检索结果-内蒙古大学图书馆

Peak-like three-dimensional CoFe_(2)O_(4)/carbon nanotube decorated bamboo fabrics for simultaneous solar-thermal evaporation of water and photocatalytic degradation of bisphenol A

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Journal of Materials science & technology 2024年第12期179卷 40-49页

作者： Rui-Jie Pan Jing Wu Jin Qu Tingting Zhang Fan-Zhen Jiao Mang Zhao Meng-Yan Han Xiaofeng Li Zhong-Zhen Yu State Key Laboratory of Organic-Inorganic Composites College of Materials Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029China Beijing Key Laboratory of Advanced Functional Polymer Composites Beijing University of Chemical TechnologyBeijing 100029China

Catalytic CoFe_(2)O_(4) and solar-thermal carbon nanotube decorated bamboo fabrics(CCBF)are fabricated for integrating efficient solar steam generation from wastewater with catalytic degradation of its organic *** to the numerous porous channels and polar groups of bamboo fabric and the efficient solar-thermal energy conversion of black carbon nanotubes,the porous and hydrophilic CCBF exhibits fast upward transport of water,efficient solar light absorption,and high solar-thermal energy conversion *** decorated CoFe_(2)O_(4) not only enhances the solar-thermal energy conversion efficiency of CCBF but also activates potassium peroxymonosulfate to generate abundant highly active species for catalytic degradation of bisphenol A(BPA).Furthermore,folding the CCBF into a peak-like 3D evaporator can en-hance solar energy utilization,and gain environmental energy for promoting solar-thermal water evapo-ration and catalytic degradation *** 3D CCBF evaporator achieves a water evaporation rate of 2.72 kg m^(-2) h^(-1) under 1-sun ***,100%of the BPA in the seawater can be degraded within 10 *** exceptional high purification efficiency of 27.72 kg m^(-2) h^(-1) is achieved with the 3D evaporator during a long-term treatment of BPA-containing seawater under 1-sun *** work demonstrates efficient purification of seawater/wastewater with both metal ions and organic pollutants by simultaneous solar-thermal evaporation of water and catalytic degradation of organic pollutants.

关键词： Solar-thermal water evaporation Seawater desalination Catalytic degradation Carbon nanotubes CoFe_(2)O_(4)

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Online preparation of high-quality BN coatings with atomic diffusion based on carbon-free water-soluble precursor

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Journal of advanced Ceramics 2024年第3期13卷 272-281页

作者： Yiang Du Bing Wang Yunbo Zhang Quzhi Song Fuwen Wang Cheng Han Xiaoshan Zhang Yingde Wang Science and Technology on Advanced Ceramic Fibers and Composites Laboratory College of Aerospace Science and EngineeringNational University of Defense TechnologyChangsha 410073China

Efficient and environmentally friendly production of high-quality continuous fiber coatings using current preparation methods is highly challenging due to issues such as scale and batch processing restrictions,low deposition rate,high energy consumption,and utilization of multiple environmentally hazardous *** address these challenges,we propose a stable and efficient wet chemical deposition coating method for high-throughput online continuous preparation of boron nitride(BN)coatings on ceramic fibers under an ambient *** process involves surface modification,in-situ wet chemical deposition,and heat treatment,and all seamlessly connecting with the ceramic fiber preparation process through continuous *** groups were introduced via surface modification enhancing wettability of the fiber surface with impregnating *** in-situ reaction and atom migration improve uniformity and binding of the *** a result,outstanding impregnation and adhesion properties are achieved.A comprehensive analysis to evaluate the impact of the BN coatings was conducted,which demonstrates that the BN-coated fibers exhibit a remarkable 36%increase in tensile strength,a 133%increase in fracture toughness,and enhanced temperature resistance of up to 1600℃.It provides a secure and efficient platform for cost-effective production of functional and high-quality coatings through targeted surface modification and rapid stretching impregnation.

