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Towards energy-efficient(bi)carbonate electrolysis:Innovation and challenges

National science Open 2024年第6期3卷 8-11页

作者： Kewen Xing Junmei Chen Yanguang Li Institute of Functional Nano&Soft Materials(FUNSOM) Soochow UniversitySuzhou 215123China Jiangsu Key Laboratory for Advanced Negative Carbon Technologies Soochow UniversitySuzhou 215123China Department of Chemical and Biomolecular Engineering National University of SingaporeSingapore 117585Singapore Macao Institute of Materials Science and Engineering(MIMSE) MUST-SUDA Joint Research Center for Advanced Functional MaterialsMacao University of Science and TechnologyMacaoChina

Electrochemical CO_(2) reduction reaction(CO_(2)RR)stands out as a promising approach for converting greenhouse gases into valuable chemicals and fuels,contributing to the closure of the artificial carbon ***,most current CO_(2)RR electrolyzers necessitate purified CO_(2) feed gases and fail to directly convert atmospheric CO_(2) or flue gases(the primary sources of CO_(2) emission).

关键词： gases closure convert

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Various topological phases and their abnormal effects of topological acoustic metamaterials

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Interdisciplinary Materials 2023年第2期2卷 179-230页

作者： Yan-Feng Chen Ze-Guo Chen Hao Ge Cheng He Xin Li Ming-Hui Lu Xiao-Chen Sun Si-Yuan Yu Xiujuan Zhang National Laboratory of Solid-State Microstructures&Department of Materials Science and Engineering Nanjing UniversityNanjingChina Collaborative Innovation Center of Advanced Microstructures Nanjing UniversityNanjingChina Jiangsu Key Laboratory of Artificial Functional Materials Nanjing UniversityNanjingChina School of Materials Science and Intelligent Engineering Nanjing UniversitySuzhouChina School of Mechanical Engineering Nanjing University of Science and TechnologyNanjingChina

The last 20 years have witnessed growing impacts of the topological concept on the branches of physics,including materials,electronics,photonics,and *** describes objects with some global invariant property under continuous deformation,which in mathematics could date back to the 17th century and mature in the 20th *** physics,it successfully underpinned the physics of the Quantum Hall effect in *** date,topology has been extensively applied to describe topological phases in acoustic *** artificial structures,acoustic metamaterials could be well theoretically analyzed,on-demand designed,and easily fabricated by modern techniques,such as three-dimensional *** new theoretical topological models were first discovered in acoustic metamaterials analogous to electronic counterparts,associated with novel effects for acoustics closer to *** this review,we focused on the concept of topology and its realization in airborne acoustic crystals,solid elastic phononic crystals,and surface acoustic wave *** also introduced emerging concepts of non-Hermitian,higher-order,and Floquet topological insulators in *** has been shown that the topology theory has such a powerful generality that among the disciplines from electron to photon and phonon,from electronic to photonics and acoustics,from acoustic topological theory to acoustic devices,could interact and be analogous to fertilize fantastic new ideas and prototype devices,which might find applications in acoustic engineering and noisevibration control engineering in the near future.

关键词： acoustic materials robust propagation topological acoustic metamaterials topological phases

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Unraveling Passivation Mechanism of Imidazolium-Based Ionic Liquids on Inorganic Perovskite to Achieve Near-Record-Efficiency CsPbI_(2)Br Solar Cells

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Nano-Micro Letters 2022年第1期14卷 152-166页

