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arXiv 2020年

作者： Li, Jiashuo Zhou, Sili Wei, Wendong Qi, Jianchuan Li, Yumeng Chen, Bin Zhang, Ning Guan, Dabo Qian, Haoqi Wu, Xiaohui Miao, Jiawen Chen, Long Liang, Sai Feng, Kuishuang Institute of Blue and Green Development Shandong University Weihai264209 State Key Laboratory of Coal Combustion School of Energy and Power Engineering Huazhong University of Science and Technology Wuhan430074 China School of International and Public Affairs Shanghai Jiao Tong University Shanghai200030 China State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Beijing Normal University Beijing100875 China Laboratory of Anthropogenic Systems Ecology College of Engineering Peking University Beijing100871 China Department of Earth System Science Tsinghua University Beijing100871 China Institute for Global Public Policy Fudan University Shanghai200433 China School of Optical-Electrical and Computer Engineering University of Shanghai for Science and Technology Shanghai200093 China Key Laboratory of Geographic Information Science Ministry of Education School of Geographic Sciences East China Normal University Shanghai200241 China

China has implemented retrofitting measures in coal-fired power plants (CFPPs) to reduce air pollution through small unit shutdown (SUS), the installation of air pollution control devices (APCDs) and power generation efficiency (PGE) improvement. The reductions in highly toxic Hg emissions and their related health impacts by these measures have not been well studied. To refine mitigation options, we evaluated the health benefits of reduced Hg emissions via retrofitting measures during China's 12th Five-Year Plan by combining plant-level Hg emission inventories with the China Hg Risk Source-Tracking Model. We found that the measures reduced Hg emissions by 23.5 tons (approximately 1/5 of that from CFPPs in 2010), preventing 0.0021 points of per-foetus intelligence quotient (IQ) decrements and 114 deaths from fatal heart attacks. These benefits were dominated by CFPP shutdowns and APCD installations. Provincial health benefits were largely attributable to Hg reductions in other regions. We also demonstrated the necessity of considering human health impacts, rather than just Hg emission reductions, in selecting Hg control devices. This study also suggests that Hg control strategies should consider various factors, such as CFPP locations, population densities and trade-offs between reductions of total Hg (THg) and Hg2+. Copyright © 2020, The Authors. All rights reserved.

关键词： Fossil fuel power plants

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Near surface camera informed agricultural land monitoring for climate smart agriculture

Climate Smart Agriculture

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Climate Smart Agriculture 2024年第1期1卷

作者： Le Yu Zhenrong Du Xiyu Li Qiang Zhao Hui Wu Duoji weise Xinqun Yuan Yuanzheng Yang Wenhua Cai Weimin Song Pei Wang Zhicong Zhao Ying Long Yongguang Zhang Jinbang Peng Xiaoping Xin Fei Xu Miaogen Shen Hui Wang Yuanmei Jiao Yong Luo Department of Earth System Science Ministry of Education Key Laboratory for Earth System Modeling Institute for Global Change Studies Tsinghua University Beijing China Ministry of Education Ecological Field Station for East Asian Migratory Birds Beijing China Tsinghua University (Department of Earth System Science)- Xi'an Institute of Surveying and Mapping Joint Research Center for Next-Generation Smart Mapping Beijing China School of Information and Communication Engineering Dalian University of Technology Dalian China Geothermal Geological Brigade Tibet Autonomous Region Geological and Mineral Exploration and Development Bureau Lhasa China International Department Beijing No. 35 High School Beijing China Key Laboratory of Environment Change and Resources Use in Beibu Gulf Ministry of Education Nanning Normal University Nanning China Guangxi Key Laboratory of Earth Surface Processes and Intelligent Simulation Nanning Normal University Nanning China Key Laboratory of Coastal Environmental Processes and Ecological Restoration Yantai Institute of Coastal Zone Research Chinese Academy of Sciences Yantai China Yellow River Delta Field Observation and Research Station of Coastal Wetland Ecosystem Chinese Academy of Sciences Dongying China Department of Landscape Architecture School of Architecture Tsinghua University Beijing China Institute for National Parks Tsinghua University Beijing China School of Architecture and Hang Lung Center for Real Estate Key Laboratory of Eco Planning & Green Building Ministry of Education Tsinghua University Beijing China International Institute for Earth System Sciences Jiangsu Center for Collaborative Innovation in Geographical Information Resource Development and Application Nanjing University Nanjing China Jiangsu Provincial Key Laboratory of Geographic Information Science and Technology Key Laboratory for Land Satellite Remote Sensing Applications of Ministry of Natural Resources School of Geography and Ocean Science Nanjing Univer

