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Aggregate 2024年第2期5卷 222-228页

作者： Zhongyu Li Kexin Fu Huangjun Deng Kaixuan Nie Zhe Pan Zhu Mao Juan Zhao Gang Li Pengli Zhu Zhenguo Chi Rong Sun National Key Laboratory of Materials for Integrated Circuits Shenzhen Institute of Advanced Electronic MaterialsShenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhenChina PCFM Lab GDHPPC LabGuangdong Engineering Technology Research Center for High-performance Organic and Polymer Photoelectric Functional FilmsState Key Laboratory of OEMTSchool of ChemistrySun Yat-sen UniversityGuangzhouChina State Key Laboratory of Optoelectronic Material and Technologies School of Materials Science and EngineeringSun Yat-sen UniversityGuangzhouChina

Polymeric ultralong organic phosphorescence(UOP)with persistent emission is of great importance in practical ***,achieving good water-resistance for long-term environmental stability is a formidable *** this contribution,through tailoring the alkyl-chain length of the hardeners and emitters,polymeric UOPs with varying crosslinking density and hydrophobic effect were ***,all the polymers show no obvious decrease in UOP emission after high temperature-humidity test(85℃/85%relative humidity for 7 days).Detailed investigations demonstrate that the rigid covalent crosslinking networks suppress the quenching of triplet excitons while the hydrophobic microenvironment affords good water/moisture-resistance ***,the polymers with superior processability are successfully applied as optical coatings,prepreg,and afterglow *** this work,we provide a new strategy to promote the long-term stability of polymeric UOP materials in high-temperature-humidity conditions.

关键词： aqueous environment hydrophobic effect long-term stability polymeric phosphorescence room temperature phosphorescence

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Wide-range color-tunable afterglow emission by the modulation of triplet exciton transition processes based on buckybowl structure

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Aggregate 2023年第4期4卷 93-99页

作者： Yongfeng Zhang Chenchen Xiong Wenbo Wang Wenbo Dai Yue Ren Junming Xia Gengchen Li Jianbing Shi Bin Tong Xiaoyan Zheng Xiangfeng Shao Zhengxu Cai Yuping Dong Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications School of Materials Science and EngineeringBeijing Institute of TechnologyBeijingChina State Key Laboratory of Applied Organic Chemistry College of Chemistry and Chemical EngineeringLanzhou UniversityLanzhouChina Beijing Key Laboratory of Photoelectronic/Electrophotonic Conversion Materials Key Laboratory of Cluster Science of the Ministry of EducationSchool of Chemistry and Chemical EngineeringBeijing Institute of TechnologyBeijingChina

Buckybowl structures as non-uniform electrostatic potential distributions of poly-cyclic aromatic materials show a unique photoelectric *** this work,OTC was utilized for dynamic modulation of triplet exciton transition *** host molecules with different functional units were selected,thus providing dif-ferent intermolecular interactions in the host/guest ***,the delayed emissions were regulated from 536 to 624 nm via the tuning of the triplet exciton transition processes of OTC in different *** data and theoretical calculations revealed that the varied triplet transition behaviors resulted from the competition between the intersystem crossing(ISC)process of OTC-monomer and the reverse intersystem crossing(RISC)process of *** work proves the superior structure of buckybowl-based luminophore for controlling triplet exciton transition processes and supplies a new perspective for persistent afterglow luminophore design.

关键词： buckybowl structure dynamic modulation host/guest doping systems room temperature phosphores-cence triplet exciton transition processes

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Yarn-based superhydrophobic wearable sensors for ammonia gas detection at room temperature

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Frontiers of materials science 2025年第1期19卷 51-62页

作者： Hao Zhao Tao Yang Hao-Kai Peng Hai-Tao Ren Bing-Chiuan Shiu Jia-Horng Lin Ting-Ting Li Ching-Wen Lou School of Textile Science and Engineering Tiangong UniversityTianjin 300387China Tianjin and Ministry of Education Key Laboratory for Advanced Textile Composite Materials Tiangong UniversityTianjin 300387China College of Materials and Chemical Engineering Minjiang UniversityFuzhou 350108China Advanced Medical Care and Protection Technology Research Center College of Textile and ClothingQingdao UniversityQingdao 266071China Shaoxing Keqiao Institute of Tiangong University Shaoxing 312030China