作者： Jie Xu Jian Cui Shaomin Yang Yu Han Xi Guo Yuhang Che Dongfang Xu Chenyang Duan Wenjing Zhao Kunpeng Guo Wanli Ma Baomin Xu Jianxi Yao Zhike Liu Shengzhong Liu Key Laboratory of Applied Surface and Colloid Chemistry Ministry of EducationShaanxi Key Laboratory for Advanced Energy Devices/Shaanxi Engineering Lab for Advanced Energy TechnologySchool of Materials Science and EngineeringShaanxi Normal UniversityXi’an 710119People’s Republic of China Dalian Institute of Chemical Physics iChEMUniversity of Chinese Academy of SciencesDalian National Laboratory for Clean EnergyChinese Academy of SciencesDalian 116023People’s Republic of China Ministry of Education Key Laboratory of Interface Science and Engineering in Advanced Materials Research Center of Advanced Materials Science and TechnologyTaiyuan University of TechnologyTaiyuan 030024People’s Republic of China Institute of Functional Nano&Soft Materials Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesJoint International Research Laboratory of Carbon-Based Functional Materials and DevicesSoochow UniversitySuzhou 215123People’s Republic of China Department of Materials Science and Engineering and Shenzhen Engineering Research and Development Center for Flexible Solar Cells Southern University of Science and TechnologyShenzhen 518055People’s Republic of China State Key Laboratory of Alternate Electrical Power System With Renewable Energy Sources North China Electric Power UniversityBeijing 102206People’s Republic of China

The application of ionic liquids in perovskite has attracted wide-spread attention for its astounding performance improvement of perovskite solar cells(PSCs).However,the detailed mechanisms behind the improvement remain ***,a series of imidazolium-based ionic liquids(IILs)with different cations and anions is systematically investigated to elucidate the passivation mechanism of IILs on inorganic *** is found that IILs display the following advantages:(1)They form ionic bonds with Cs^(+)and Pb^(2+)cations on the surface and at the grain boundaries of perovskite films,which could effectively heal/reduce the Cs^(+)/I−vacancies and Pb-related defects;(2)They serve as a bridge between the perovskite and the hole-transport-layer for effective charge extraction and transfer;and(3)They increase the hydrophobicity of the perovskite surface to further improve the stability of the CsPbI_(2)Br *** combination of the above effects results in suppressed non-radiative recombination loss in CsPbI_(2)Br PSCs and an impressive power conversion efficiency of 17.02%.Additionally,the CsPbI_(2)Br PSCs with IILs surface modification exhibited improved ambient and light illumination *** results provide guidance for an indepth understanding of the passivation mechanism of IILs in inorganic perovskites.

关键词： Ionic liquids Inorganic perovskite Imidazolium Passivation High efficiency

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Temperature Effect on Early Oxidation Behavior of NiCoCrAlY Coatings: Microstructure and Phase Transformation

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Acta Metallurgica Sinica(English Letters) 2022年第6期35卷 975-984页

作者： A.Ullah A.Khan Z.B.Bao Y.F.Yang M.M.Xu S.L.Zhu F.H.Wang University of Chinese Academy of Sciences Beijing 100049China Shi-Changxu Innovation Center for Advanced Materials Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China Key Laboratory of Green Fabrication and Surface Technology of Advanced Metal Materials Ministry of EducationSchool of Materials Science and EngineeringAnhui University of TechnologyMaanshan 243000China Institute of Advanced Wear and Corrosion Resistant and Functional Material Jinan UniversityGuangzhou 510632China Shenyang National Laboratory for Materials Science Northeastern UniversityShenyang 110819China

Initial oxidation behavior of NiCoCrAlY coating prepared by arc-ion plating has been studied in air at 900, 1000 and 1100 ℃. The results showed that phase transformation from transient θ-Al_(2)O_(3) to α-Al_(2)O_(3) was highly related to the temperature and oxidation time. The oxide scale in the initial stage was mainly composed of θ-Al_(2)O_(3) at 900 ℃. Instead, more amount of α-Al_(2)O_(3) emerged out with increasing oxidation temperature. The elemental distribution after oxidation confirmed that faster chromium diffusion to the oxide scale played an important role in the speedy transformation from θ-Al_(2)O_(3) to α-Al_(2)O_(3). Y segregation at scale/coating interface resulted in less cavity formation and hence improved the oxide scale adherence.