Continuous and accurate monitoring of agricultural landscapes is crucial for understanding crop phenology and responding to climatic and anthropogenic changes. However, the widely used optical satellite remote sensing is limited by revisit cycles and weather conditions, leading to gaps in agricultural monitoring. To address these limitations, we designed and deployed a Near Surface Camera (NSCam) Network across China, and explored its application in agricultural land monitoring and achieving climate-smart agriculture (CSA). By analyzing the image data captured by the NSCam Network, we can accurately assess long-term or abrupt agricultural land changes. According to the preliminary monitoring results, integrating NSCam data with remote sensing imagery greatly enhances the temporal details and accuracy of agricultural monitoring, aiding agricultural managers in making informed decisions. The impacts of abnormal weather conditions and human activities on agricultural land, which are not captured by remote sensing imagery, can be complemented by incorporating our NSCam Network. The successful implementation of this method underscores its potential for broader application in CSA, promoting resilient and sustainable agricultural practices.

关键词： Near surface camera (NSCam) Climate-smart agriculture (CSA) Agricultural monitoring Data fusion Sentinel-2

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Coalition game based user association for mmWave mobile relay systems in rail traffic scenarios

arXiv

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arXiv 2021年

作者： Chen, Chen Niu, Yong Mao, Shiwen Zhang, Xiaodan Han, Zhu Ai, Bo Gao, Meilin Xiao, Huahua Wang, Ning The State Key Laboratory of Rail Traffic Control and Safety Beijing Jiaotong University Beijing100044 China The Frontiers Science Center for Smart High-Speed Railway System Beijing Jiaotong University Beijing100044 China The National Mobile Communications Research Laboratory Southeast University Nanjing211189 China The Department of Electrical and Computer Engineering Auburn University AuburnAL36849-5201 United States The School of Management Shenzhen Institute of Information Technology Shenzhen518172 China The Department of Electrical and Computer Engineering The University of Houston HoustonTX77004 United States The Department of Computer Science and Engineering Kyung Hee University Seoul446-701 Korea Republic of The Beijing Engineering Research Center of High-Speed Railway Broadband Mobile Communications Beijing Jiaotong University Beijing100044 China The Tsinghua Space Center Tsinghua University Beijing100091 China The ZTE Corporation State Key Laboratory of Mobile Network Mobile Multimedia Technology Shenzhen518057 China The School of Information Engineering Zhengzhou University Zhengzhou450001 China

Rail transportation, especially, high-speed rails (HSR), is an important infrastructure for the development of national economy and the promotion of passenger experience. Due to the large bandwidth, millimeter wave (mmWave) communication is regarded as a promising technology to meet the demand of high data rates. However, since mmWave communication has the characteristic of high attenuation, mobile relay (MR) is considered in this paper. Also, full-duplex (FD) communications have been proposed to improve the spectral efficiency. However, because of the high speed, as well as the problem of penetration loss, passengers on the train have a poor quality of service. Consequently, an effective user association scheme for HSR in mmWave band is necessary. In this paper, we investigate the user association optimization problem in mmWave mobile relay systems where the MRs operate in the FD mode. To maximize the system capacity, we propose a cooperative user association approach based on coalition formation game, and develop a coalition formation algorithm to solve the challenging NP-hard problem. We also prove the convergence and Nash-stable property of the proposed algorithm. Extensive simulations are done to show the system performance of the proposed scheme under various network settings. It is demonstrated that the proposed distributed low complexity scheme achieves a near-optimal performance and outperforms two baseline schemes in terms of average system throughput. Copyright © 2021, The Authors. All rights reserved.

关键词： Game theory

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Modular Design of A Radial Scalled Hall Thruster for Different Magnetic Configurations

Modular Design of A Radial Scalled Hall Thruster for Differe...