Conventional metal-oxide-semiconductor(MOS)gas sensors are limited in wearable gas detection due to their non-flexibility,high operating temperature,and less *** this study,a yarn-based superhydrophobic flexible wearable sensor for room-temperature ammonia gas detection was prepared based on the nano-size effect of both nanocore yarns prepared through electrostatic spinning and MOS gas-sensitive materials synthesized via a two-step hydrothermal synthesis *** yarn sensor has a response sensitivity of 13.11 towards 100 ppm(1 ppm=10^(−6))ammonia at room temperature,a response time and a recovery time of 36 and 21 s,respectively,and a detection limit as low as 10 ppm with the sensitivity of up to 4.76 towards *** addition,it displays commendable linearity within the concentration range of 10‒100 ppm,accompanied by remarkable selectivity and stability,while the hydrophobicity angle reaches 155.74°.Furthermore,its sensing performance still maintains stability even after repeated bending and prolonged *** sensor also has stable mechanical properties and flexibility,and can be affixed onto the fabric surface through sewing,which has a specific potential for clothing use.

关键词： ammonia sensor superhydrophobicity metal oxide semiconductor flexible wearable sensor

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Large enhancement of magnetocaloric effect induced by dual regulation effects of hydrostatic pressure in Mn_(0.94)Fe_(0.06)NiGe compound

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Journal of materials science & technology 2022年第19期114卷 73-80页

作者： He Zhou Dekun Wang Zhe Li Junzhuang Cong Ziyuan Yu Shuo Zhao Peng Jiang Daoyong Cong Xinqi Zheng Kaiming Qiao Hu Zhang School of Materials Science and Engineering University of Science and Technology BeijingBeijing 100083China College of Physics and Electronic Engineering Key Laboratory for Advanced Functional and Low Dimensional Materials of Yunnan Higher Education InstituteQujing Normal UniversityQujing 655011China MultiFields Technologies(Beijing)Co.Ltd. Beijing 100190China State Key Laboratory for Advanced Metals and Materials University of Science and Technology BeijingBeijing 100083China

MM'X(M,M'=transition metals,X=carbon or boron group elements)compounds could exhibit large magnetocaloric effect due to the magnetostructural transition,and the composition regulation has been widely studied to realize the magnetostructural ***,the magnetostructural transition is also sensitive to the ***,the effect of hydrostatic pressure on magnetostructural transformation and magnetocaloric effect has been investigated in Mn_(0.94)Fe_(0.06)NiGe *** regulation effect of lowering structural transition temperature and strengthening ferromagnetic(FM)state of martensite is realized by applying hydrostatic pressure,which would greatly improve the magnetocaloric effect of Mn_(0.94)Fe_(0.06)NiGe ***,the first-principles calculations have also been performed to discuss the origin of the regulation effect under hydrostatic pressure,and it indicates that the hydrostatic pressure can stabilize the hexagonal structure and decrease the structural transition *** maximum isothermal entropy change increases by 109%from 4.3 J/(kg K)under 0 GPa to 9.0 J/(kg K)under 0.402 GPa for a magnetic field change of 0-3 *** work proves that the hydrostatic pressure is an effective method to regulate the magnetostructural transition and enhance magnetocaloric effect in MM'X compounds.

