal) Investigation (supporting) Supervision (equal) Writing - original draft (equal) Writing - review & editing (equal) Contribution: Conceptualization (equal) Funding acquisition (equal) Supervision (equal) Writing - review & editing (equal)

Expensive gold-based catalysts are frequently used for electrochemical CO 2 reduction into CO. A feasible approach to obtain low-cost Au-based catalysts is needed. Herein, a novel framework 1 assembled from [Zr 48 Ni 6 ] nano-cages is prepared. It exhibits a high BET surface area of 1569 m 2 g −1 and high solvents/pH stability. 1 can not only selectively extract AuCl 4 − from artificial electronic waste, but can then be transformed into low-cost catalyst Au nanoparticle@ 1 - x (Au NPs@ 1 - x , x =1, 2, 3, 4) with tuneable Au NPs sizes. The CO 2 RR investigations revealed that the Au NPs@ 1 -3 displayed an excellent FE CO of 95.2 % with a current density of 102.9 mA cm −2 at −1.1 V, and such high catalytic activity can be maintained for at least 15 h without obvious decrease because the confinement effect of [Zr 48 Ni 6 ] nano-cages prevents Au NPs agglomeration. This work offers a facile strategy to obtain low-cost and high-performance Au-based catalysts for various reactions activated by Au.

关键词： CO CO2 Electroreduction Gold Enrichment Low-Cost Catalysts MOFs

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Red Room Temperature Phosphorescence from Lignin

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Angewandte Chemie 2024年第10期137卷

作者： Hongda Guo Huanjie Cheng Ruixia Liu Xiaoxia Chen Luyao Wang Chenhui Yang Shujun Li Shouxin Liu Jian Li Qingjiang Pan Tony D. James Zhijun Chen Key Laboratory of Bio-based Material Science and Technology of Ministry of Education Northeast Forestry University Harbin 150040 P. R. China International joint lab of advanced biomass materials Northeast Forestry University Heilongjiang Province Harbin 150040 P. R. China Key Laboratory of Functional Inorganic Material Chemistry (Ministry of Education) School of Chemistry and Materials Science Heilongjiang University Harbin 150080 P. R. China Department of Chemistry University of Bath Bath BA2 7AY United Kingdom School of Chemistry and Chemical Engineering Henan Normal University Xinxiang 453007 P. R. China

Materials with red room-temperature phosphorescence (RTP) derived from sustainable resources are crucial but rarely reported. Here, we produced red RTP materials from lignin. Lignin was covalently modified with Upy (1-(6-isocyanatohexyl)-3-(6-methyl-4-oxo-1,4-dihydropyrimidin-2-yl) urea) to obtain Lig-Upy. The Upy in the Lig-Upy promoted the interaction between the aromatic units of lignin and reduced energy gaps of these molecules. As a result, Lig-Upy exhibited red RTP centered at 625 nm with a lifetime of 24.2 ms. Moreover, the hydrogen bonding interactions in Lig-Upy varied when embedded into different matrices, such as polyvinyl alcohol (PVA) or sodium montmorillonite (MTM), inducing a change in RTP wavelength and lifetime. Utilizing these properties, Lig-Upy was used as building blocks for producing materials exhibiting time-dependent phosphorescent colors (TDPCs). Such TDPCs materials have exhibited great potential for visual decorations, information encryption and anti-counterfeiting logos for medicine bottles.

关键词： Lignin Red RTP materials Multiple hydrogen bonds TDPCs

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