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Recycling the spent electronic materials to construct a highperformance Cu_(1.94)S/ZnS heterostructure anode of sodium-ion batteries

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Nano Research 2024年第5期17卷 4006-4015页

作者： Xiaowei He Tianshuai Wang Lidong Tian Qiuyu Zhang School of Chemistry and Chemical Engineering Xi’an Key Laboratory of Functional Organic Porous MaterialsKey Laboratory of Special Functional and Smart Polymer Materials of Ministry of Industry and Information TechnologyNorthwestern Polytechnical UniversityXi’an 710072China Chongqing Science and Technology Innovation Center of Northwestern Polytechnical University Chongqing 401135China College of Materials Science and Engineering Xi’an University Science and TechnologyXi’an 710054China

Heterostructure engineering by coupling different nanocrystals has received extensive attention because it can enhance the reaction kinetics of the anode of sodium-ion batteries(SIBs).However,constructing high-quality heterostructure anode materials through green and environmentally friendly methods remains a ***,we have proposed a simple one-step method by recycling the electronic waste metal materials to synthesize the Cu_(1.94)S/ZnS heterostructure *** with the experimental analysis and first principle calculations,we find that the synergistic effect of different components in heterostructure structures can significantly enhance the reversible capacity and rate performance of anode *** on the constructed Cu_(1.94)S/ZnS anode,we obtain a superior reversible capacity of 440 mAh·g^(-1) at 100 mA·g^(-1) and 335 mAh·g^(-1) after 3000 cycles at 2000 mA·g^(-1).Our work sheds new light on designing high-rate and capacity anodes for SIBs through the greenness synthesis method.

关键词： sodium-ion batteries heterostructure reversible capacity environmentally synthesis process

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Co-regulation effect of solvation and interface of pyridine derivative enabling highly reversible zinc anode

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材料科学技术（英文版） 2025年第1期204卷 1-9页

作者： Binrui Xu Guangbin Wang Yong Liu Quanan Li Fengzhang Ren Jianmin Ma School of Information Engineering Henan University of Science and TechnologyLuoyang 471023China School of Materials Science and Engineering Provincial and Ministerial Coconstruction of Collaborative Innovation Center for Non-ferrous Metal New Materials and Advanced Processing TechnologyHenan University of Science and TechnologyLuoyang 471023China Longmen laboratory Luoyang 471000China School of Chemistry Tiangong UniversityTianjin 300387China

The poor reversibility and stability of Zn anodes greatly restrict the practical application of aqueous Zn-ion batteries(AZIBs),resulting from the uncontrollable dendrite growth and H2O-induced side reactions during *** additive modification is considered one of the most effective and simplest methods for solving the aforementioned ***,the pyridine derivatives(PD)including 2,4-dihydroxypyridine(2,4-DHP),2,3-dihydroxypyridine(2,3-DHP),and 2-hydroxypyrdine(2-DHP),were em-ployed as novel electrolyte additives in ZnSO4 *** density functional theory calculation and experimental findings demonstrated that the incorporation of PD additives into the electrolyte effectively modulates the solvation structure of hydrated Zn ions,thereby suppressing side reactions in ***-ditionally,the adsorption of PD molecules on the zinc anode surface contributed to uniform Zn deposi-tion and dendrite growth ***,a 2,4-DHP-modified Zn/Zn symmetrical cell achieved an extremely long cyclic stability up to 5650 h at 1 mA ***,the Zn/NH4V4O10 full cell with 2,4-DHP-containing electrolyte exhibited an outstanding initial capacity of 204 mAh g-1,with a no-table capacity retention of 79％after 1000 cycles at 5 A ***,this study expands the selection of electrolyte additives for AZIBs,and the working mechanism of PD additives provides new insights for electrolyte modification enabling highly reversible zinc anode.

关键词： Zn anode Pyridine derivative Electrolyte additive Solvation regulation Interface modification

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Femtosecond laser-induced periodic surface structures on hard and brittle materials

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science China(Technological sciences) 2024年第1期67卷 19-36页

作者： ZHAO GuoXu WANG Gong LI YunFei WANG Lei LIAN YuDong YU Yu ZHAO Hui WANG YuLei LU ZhiWei Center for Advanced Laser Technology Hebei University of TechnologyTianjin 300401China Hebei Key Laboratory of Advanced Laser Technology and Equipment Tianjin 300401China State Key Laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130012China School of Information and Electrical Engineering Hebei University of EngineeringHandan 056038China