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International Conference on Pulsed Power

作者： A. Olano H. Tang J. Ren G. Zhang J. Li Key Laboratory of Spacecraft Design Optimization & Dynamic Simulation Technologies of Ministry of Education School of Astronautics Beihang University Beijing People's Republic of China Key Laboratory of Spacecraft Design Optimization & Dynamic Simulation Technologies of Ministry of Education School of Space and Environment Beihang University Beijing People's Republic of China Science and Technology on Vacuum Technology and Physics Laboratory Lanzhou Institute of Physics Lanzhou People's Republic of China

ISBN: (数字)9781538679692

ISBN: (纸本)9781538679708

A 100 W radial scaled Hall Thruster has been designed and manufactured using as reference design the D-55 thruster with anode layer (TAL). The magnetic field required is provided by permanent magnets following a modular design in order to compare three different magnetic field configurations: A) nominal, B) orthogonal magnetic field and C) high magnetic field. In Hall Thrusters the magnetic field is used to confine the electrons and create highly ionized plasma. Configuration A and configuration B were chosen to compare two different topographies of the magnetic field with two different magnetic field gradients and to study their influence in the plasma discharge and thruster performance. Both configurations where derived assuming Bohm diffusion as the dominant process in the plasma discharge. If instead of Bohm diffusion it is considered electron-wall collisions as main mechanism in the electron transport then a higher magnetic field is required and in consequence configuration C was designed. These three configurations are intended to provide a better understanding of the influence of the magnetic field in the thruster discharge.

关键词： Magnetic fields Discharges (electric) Plasmas Anodes Surfaces Permanent magnets Propulsion

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A Phase Unwrapping Method for Large Scale Interferometric Phase Images 2017

A Phase Unwrapping Method for Large Scale Interferometric Ph...

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Proceedings of the International Conference on Imaging, Signal Processing and Communication

作者： Hao Hongxing Wu Lingda Song Xiaorui Science and Technology on Complex Electronic System Simulation Laboratory Equipment Academy

ISBN: (纸本)9781450352895

Optical interferometry images are widely used in many research areas such as geoscience and remote sensing. However, the phase image which gets from the sensors is modulo-2π, and an important process is to estimate the absolute phase from the observation which is termed phase unwrapping. This paper addresses the absolute phase estimation of large scale images. The proposed phase unwrapping method is patch based which divides the large interferogram into small patches and does the unwrapping based on Markov Random Field for each small patch. This paper also analyzes the two types of errors that may be caused in the combination of the patches and studies how to get rid of these errors. The advantage of the proposal is that the method can be used for the wrapped phase images with discontinuous areas. Experiments in the paper show the efficiency of the proposed algorithm.

关键词： Phase Unwrapping InSAR image processing Remote sensing Digital Elevation Model data

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Design of ELF/VLF Chirp-BOK communication based on modulated heating low ionosphere

Design of ELF/VLF Chirp-BOK communication based on modulated...

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作者： Zhou, Kaijie Wang, Huali Cao, Peipei Luo, Zhangkai Institute of Communications Engineering PLA Army Engineering University Nanjing210007 China College of Physics and Electrical Engineering Huaiyin Normal University Huai'an223300 China School of Electronic and Optical Engineering Nanjing University of Science and Technology Nanjing210094 China Science and Technology on Complex Electronic System Simulation Laboratory Space Engineering University Beijing101400 China

Excitation of Extremely Low Frequency (ELF)/Very Low Frequency (VLF) from ionosphere,which is artificial modulated by High Frequency (HF) waves can provide a way of antenna generation for deep submarine communication. In this paper, based on plasma energy conservation equation, the theoretical model of amplitude modulation HF pump heating low ionosphere for ELF/VLF generation is established. The linear frequency modulation technique of up-chirp and down-chirp have good self-correlation and cross-correlation, by which information can be transmitted by up-chirp and down-chirp. Thus, the linear frequency modulation technique can be applied to the ionosphere ELF/VLF communication. Based on this, a Chirp-BOK (Binary Orthogonal Keying) communication scheme is proposed. Indeed the Chirp-BOK amplitude and power modulation function are designed by combining the linear frequency modulation technique with the square wave amplitude modulation technique. The simulation results show in the condition that the ionosphere is heated by the Chirp-BOK power modulation HF waves, the temperature of ionospheric electronic and the variations of conductivity have obvious frequency modulation characteristics which are the same as that of power modulation, so does the variation of ionospheric current. Thus, when the ionosphere is heated by Chirp-BOK power modulation HF waves, the up-chirp (symbol '0') and down-chirp (symbol '1') ELF/VLF signals can be generated. Copyright © 2018 The Institute of Electronics, Information and Communication Engineers.

关键词： Ionosphere

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Control of Stray Currents in Pipeline system based on Melnikov Theory 36

Control of Stray Currents in Pipeline System based on Melnik...

