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Point-defect-driven flattened polar phonon bands in fluorite ferroelectrics

npj Computational Materials 2023年第1期9卷 1120-1128页

作者： Pu Ai Fengjun Yan Wen Dong Shi Liu Junlei Zhao Kan-Hao Xue Syed Ul Hasnain Bakhtiar Yilong Liu Qi Ma Ling Miao Mengyuan Hua Guangzu Zhang Shenglin Jiang Wei Luo Qiuyun Fu School of Integrated Circuits Engineering Research Centre for Functional Ceramics of the Ministry of Education&Wuhan National Lab for Optoelectronics&Optical Valley Laboratory Huazhong University of Science and Technology430074 WuhanChina Department of Physics School of ScienceWestlake UniversityHangzhou310024 ZhejiangChina School of Optical and Electronic Information Research Centre&Wuhan National Lab for Optoelectronics&Optical Valley Laboratory Huazhong University of Science and Technology430074 WuhanChina Department of Electrical and Electronic Engineering Southern University of Science and Technology518055 ShenzhenChina Shenzhen Huazhong University of Science and Technology Research Institute 518000 ShenzhenP.R.China

The scale-free ferroelectric polarization of fluorite MO_(2)(M=Hf,Zr)due to flat polar phonon bands are promising for nonvolatile *** are also widely introduced to improve the emergent ***,their roles are still not fully understood at the ***,we report a significant effect of point-defect-driven flattening of polar phonon bands with more polar modes and polarization contribution in doped MO_(2).The polar phonon bands in La-doped MO_(2)(M=Hf,Zr)can be significantly flattened,compared with pure ***,the lower energy barrier with larger polarization of VO-only doped MO_(2) compared with La-doped cases suggest that VO and local lattice distortion should be balanced for high-performance fluorite *** work is believed to bridge the relation between point defects and the generally enhanced induced ferroelectricity in fluorite ferroelectrics at the atomic-level and inspire their further property optimization via defect-engineering.

关键词： bands phonon ferroelectric

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Enhancing hydrogen evolution and oxidation kinetics through oxygen insertion into nickel lattice

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Journal of Energy Chemistry 2024年第8期95卷 529-539,I0012页

作者： Wanli Liang Xiyu Gong Jinchang Xu Zixuan Dan Fanyan Xie Hulei Yu Hao-Fan Wang Yanshuo Jin Hongjuan Wang Yonghai Cao Hui Meng Hao Yu School of Chemistry and Chemical Engineering South China University of TechnologyGuangzhou 510641GuangdongChina Siyuan Laboratory Guangzhou Key Laboratory of Vacuum Coating Technologies and New Energy MaterialsGuangdong Provincial Engineering Technology Research Center of Vacuum Coating Technologies and New Energy MaterialsGuangdong Provincial Key Laboratory of Optical Fiber Sensing and CommunicationsDepartment of PhysicsJinan UniversityGuangzhou 510632GuangdongChina GBA Branch of Aerospace Information Research Institute Chinese Academy of SciencesGuangzhou 510700GuangdongChina Instrumental Analysis&Research Center Sun Yat-sen UniversityGuangzhou 510275GuangdongChina School of Materials Science and Engineering South China University of TechnologyGuangzhou 510641GuangdongChina

Nickel-based materials,including metallic Ni and Ni oxide,have been widely studied in the exploration of non-precious-metal hydrogen electrocatalysts,but neither pure Ni nor NiO is ideal for the hydrogen evolution reaction(HER)and hydrogen oxidation reaction(HOR).In this paper,an oxygen insertion strategy was applied on nickel to regulate its hydrogen electrocatalytic performance,and the oxygen-inserted nickel catalyst was successfully obtained with the assistance of tungsten dioxide support(denoted as O-Ni/WO_(2)).The partial insertion of oxygen in Ni maintains the face-centered cubic arrangement of Ni atoms,simultaneously expanding the lattice and increasing the lattice ***,the adsorption strength of^(*)H and^(*)OH on Ni is optimized,thus resulting in superior electrocatalytic performance of0-Ni/WO_(2)in alkaline HER/*** Tafel slope of O-Ni/WO_(2)@NF for HER is 56 mV dec^(-1),and the kinetic current density of O-Ni/WO_(2)for HOR reaches 4.85 mA cm^(-2),which is ahead of most currently reported *** proposed strategy of inserting an appropriate amount of anions into the metal lattice could provide more possibilities for the design of high-performance catalysts.