关键词： polymer-derived ceramics SiC fibers wet chemical deposition atomic diffusion boron nitride(BN)coatings

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Multifunctional Waterborne Polyurethane Nanocomposite Films with Remarkable Electromagnetic Interference Shielding,Electrothermal and Solarthermal Performances

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Chinese Journal of Polymer science 2023年第2期41卷 267-277页

作者： Ming-Ke Xu Xin-Jie Luo Hao-Bin Zhang Yu Zhang Lulu Li Xin-Feng Zhou Zhong-Zhen Yu Beijing Key Laboratory of Advanced Functional Polymer Composites Beijing University of Chemical TechnologyBeijing100029China State Key Laboratory of Organic-Inorganic Composites College of Materials Science and EngineeringBeijing University of Chemical TechnologyBeijing100029China

To impart polymers with high electrical conductivity and satisfactory electromagnetic interference shielding efficiency,it is crucial to efficiently construct interconnecting networks of conductive nanofillers in polymer ***,on the basis of the three-dimensional(3D)skeleton and volume-exclusion effect of silane-modified tetra-needle ZnO(ST-ZnO)whiskers and the high conductivity of two-dimensional MXene nanosheets,multifunctional MXene/ST-ZnO/waterborne polyurethane(MTW)nanocomposite films are fabricated by coating of MXene on ST-ZnO followed by compounding with waterborne *** 3D four-needles of the whiskers facilitate the formation of an interconnecting network in the waterborne polyurethane matrix,while the coating of MXene efficiently makes the interconnecting network of the whiskers conductive at a low amount of the *** resultant MTW ternary nanocomposite film exhibits not only a high electrical conductivity of 4.8×10^(4)S/m,but also an excellent electromagnetic interference shielding effectiveness of over 70 dB in the X-band at a low thickness of 100µ*** addition,the ternary film also exhibits outstanding Joule heating performances with an equilibrium temperature of 113℃at a low driving voltage of 3 *** multifunctional nanocomposite films are promising for applications in portable and wearable electronics and flexible electromagnetic interference shielding devices.

关键词： Electrical conductivity Electromagnetic interference shielding Nanocomposite films Waterborne polyurethane MXene nanosheets

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Synergistic Enhancement of Mechanical Properties and Electrical Conductivity of Immiscible Bimetal:A Case Study on W–Cu

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Engineering 2025年第3期46卷 224-235页

作者： Qixiang Duan Chao Hou Tielong Han Yurong Li Haibin Wang Xiaoyan Song Zuoren Nie Key Laboratory of Advanced Functional Materials Ministry of EducationCollege of Materials Science and EngineeringBeijing University of TechnologyBeijing 100124China

Immiscible bimetal systems,of which tungsten–copper(W–Cu)is a typical representative,have crucial applications in fields requiring both mechanical and physical ***,it is a major challenge to determine how to give full play to the advantages of the two phases of the bimetal and achieve outstanding comprehensive *** this study,an ultrafine-grained W–Cu bimetal with spatially connected Cu and specific Wislands was fabricated through a designed powder-mixing process and subsequent rapid low-temperature *** prepared bimetal concurrently has a high yield strength,large plastic strain,and high electrical *** stress distribution and strain response of individual phases in different types of W–Cu bimetals under loading were quantified by means of a *** high yield strength of the reported bimetal results from the microstructure refinement and high contiguity of the grains in the W islands,which enhance the contribution of W to the total plastic deformation of the *** high electrical conductivity is attributed to the increased mean free path of the Cu and the reduced proportion of phase boundaries due to the specific phase combination of W islands and *** work provides new insight into modulating phase configuration in immiscible metallic composites to achieve high-level multi-objective properties.

