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Operando modeling and measurements:powerful tools for revealing the mechanism of alkali carbonate-based sorbents for CO_(2)capture in real conditions

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Frontiers in Energy 2023年第3期17卷 380-389页

作者： Tianyi CAI Mengshi WANG Xiaoping CHEN Ye WU Jiliang MA Wu ZHOU School of Energy and Power Engineering Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power EngineeringUniversity of Shanghai for Science and TechnologyShanghai 200093China Key Laboratory of Energy Thermal Conversion and Control of the Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 210096China Key Laboratory of Thermal Control of Electronic Equipment and Advanced Combustion Laboratory of the Ministry of Industry and Information Technology School of Energy and Power EngineeringNanjing University of Science and TechnologyNanjing 210094China

Alkalicarbonate-based sorbents(ACSs),including Na_(2)CO_(3)-and K2CO_(3)-based sorbents,are promising for CO_(2)***,the complex sorbent components and operation conditions lead to the versatile kinetics of CO_(2)sorption on these *** paper proposed that operando modeling and measurements are powerful tools to understand the mechanism of sorbents in real operating conditions,facilitating the sorbent development,reactor design,and operation parameter *** reviewed the theoretical simulation achievements during the development of *** elucidated the findings obtained by utilizing density functional theory(DFT)calculations,ab initio molecular dynamics(AIMD)simulations,and classical molecular dynamics(CMD)simulations as *** hygroscopicity of sorbent and the humidity of gas flow are crucial to shifting the carbonation reaction from the gas-solid mode to the gas-liquid mode,boosting the ***,it briefly introduced a machine learning(ML)approach as a promising method to aid sorbent ***,it demonstrated a conceptual compact operando measurement system in order to understand the behavior of ACSs in the real operation *** proposed measurement system includes a micro fluidizedbed(MFB)reactor for kinetic analysis,a multi-camera sub-system for 3D particle movement tracking,and a combined Raman and IR sub-system for solid/gas components and temperature *** is believed that this system is useful to evaluate the real-time sorbent performance,validating the theoretical prediction and promoting the industrial scale-up of ACSs for CO_(2)capture.

关键词： CO_(2)capture carbonation theoretical modeling operando techniques reaction visualization

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Deformation Analysis and Prediction of Pneumatic Probe Based on Fluid-structure Interaction

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International Journal of Fluid Machinery and Systems 2023年第1期16卷 1-13页

作者： Fan, Yang Dexin, Qiu Xinwei, Zhao Qingyi, Sai Xiaoshu, Cai School of Energy and Power Engineering University of Shanghai for Science and Technology No. 516 Jungong Road Shanghai200093 China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering University of Sh anghai for Science and Technology No. 516 Jungong Road Shanghai200093 China

As an essential tool for measuring flow field, pneumatic probes have gained a wide range of applications. In order to obtain the flow field parameters accurately, it is also crucial to study the deformation of the pneumatic probe structure in flow field. In this paper, the deformation of the conical probe is numerically simulated under the condition of steady incoming flow in the transonic flow field. The fluid-structure interaction and modal analysis methods are used to obtain the deformation and vibration frequency of the probe. The results show that the vibration of the probe is underdamped under the action of two-way fluid-structure interaction, and the total deformation decays exponentially, and the total deformation after stabilization is the same as the result of one-way fluid-structure interaction. For the same material probe, the total deformation changes with time in the same dimensionless expression, and the vibration frequency as well as damping factor do not change due to the variation of flow field. The accuracy of the dimensionless expressions was verified by different incoming flow conditions and the probe material. For the cases studied in this paper, the maximum total deformation, vibration frequency and damping factor of the probe in the flow field can be obtained by using one-way fluid-structure interaction, modal analysis and two-way fluid-structure interaction with a small number of cycles, respectively, so that the total deformation of the probe in the flow field can be predicted over time. The method obtained in this paper can significantly reduce the calculation time for obtaining the probe deformation data in the flow field and improve the work efficiency, which can provide a reference for the design, calibration and application of probes in engineering applications. © 2023, Turbomachinery Society of Japan. All rights reserved.