关键词： Hydrogen evolution Hydrogen oxidation Nickel Oxygen insertion Adsorption free energy

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A multifunctional flexible sensor based on PI-MXene/SrTiO_(3) hybrid aerogel for tactile perception

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The Innovation 2024年第3期5卷 44-54页

作者： Shihao Deng Yue Li Shengzhao Li Shen Yuan Hao Zhu Ju Bai Jingyi Xu Lu Peng Tie Li Ting Zhang Nano Science and Technology Institute University of Science and Technology of China(USTC)Suzhou 215123China i-lab Nano-X Vacuum Interconnected WorkstationKey Laboratory of Multifunctional Nanomaterials and Smart SystemsSuzhou Institute of Nano-Tech and Nano-Bionics(SINANO)Chinese Academy of Sciences(CAS)Suzhou 215123China School of Nano-Tech and Nano-Bionics University of Science and Technology of China(USTC)Hefei 230026China Jiangxi Institute of Nanotechnology 278 Luozhu RoadXiaolan Economic and Technological Development ZoneNanchang 330200China

The inadequacy of tactile perception systems in humanoid robotic manipulators limits the breadth of available robotic ***,we designed a multifunctional flexible tactile sensor for robotic fingers that provides capabilities similar to those of human skin sensing *** sensor utilizes a novel PI-MXene/SrTiO_(3) hybrid aerogel developed as a sensing unit with the additional abilities of electromagnetic transmission and thermal insulation to adapt to certain complex ***,polyimide(PI)provides a high-strength skeleton,MXene realizes a pressure-sensing function,and MXene/SrTiO_(3) achieves both thermoelectric and infrared radiation response ***,via the pressure response mechanism and unsteady-state heat transfer,these aerogel-derived flexible sensors realize multimodal sensing and recognition capabilities with minimal *** can differentiate among 13 types of hardness and four types of material from objects with accuracies of 94%and 85%,respectively,using a decision tree *** addition,based on the infrared radiation-sensing function,a sensory array was assembled,and different shapes of objects were successfully *** findings demonstrate that this PI-MXene/SrTiO_(3) aerogel provides a new concept for expanding the multifunctionality of flexible sensors such that the manipulator can more closely reach the tactile level of the human *** advancement reduces the difficulty of integrating humanoid robots and provides a new breadth of application scenarios for their possibility.

关键词： utilize integrating insulation

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Improving electrical and thermal properties synchronously via introducing CsPbBr_(3)QDs into higher manganese silicides

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Journal of Materials science & technology 2022年第16期111卷 279-286页

作者： Qing Wang Zhiliang Li Xiaofeng Yang Xin Qian Linjuan Guo Jianglong Wang Dan Zhang Shu-Fang Wang Key Laboratory of High-precision Computation and Application of Quantum Field Theory of Hebei Province College of Physics Science and TechnologyHebei UniversityBaoding 071002China Hebei Key Lab of Optic-Electronic Information and Materials College of Physics Science and TechnologyHebei UniversityBaoding 071002China

