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CLEO: science and Innovations in CLEO 2024, CLEO: S and I 2024 - Part of Conference on Lasers and Electro-Optics

作者： Anderson, B.E. Zhao, J. Zhou, Z. Speirs, R. Jones, K.M. Lett, P.D. Department of Physics American University 4400 Massachusetts Ave. NW WashingtonDC20016 United States Joint Quantum Institute National Institute of Standards and Technology The University of Maryland College ParkMD20742 United States Centre for Quantum Computation and Communication Technology Department of Quantum Science and Technology Research School of Physics The Australian National University CanberraACT2601 Australia Department of Physics Williams College 33 Lab Campus Drive WilliamstownMA01267 United States

We construct a phase-conjugate resonator which passively mode-locks, produces pulsing, and is unconditionally stable. The resonator uses non-degenerate four-wave mixing in rubidium vapor and the output switches betwee... 详细信息

关键词： Four wave mixing

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Color Switching in a Mode-Locked Optical Phase-Conjugate Resonator

Color Switching in a Mode-Locked Optical Phase-Conjugate Res...

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2024 Conference on Lasers and Electro-Optics, CLEO 2024

ISBN: (纸本)9781957171395

关键词： Four wave mixing

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Nonlinear defect theory of thermal relaxation in complex multimoded systems

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Physical Review Research 2024年第3期6卷 033114-033114页

作者： Emily Kabat Alba Y. Ramos Lucas J. Fernández-Alcázar Tsampikos Kottos Wave Transport in Complex Systems Lab Department of Physics Institute for Modeling and Innovative Technology IMIT ( Physics Department Natural and Exact Science Faculty

We show that a single nonlinear defect can thermalize an initial excitation towards a Rayleigh-Jeans (RJ) state in complex multimoded systems. The thermalization can be hindered by disorder-induced localization phenomena, which drive the system into a metastable RJ state. It can differ dramatically from the thermal RJ and it involves only a (quasi)isolated set of prethermal modes whose density can be predicted using a renormalization group theory. Importantly, we establish a connection between the modal relaxation rates that dictate the dynamics towards (quasi)equilibrium and the Thouless conductance. This connection allows us to derive the whole modal relaxation rate distribution. Our results are relevant to photonics, optomechanics, and cold atoms.

关键词： Anderson localization Dynamics of networks Kinetic theory Nonlinear optics Photonics Wave chaos Collective dynamics Complex media Complex networks Coupled oscillators Disordered systems Dynamical systems Fibers Nonequilibrium systems Nonlinear waves Optical fibers Waveguides Computational complexity Data analysis Finite-size scaling Numerical approximation & analysis Perturbative methods Random matrix theory Renormalization group Scaling methods Schroedinger equation

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High-Efficiency and Low-Energy-Loss Organic Solar Cells Enabled by Tuning Conformations of Dimeric Electron Acceptors

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CCS Chemistry 2023年第11期5卷 2576-2588页

作者： Xiaobin Gu Yanan Wei Na Yu Jiawei Qiao Ziyang Han Qijie Lin Xiao Han Jinhua Gao Congqi Li Jianqi Zhang Xiaotao Hao Zhixiang Wei Zheng Tang Yunhao Cai Xin Zhang Hui Huang College of Materials Science and Opto-Electronic Technology Center of Materials Science and Optoelectronics EngineeringCAS Center for Excellence in Topological Quantum ComputationCAS Key Laboratory of Vacuum PhysicsUniversity of Chinese Academy of SciencesBeijing 100049 Center for Advanced Low-Dimension Materials State Key Laboratory for Modification of Chemical Fibers and Polymer MaterialsCollege of Materials Science and EngineeringDonghua UniversityShanghai 201620 School of Physics State Key Laboratory of Crystal MaterialsShandong UniversityJinan 250100 Center for Excellence in Nanoscience(CAS) Key Laboratory of Nanosystem and Hierarchical Fabrication(CAS)National Center for Nanoscience and TechnologyBeijing 100190