关键词： MCrAlY coating Phase transformation Isothermal oxidation Temperature effect

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In-situ study of damage mechanisms in Mg-6Li dual-phase alloy

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Journal of Materials science & technology 2024年第12期179卷 114-124页

作者： Jing Li Li Jin Sangbong Yi Xin Zhang Jie Dong Ming Luo Key Laboratory of High Performance Manufacturing for Aero Engine(Northwestern Polytechnical University) Ministry of Industry and Information TechnologyXi'an 710072China Engineering Research Center of Advanced Manufacturing Technology for Aero Engine Ministry of EducationNorthwestern Polytechnical UniversityXi'an 710072China National Engineering Research Center of Light Alloy Net Forming and State Key Laboratory of Metal Matrix Composite School of Materials Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240China Institute of Materials and Process Design Helmholtz-Zentrum HereonGeesthacht 21502Germany

Interfaces play a crucial role in influencing the mechanical properties of Mg *** Mg-Li dual-phase alloy,the type of interfaces is complex,which includes both grain boundary and phase boundary,and the influence of such interfaces on the damage nucleation is yet to be *** this paper,in-situ scanning electron microscopy(SEM)based measurements were carried out to investigate the meso-scale damage nucleation mechanisms of the Mg-6Li dual-phase *** show that 94.8%of cracks are nucleated at the α-Mg grain boundary in the post-uniform elongation stage,while 5.2%are at phase boundary and almost no crack at the β-Li grain *** initiation of α-Mg grain boundary cracks is attributed to strain incompatibility,which induces micro-strain localization,and then causes grain boundary sliding(GBS)and crack *** compatibility analysis reveals that the geometric compatibility factor(Mk)can be used to predict the nucleation of α-Mg grain boundary *** Mk is lower than 0.075,α-Mg grain boundary cracks tend to *** cracks are generated at the phase boundary is due to the mild strain partitioning between α-Mg phase and β-Li phase and may also be partly attributed to multiple slip systems in body-centered cubic(BCC)-structured β-Li phase,which can accommodate well with the deformation of adjacent α-Mg phase.

关键词： Crack nucleation Strain localization Grain boundary sliding Phase boundary Mg–6Li dual-phase alloy

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Nitrogen and oxygen co-doped mesoporous carbon spheres as capacitive anode for high performance sodium-ion capacitors

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Journal of Materials science & technology 2021年第24期83卷 188-195页

作者： Chunhai Jiang Wenyang Zhou Zhimin Zou Fujian Provincial Key Laboratory of Functional Materials and Applications Institute of Advanced Energy MaterialsSchool of Materials Science and EngineeringXiamen University of TechnologyXiamen361024China

The poor rate capability of battery-type anode is usually the bottleneck of the power-energy outputs of a hybrid alkaline metal ion *** this work,nitrogen and oxygen co-doped mesoporous carbon spheres with excellent rate performance and cycle stability are used as anode materials of sodium ion capacitors(SICs).The high N and O element doping levels as well as the amorphous and mesoporous structure have enabled prominent capacitive Na ion storage behavior,which in turn match well with the capacitive cathode in the hybrid *** optimum conditions,the SIC delivers a high energy density of 103.1 Wh kg^(-1)at a power density of 205.6 W kg^(-1).Even at a high power density of 7520 W kg^(-1),an energy density of 23.5 Wh kg^(-1)is still ***,a robust cycle stability with capacity retention of 84.6%after 2500 cycles at 1 A g^(-1)is *** excellent electrochemical performances convincingly demonstrate that the all-carbon based SICs with the highly capacitive N and O co-doped mesoporous carbon anode can be promising Na ion-based energy storage devices alternative to their Li ion-based counterparts.

