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A novel fluorescent probe for volatile amine vapor detection

Chinese Chemical Letters 2024年第3期35卷 3-4页

作者： Lulu Bu Daofu Liu Longde Wang Mei Sun Chao Gao Yongshu Xie School of Chemistry and Materials Engineering Anhui Province Key Laboratory of Low Temperature Co-Fired MaterialsHuainan Normal UniversityHuainan 232038China College of Material Chemistry and Chemical EngineeringKey Laboratory of Organosilicon Chemistry and Material Technology of Ministry of EducationHangzhou Normal UniversityHangzhou 311121China Shanghai Key Laboratory of Functional Materials Chemistry Key Laboratory for Advanced Materials and Institute of Fine ChemicalsSchool of Chemistry&Molecular EngineeringEast China University of Science&TechnologyShanghai 200237China

In recent years,fluorescent probes have gained significant prominence in the field of substance analysis and detection[1–4].The development of high-performance volatile amine gas sensors is crucial for applications i... 详细信息

关键词： volatile gained probe

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Strain engineering in electrocatalysis:Strategies,characterization,and insights

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Nano Research 2024年第5期17卷 3603-3621页

作者： Qibo Deng Peng Xu Hassanien Gomaa Mohamed A.Shenashen Sherif A.El-Safty Cuihua An Li-Hua Shao Ning Hu School of Mechanical Engineering Hebei University of TechnologyTianjin 300401China Department of Chemistry Faculty of ScienceAl-Azhar University71524AssiutEgypt Department of Petrochemical Egyptian Petroleum Research Institute(EPRI)Nasr City11727CairoEgypt Center for Functional Materials National Institute for Materials Science(NIMS)1-2-1 SengenTsukubaIbaraki-ken305-0047Japan State Key Laboratory of Reliability and Intelligence Electrical Equipment Key Laboratory of Advanced Intelligent Protective Equipment TechnologyMinistry of Educationand School of Mechanical EngineeringHebei University of TechnologyTianjin 300401China National Key Laboratory of Strength and Structural Integrity Institute of Solid MechanicsSchool of Aeronautic Science and EngineeringBeihang UniversityBeijing100191China Advanced Equipment Research Institute Co. Ltd.of HEBUTTianjin 300401China

Strain engineering,as a cutting-edge method for modulating the electronic structure of catalysts,plays a crucial role in regulating the interaction between the catalytic surface and the adsorbed *** electrocatalytic performance is influenced by the electronic structure,which can be achieved by introducing the external forces or stresses to adjust interatomic spacing between surface *** challenges in strain engineering research lie in accurately understanding the mechanical impact of strain on *** paper first introduces the basic strategy for generating the strain,summarizes the different strain generation forms and their advantages and *** progress in researching the characterization means for the lattice strains and their applications in the field of electrocatalysis is also ***,the challenges of strain engineering are introduced,and an outlook on the future research directions is provided.

关键词： strain electrocatalysis characterization chemical reaction kinetics lattice mismatch

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Chip-integrated quantum signature network over 200 km

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Light(science & Applications) 2025年第4期14卷 1061-1069页

作者： Yongqiang Du Bing-Hong Li Xin Hua Xiao-Yu Cao Zhengeng Zhao Feng Xie Zhenrong Zhang Hua-Lei Yin Xi Xiao Kejin Wei Guangxi Key Laboratory for Relativistic Astrophysics School of Physical Science and TechnologyGuangxi UniversityNanning 530004China National Laboratory of Solid State Microstructures and School of Physics Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210093China National Information Optoelectronics Innovation Center(NOEIC) Wuhan 430074China Guangxi Key Laboratory of Multimedia Communications and Network Technology School of ComputerElectronicsand InformationGuangxi UniversityNanning 530004China Department of Physics and Beijing Key Laboratory of Opto-electronic Functional Materials and Micro-nano Devices Key Laboratory of Quantum State Construction and Manipulation(Ministry of Education)Renmin University of ChinaBeijing 100872China Peng Cheng Laboratory Shenzhen 518055China