Dimeric fused-ring electron acceptors(DFREAs)have attracted much attention due to the combined advantages of their monomeric and polymeric acceptors,including a well-defined molecular structure,excellent repeatability,and stable ***,the additionally introduced single-bonds during dimerization may result in a twisted backbone of DFREAs,which is detrimental to intermolecular packing and charge ***,three DFREAs are designed and synthesized,in which DFREA conformations were systematically tuned via adjusting the intensities of intramolecular noncovalent interactions(INIs)to achieve high-performance organic solar cells(OSCs).Theoretical and experimental results show that the gradual introduction of S…F INIs can continuously improve molecular planarity and rigidity,resulting in reduced reorganization energies,ordered packing mode,and enhanced crystallization of *** from the incorporation of fourfold S…F INIs,DYF-TF-based binary OSCs show a record high efficiency of 18.26%with an extremely low energy loss(0.493 eV)for DFREAbased *** addition,DYF-TF-based OSCs exhibited good long-term stability with a T_(80%)lifetime of 2681 h,and the power conversion efficiency of the DYF-TF-based ternary device is further enhanced to 18.73%.This contribution demonstrates the great potential of the INIs strategy in achieving excellent DFREAs materials.

关键词： organic solar cells dimeric fused-ring electron acceptors intramolecular noncovalent interactions molecular planarity and rigidity reorganization energies

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Effect of pH and applied stress on hydrogen sulfide stress corrosion behavior of HSLA steel based on electrochemical noise analysis

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Journal of Iron and Steel Research International 2023年第12期30卷 2531-2540页

作者： Xiao-hua Li Chen-xi Liu Teng Zhang Chuan-tao Lv Jiang-cheng Liu Ran Ding Zhi-ming Gao Rui Wang Yong-chang Liu School of Mechanical Engineering Tianjin University of Technology and EducationTianjin300222China State Key Lab of Hydraulic Engineering Simulation and Safety School of Materials Science&EngineeringTianjin UniversityTianjin300350China Southwestern Institute of Physics Chengdu610041SichuanChina Tianjin Pipe Corporation Tianjin300301China

The influence mechanism of pH and the externally applied stress on sulfide stress corrosion cracking behavior based on the joint analysis of the in situ electrochemical noise and microstructure was *** results showed that{\mathrm{H}}^{+}in solution changes the composition and structure of corrosion product film by affecting the concentration of{\mathrm{S}}^{2-}and{\mathrm{Fe}}^{2+}near the anode *** the pH increased from 2.6 to 3.6 and 4.6,the corrosion product film changed from porous Mackinawite to dense and stable *** change in corrosion product type delayed the crack initiation time by 10.5 and 45.5 h,while the uniform corrosion time was prolonged by 6.1 and 46 h,respectively,delaying SSC *** increasing the applied stress,the local plastic deformation on the material surface increases the porosity and crack rate of the corrosion product film and becomes a fast propagation channel for SSC *** the applied stress is 110%of the actual yield strength of the material,the initiation time of stress corrosion cracking is 6 and 18.1 h earlier than that of 90%and 100%,*** local corrosion time was extended by 23.5 and 8.2 h,respectively,accelerating SSC behavior.

关键词： Sulfide stress cracking Electrochemical noise pH-Stress High strength low alloy steel

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Self‑Generated Buried Submicrocavities for High‑Performance Near‑Infrared Perovskite Light‑Emitting Diode

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Nano-Micro Letters 2023年第8期15卷 355-367页