Hard and brittle materials have high hardness,excellent optical stability,chemical stability,and high thermal ***,they have huge application potential in various fields,such as optical components,substrate materials,and quantum information,especially under harsh conditions,such as high temperatures and high *** laser direct writing technology has greatly promoted the development of femtosecond laser-induced periodic surface structure(Fs-LIPSS or LIPSS by a femtosecond laser)applications of hard and brittle materials due to its high precision,controllability,and three-dimensional processing *** far,LIPSSs have been widely used in material surface treatment,optoelectronic devices,and ***,a consensus has not been reached regarding the formation mechanism of LIPSSs on hard and brittle *** this paper,three widely accepted LIPSS formation mechanisms are introduced,and the characteristics and applications of LIPSSs on diamonds,silicon,silicon carbide,and fused silica surfaces in recent years are *** addition,the application prospects and challenges of LIPSSs on hard and brittle materials by a femtosecond laser are discussed.

关键词： laser-induced periodic surface structures hard and brittle materials femtosecond laser

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ViGT: proposal-free video grounding with a learnable token in the transformer

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science China(information sciences) 2023年第10期66卷 196-212页

作者： Kun LI Dan GUO Meng WANG School of Computer Science and Information Engineering Hefei University of Technology Key Laboratory of Knowledge Engineering with Big Data Ministry of Education Intelligent Interconnected Systems Laboratory of Anhui Province Institute of Artificial Intelligence Hefei Comprehensive National Science Center

The video grounding(VG) task aims to locate the queried action or event in an untrimmed video based on rich linguistic descriptions. Existing proposal-free methods are trapped in the complex interaction between video and query, overemphasizing cross-modal feature fusion and feature correlation for VG. In this paper, we propose a novel boundary regression paradigm that performs regression token learning in a transformer. Particularly, we present a simple but effective proposal-free framework, namely video grounding transformer(ViGT), which predicts the temporal boundary using a learnable regression token rather than multi-modal or cross-modal features. In ViGT, the benefits of a learnable token are manifested as follows.(1) The token is unrelated to the video or the query and avoids data bias toward the original video and query.(2) The token simultaneously performs global context aggregation from video and query ***, we employed a sharing feature encoder to project both video and query into a joint feature space before performing cross-modal co-attention(i.e., video-to-query attention and query-to-video attention) to highlight discriminative features in each modality. Furthermore, we concatenated a learnable regression token [REG] with the video and query features as the input of a vision-language transformer. Finally, we utilized the token [REG] to predict the target moment and visual features to constrain the foreground and background probabilities at each timestamp. The proposed ViGT performed well on three public datasets:ANet-Captions, TACoS, and YouCookⅡ. Extensive ablation studies and qualitative analysis further validated the interpretability of ViGT.

关键词： video grounding temporal sentence grounding boundary regression token learning proposal-free

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Towards optimized tensor code generation for deep learning on sunway many-core processor

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Frontiers of Computer science 2024年第2期18卷 1-15页

作者： Mingzhen LI Changxi LIU Jianjin LIAO Xuegui ZHENG Hailong YANG Rujun SUN Jun XU Lin GAN Guangwen YANG Zhongzhi LUAN Depei QIAN State Key Laboratory of Software Development Environment Beijing 100191China School of Computer Science and Engineering Beihang UniversityBeijing 100191China National University of Singapore Singapore 119077Singapore State Key Laboratory of Mathematical Engineering and Advanced Computing Wuxi 214000China Science and Technology on Special System Simulation Laboratory Beijing Simulation Center Beijing 100854China Department of Computer Science and Technology Tsinghua UniversityBeijing 100084China

The flourish of deep learning frameworks and hardware platforms has been demanding an efficient compiler that can shield the diversity in both software and hardware in order to provide application *** the existing deep learning compilers,TVM is well known for its efficiency in code generation and optimization across diverse hardware *** the meanwhile,the Sunway many-core processor renders itself as a competitive candidate for its attractive computational power in both scientific computing and deep learning *** paper combines the trends in these two ***,we propose swTVM that extends the original TVM to support ahead-of-time compilation for architecture requiring cross-compilation such as *** addition,we leverage the architecture features during the compilation such as core group for massive parallelism,DMA for high bandwidth memory transfer and local device memory for data locality,in order to generate efficient codes for deep learning workloads on *** experiment results show that the codes generated by swTVM achieve 1.79x improvement of inference latency on average compared to the state-of-the-art deep learning framework on Sunway,across eight representative *** work is the first attempt from the compiler perspective to bridge the gap of deep learning and Sunway processor particularly with productivity and efficiency in *** believe this work will encourage more people to embrace the power of deep learning and Sunwaymany-coreprocessor.