The development of quantum networks is paramount towards practical and secure *** digital signatures(QDS)offer an information-theoretically secure solution for ensuring data integrity,authenticity,and nonrepudiation,rapidly growing from proof-of-concept to robust ***,previous QDS systems relied on expensive and bulky optical equipment,limiting large-scale deployment and reconfigurable networking ***,we introduce and verify a chip-based QDS network,placing the complicated and expensive measurement devices in the central relay while each user needs only a low-cost *** demonstrate the network with a three-node setup using an integrated encoder chip and decoder *** developing a 1-decoy-state one-time universal hashing-QDS protocol,we achieve a maximum signature rate of 0.0414 times per second for a 1 Mbit messages over fiber distances up to 200 km,surpassing all current state-of-the-art QDS *** study validates the feasibility of chip-based QDS,paving the way for large-scale deployment and integration with existing fiber infrastructure.

关键词： secure communications quantum networks chip based network large scale deployment digital signatures qds offer quantum digital signatures fiber distances decoy state protocol

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A case study of comparing two dimerized acceptor molecules built by different branch-connected and terminal-connected approaches

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science China Chemistry 2024年第5期67卷 1687-1696页

作者： Kangqiao Ma Huazhe Liang Yuxin Wang Tengfei He Tainan Duan Xiaodong Si Wendi Shi Guankui Long Xiangjian Cao Zhaoyang Yao Xiangjian Wan Chenxi Li Bin Kan Yongsheng Chen State Key Laboratory and Institute of Elemento-Organic Chemistry Frontiers Science Center for New Organic MatterThe Centre of Nanoscale Science and Technology and Key Laboratory of Functional Polymer MaterialsInstitute of Polymer ChemistryRenewable Energy Conversion and Storage Center(RECAST)College of ChemistryNankai UniversityTianjin 300071China School of Materials Science and Engineering National Institute for Advanced MaterialsRenewable Energy Conversion and Storage Center(RECAST)Nankai UniversityTianjin 300350China Chongqing Institute of Green and Intelligent Technology Chongqing SchoolUniversity of Chinese Academy of Sciences(UCAS Chongqing)Chinese Academy of SciencesChongqing 400015China

Dimerized small-molecule acceptors(SMAs) built by the conventional connection of terminal groups of monomers have contributed to exciting long-term stabilities of organic solar cells(OSCs). However, device efficiencies, especially fill factors(FFs), still need to be improved. This probably originates from unsymmetrical molecular structure/conformation-determined less compact/ordered molecular stackings, such as ineffective stackings of constraint terminals. Herein, an exotic dimerized SMA of BC-Th is established by bridging the branched groups(BC-type, branch coupling) of two monomers rather than conventional terminal units(TC-type, terminal coupling). Benefiting from the three-dimensional conformation and more uncurbed terminals,BC-Th exhibits multiple molecular orientations along with a larger dielectric constant and electron mobility compared with TCTh. Finally, an efficiency of 17.43% is achieved by BC-Th-based OSCs, along with the highest FF of 79.13% among all dimerized SMAs-based OSCs to date. When introducing L8-BO as the third component, overall enhanced efficiency of 18.05%and FF of 80.11% are further afforded. Contrarily, TC-Th-based OSCs exhibit much inferior PCE of 16.29% and FF of 74.81%,demonstrating the great advantages of “branch coupling” over “terminal coupling” when building dimerized SMAs.

关键词： organic solar cells dimerized acceptor molecules branch coupling morphology control stability

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Graphitic carbon nitride-based photocatalysts in the applications of environmental catalysis

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Journal of Environmental sciences 2023年第2期124卷 570-590页

作者： Hongxia Lin JinmoWu Fan Zhou Xiaolong Zhao Pengfei Lu Guanghui Sun Yuhan Song Yayun Li Xiaoyong Liu Hongxing Dai Hefei Institute for Public Safety Research Tsinghua UniversityHefei 230601China Anhui Province Key Laboratory of Human Safety Hefei 230601China Beijing Key Laboratory for Green Catalysis and Separation Key Laboratory of Beijing on Regional Air Pollution ControlKey Laboratory of Advanced Functional MaterialsEducation Ministry of ChinaLaboratory of Catalysis Chemistry and NanoscienceDepartment of Environmental Chemical EngineeringSchool of Environmental and Chemical EngineeringFaculty of Environment and Life ScienceBeijing University of TechnologyBeijing 100124China