作者： Jiong Li Chenghao Duan Qianpeng Zhang Chang Chen Qiaoyun Wen Minchao Qin Christopher C.S.Chan Shibing Zou Jianwu Wei Zuo Xiao Chuantian Zuo Xinhui Lu Kam Sing Wong Zhiyong Fan Keyou Yan School of Environment and Energy State Key Lab of Luminescent Materials and DevicesGuangdong Provincial Key Laboratory of Solid Wastes Pollution Control and RecyclingSouth China University of TechnologyGuangzhou 510000People’s Republic of China Department of Electronic and Computer Engineering The Hong Kong University of Science and TechnologyClear Water BayKowloonHong KongPeople’s Republic of China Department of Physics The Chinese University of Hong KongShatinHong KongPeople’s Republic of China Department of Physics The Hong Kong University of Science and TechnologyClear Water BayKowloon 999077Hong KongPeople’s Republic of China School of Chemistry and Chemical Engineering Guangxi UniversityNanning 530004People’s Republic of China Center for Excellence in Nanoscience(CAS) Key Laboratory of Nanosystem and Hierarchical Fabrication(CAS)National Center for Nanoscience and TechnologyBeijing 100190People’s Republic of China

ABSTRACT Embedding submicrocavities is an effective approach to improve the light out-coupling efficiency(LOCE)for planar perovskite light-emitting diodes(PeLEDs).In this work,we employ phenethylammonium iodide(PEAI)to trigger the Ostwald ripening for the downward recrystallization of perovskite,resulting in spontaneous formation of buried submicrocavities as light output *** simulation suggests the buried submicrocavities can improve the LOCE from 26.8 to 36.2%for near-infrared ***,PeLED yields peak external quantum efficiency(EQE)increasing from 17.3%at current density of 114 mA cm^(−2)to 25.5%at current density of 109 mA cm^(−2)and a radiance increasing from 109 to 487 W sr^(−1)m^(−2)with low *** turn-on voltage decreased from 1.25 to 1.15 V at 0.1 W sr^(−1)m^(−2).Besides,downward recrystallization process slightly reduces the trap density from 8.90×10^(15)to 7.27×10^(15)cm^(−3).This work provides a self-assembly method to integrate buried output coupler for boosting the performance of PeLEDs.

关键词： Perovskite light-emitting diodes Downward recrystallization Buried submicrocavities Light out-coupling efficiency Radiative recombination

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Probing the Gamma-Ray Emission Region of Five TeV Flat Spectrum Radio Quasars

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Research in Astronomy and Astrophysics 2024年第6期24卷 156-169页

作者： Hu-Bing Xiao Hai-Tao Cao Rui Xue Jin-Ting Cai Ge-Ge Wang Marina Manganaro Shao-Hua Zhang Zhi-Hao Ouyang Li-Ping Fu Jun-Hui Fan Shanghai Key Lab for Astrophysics Shanghai Normal UniversityShanghai 200234China School of Information Engineering Guangzhou Panyu PolytechnicGuangzhou 511483China Department of Physics Zhejiang Normal UniversityJinhua 321004China College of Mathematics and Physics Guangxi Minzu UniversityNanning 530006China Key Laboratory of Cosmology and Astrophysics(Liaoning) College of SciencesNortheastern UniversityShenyang 110819China Department of Physics University of RijekaRijeka 51000Croatia Center for Astrophysics Guangzhou UniversityGuangzhou 510006China Key Laboratory for Astronomical Observation and Technology of Guangzhou Guangzhou 510006China Astronomy Science and Technology Research Laboratory of Department of Education of Guangdong Province Guangzhou 510006China