关键词： Modal analysis

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A universal charge-compensating strategy for high-energy-density pseudocapacitors

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Journal of Energy Chemistry 2023年第3期78卷 333-339,I0010页

作者： Baoyi Yin Jiaqi Zhang Yuanhui Su Yu Huan Liang Hao Chen Wang Xun Hu Tao Wei School of Material Science and Engineering University of Jinan336 Nanxinzhuang West RoadJinan 250022ShandongChina School of Microelectronics Dalian University of TechnologyDalian 116024LiaoningChina Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering School of Energy and Power EngineeringUniversity of Shanghai for Science and TechnologyShanghai 200093China State Key Laboratory of ASIC and Systems School of MicroelectronicsFudan UniversityShanghai 200433China

For pseudocapacitive electrode materials(PseEMs),despite much progress having been made in achieving both high power density and high energy density,a general strategy to guide the enhancement of intrinsic capacitive properties of PseEMs remains ***,we demonstrate a universal chargecompensating strategy to improve the charge-storage capability of PseEMs intrinsically:ⅰ) in the electrolyte with anion as charge carriers(such as OH-),reducing the multivalent cations of PseEMs into lower valences could create more reversible low-to-high valence redox cou ples to promote the intercalation of the anions;ⅱ) in the electrolytes with cation as charge carriers(such as H^(+),Li^(+),Na^(+)),oxidizing the multivalent cations of PseEMs into higher valences could introduce more reversible high-to-low valence redox couples to promote the intercalation of the *** we demonstrated that the improved intrinsic charge-storage capability for PseEMs originates from the increased Faradaic charge storage sites.

关键词： Supercapacitors Universal charge-compensating strategy Changed valence state Increased Faradaic charge storage sites

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Numerical and experimental research of the characteristics of concentration solar cells

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Frontiers in Energy 2021年第2期15卷 279-291页

作者： Zilong WANG Hua ZHANG Binlin DOU Weidong WU Guanhua ZHANG Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering School of Energy and Power EngineeringUniversity of Shanghai for Science and TechnologyShanghai 200093China

The development of automatic tracking solar concentrator photovoltaic systems is currently attracting growing *** concentration photovoltaic systems(HCPVs)combining triple-junction InGaP/lnGaAs/Ge solar cells with a concentrator provide high conversion *** mathematical model for triple-junction solar cells,having a higher efficiency and superior temperature characteristics,was established based on the one-diode equivalent circuit cell model.A paraboloidal concentrator with a secondary optic system and a concentration ratio in the range of 100X–150X along with a sun tracking system was developed in this *** GaInP/GalnAs/Ge triple-junction solar cell,produced by AZUR SPACE Solar power,was also used in this *** solar cells produced by shanghai Solar Youth Energy(SY)and Shenzhen Yinshengsheng Technology ***.(YXS)were used as comparison samples in a further comparative study at different concentration ratios(200X–1000X).A detailed analysis on the factors that influence the electrical output characteristics of the InGaP/lnGaAs/Ge solar cell was conducted with a dish-style concentrating photovoltaic *** results show that the short-circuit current(Isc)and the open-circuit voltage(Voc)of multi-junction solar cells increases with the increasing concentration ratio,while the cell efficiency(ηc)of the solar cells increases first and then decreases with increasing concentration *** increasing solar cell temperature,Isc increases,while Voc andηc decrease.A comparison of the experimental and simulation results indicate that the maximum root mean square error is less than 10%,which provides a certain theoretical basis for the study of the characteristics of triple-junction solar cell that can be applied in the analysis and discussion regarding the influence of the relevant parameters on the performance of high concentration photovoltaic systems.