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第36届中国控制会议

作者： Peng Wang Bohu Li Guoqiang Shi Junhua Zhou School of Automation Science and Electrical Engineering BeiHang University Beijing Complex Product Advanced Manufacturing Engineering Research Center Beijing Simulation Center State Key Laboratory of Intelligent Manufacturing System Technology Beijing Institute of Electronic System Science and Technology on Space System Simulation Laboratory Beijing Simulation Center

ISBN: (纸本)9781538629185

The pipeline network interfered by the stray currents has been verified to be a complex nonlinear dynamical *** paper shows that the chaotic characteristic could be utilized in the stray currents *** prove this,this paper establishes an equivalent chaotic control *** we analyze this model by using Melnikov method and find out the condition under which the chaotic phenomenon will be *** order to get a sufficient proof for identifying the conclusion,simulation experiments are used to verify the validity of the control method.

关键词： stray currents chaos control Melnikov

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State of the climate in 2022

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Bulletin of the American Meteorological Society 2023年第9期104卷 1-516页

作者： Abida, A. Ades, Melanie Adler, Robert Adusumilli, Susheel Agyakwah, W. Ahmasuk, Brandon Aldeco, Laura S. Alexe, Mihai Alfaro, Eric J. Allan, Richard P. Allgood, Adam Alves, Lincoln M. Amador, Jorge A. Anderson, John Andrade, B. Anneville, Orlane Aono, Yasuyuki Arguez, Anthony Arosio, Carlo Atkinson, C. Augustine, John A. Avalos, Grinia Azorin-Molina, Cesar Backensto, Stacia A. Bader, Stephan Baez, Julian Baiman, Rebecca Ballinger, Thomas J. Banwell, Alison F. Bardin, M.Yu. Barichivich, Jonathan Barnes, John E. Barreira, Sandra Bartow-Gillies, Ellen Beadling, Rebecca L. Beck, Hylke E. Becker, Emily J. Bekele, E. Bellido, Guillem Martín Bellouin, Nicolas Benedetti, Angela Benestad, Rasmus Berne, Christine Berner, Logan T. Bernhard, Germar H. Bhatt, Uma S. Bhuiyan, A.E. Bigalke, Siiri Biló, Tiago Bissolli, Peter Bjerke Jarle, W. Blagrave, Kevin Blake, Eric S. Blenkinsop, Stephen Blunden, Jessica Bochníček, Oliver Bock, Olivier Bodin, Xavier Bosilovich, Michael Boucher, Olivier Boyer, Tim Bozkurt, Deniz Brettschneider, Brian Bringas, Francis G. Bringas, Francis Buechler, Dennis Buehler, Stefan A. Bukunt, Brandon Calderón, Blanca Camargo, Suzana J. Campbell, Jayaka Campos, Diego Carrea, Laura Carter, Brendan R. Cetinić, Ivona Chambers, Don P. Chan, Duo Chandler, Elise Chang, Kai-Lan Chen, Hua Chen, Lin Cheng, Lijing Cheng, Vincent Y.S. Chomiak, Leah Christiansen, Hanne H. Christy, John R. Chung, Eui-Seok Ciasto, Laura M. Clarke, Leonardo Clem, Kyle R. Clingan, Scott Coelho, Caio A.S. Cohen, Judah L. Coldewey-Egbers, Melanie Colwell, Steve Cooper, Owen R. Cornes, Richard C. Correa, Kris Costa, Felipe Covey, Curt Coy, Lawrence Créatux, Jean-François Crhova, Lenka Crimmins, Theresa Cronin, Meghan F. Cropper, Thomas Crotwell, Molly Culpepper, Joshua Cunha, Ana P. Cusicanqui, Diego Datta, Rajashree T. Davis, Sean M. De Bock, Veerle de Jeu, Richard A.M. De Laat, Jos Decharme, Bertrand Degenstein, Doug Delaloye, Reynald Demircan, Mesut Derksen, Chris Deus, Ricardo Dhurmea, K.R. Diamond, Howard J. Dirkse, S. Divine, Dmitry Do Agence Nationale de l’Aviation Civile et de la Météorologie Moroni Comoros European Centre for Medium-Range Weather Forecasts Reading United Kingdom CMNS-Earth System Science Interdisciplinary Center University of Maryland College ParkMD United States Scripps-Institution of Oceanography University of California La Jolla San DiegoCA United States NOAA NWS National Centers for Environmental Prediction Climate Prediction Center College ParkMD United States Kawerak Inc. NomeAK United States Servicio Meteorológico Nacional Buenos Aires Argentina European Centre for Medium-Range Weather Forecasts Bonn Germany Center for Geophysical Research School of Physics University of Costa Rica San José Costa Rica Department of Meteorology National Centre for Earth Observation University of Reading Reading United Kingdom Centro Nacional de Monitoramento e Alertas de Desastres Naturais CEMADEN São Paulo Brazil Hampton University HamptonVA United States Seychelles Meteorological Authority Mahe Seychelles CARRTEL Université Savoie Mont Blanc Chambéry France Graduate School of Agriculture Osaka Metropolitan University Sakai Japan NOAA/NESDIS National Centers for Environmental Information AshevilleNC United States University of Bremen Bremen Germany Met Office Hadley Center Exeter United Kingdom NOAA Global Monitoring Laboratory BoulderCO United States Servicio Nacional de Meteorología e Hidrología del Perú Lima Peru Valencia Spain National Park Service FairbanksAK United States Federal Office of Meteorology and Climatology MeteoSwiss Switzerland Universidad Católica Nuestra Señora de la Asunción Asunción Paraguay Department of Atmospheric and Oceanic Sciences University of Colorado Boulder BoulderCO United States International Arctic Research Center University of Alaska Fairbanks FairbanksAK United States University of Colorado Boulder BoulderCO United States Yu. A. Izrael Institute of Global Climate and Ecology Institute of Geography Russian Academy of