关键词： N and O co-doping Carbon anode Na-ion capacitors Energy density Cycle stability

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Surface-patterned chalcogenide glasses with high-aspect-ratio microstructures for long-wave infrared metalenses

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Opto-Electronic science 2024年第10期3卷 1-13页

作者： Zhaofeng Gu Yixiao Gao Kongsi Zhou Junyang Ge Chen Xu Lei Xu Mohsen Rahmani Ran Jiang Yimin Chen Zijun Liu Chenjie Gu Yaoguang Ma Jianrong Qiu Xiang Shen Laboratory of Infrared Materials and Devices Research Institute of Advanced TechnologiesNingbo UniversityNingbo 315211China Zhejiang Key Laboratory of Advanced Optical Functional Materials and Devices Ningbo 315211China Advanced Optics&Photonics Laboratory Department of EngineeringSchool of Science and TechnologyNottingham Trent UniversityNottingham NG118NSUnited Kingdom Faculty of Electrical Engineering and Computer Science Ningbo UniversityNingbo 315211China State Key Laboratory of Extreme Photonics and Instrumentation College of Optical Science and EngineeringInternational ResearchCenter for Advanced PhotonicsZhejiang UniversityHangzhou 310027China Ningbo Institute of Oceanography Ningbo 315832China

Multidimensional-engineering chalcogenide glasses is widely explored to construct various infrared photonic devices,with their surface as a key dimension for wavefront ***,we demonstrate direct patterning high-aspect-ratio microstructures on the surface of chalcogenide glasses offers an efficient and robust method to manipulate longwave infrared *** chalcogenide glass being considered soft in terms of its mechanical properties,we successfully fabricate high-aspect-ratio micropillars with a height of 8μm using optimized deep etching process,and we demonstrate a 2-mm-diameter all-chalcogenide metalens with a numerical aperture of 0.45 on the surface of a 1.5-mm-thick As2Se3 *** the exceptional longwave infrared(LWIR)transparency and moderate refractive index of As2Se3 glass,the all-chalcogenide metalens produces a focal spot size of~1.39λ0 with a focusing efficiency of 47%at the wavelength of 9.78μm,while also exhibiting high-resolution imaging *** work provides a promising route to realize easy-to-fabricate,mass-producible planar infrared optics for compact,light-weight LWIR imaging systems.

关键词： chalcogenide glasses long wave infrared metalens

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Magnetic Topological Dirac Semimetal Transition Driven by SOC in EuMg_(2)Bi_(2)

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Chinese Physics Letters 2024年第1期41卷 63-67页

作者：王佳萌钱浩吉姜琦乔山叶茂 State Key Laboratory of Functional Materials for Informatics Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesShanghai 200050China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Research Center for Intelligent Chips and Devices Zhejiang LabHangzhou 311121China Center for Transformative Science ShanghaiTech UniversityShanghai 201210China School of Physical Science and Technology ShanghaiTech UniversityShanghai 201210China Shanghai Synchrotron Radiation Facility Shanghai Advanced Research InstituteChinese Academy of SciencesShanghai 201204China

Magnetic topological semimetals have been at the forefront of condensed matter physics due to their ability to exhibit exotic transport *** the interplay between magnetic and topological orders in systems with broken time-reversal symmetry is crucial for realizing non-trivial quantum *** delve into the electronic structure of the rare-earth-based antiferromagnetic Dirac semimetal EuMg_(2)Bi_(2) using first-principles calculations and angle-resolved photoemission *** calculations reveal that the spin-orbit coupling(SOC)in EuMg_(2)Bi_(2) prompts an insulator to topological semimetal transition,with the Dirac bands protected by crystal *** linearly dispersive states near the Fermi level,primarily originating from Bi 6p orbitals,are observed on both the(001)and(100)surfaces,confirming that EuMg_(2)Bi_(2) is a three-dimensional topological Dirac *** research offers pivotal insights into the interplay between magnetism,SOC and topological phase transitions in spintronics applications.