The location ofγ-ray emission of blazars remains a contested topic,inspiring the development of numerous investigative techniques to address this *** this work,we analyzed Fermiγ-ray light curves in the GeV and MeV bands,employing the discrete cross-correlation function method to discern time lags between the two *** 4C+21.35,Ton 599,B21420+32,and PKS 1510-089,we identified a time lag spanning several days,while for PKS 1441+25,the time lag was not statistically *** results imply that the soft photons necessary for inverse Compton scattering predominantly originate from the dusty torus in the first four sources,whereas for PKS1441+25,they seem to be sourced mainly from the broad-line *** analysis of the opacity(τγγ)and the GeV spectra study supports the conclusion that the location of the dissipation region must be beyond the BLR to avoid significant ***,for PKS 1441+25,the emission region is also posited to lie outside yet proximate to the *** parameters of describing the emission region were obtained by fitting broadband spectral energy distribution with contemporaneous observation *** findings suggest that for the five TeV FSRQs,during Te V flaring events,the jet appears to maintain an equilibrium between the energy density of the magnetic field and that of the particles for all investigated sources,with the exceptions of 4C+21.35 and PKS1441+*** terms of the overall jet power,particle energy is the dominant contributor,and the observed blazar radiation cannot be solely attributed to the magnetic field,except in the case of 4C+***,magnetic reconnection is unlikely to be the primary mechanism behind particle acceleration in these systems.

关键词： galaxies:active gamma-rays:galaxies galaxies:jets

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Beam normal single-spin asymmetry in electron-proton scattering with intermediate state resonances 25

Beam normal single-spin asymmetry in electron-proton scatter...

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25th International Symposium on Spin physics, SPIN 2023

作者： Ahmed, Jaseer Blunden, Peter Melnitchouk, Wally Department of Physics Shahjalal University of Science and Technology Sylhet3114 Bangladesh Department of Physics and Astronomy University of Manitoba WinnipegMBR3T 2N2 Canada Jefferson Lab Newport NewsVA23606 United States

This contribution highlights results from our recent calculations of beam normal single-spin asymmetries in electron–proton elastic scattering that depend on the imaginary (absorptive) part of two-photon exchange amplitudes. The intermediate hadronic states are modelled by spin 1/2 and 3/2 resonance states below 1.8 GeV in mass. CLAS exclusive meson electroproduction data are used as input for the transition amplitudes from the proton to the resonance states, and we also include the effect of resonance widths. We compare results with data from the SAMPLE, A4, and Qweak experiments. © Copyright owned by the author(s) under the terms of the Creative Commons.

关键词： Germanium compounds

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Recent progress on surface chemistryⅡ:Property and characterization

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Chinese Chemical Letters 2025年第1期36卷 8-57页

作者： Xin Li Zhen Xu Donglei Bu Jinming Cai Huamei Chen Qi Chen Ting Chen Fang Cheng Lifeng Chi Wenjie Dong Zhenchao Dong Shixuan Du Qitang Fan Xing Fan Qiang Fu Song Gao Jing Guo Weijun Guo Yang He Shimin Hou Ying Jiang Huihui Kong Baojun Li Dengyuan Li Jie Li Qing Li Ruoning Li Shuying Li Yuxuan Lin Mengxi Liu Peinian Liu Yanyan Liu Jingtao Lü Chuanxu Ma Haoyang Pan JinLiang Pan Minghu Pan Xiaohui Qiu Ziyong Shen Qiang Sun Shijing Tan Bing Wang Dong Wang Li Wang Lili Wang Tao Wang Xiang Wang Xingyue Wang Xueyan Wang Yansong Wang Yu Wang Kai Wu Wei Xu Na Xue Linghao Yan Fan Yang Zhiyong Yang Chi Zhang Xue Zhang Yang Zhang Yao Zhang Xiong Zhou Junfa Zhu Yajie Zhang Feixue Gao Yongfeng Wang Center for Carbon-based Electronics and Key Laboratory for the Physics and Chemistry of Nanodevices School of ElectronicsPeking UniversityBeijing 100871China Spin-X Institute School of MicroelectronicsSouth China University of TechnologyGuangzhou 511442China School of Materials and Energy Guangzhou Key Laboratory of Low-Dimensional Materials and Energy Storage DevicesGuangdong University of TechnologyGuangzhou 510006China Faculty of Materials Science and Engineering Kunming University of Science and TechnologyKunming 650093China i-Lab CAS Key Laboratory of Nanophotonic Materials and DevicesSuzhou Institute of Nano-Tech and Nano-BionicsChinese Academy of SciencesSuzhou 215123China CAS Key Laboratory of Molecular Nanostructure and Nanotechnology CAS Research/Education Center for Excellence in Molecular SciencesBeijing National Laboratory for Molecular Sciences(BNLMS)Institute of ChemistryChinese Academy of SciencesBeijing 100190China State Key Laboratory for Organic Electronics and Information Displays&Jiangsu Key Laboratory for Biosensors Institute of Advanced MaterialsJiangsu National Synergetic Innovation Center for Advanced MaterialsNanjing University of Posts and TelecommunicationsNanjing 210023China Institute of Functional Nano and Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials and DevicesSoochow UniversitySuzhou 215123China Hefei National Research Center for Physical Sciences at the Microscale and Synergetic Innovation Center of Quantum Information and Quantum Physics University of Science and Technology of ChinaHefei 230026China Institute of Physics&University of Chinese Academy of Sciences Beijing 100190China State Key Laboratory of Catalysis Dalian Institute of Chemical PhysicsChinese Academy of SciencesDalian 116023China College of Chemistry Beijing Normal UniversityBeijing 100875China Beijing National Laboratory for Molecular Sciences(BNLMS) College of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China School