Earth’s global climate system is vast, complex, and intricately interrelated. Many areas are influenced by global-scale phenomena, including the "triple dip" La Niña conditions that prevailed in the eastern Pacific Ocean nearly continuously from mid-2020 through all of 2022;by regional phenomena such as the positive winter and summer North Atlantic Oscillation that impacted weather in parts the Northern Hemisphere and the negative Indian Ocean dipole that impacted weather in parts of the Southern Hemisphere;and by more localized systems such as high-pressure heat domes that caused extreme heat in different areas of the world. Underlying all these natural short-term variabilities are long-term climate trends due to continuous increases since the beginning of the Industrial Revolution in the atmospheric concentrations of Earth’s major greenhouse gases. In 2022, the annual global average carbon dioxide concentration in the atmosphere rose to 417.1±0.1 ppm, which is 50% greater than the pre-industrial level. Global mean tropospheric methane abundance was 165% higher than its pre-industrial level, and nitrous oxide was 24% higher. All three gases set new record-high atmospheric concentration levels in 2022. Sea-surface temperature patterns in the tropical Pacific characteristic of La Niña and attendant atmospheric patterns tend to mitigate atmospheric heat gain at the global scale, but the annual global surface temperature across land and oceans was still among the six highest in records dating as far back as the mid-1800s. It was the warmest La Niña year on record. Many areas observed record or near-record heat. Europe as a whole observed its second-warmest year on record, with sixteen individual countries observing record warmth at the national scale. Records were shattered across the continent during the summer months as heatwaves plagued the region. On 18 July, 104 stations in France broke their all-time records. One day later, England recorded a temperature of 40°C

关键词： Atmospheric temperature

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INTRODUCTION

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Bulletin of the American Meteorological Society 2024年第8期105卷 S1-S11页

作者： Boyer, T. Blunden, J. Dunn, R.J.H. NOAA/NESDIS National Centers for Environmental Information Silver Spring Maryland NOAA/NESDIS National Centers for Environmental Information Asheville North Carolina Met Office Hadley Centre Exeter United Kingdom European Centre for Medium-Range Weather Forecasts Reading United Kingdom University of Maryland College Park Maryland Scripps Institution of Oceanography University of California San Diego La Jolla California NOAA/NWS National Centers for Environmental Prediction Climate Prediction Center College Park Maryland Brandenburg University of Technology (BTU) Cottbus-Senftenberg Germany Servicio Meteorológico Nacional Buenos Aires Argentina NOAA/OAR Physical Sciences Laboratory Boulder Colorado European Centre for Medium-Range Weather Forecasts Bonn Germany Center for Geophysical Research and School of Physics University of Costa Rica San José Costa Rica Department of Meteorology and National Centre for Earth Observation University of Reading Reading United Kingdom Centro Nacional de Monitoramento e Alertas de Desastres Naturais CEMADEN São Paulo Brazil Université Grenoble Alpes Institut des Géosciences de l’Environnement IRD CNRS Grenoble INP Grenoble France Hampton University Hampton Virginia Seychelles Meteorological Authority Mahe Seychelles Section for Glaciers Ice and Snow Norwegian Water Resources and Energy Directorate Oslo Norway National Research Institute for Agriculture Food and Environment (INRAE) CARRTEL Université Savoie Mont Blanc Thonon les Bains France Graduate School of Agriculture Osaka Metropolitan University Sakai Japan Science Faculty Universidad Nacional de Colombia Bogotá Colombia University of Bremen Bremen Germany NOAA Global Monitoring Laboratory Boulder Colorado Servicio Nacional de Meteorología e Hidrología del Perú Lima Perú Centro de Investigaciones sobre Desertificación – Spanish National Research Council (CSIC-UV-GVA) Valencia Spain Hydro-Climate Extremes Lab (H-CEL) Ghent University Ghent Belgium Department o