关键词： Magnetocaloric effect Magnetostructural transition Hydrostatic pressure Magnetic properties

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Improved material descriptors for bulk modulus in intermetallic compounds via machine learning

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Rare Metals 2023年第7期42卷 2396-2405页

作者： De-Xin Zhu Kun-Ming Pan Yuan Wu Xiao-Ye Zhou Xiang-Yue Li Yong-Peng Ren Sai-Ru Shi Hua Yu Shi-Zhong Wei Hong-Hui Wu Xu-Sheng Yang National Joint Engineering Research Center for Abrasion Control and Molding of Metal Materials Henan Key Laboratory of High-Temperature Structural and Functional MaterialsHenan University of Science and TechnologyLuoyang471003China Longmen Laboratory Luoyang471003China State Key Laboratory for Advanced Metals and Materials University of Science and Technology BeijingBeijing100083China Guangdong Province Key Laboratory of Durability for Marine Civil Engineering School of Civil EngineeringShenzhen UniversityShenzhen518060China Department of Industrial and Systems Engineering The Hong Kong Polytechnic UniversityHong Kong999077China

Bulk modulus is an important mechanical property in the optimal design and selection of intermetallic *** this study,bulk modulus datasets of intermetallic compounds were collected,and the features affecting the bulk modulus of intermetallics were screened via feature *** features B_(cal),dB_(avg),and TIE(corresponding to calculated bulk modulus,mean bulk modulus,and third ionization energy,respectively)were found to be the dominant factors influencing bulk modulus and can be extended to other multi-component ***,we predicted the bulk modulus with an accuracy of 95%using surrogate machine learning models with the selected features,and these features were also demonstrated to be effective for high-entropy ***,symbolic regression provided an expression for the relationship between bulk modulus and the screened *** machine learning models provide a new approach for optimizing and predicting the bulk moduli of intermetallic compounds.

关键词： Bulk modulus Intermetallic compounds Machine learning Symbolic regression

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A facile process to optimize performance of regenerated Nd-Fe-B sintered magnets:Chemo-selective dissolution washing

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Journal of Rare Earths 2023年第12期41卷 1976-1983,I0006页

作者： Haibo Xu Qingmei Lu Lichao Yu Liying Cong Haowen Tian Weiqiang Liu Youhao Liu Yunqiao Wang Jingwu Chen Xiaofei Yi Qiong Wu Ming Yue College of Materials Science&Engineering Key Lab of Advanced Functional MaterialsBeijing University of TechnologyBeijing100124China Ganjiang Innovation Academy Chinese Academy of SciencesGanzhou341119China State Key Laboratory of Rare Earth Permanent Magnetic Materials Hefei231500China Earth-Panda Advanced Magnetic Materials Co. Ltd.Hefei231500China Beijing Zhong Ke San Huan Research Beijing102200China

In this work,the recycled Nd-Fe-B powders and regenerated Nd-Fe-B sintered magnets with low impurity content were successfully prepared from Nd-Fe-B magnet sludge via reduction diffusion(RD)method followed by a chemo-selective dissolution washing proc *** chemo-selective dissolution effect of various solution(deionized water,dilute acetic acid solution,NH_(4)Cl-methanol solution) was evaluated by impurity content and magnetic properties of the recycled Nd-Fe-B *** NH_(4)Cl-methanol solution can selectively remove impurities with minimal damage to the magnetic ***,the optimal NH_(4)Cl concentration and liquid-to-solid ratio were *** a consequence,the contents of Ca,O,and H after optimal washing process are reduced to 0.07 wt%,0.31 wt% and 0.22 wt%,***,M_(3) Tis increased to 146.72 emu/g,which is 33% higher than that of the initial ***,the regenerated Nd-Fe-B sintered magnets with properties of B_(r)=11.66 kG,H_(cj)=16.49 kOe,and(BH)_(m)=31.78 MGOe were successfully prepared by mixing with 40 wt% Nd4Fe14B alloy *** with the corresponding regenerated magnets washed with deionized water,the remanence and coercivity are increased by 18% and 59%,respectively.