关键词： sunway processor deep learning compiler code generation performance optimization

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Geometry-Based Stochastic MIMO Channel Model for Near-Field and Far-Field Scenarios of Integrated Sensing and Communications

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IEEE Transactions on Vehicular technology 2025年第5期74卷 6928-6940页

作者： Jin, Yunwei He, Ruisi Ai, Bo Yuan, Yuan Niu, Yong Zhang, Haoxiang Beijing Jiaotong University State Key Laboratory of Advanced Rail Autonomous Operation School of Electronics and Information Engineering Frontiers Science Center for Smart High-speed Railway System Beijing100044 China Ministry of Industry and Information Technology China Academy of Industrial Internet Beijing100804 China

Integrated sensing and communication (ISAC) has become a promising technology in current sixth-generation (6G) wireless communications due to its ability to support both communication and sensing. Existing works regarding ISAC channels mainly focus on far-field propagation conditions based on plane wave assumption. However, with the deployment of ultra-massive multiple-input multiple-output (MIMO), the far-field assumption may no longer hold, as the communication and sensing propagation distances distances may be comparable to the array aperture size. To address this issue, we propose a three-dimensional MIMO channel model that simultaneously considers near-field and far-field propagation conditions in ISAC environments. Additionally, we distinguish the communication and sensing propagation environments by employing different effective scatterer distributions. In the model, the sensing channel is divided into target sensing and environmental sensing components, whereas the communication channel is divided into line-of-sight and non-line-of-sight components. The weighted sum of each component in communication and sensing channels results in accurate channel representations. Based on the proposed model, we derive and thoroughly investigate space-time-frequency correlation function, normalized absolute error function, and channel capacity. A key observation is that the channel correlation strongly depends on scatterer distribution. In certain conditions, the sensing channel can effectively capture the behavior of the communication channel. Error function results indicate that the proposed channel model achieves fairly high accuracy in ultra-massive MIMO scenarios. These findings provide essential support for the development of ISAC systems in future 6G wireless communications. © 1967-2012 IEEE.

关键词： Stochastic systems

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BayProNet: Advancing Few-Shot Learning with Bayesian Prototype Network 24

BayProNet: Advancing Few-Shot Learning with Bayesian Prototy...

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8th International Conference on Computer science and Artificial Intelligence, CSAI 2024

作者： Gao, Cheng Lang Miao, Jiang Hui, Chen Hong Science and Technology on Information Systems Engineering Laboratory National University of Defense Technology HuNan ChangSha China

ISBN: (纸本)9798400718182

Text classification is a challenging task in the field of Natural Language Processing (NLP), and significant progress has been made using deep learning methods. Traditional deep-learning approaches for text classification require large amounts of data, thereby performing suboptimally in few-shot data scenarios. To alleviate this bottleneck, this study proposes a Bayesian Prototypical Network with Hybrid Attention (BayProNet) to improve the accuracy of few-shot text classification. Experimental results on the Clinc150 dataset show that the model significantly outperforms existing SOTA baseline models in terms of classification accuracy and also exhibits strong stability when handling noisy data. This research validates the effectiveness and superiority of Bayesian Prototypical Networks in few-shot text classification tasks. © 2024 Copyright held by the owner/author(s).

关键词： Zero-shot learning

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Closed-loop scheduling optimization strategy based on particle swarm optimization with niche technology and soft sensor method of attributes-applied to gasoline blending process

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Chinese Journal of Chemical engineering 2023年第9期61卷 43-57页

作者： Jian Long Kai Deng Renchu He Key Laboratory of Smart Manufacturing in Energy Chemical Process Ministry of EducationEast China University of Science and TechnologyShanghaiChina Engineering Research Center of Process System Engineering Ministry of EducationEast China University of Science and TechnologyShanghai 200237China

Gasoline blending scheduling optimization can bring significant economic and efficient benefits to ***,the optimization model is complex and difficult to build,which is a typical mixed integer nonlinear programming(MINLP)*** the large scale of the MINLP model,in order to improve the efficiency of the solution,the mixed integer linear programming-nonlinear programming(MILP-NLP)strategy is used to solve the *** paper uses the linear blending rules plus the blending effect correction to build the gasoline blending model,and a relaxed MILP model is constructed on this *** particle swarm optimization algorithm with niche technology(NPSO)is proposed to optimize the solution,and the high-precision soft-sensor method is used to calculate the deviation of gasoline attributes,the blending effect is dynamically corrected to ensure the accuracy of the blending effect and optimization results,thus forming a prediction-verification-reprediction closed-loop scheduling optimization strategy suitable for engineering *** optimization result of the MILP model provides a good initial *** fixing the integer variables to the MILPoptimal value,the approximate MINLP optimal solution can be obtained through a NLP *** above solution strategy has been successfully applied to the actual gasoline production case of a refinery(3.5 million tons per year),and the results show that the strategy is effective and *** optimization results based on the closed-loop scheduling optimization strategy have higher *** with the standard particle swarm optimization algorithm,NPSO algorithm improves the optimization ability and efficiency to a certain extent,effectively reduces the blending cost while ensuring the convergence speed.