Semiconductor photocatalytic technology has shown great prospects in converting solar energy into chemical energy to mitigate energy crisis and solve environmental pollution *** key issue is the development of high-efficiency *** strategies in the state-of-the-art advancements,such as heterostructure construction,heteroatom doping,metal/single atom loading,and defect engineering,have been presented for the graphitic carbon nitride(g-C3N4)-based nanocomposite catalysts to design their surface chemical environments and internal electronic structures to make them more suitable for different photocatalytic *** this review,nanoarchitecture design,synthesis methods,photochemical properties,potential photocatalytic applications,and related reaction mechanisms of the modified high-efficiency carbon nitride-based photocatalysts were briefly *** superior photocatalytic performance was identified to be associated with the enhanced visible-light response,fast photoinduced electron-hole separation,efficient charge migration,and increased unsaturated active ***,the further advance of the visible-light harvesting and solar-to-energy conversions are proposed.

关键词： Graphitic carbon nitride-based photocatalyst Photocatalytic reduction Photocatalytic degradation Chemical modification Heterostructure construction Metal doping

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Highly Thermoconductive,Strong Graphene‑Based composite Films by Eliminating Nanosheets Wrinkles

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Nano-Micro Letters 2024年第1期16卷 328-340页

作者： Guang Xiao Hao Li Zhizhou Yu Haoting Niu Yagang Yao College of Engineering and Applied Sciences Jiangsu Key Laboratory of Artificial Functional Materialsand Collaborative Innovation Center of Advanced MicrostructuresNational Laboratory of Solid State MicrostructuresNanjing UniversityNanjing 210093People’s Republic of China Institute of Laser Manufacturing Henan Academy of SciencesZhengzhou 450052People’s Republic of China Center for Quantum Transport and Thermal Energy Science School of Physics and TechnologyNanjing Normal UniversityNanjing 210023People’s Republic of China

Graphene-based thermally conductive composites have been proposed as effective thermal management materials for cooling high-power electronic ***,when flexible graphene nanosheets are assembled into macroscopic thermally conductive composites,capillary forces induce shrinkage of graphene nanosheets to form wrinkles during solution-based spontaneous drying,which greatly reduces the thermal conductivity of the ***,graphene nanosheets/aramid nanofiber(GNS/ANF)composite films with high thermal conductivity were prepared by in-plane stretching of GNS/ANF composite hydrogel networks with hydrogen bonds andπ-π*** in-plane mechanical stretching eliminates graphene nanosheets wrinkles by suppressing inward shrinkage due to capillary forces during drying and achieves a high in-plane orientation of graphene nanosheets,thereby creating a fast in-plane heat transfer *** composite films(GNS/ANF-60 wt%)with eliminated graphene nanosheets wrinkles showed a significant increase in thermal conductivity(146 W m^(−1)K^(−1))and tensile strength(207 MPa).The combination of these excellent properties enables the GNS/ANF composite films to be effectively used for cooling flexible LED chips and smartphones,showing promising applications in the thermal management of high-power electronic devices.

关键词： Graphene Aramid nanofiber Wrinkles elimination In-plane stretching Thermal conductivity

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Dealloyed TiCuMn efficiently catalyze the NO reduction and Zn-NO batteries

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Frontiers of Chemical science and Engineering 2024年第9期18卷 51-59页

作者： Lang Zhang Tong Hou Weijia Liu Yeyu Wu Tianran Wei Junyang Ding Qian Liu Jun Luo Xijun Liu State Key Laboratory of Featured Metal Materials and Life-Cycle Safety for Composite Structures MOE Key Laboratory of New Processing Technology for Nonferrous Metals and MaterialsSchool of ResourcesEnvironment and MaterialsGuangxi UniversityNanning 530004China Education Department of Guangxi Zhuang Autonomous Region Key Laboratory of Applied Analytical ChemistryGuangxi Collaborative Innovation Center for Chemistry and Engineering of Forest ProductsGuangxi Key Laboratory of Chemistry and Engineering of Forest ProductsKey Laboratory of Chemistry and Engineering of Forest ProductsState Ethnic Affairs CommissionSchool of Chemistry and Chemical EngineeringGuangxi Minzu UniversityNanning 530006China Institute for New Energy Materials&Low-Carbon Technologies School of Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China Institute for Advanced Study Chengdu UniversityChengdu 610106China ShenSi Lab Shenzhen Institute for Advanced StudyUniversity of Electronic Science and Technology of ChinaShenzhen 518110China