关键词： Recycling Nd-Fe-B magnet Sludge Chemo-selective dissolution Washing process Magnetic properties Reduction diffusion Rare earths

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Revealing the role of electrode potential micro-environments in single Mn atoms for carbon dioxide and oxygen electrolysis

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Nano Research 2024年第9期17卷 7957-7966页

作者： Pengcheng Liu anyi Liu Kaili Wang Shuai Shi Mengmeng Jin Jingxiu Liu Tao Qin Qian Liu Xijun Liu Jia He Tianjin Key Laboratory of Organic Solar Cells and Photochemical Conversion School of Chemistry and Chemical EngineeringInstitute of New-Energy Materials and Low-Carbon TechnologiesSchool of Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China School of Chemistry and Chemical Engineering and Environmental Engineering Weifang UniversityWeifang 261061China Department of Electrical Engineering and Automation Luoyang Institute of Science and TechnologyLuoyang 471023China Institute for Advanced Study Chengdu UniversityChengdu 610106China State Key Laboratory of Featured Metal Materials and Life-cycle Safety for Composite Structures Guangxi Key Laboratory of Processing for Non-ferrous Metals and Featured MaterialsSchool of ResourcesEnvironment and MaterialsGuangxi UniversityNanning 530004China

Elucidation the relationship between electrode potentials and heterogeneous electrocatalytic reactions has attracted widespread *** we construct the well-defined Mn single-atom(MnSA)catalyst with four N-coordination through a simple thermal pyrolysis preparation method to investigate the electrode potential micro-environments effect on carbon dioxide reduction reactions(CO_(2)RR)and oxygen reduction reactions(ORR).MnSA catalysts generate higher CO production Faradaic efficiency of exceeding 90%at-0.9 V for CO_(2)RR and higher H_(2)O_(2)yield from 0.1 to 0.6 V with excellent ORR *** functional theory(DFT)calculations based on constant potential models were performed to study the mechanism of MnSA on CO_(2)*** thermodynamic energy barrier of CO_(2)RR is lowest at-0.9 V *** hydrogen electrode(RHE).Similar DFT calculations on the H_(2)O_(2)yield of ORR showed that the H_(2)O_(2)yield at 0.2 V was *** study provides a reasonable explanation for the role of electrode potential micro-environments.

关键词： electrode potential micro-environments Mn single-atom catalyst carbon dioxide reduction reaction oxygen reduction reaction constant potential models

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Morphology and magnetic properties of Sm_(2)Co_(7)/α-Fe nanocomposite magnets produced by high energy ball milling and spark plasma sintering

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Journal of Rare Earths 2021年第3期39卷 312-316,I0003页

作者： Yitong Zhuge Yuqing Li Xiaochang Xu Dongtao Zhang Hongguo Zhang Weiqiang Liu Ming Yue Key Laboratory of Advanced Functional Materials Ministry of Education of ChinaCollege of Materials Science and EngineeringBeijing University of TechnologyBeijing 100124China

In this article,the Sm_(2)Co_(7)/α-Fe nanocomposite magnets were prepared by high energy ball milling and spark plasma sintering *** effect of soft phase content on the magnetic properties was *** to 30 wt% α-Fe was added into Sm_(2)Co_(7) matrix without the decrease of *** energy product(BH)max of 9.2 MGOe was obtained with 20 wt% α-*** observation shows that the grain size of α-Fe is 20-50 nm which ensures a good coupling effect between soft and hard *** more thing needs to be mentioned is that there exists inter-diffusion between Sm-Co phase and α-Fe ***,our results can also illustrate that the Sm_(2)Co_(7)/α-Fe nanocomposite magnets are able to acquire better magnetic properties than the SmCo_(5)/α-Fe magnets prepared by the same process due to the large domain width of Sm_(2)Co_(7) phase.

关键词： Nanocomposite magnet Microstructure Interdiffusion Exchange coupling effect Spark plasma sintering Rare earths

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Effects of copper and zirconium contents on microstructure and magnetic properties of Sm(Co,Fe,Cu,Zr)_(z)magnets with high iron content

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Journal of Rare Earths 2021年第2期39卷 160-166页

作者： Zhifeng Shang Dongtao Zhang Zhihong Xie Yunqiao Wang Muhammad Haseeb Pengbiao Qiao Weiqiang Liu Ming Yue College of Materials Science and Engineering Key Laboratory of Advanced Functional MaterialsMinistry of Education of ChinaBeijing University of TechnologyBeijing 100124China