Higher manganese silicide(HMS)is a P-type medium temperature thermoelectric(TE)material,which has attracted widespread attention over the past few decades due to its remarkable mechanical properties,excellent chemical and thermal stability,as well as the non-toxicity,abundance and competitive *** peak power factor(PF)of HMS is as high as~1.50×10^(-3)W m^(-1)K^(-2)because of its intrinsic high electrical conductivity and Seebeck ***,the thermal conductivity of HMS is also high,resulting in relatively low z T *** nano-dispersion in the matrix is one of the most effective methods to enhance the TE properties via reducing the lattice thermal conductivity significantly without drastic changes on the other *** this study,Cs Pb BrQDs with uniform size were synthesized and introduced into HMS *** PF(at 823 K)was enhanced to 1.71×10^(-3)W m^(-1)K^(-2),which is improved 14.0%approximately compared with that of pure HMS owing to the combined effect of element doping and energy *** lattice thermal conductivity(at 823 K)decreased from 2.56W mKto 1.99 W mKsynchronously(~22.0%)due to the intensive phonon scattering caused by Cs doping,and the embedding of Pb riched CsPbBr_(3)QDs and Pb QDs.A maximum z T value of 0.57(823 K)is achieved in Cs Pb BrQDs/HMS composites,which is 36.0%higher than that of pure ***,for other TE materials,it is also feasible to improve the TE properties via introducing metastable quantum dots.

关键词： Thermoelectric material Higher manganese silicide Quantum dot Figure of merit Inclusion

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Multifunctional Carbon Foam with Nanoscale Chiral Magnetic Heterostructures for Broadband Microwave Absorption in Low Frequency

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Nano-Micro Letters 2025年第6期17卷 181-197页

作者： Hao Zhang Kaili Kuang Yifeng Zhang Chen Sun Tingkang Yuan Ruilin Yin Zeng Fan Renchao Che Lujun Pan School of Physics Dalian University of TechnologyDalian 116024LiaoningPeople’s Republic of China Laboratory of Advanced Materials Shanghai Key Lab of Molecular Catalysis and Innovative MaterialsDepartment of Materials ScienceFudan UniversityShanghai 200438People’s Republic of China

The construction of carbon nanocoil(CNC)-based chiral-dielectric-magnetic trinity composites is considered as a promising approach to achieve excellent low-frequency microwave ***,it is still challenging to further enhance the low frequency microwave absorption and elucidate the related loss ***,the chiral CNCs are first synthesized on a threedimensional(3D)carbon foam and then combined with the FeNi/NiFe_(2)O_(4) nanoparticles to form a novel chiral-dielectric-magnetic trinity *** 3D porous CNC-carbon foam network provides excellent impedance matching and strong conduction *** formation of the FeNi-carbon interfaces induces interfacial polarization loss,which is confirmed by the density functional theory *** permeability analysis and the micromagnetic simulation indicate that the nanoscale chiral magnetic heterostructures achieve magnetic pinning and coupling effects,which enhance the magnetic anisotropy and magnetic loss *** to the synergistic effect between dielectricity,chirality,and magnetism,the trinity composite foam exhibits excellent microwave absorption performance with an ultrabroad effective absorption bandwidth(EAB)of 14 GHz and a minimum reflection of loss less than-50 *** importantly,the C-band EAB of the foam is extended to 4 GHz,achieving the full C-band *** study provides further guidelines for the microstructure design of the chiral-dielectric-magnetic trinity composites to achieve broadband microwave absorption.

关键词： Carbon nanocoils Chiral magnetic structures 3D conductive networks Magnetic pinning effect Broadband microwave absorption

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Mesoporous polymers:soft-template self-assembly synthesis and applications

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science China Chemistry 2024年第5期67卷 1442-1464页

作者： Facai Wei Tingting Zhang Jianwei Fu Chengbin Jing Jiangong Cheng Shaohua Liu State Key Laboratory of Precision Spectroscopy Engineering Research Center of Nanophotonics&Advanced Instrument(Ministry of Education)School of Physics and Electronic ScienceEast China Normal UniversityShanghai 200241China School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450052China State Key Lab of Transducer Technology Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesShanghai 200050China