Electrocatalytic NO reduction reaction offers a sustainable route to achieving environmental protection and NH3 production targets as *** this work,a class of dealloyed Ti_(60)Cu_(33)Mn_(7)ribbons with enough nanoparticles for the high-efficient NO reduction reaction to NH_(3)is fabricated,reaching an excellent Faradaic efficiency of 93.2%at–0.5 V vs reversible hydrogen electrode and a high NH_(3) synthesis rate of 717.4μmol·h^(-1)·mg_(cat).^(-1) at–0.6 V vs reversible hydrogen *** formed nanoparticles on the surface of the catalyst could facilitate the exposure of active sites and the transportation of various reactive ions and ***,the Mn content in the TiCuMn ribbons modulates the chemical and physical properties of its surface,such as modifying the electronic structure of the Cu species,optimizing the adsorption energy of N^(*)atoms,decreasing the strength of the NO adsorption,and eliminating the thermodynamic energy barrier,thus improving the NO reduction reaction catalytic ***,a Zn-NO battery was fabricated using the catalyst and Zn plates,generating an NH_(3) yield of 129.1µmol·h^(-1)·cm^(-2)while offering a peak power density of 1.45 mW·cm^(-2).

关键词： nitric oxide reduction NH_(3)electrosynthesis TiCuMn alloy Mn modulation Zn-NO battery

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Diameter-dependent photoelectric performances of semiconducting carbon nanotubes/perovskite heterojunctions

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Nano Research 2023年第11期16卷 12662-12669页

作者： Yayang Yu Wenke Wang Xiao Li Linhai Li Shilong Li Xiaojun Wei Weiya Zhou Jing Lin Yang Huang Huaping Liu School of Materials Science and Engineering Hebei Key Laboratory of Boron Nitride Micro and Nano MaterialsHebei University of TechnologyTianjin 300130China Beijing National Laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China Center of Materials Science and Optoelectronics Engineering School of Physical SciencesUniversity of Chinese Academy of SciencesBeijing 100049China Beijing Key Laboratory for Advanced Functional Materials and Structure Research Beijing 100190China Songshan Lake Materials Laboratory Dongguan 523808China

The heterojunction of single-wall carbon nanotubes(SWCNTs)and perovskite quantum dots(QDs)shows excellent photodetection performances due to the combination of the advantages of high carrier mobility of SWCNTs and high absorption coefficient of perovskite ***,the band structure of a SWCNT is determined by its atomic arrangement *** the structure of SWCNTs affects the photoelectric performance of the composite film remains ***,we systematically explored the diameter effect of SWCNTs with different bandgaps on the photodetection performances of SWCNTs/perovskite QDs heterojunction films by integrating semiconducting SWCNTs(s-SWCNTs)with different diameters with CsPbBr3 *** results show that with an increase in diameter of s-SWCNTs,the heterojunction exhibits increasing responsivity(R),detectivity(D*),and faster response *** great improvement in the optoelectronic performances of devices should be attributed to the higher carrier mobility of larger-diameter SWCNT films and the increasing built-in electric field at the heterojunction interfaces between larger-diameter SWCNTs and CsPbBr3 QDs,which enhances the separation of the photogenerated excitons and the transport of the resulted carriers in SWCNT films.

关键词： carbon nanotubes perovskite quantum dots diameter effect responsivity detectivity

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Continuum of spin excitations in an ordered magnet

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The Innovation 2025年第4期6卷 83-88,82页