The evolution of the microstructure,microchemistry and magnetic properties of the Sm(CobalFe_(0.28)-CuyZrx)_(7.6)magnets with different Zr and Cu contents was *** is found that the coercivity of the Sm(Co,Fe,Cu,Zr)_(z)magnets is sensitive to Zr *** deficiency of Zr content causes heterogeneity of Cu and Fe distributions,while an excessive Zr content leads to the formation of a SmCoZr impurity *** cellular structure and distribution of Cu *** between the cell boundary phase and cell pha se are destroyed by inappropriate Zr content,which results in a reduction of *** Cu concentration difference between the cell boundary phase and cell phase increases with increasing Cu *** coercivity of the Sm(CobalFe_(0.28)CuyZ_(r0.02))_(7.6)magnets increases from 10.4 to 25.4 kOe for y=0.05 and y=***,the excess of Cu element destroys the cell boundary phase and enlarges the cell size,resulting in a significant decrease of squareness and energy *** optimum performance(remanence of 11.4 kG,coercivity of 25.4 kOe,maximum magnetic ene rgy product of 30.4 MGOe)was obtained for the Sm(Co_(0.63)Fe_(0.28)Cu_(0.07)Zr_(0.02))_(7.6)magnet.

关键词： Sm(CoFeCuZr)_(z)permanent magnets Cu Zr Microstructure Magnetic properties Composition distribution

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Theoretical predictions and experimental verification on the phase stability of enthalpy-stabilized HE TMREB_(2)s

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Journal of materials science & technology 2022年第26期121卷 154-162页

作者： Ze Zhang Shizhen Zhu Fu-Zhi Dai Huimin Xiang Yanbo Liu Ling Liu Zhuang Ma Shijiang Wu Fei Liu Kuang Sun Yanchun Zhou School of Materials Science and Engineering Beijing Institute of TechnologyBeijing 100081China Science and Technology on Advanced Functional Composite Laboratory Aerospace Research Institute of Materials and Processing TechnologyBeijing 100076China National Key Laboratory of Science and Technology on Materials Under Shock and Impact Beijing 100081China Beijing Institute of Technology Chongqing Innovation Center Chongqing 401120China Yangtze Delta Region Academy of Beijing Institute of Technology Jiaxing 314019China Zibo Firststar New Material Incorporated Co. Ltd.Zibo 255000China Shanghai Chenhua Science and Technology Corporation Ltd. Shanghai 201804China

Transition metal diborides(TMB_(2)s)are the materials of choice in extreme environments due to their excellent thermal and chemical ***,the degradation of oxidation resistance of TMB_(2)s at elevated temperature still hinders their *** cope with this challenge,it is effective to incorporate rare earth elements to form high-entropy transition and rare-earth metal diborides(HE TMREBs).To obtain thermodynamically stable single-phase structures for HE TMREB_(2)s,a“16×16 mixed enthalpy matrix”is constructed using first-principles calculations to predict the single-phase formation ability of120 two-component diborides(TCBs).Through the use of the“16×16 mixed enthalpy matrix”of TCBs,specific combinations of TMB_(2)s and REB_(2)s that are most likely to form single-phase HE TMREB_(2)s are ***,based on the energy distribution of the local mixing enthalpies of all possible configurations,the enthalpy and entropy descriptors of HE TMREB_(2)s(RE=Sc,Lu,Tm,Er,Ho and Dy)are *** is found that the mixing enthalpy plays a critical role in the stability of the single-phase HE TMREB_(2)s,i.e.,HE TMREB_(2)s are enthalpy-stabilized *** experimental results further confirm that enthalpy dominates the thermodynamic domain and drives the stability of REB_(2)s in HE TMREB_(2)*** study validates that enthalpy-stabilized HE TMREB_(2)s can further expand the compositional space of ultrahigh temperature ceramics(UHTCs)and is expected to further improve the oxidation resistance and high temperature properties of UHTCs.

关键词： High-entropy ceramics Ultrahigh temperature ceramics First-principles calculation Mixing enthalpy Transition and rare earth metal diborides

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