In 2023, La Niña conditions that generally prevailed in the eastern Pacific Ocean from mid-2020 into early 2023 gave way to a strong El Niño by October. Atmospheric concentrations of Earth’s major greenhouse gases—carbon dioxide, methane, and nitrous oxide—all increased to record-high levels. The annual global average carbon dioxide concentration in the atmosphere rose to 419.3±0.1 ppm, which is 50% greater than the pre-industrial level. The growth from 2022 to 2023 was 2.8 ppm, the fourth highest in the record since the 1960s. The combined short-term effects of El Niño and the long-term effects of increasing levels of heat-trapping gases in the atmosphere contributed to new records for many essential climate variables reported here. The annual global temperature across land and oceans was the highest in records dating as far back as 1850, with the last seven months (June–December) having each been record warm. Over land, the globally averaged temperature was also record high. Dozens of countries reported record or near-record warmth for the year, including China and continental Europe as a whole (warmest on record), India and Russia (second warmest), and Canada (third warmest). Intense and widespread heatwaves were reported around the world. In Vietnam, an all-time national maximum temperature record of 44.2°C was observed at Tuong Duong on 7 May, surpassing the previous record of 43.4°C at Huong Khe on 20 April 2019. In Brazil, the air temperature reached 44.8°C in Araçuaí in Minas Gerais on 20 November, potentially a new national record and 12.8°C above normal. The effect of rising temperatures was apparent in the cryosphere, where snow cover extent by June 2023 was the smallest in the 56-year record for North America and seventh smallest for the Northern Hemisphere overall. Heatwaves contributed to the greatest average mass balance loss for Alpine glaciers around the world since the start of the record in 1970. Due to rapid volume loss beginning in 2021, St. A

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reversible in-situ exsolution of Fe catalyst in La0.5Sr1.5Fe1.5Mo0.5O6-δ anode for SOFCs 16

reversible in-situ exsolution of Fe catalyst in La0.5Sr1.5Fe...

引用

16th International Symposium on Solid Oxide Fuel Cells, SOFC 2019

作者： Qi, H. Yang, T. Li, W. Ma, L. Hu, S. Shi, W. Sabolsky, E.M. Zondlo, J. Hart, R. Hackett, G.A. Liu, X. Department of Mechanical and Aerospace Engineering West Virginia University MorgantownWV26506 United States National Energy Technology Laboratory MorgantownWV26505 United States Oak Ridge Institute for Science and Education P.O. Box 117 Oak RidgeTN37830 United States Department of Energy and Power Engineering State Key Laboratory of Control and Simulation of Power System and Generation Equipments Tsinghua University Beijing10083 China GE Global Research Centre NiskayunaNY12309 United States

ISBN: (纸本)9781607688747

In-situ exsolution is widely considered to be an efficient and cost-effective method to enhance the electrochemical performance of a ceramic anode in solid oxide fuel cells (SOFCs). In this study, by controlling the non-stoichiometry of Sr2Fe1.5Mo0.5O6-δ with A-site doping, evenly distributed Fe nano-particles (~100 nm) were obtained on surface of La0.5Sr1.5Fe1.5Mo0.5O6-δ (LSFM) when treated in hydrogen. In a redox environment, excellent exsolution-dissolution reversibility was also demonstrated. Electrical conductivity relaxation (ECR) and electrochemical impedance spectroscopy (EIS) were employed to evaluate the surface reaction kinetics change during exsolution. The surface exchange coefficient (kex) was increased by 1.5 to 2 times with Fe exsolution. Based on distribution of relaxation time (DRT) analysis, the polarization resistance (Rp) associating with surface process was reduced in the first few hours. Both results revealed an enhanced surface reaction kinetics which mainly benefits from the high catalytic activity of exsolved nano-particles to H2 adsorption and dissociation process. © The Electrochemical Society.

关键词： Electrochemical impedance spectroscopy

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