关键词： Immiscible bimetal Phase configuration Mechanical property Electrical conductivity Strain response

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Nano-TiO_(2) coate d nee dle carbon fib er reinforced phenolic aerogel composite with low density, excellent heat-insulating and infrared radiation shielding performance

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Journal of Materials science & technology 2023年第21期152卷 181-189页

作者： Yiwu Pan Xiangyu Jin Hebing Wang He Huang Can Wu Xiaojie Yan Changqing Hong Xinghong Zhang National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of TechnologyHarbin 150001China

High-performance thermal protection materials(TPMs)for spacecraft are becoming current research *** polymer-based ablators are considered to be the most promising candidates for TPMs due to their excellent designability and *** this study,a unique nano-TiO_(2) coated needled carbon fiber felt/phenolic resin aerogel composite(TiCF/PR)is *** the anatase nano-TiO_(2) was in-situ coated on the surface of carbon fibers uniformly through the sol-gel and calcination method,then,the phenolic resin aerogel was in-situ synthesized in the nano-TiO_(2) coated needled carbon fiber felt(TiCF)preform through vacuum impregnation and solvothermal *** as-prepared aerogel com-posite possesses a low density(0.30–0.32 g/cm^(3)),low thermal conductivity(0.034 and 0.312 W/(m K)in the z and xy directions),and excellent thermal stability with 13.86%residual weight at 1300℃ in *** is worthwhile to note that the TiCF/PR composite exhibits excellent antioxidant ablation and infrared(IR)radiation shielding properties in a high-temperature heating *** an oxygen-acetylene blaze heating of 1.5 MW/m^(2) for 150 s,the linear ablation rates decreased by 13.4%,and the backside temperature reduced from 322.3 to 179.1℃ compared to that of the sample without nano-TiO_(2) *** experimental and theoretical analysis showed that the present TiCF/PR nanocomposite has competitive and potential application prospects in the field of future TPMs.

关键词： Carbon fiber Opacifier Mechanical properties Thermal properties Ablation performance

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Constructing central hollow cylindrical reduced graphene oxide foams with vertically and radially orientated porous channels for highly efficient solar-driven water evaporation and purification

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Nano Research 2023年第5期16卷 6343-6352页

作者： Changjun Li Wei Li Hao-Yu Zhao Xin-Yue Feng Xiaofeng Li Zhong-Zhen Yu State Key Laboratory of Organic-Inorganic Composites College of Materials Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029China Beijing Key Laboratory of Advanced Functional Polymer Composites Beijing University of Chemical TechnologyBeijing 100029China College of Materials Science and Engineering Shandong University of Science and TechnologyQingdao 266590China

Although solar steam generation is an eco-friendly approach for desalinating seawater and purifying wastewater,there are still issues on how to improve the efficiency of solar energy utilization and accelerate the water and heat transport inside the solardriven water ***,we design a central hollow cylindrical reduced graphene oxide(RGO)foam with vertically and radially orientated channels as a solar steam generation device for efficient water evaporation and *** vertically aligned porous channels accelerate upward transport of water to the top evaporation surface,while the radially aligned porous channels facilitate water transport and heat transfer along the radial directions for fully utilizing the heat accumulated inside the central cylindrical hole of the *** central hole of the foam plays a highly positive role in accumulating more heat for accelerating the water evaporation,the newly generated inner sidewall resulted from the central hole can gain extra thermal energy from surrounding environment in the same way as the outer sidewall of the foam due to the surface cooling effect of the water *** a result,the vertically and radially aligned RGO foam evaporator with central hollow cylinder achieves a high solar steam generation rate of 2.32 kg·m^(−2)·h^(−1)with an exceptional energy conversion efficiency of 120.9%under 1-sun irradiation,superior to the vertically aligned RGO foam without the central hole(1.83 kg·m^(−2)·h^(−1),96.9%)because of the enhanced water and heat transfer inside the porous channels,the efficient utilization of environmental energy.