Mesoporous polymers combine the advantages of polymer materials(abundant polar functional groups,lightweight,flexibility,and processability)and mesoporous structures(high specific surface area,adjustable pore structure,and large pore volume);hence,they have great application potential in sensing,adsorption,catalysis,energy storage,biomedicine,***,developing advanced synthetic strategies for mesoporous polymers and investigating their intrinsic applications have become hot research ***-template-based self-assembly is regarded as a promising approach for synthesizing mesoporous *** work reviews recent progress in the synthetic strategy for producing various mesoporous polymers using soft-template selfassembly,focusing on the synthesis of conductive polymers,phenol-based polymers,and resin-based polymers and their potential ***,perspectives on future applications of mesoporous polymers,along with a few challenges that need to be resolved,are also discussed in this review.

关键词： mesoporous polymer porous material self-assembly soft templates interface synthesis

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Emerging hierarchical mesoporous materials of covalent organic frameworks

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science China Chemistry 2024年第9期67卷 2796-2802页

作者： Lingyan Huang Wenda Li Hongyi Zhang Shanzhe Ke Hao Chen Jianwei Fu Chengbin Jing Jiangong Cheng Shaohua Liu State Key Laboratory of Precision Spectroscopy/Engineering Research Center of Nanophotonics&Advanced Instrument(Ministry of Education) School of Physics and Electronic ScienceEast China Normal UniversityShanghai 200241China School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450052China State Key Lab of Transducer Technology Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesShanghai 200050China

Benefiting from abundant exposed active sites,minimized diffusion resistance of guest molecules,facilitated mass transfer process and enhanced storage capacity,covalent organic frameworks(COFs)have gained widespread scientific attention[1–4].Further construction of mesopores regarding pore engineering(pore size,pore geometry,pore volume,and framework compositions)in COFs can improve mass transport,accessibility as well as size-selectivity of the special guest moieties,thus exhibiting potential in catalysis,energy storage and separation and so on[5,6].

关键词： gained catalysis separation

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Engineering strong spin-frustration at the surface of three-dimensional graphene

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science Bulletin 2024年第18期69卷 2816-2819页

作者： Wenjing Li Ken Chen Menglei Li Huiying Gao Jize Zhao Fawei Zheng Wenhui Duan Center for Quantum Physics Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement(MOE)School of PhysicsBeijing Institute of TechnologyBeijing 100081China Beijing Key Lab of Nanophotonics&Ultrafine Optoelectronic Systems School of PhysicsBeijing Institute of TechnologyBeijing 100081China School of Physical Science and Technology Key Laboratory of Quantum Theory and Applications of MOELanzhou UniversityLanzhou 730000China Lanzhou Center for Theoretical Physics Key Laboratory of Theoretical Physics of Gansu ProvinceLanzhou UniversityLanzhou 730000China Department of Physics Capital Normal UniversityBeijing 100048China State Key Laboratory of Low Dimensional Quantum Physics Department of PhysicsTsinghua UniversityBeijing 100084China Institute for Advanced Study Tsinghua UniversityBeijing 100084China Frontier Science Center for Quantum Information Beijing 100084China Beijing Academy of Quantum Information Sciences Beijing 100193China

Since the first successful fabrication in 2004[1],graphene has received tremendous attention due to its extremely simple atomic structure and alluring physical *** example,its massless low energy excitations have a linear dispersion and thus its transport property is governed by Dirac equation instead of Schr?dinger *** special electronic structures suppress the intra-valley and inter-valley backscatterings,leading to the half-integer and fractional quantum Hall effect[2]under magnetic field and the relativistic quantum tunneling described by the Klein paradox[3].