作者： Jieming Sheng Le Wang Wenrui Jiang Han Ge Nan Zhao Tiantian Li Maiko Kofu Dehong Yu Wei Zhu Jia-Wei Mei Zhentao Wang Liusuo Wu Department of Physics Southern University of Science and TechnologyShenzhen 518055China School of Physical Sciences Great Bay University and Great Bay Institute for Advanced StudyDongguan 523000China Shenzhen Institute for Quantum Science and Engineering Southern University of Science and TechnologyShenzhen 518055China International Quantum Academy Shenzhen 518048China J-PARC Center Japan Atomic Energy AgencyTokaiIbaraki 319-1195Japan Australian Nuclear Science and Technology Organisation Lucas HeightsNSW 2234Australia School of Science Westlake UniversityHangzhou 310030China Institute of Natural Sciences Westlake Institute of Advanced StudyHangzhou 310024China Shenzhen Key Laboratory of Advanced Quantum Functional Materials and Devices Southern University of Science and TechnologyShenzhen 518055China Center for Correlated Matter and School of Physics Zhejiang UniversityHangzhou 310058China

Spin excitation continua observed in neutron scattering studies are often considered to be strong evidence of quantum spin liquid *** a disorder-free magnetic compound with a quantum spin liquid ground state,the elementary excitation is no longer the conventional spin waves(magnons).Instead,the magnons fractionalize into spinons,producing a characteristic two-spinon ***,it remained uncertain whether a clean,ordered antiferromagnet could exhibit a continuous spectrum similar to that of a quantum spin *** paper presents evidence of a spin excitation continuum in the magnetically ordered state of Na_(2)BaCo(PO_(4))_(2),where free spinons are *** challenges the interpretation of such a continuum as a definitive signature of a quantum spin liquid in new material studies.

关键词： spin excitation continua spin excitation continuum neutron scattering studies spin waves magnons insteadthe quantum spin liquid ordered antiferromagnet magnons spinons

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The first chiral cerium halide towards circularly-polarized luminescence in the UV region

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science China Chemistry 2024年第6期67卷 1961-1968页

作者： Xinyi Niu Zhichao Zeng Zhaoyu Wang Haolin Lu Bing Sun Hao-Li Zhang Yongsheng Chen Yaping Du Guankui Long Tianjin Key Lab for Rare Earth Materials and Applications Renewable Energy Conversion and Storage CenterSmart Sensing Interdisciplinary Science CenterSchool of Materials Science and EngineeringNational Institute for Advanced MaterialsNankai UniversityTianjin300350China Tianjin Key Lab for Rare Earth Materials and Applications Center for Rare Earth and Inorganic Functional MaterialsHaihe Laboratory of Sustainable Chemical TransformationsSmart Sensing Interdisciplinary Science CenterSchool of Materials Science and EngineeringNational Institute for Advanced MaterialsNankai UniversityTianjin300350China State Key Laboratory of Applied Organic Chemistry Key Laboratory of Special Function Materials and Structure Design(Ministry of Education)College of Chemistry and Chemical EngineeringLanzhou UniversityLanzhou730000China The Centre of Nanoscale Science and Technology and State Key Laboratory of Elemento-Organic Chemistry Frontiers Science Center for New Organic MatterCollege of ChemistryNankai UniversityTianjin300071China

Chiral organic-inorganic hybrid metal halides(OIHMHs)have attracted broader scientific community recently in spin lightemitting diodes,and circularly polarized light-emitting ***,the emission peaks of the reported chiral OIHMHs mainly locate in the visible region,and chiral OIHMH with ultraviolet(UV)circularly polarized luminescence(CPL)has been rarely *** fill this gap,cerium,a unique rare-earth(RE)element with tunable luminescence from UV to the visible region owing to the 4 f-related electronic transition,was introduced to construct the first RE-based chiral OIHMHs,R/*** chirality is successfully transferred from the chiral organic cations to the inorganic cerium chloride framework in R/S-MCC,as confirmed by the single crystal structures,circular dichroism,and *** emission spectra of R/S-MCC are in the UV region,originating from the characteristic d-f transition of Ce^(3+),which making the Ce-based metal halides are ideal candidates towards CPL light sources in the UV ***,R-and S-MCC are the first RE-based OIHMHs,also the first chiral metalhalides with UV *** work opens a new avenue for the development of the chiral OIHMH family towards RE-based chiral *** RE-based chiral metal halides couple the unique and superior optical,electrical,magnetic,and spintronic properties of RE elements with chirality could accelerate the development of chiral optoelectronics and spintronics toward real applications.

关键词： chiral rare-earth halide ultraviolet circularly-polarized luminescence d-f transition rare-earth halide perovskite chiral perovskite

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