关键词： hollow cylindrical foams reduced graphene oxide solar steam generation water evaporation rate seawater desalination

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Constructing in-situ polymerized electrolyte for room-temperature solid-state chloride ion battery with enhanced electrochemical performance

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材料科学技术（英文版） 2025年第3期206卷 185-192页

作者： Yuling Xu Tiantian Zhu Haiyang Xu Xiangyu Zhao State Key Laboratory of Materials-Oriented Chemical Engineering Jiangsu Collaborative Innovation Center for Advanced Inorganic Functional CompositesCollege of Materials Science and EngineeringNanjing Tech UniversityNanjing211816China

Considering large volume variation and dissolution issues of some promising electrode materials for chloride ion batteries(CIB),the construction of solid polymer electrolytes(SPE)for efficient chloride ion transport is ***,this is hindered by low ionic conductivity of chloride SPEs and poor cycling performance of ***,an in-situ polymerized and cross-linked poly(ethylene gly-col)diacrylate-based chloride SPE with a low plasticizer content of succinonitrile is designed,yielding a room-temperature ionic conductivity of 7.6 × 10-5 S cm-1,which is higher than that of previously re-ported SPEs for ***,the use of the as-prepared SPE achieves an integrated organic cathode with significantly enhanced rate performance and capacity retention of 96.1％after 100 cycles at room temperature,which is much higher than 49.9％(80 cycles)of the cathode in the CIB with a sandwiched *** improved properties are also superior to that of other reported cathodes coupled with different chloride *** chloride ion transfer mechanism of the cathode is revealed by X-ray photo-electron spectroscopy and energy dispersive spectroscopy.

关键词： Chloride ion batteries Polymer electrolytes Poly(ethylene glycol)diacrylate Ionic conductivity Integrated cathode Cycling stability

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Machine learning-driven insights into biaxial strain-induced anomalous thermal conductivity enhancement of boron arsenide

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science China Technological sciences 2025年第5期68卷 5-18页

作者： Yikun LIU Yurong HE Tianqi TANG Jiaqi ZHU School of Energy Science and Engineering Harbin Institute of Technology Zhengzhou Research Institute Harbin Institute of Technology Heilongjiang Key Laboratory of New Energy Storage Materials and Processes National Key Laboratory of Science and Technology on Advanced Composites in Special Environments

Boron arsenide(BAs) is a promising integrated circuit thermal management material with ultra-high thermal conductivity(κ) and exceptional semiconductor properties. In practical devices, mechanical stress and strain caused by thermal expansion inevitably affect the thermodynamic properties of heat sink materials. Consequently, investigation of the effects of stress and strain on the κ of BAs is essential. Accurate assessment and regulation of the κ and phonon heat transport of BAs requires consideration of both three-phonon(3ph) and four-phonon(4ph) interactions. However, anharmonicity computation using density functional theory is computationally expensive, particularly for the fourth-order interatomic force constants. This work uses a machine learning-driven moment tensor potential method to evaluate higher-order anharmonicity and extends it to include fourth-order forces, accelerating the calculations significantly. Results show that the κ of BAs calculated using the moment tensor potential method when considering both 3ph and 4ph processes agrees well with experimental data. In contrast,considering the 3ph interaction alone causes κ to be overestimated. The machine learning approach reduces computational costs by approximately 94% while maintaining comparable accuracy to density functional theory. By solving the phonon Boltzmann transport equation, the thermal transport properties of BAs under biaxial tensile strains ranging up to 7% are evaluated. BAs shows an anomalous κ enhancement when including both 3ph and 4ph interactions, with a maximum enhancement of 15% at a small strain of 1%, primarily because of the weakening of the 3ph scattering. Beyond 2% strain, both the 3ph and 4ph scattering rates increase significantly, causing shorter phonon lifetimes and a monotonic reduction in κ. Additionally, the κ temperature dependence under strain is explored, highlighting temperature's role in modulating phonon scattering. This study provides machine learning-driven i

关键词： boron arsenide machine learning potential biaxial strain thermal conductivity enhancement phonon transport

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Robust,fire-resistant,and thermal-stable SiZrNOC nanofiber membranes with amorphous microstructure for high-temperature thermal superinsulation