关键词： spectroscopy topological Dirac

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Microstructural evolution of h-BN matrix composite ceramics with La-Al-Si-O glass phase during hot-pressed sintering

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Journal of advanced Ceramics 2021年第3期10卷 493-501页

作者： Baofu QIU Xiaoming DUAN Zhuo ZHANG Chen ZHAO Bo NIU Peigang HE Delong CAI Lei CHEN Zhihua YANG Yujin WANG Dechang JIA Yu ZHOU Key Laboratory of Advanced Structural-Functional Integration Materials&Green Manufacturing Technology Harbin Institute of TechnologyHarbin 150001China Institute for Advanced Ceramics School of Materials Science and EngineeringHarbin Institute of TechnologyHarbin 150001China State Key Laboratory of Advanced Welding and Joining Harbin Institute of TechnologyHarbin 150001China

BN/La-Al-Si-O composite ceramics were fabricated by hot-pressed sintering using hexagonal boron nitride(h-BN),lanthanum oxide(La_(2)O_(3)),aluminia(Al_(2)O_(3)),and amorphous silica(SiO_(2))as the raw *** effects of sintering temperature on microstructural evolution,bulk density,apparent porosity,and mechanical properties of the h-BN composite ceramics were *** results indicated that La-Al-Si-O liquid phase was formed during sintering process,which provided an environment for the growth of h-BN *** increasing sintering temperature,the cristobalite phase precipitation and h-BN grain growth occurred at the same time,which had a significant influence on the densification and mechanical properties of h-BN composite *** best mechanical properties of BN/La-Al-Si-O composite ceramics were obtained under the sintering temperature of 1700℃.The elastic modulus,flexural strength,and fracture toughness were 80.5 GPa,266.4 MPa,and 3.25 MPa·m^(1/2),respectively.

关键词： h-BN matrix composite ceramics La-A1-Si-O glass phase microstructural evolution nanocrystalline precipitation mechanical properties

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Ultra-small platinum nanoparticles segregated by nickle sites for efficient ORR and HER processes

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Journal of Energy Chemistry 2022年第2期31卷 48-54页

作者： Lvhan Liang Huihui jin Huang Zhou Bingshuai Liu Chenxi Hu Ding Chen Jiawei Zhu Zhe Wang Hai-Wen Li Suli Liu Daping He Shichun Mu State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070HubeiChina Foshan Xianhu Laboratory of the Advanced Energy Science and Technology Guangdong LaboratoryXianhu Hydrogen ValleyFoshan 528200GuangdongChina Hubei Engineering Research Center of RF-Microwave Technology and Application Wuhan University of TechnologyWuhan 430070HubeiChina Platform of Inter/Transdisciplinary Energy Research International Research Center for Hydrogen EnergyInternational Institute for Carbon-Neutral Energy ResearchYushu UniversityFukuoka 819-0395Japan Key Laboratory of Advanced Functional Materials of Nanjing Nanjing Xiaozhuang UniversityNanjing 211171JiangsuChina

In the electrochemical process,Pt nanoparticles(NPs)in Pt-based catalysts usually agglomerate due to Oswald ripening or lack of restraint,ultimately resulting in reduction of the active sites and catalytic *** to uniformly disperse and firmly fix Pt NPs on carbon matrix with suitable particle size for catalysis is still a big ***,to prevent the agglomeration and shedding of Pt NPs,Ni species is introduced and are evenly dispersed in the surface of carbon matrix in the form of Ni-N-C active sites(Ni ZIF-NC).The Ni sites can be used to anchor Pt NPs,and then effectively limit the further growth and agglomeration of Pt NPs during the reaction *** with commercial Pt/C catalyst,Pt@Ni ZIF-NC,with ultralow Pt loading(7 wt%)and ideal particle size(2.3 nm),not only increases the active center,but also promotes the catalysis kinetics,greatly improving the ORR and HER catalytic *** acidic conditions,its half-wave potential(0.902 V)is superior to commercial Pt/C(0.861 V),and the mass activity(0.38 A per mg Pt)at 0.9 V is 4.7 times that of Pt/C(0.08 A per mg Pt).Besides,it also shows outstanding HER *** 20 and 30 mV,its mass activity is even 2 and 6 times that of Pt/C,*** it is under ORR or HER conditions,it still shows excellent *** undoubtedly indicate the realization of dual-functional catalysts with low-Pt and high-efficiency properties.

关键词： Oxygen reduction reaction Hydrogen evolution reaction Zeolitic imidazolate frameworks Nickle site Pt nanoparticles

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