关键词： Blend Optimization algorithm Neural networks Particle swarm optimization Mixed integer programming

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Glycine betaine modulates extracellular polymeric substances to enhance microbial salinity tolerance

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Environmental science and Ecotechnology 2024年第4期20卷 259-268页

作者： Yan Xia Xinbai Jiang Shuaishuai Guo Yuxuan Wang Yang Mu Jinyou Shen Key Laboratory of Environmental Remediation and Ecological Health Ministry of Industry and Information TechnologySchool of Environmental and Biological EngineeringNanjing University of Science and TechnologyNanjing210094China CAS Key Laboratory of Urban Pollutant Conversion Department of Environmental Science and EngineeringUniversity of Science&Technology of ChinaHefei230026China

High salinity inhibits microbial activity in the bioremediation of saline *** alleviate osmotic stress,glycine betaine(GB),an osmoprotectant,is added to enhance the secretion of extracellular polymeric substances(EPS).These EPS are pivotal in withstanding environmental stressors,yet the intricate interplay between GB supplementation and microbial responses through EPS modificationsdencompassing composition,molecular architecture,and electrochemical featuresdremains elusive in hypersaline *** we show microbial strategies for salinity endurance by investigating the impact of GB on the dynamic alterations of EPS *** findings reveal that GB supplementation at 3.5%salinity elevates the total EPS(T-EPS)content from 12.50±0.05 to 24.58±0.96 mg per g dry cell *** observed shift in zeta potential from-28.95 to-6.25 mV at 0%and 3.5%salinity,respectively,with GB treatment,indicates a reduction in electrostatic repulsion and ***,the EPS protein secondary structure transition from b-sheet to a-helix,with GB addition,signifies a more compact protein configuration,less susceptible to salinity *** analyses,including cyclic voltammetry(CV)and differential pulse voltammetry(DPV),reveal GB's role in promoting the release of exogenous electron shuttles,such as flavins and c-type cytochromes(c-Cyts).The enhancement in DPV peak areas(Q_(DPV))with GB addition implies an increase in available extracellular electron transfer *** investigation advances our comprehension of microbial adaptation mechanisms to salinity through EPS modifications facilitated by GB in saline habitats.

关键词： High salinity Extracellular polymeric substances Glycine betaine Protein secondary structure Extracellular electron transfer

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Representation learning via an integrated autoencoder for unsupervised domain adaptation

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Frontiers of Computer science 2023年第5期17卷 75-87页

作者： Yi ZHU Xindong WU Jipeng QIANG Yunhao YUAN Yun LI School of Information Engineering Yangzhou UniversityYangzhou 225127China Key Laboratory of Knowledge Engineering with Big Data(Ministry of Education of China) Hefei University of TechnologyHefei 230009China School of Computer Science and Information Engineering Hefei University of TechnologyHefei 230601China

The purpose of unsupervised domain adaptation is to use the knowledge of the source domain whose data distribution is different from that of the target domain for promoting the learning task in the target *** key bottleneck in unsupervised domain adaptation is how to obtain higher-level and more abstract feature representations between source and target domains which can bridge the chasm of domain ***,deep learning methods based on autoencoder have achieved sound performance in representation learning,and many dual or serial autoencoderbased methods take different characteristics of data into consideration for improving the effectiveness of unsupervised domain ***,most existing methods of autoencoders just serially connect the features generated by different autoencoders,which pose challenges for the discriminative representation learning and fail to find the real cross-domain *** address this problem,we propose a novel representation learning method based on an integrated autoencoders for unsupervised domain adaptation,called *** capture the inter-and inner-domain features of the raw data,two different autoencoders,which are the marginalized autoencoder with maximum mean discrepancy(mAE)and convolutional autoencoder(CAE)respectively,are proposed to learn different feature *** higher-level features are obtained by these two different autoencoders,a sparse autoencoder is introduced to compact these inter-and inner-domain *** addition,a whitening layer is embedded for features processed before the mAE to reduce redundant features inside a local *** results demonstrate the effectiveness of our proposed method compared with several state-of-the-art baseline methods.

关键词： unsupervised domain adaptation representation learning marginalized autoencoder convolutional autoen-coder sparse autoencoder

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