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Journal of advanced Ceramics 2023年第1期12卷 36-48页

作者： Xiaoshan ZHANG Nana XU Yonggang JIANG Haiyan LIU Hui XU Cheng HAN Bing WANG Yingde WANG Science and Technology on Advanced Ceramic Fiber and Composites Laboratory College of Aerospace Science and EngineeringNational University of Defense TechnologyChangsha 410073China

Ceramic nanofibers with robust mechanical properties,high-temperature resistance,and superior thermal insulation performance are promising thermal insulators used under extreme ***,developing of ceramic fibers with both low solid thermal conductivity(λs)and low infrared radiation thermal conductivity(λr)is still a great ***,according to the Ioffe-Regel limit theory,we report a novel SiZrNOC nanofiber membrane(NFM)with a typically amorphous structure by combining the electrospinning method and high-temperature pyrolysis technique in a NH3 *** prepared SiZrNOC NFM has a high tensile strength(1.98±0.09 MPa),excellent thermal stability(1100℃in air),and superior thermal insulation *** thermal conductivity of SiZrNOC NFM was 0.112 W·m^(−1)·K^(−1) at 1000℃,which is obviously lower than that of the traditional ceramic fiber membranes(>0.2 W·m^(−1)·K^(−1) at 1000℃).In addition,the prepared SiZrNOC NFM-reinforced SiO2 aerogel composites(SiZrNOCf/SiO2 ACs)exhibited ultralow thermal conductivity of 0.044 W·m^(−1)·K^(−1) at 1000℃,which was the lowest value for SiO2-based aerogel composites ever *** superior thermal insulation performance of SiZrNOC NFMs was mainly due to significant decreasing of solid heat conduction and thermal radiation by the fancy amorphous microstructure and high infrared shielding *** work not only provides a promising high-temperature thermal insulator,but also offers a novel route to develop other high-performance thermal insulating materials.

关键词： amorphous microstructure SiZrNOC nanofiber thermal stability thermal insulation

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Ultralight and superelastic MXene/reduced graphene oxide aerogels for electromagnetic interference shielding

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Nano Research 2025年第1期18卷 1-9页

作者： Xinfeng Zhou Yang Dai Guoyao Yue Yiman Zhang Lulu Li Zhong-Zhen Yu Peng Min Hao-Bin Zhang State Key Laboratory of Organic-Inorganic Composites College of Materials Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029China Beijing Key Laboratory of Advanced Functional Polymer Composites College of Materials Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029China Present address:BOE Technology Innovation Center BOE Technology Group Co.Ltd.Beijing 100176China Xi’an Modern Chemistry Research Institute Xi’an 710065China

Lightweight aerogels feature multifunctionality and a high porosity,yet accompanied with poor structure recovery under large strain *** this work,we develop an air bubble-ice crystal dual template and annealing strategy to integrate low density and high resilience for the conductive transition metal carbides/nitrides(MXene)composite *** air bubbles and ice crystals synergistically exclude the nanosheets to the gas-liquid interfaces,thereby constructing unique Y-shaped junctions and robust *** annealing process greatly enhances the interlayer *** external load,the Yshaped structures prevent the stress concentration at the junctions by transferring the forces to the skeleton for maintaining structural *** addition,the wrinkled and thick cell walls,together with the enhanced interlayer interactions,endow the aerogel with exceptional structural stability and *** a result,the MXene/reduced graphene oxide(RGO)composite aerogels exhibit superelasticity with reversible compressive strains of up to 95%.In addition,the electron bridging effect of the RGO sheets affords the aerogel to deliver excellent electromagnetic interference shielding performance,as high as 46.3 dB at 2.5 ***,the remarkable reshapeability of the aerogels allows for precise regulation of structure and performance(33.5-75.1 dB)by a simple wetting compression *** summary,this work offers helpful inspirations for developing lightweight and superelasticity aerogels for extensive applications.

关键词： lightweight superelasticity MXene aerogel electromagnetic interference shielding reshapeability

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