关键词： properties equation quantum

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Quantum dots enhanced stability of in-situ fabricated perovskite nanocrystals based light-emitting diodes:Electrical field distribution effects

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Fundamental Research 2025年第1期5卷 347-353页

作者： Xulan Xue Menglin Li Zhenjie Liu Chenhui Wang Jincheng Xu Shuangpeng Wang Hanzhuang Zhang Haizheng Zhong Wenyu Ji Key Lab of Physics and Technology for Advanced Batteries(Ministry of Education) College of PhysicsJilin UniversityChangchun 130012China MIIT Key Laboratory for Low-Dimensional Quantum Structure and Devices School of Materials Science&EngineeringBeijing Institute of TechnologyBeijing 100081China Institute of Applied Physics and Materials Engineering University of MacaoTaipa 999078China

With the development in fabricating efficient perovskite light emitting diodes(PeLEDs),improving the operating stability becomes an urgent *** we report quantum dot(QD)enhanced stability of PeLEDs by introducing CdSe/ZnS core-shell QDs in toluene anti-solvent during in-situ fabrication of FAPbBr3 perovskite nanocrystals(PNCs)*** comparison with PNC films with pristine toluene as the anti-solvent,the as-prepared FAPbBr3 PNC films with a QD monolayer on the surface exhibit improved photoluminescence quantum yield,enhanced photostability and better *** from these advantages,the peak luminance and the maximum external quantum efficiency of the PeLED containing QD monolayer are increased from 6807 cd/m^(2)to 86,670 cd/m^(2)and 2.4%to 7.1%,*** T50 lifetime under the initial luminance of 1021 cd/m^(2)approaches 83 *** on electrical field simulation and transient electroluminescence measurements,the enhanced stability can be mainly attributed to the electrical field redistribution induced by the QD *** work demonstrates that the combination of QDs and perovskites provides an effective strategy to address the operational stability of *** insights into electrical field distribution effect will make great impact on stability improvement of other perovskite based devices.

关键词： Perovskite nanocrystals Quantum dots Electrical field distribution Light-emitting diodes Operational stability

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A Simple Building Block with Noncovalently Conformational Locks towards Constructing Low-Cost and High-Performance Nonfused Ring Electron Acceptors

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Chinese Journal of Polymer science 2023年第4期41卷 556-563,I0008页

作者： Xiao-Bin Gu Jin-Hua Gao Zi-Yang Han Yu-Hao Shi Ya-Nan Wei Yin-Cheng Zhang Qian Peng Zhi-Xiang Wei Xin Zhang Hui Huang College of Materials Science and Opto-Electronic Technology Center of Materials Science and Optoelectronics EngineeringCAS Center for Excellence in Topological Quantum ComputationCAS Key Laboratory of Vacuum PhysicsUniversity of Chinese Academy of SciencesBeijing100049China School of Chemical Sciences University of Chinese Academy of SciencesBeijing100049China CAS Key Laboratory of Nanosystem and Hierarchical Fabrication CAS Center for Excellence in NanoscienceNational Center for Nanoscience and TechnologyBeijing100190China

Nonfused ring electron acceptors(NFREAs)have attracted much attention due to their concise synthetic routes and low ***,developing high-performance NFREAs with simple structure remains a great *** this work,a simple building block(POBT)with noncovalently conformational locks(No CLs)was designed and ***-crystal X-ray study indicated the presence of S…O NOCLs in POBT,thus enabling it to possess a coplanar conformation comparable to that of fused-ring *** novel NFREAs based on CPT and POBT were developed,namely TT-CPT and TT-POBT,***,TT-POBT possessed a smaller Stokes shift and a reduced reorganization energy compared with TT-CPT,indicating the introduction of S…O No CLs can enhance the molecular rigidity even if simplifying the molecular *** a result,the TT-POBT-based PSC device afforded an impressive power conversion efficiency of 11.15%,much higher than that of TT-CPT counterpart(7.03%),mainly resulting from the tighterπ-πstacking,improved and balanced charge transport,and more favorable film *** work demonstrates the potential of the simple building block POBT with No CLs towards constructing low-cost and highperformance NFREAs.

关键词： Polymer solar cells Nonfused ring electron acceptors Simple building block Noncovalent conformation locks Reorganization energy

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