Surface with well-defined components and structures possesses unique electronic,magnetic,optical and chemical *** a result,surface chemistry research plays a crucial role in various fields such as catalysis,energy,materials,quantum,and *** science mainly investigates the correspondence between surface property and *** probe microscopy(SPM)techniques are important tools to characterize surface properties because of the capability of atomic-scale imaging,spectroscopy and manipulation at the single-atom *** this review,we summarize recent advances in surface electronic,magnetic and optical properties characterized mainly by SPM-based *** focus on elucidating theπ-magnetism in graphene-based nanostructures,construction of spin qubits on surfaces,topology properties of surface organic structures,STM-based light emission,tip-enhanced Raman spectroscopy and integration of machine learning in SPM studies.

关键词： Surface chemistry Scanning probe microscopy π-Magnetism Spin qubits Tip-enhanced Raman spectroscopy

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用于高效电磁波吸收的3D打印超材料

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science China Materials 2023年第4期66卷 1283-1312页

作者：周睿于震吴蓁蓁曲畅宋燕邢瑞哲孔杰 Shaanxi Key Lab of Macromolecular Science and Technology MOE Key Lab of Materials Physics and Chemistry in Extraordinary ConditionsSchool of Chemistry and Chemical EngineeringNorthwestern Polytechnical UniversityXi’an 710072China

由人工结构组成的超材料具有传统材料不具备的卓越性能.通过设计和排列具有特殊物理性质的单元结构可制备用于高效电磁波吸收的吸波超材料.这些亚波长尺度的单元结构是吸波超材料超越传统材料性能极限的基础,因此制造工艺的匹配尤为重要... 详细信息

由人工结构组成的超材料具有传统材料不具备的卓越性能.通过设计和排列具有特殊物理性质的单元结构可制备用于高效电磁波吸收的吸波超材料.这些亚波长尺度的单元结构是吸波超材料超越传统材料性能极限的基础,因此制造工艺的匹配尤为重要.快速发展的3D打印技术在制造具有复杂结构的材料方面展现出巨大的优势和潜力,为研究和制备吸波超材料提供了一种简单、快速、高效的方法.在这篇综述中,我们介绍了吸波超材料的概念和发展,重点介绍了利用3D打印技术制造吸波超材料的研究现状.此外,还简要介绍了超材料的典型应用,讨论了当前超材料发展的不足和3D打印技术制备吸波超材料的局限性,并提出了超材料和3D打印技术结合的发展前景.

关键词：电磁波吸收单元结构超材料典型应用制造工艺性能极限发展前景亚波长

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