关键词： concentration three-junction solar cell mathematical model electrical properties solar energy

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Influence of suction flow control on energy extraction characteristics of flapping foil

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INTERNATIONAL JOURNAL OF GREEN ENERGY 2022年第8期19卷 888-903页

作者： Wang, Jiayue Huang, Shengxian Hou, Longfeng Wang, Ying Univ Shanghai Sci & Technol Sch Energy & Power Engn Shanghai Key Lab Multiphase Flow & Heat Transfer Shanghai 200093 Peoples R China

Flapping foil (FF) is a relatively new renewable energy extraction device, which has the advantages of simple structure, strong environmental adaptability and little impact on the environment. This study proposed a new FF energy extraction equipment with suction control added to the surface. Based on the moving grid technology, the effect of different suction control methods on energy extraction characteristics of FF was numerically investigated. In this paper, taking NACA0012 as the reference airfoil, the influence laws of key parameters, such as suction velocity, suction port position and suction mode on the energy extraction efficiency of FF were studied respectively. The results show that, compared with the original FF, the addition of suction control can effectively control the size of the leading edge negative effect vortex, increase the force consistent with the motion direction of the FF and its surface pressure difference, thus improving the energy extraction efficiency. In addition, the innovative change of suction mode to sinusoidal suction mode in this paper can not only enhance the stability and safety of FF operation structure, but also its energy extraction efficiency is not much different from that of FF with sudden suction control.

关键词： flapping foil energy extraction suction flow control simulation

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Theoretical and experimental evaluation on the electrical properties of multi-junction solar cells in a reflective concentration photovoltaic system

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ENERGY REPORTS 2022年 8卷 820-831页

作者： Wang, Zilong Zhang, Hua Dou, Binlin Zhang, Guanhua Wu, Weidong Univ Shanghai Sci & Technol Sch Energy & Power Engn Shanghai Key Lab Multiphase Flow & Heat Transfer Shanghai 200093 Peoples R China

Solar photovoltaic systems represent an important technology for renewable energy utilization and have broad potential for application and development. However, the further development of solar photovoltaic systems is hindered by their higher generation costs. A high-concentration photovoltaic system (HCPVs) can use an inexpensive concentrator to replace solar cells;this, in turn, reduces the cost of electricity generation, because the solar cell requirement decreases for a given power. This study developed a mathematical model for multi-junction solar cell (MJSC) based on single-diode equivalent circuit, furthermore, an HCPVs with hyperboloid mirrors was established. The electrical properties for an MJSC module, including the short-circuit current (I-sc), peak power (P-m), open-circuit voltage (V-oc), fill factor (FF), and efficiency (eta) were investigated at concentration ratios between 650 X and 800 X and direct solar radiation intensities between approximately 400 W/m(2) and 730 W/m(2). Furthermore, the experimental results and theoretical values were comparatively analyzed. The results demonstrated that I-sc, V-oc,V- and P-m of MJSC module increased as the direct solar radiation raised. In contrast, the FF and eta of an MJSC module decreased as the direct solar radiation raised. As the direct solar radiation intensity was 700 W/m(2) and concentration ratio increased from 650 X to 800 X, I-sc, V-oc, and P-m increased from 1.002 A to 1.243 A, 11.095 V to 11.158 V, and 9.466 W to 11.358 W, respectively. Conversely, the FF and eta of the MJSC module decreased from 32.51 % to 31.33 % and 0.851 to 0.819, respectively. The tallied between the numerical and experimental results was evaluated, which indicated that root-mean-square error between the experimental and calculated values increased as the direct solar radiation increased.(c) 2021 The Author(s). Published by Elsevier Ltd.

关键词： Solar energy Triple-junction solar cell High-concentration photovoltaic system Hyperboloid mirrors Mathematical model

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The airfoil design and parameter optimization of the deformable micro air vehicle

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engineering COMPUTATIONS 2023年第9/10期40卷 2029-2048页

作者： Huang, Shengxian Qiu, Huihe Wang, Ying Univ Shanghai Sci & Technol Sch Energy & Power Engn Shanghai Key Lab Multiphase Flow & Heat Transfer P Shanghai Peoples R China Dept Mech & Aerosp Engn Hong Kong Peoples R China

Purpose - Since most of the existing literature do not disclose the node coordinate data of its fixed-wing aircraft airfoil, in order to develop and obtain a practical and suitable deformation airfoil for fixed-wing micro air vehicle (MAV), this paper proposes an improved airfoil design method of fixed-wing MAV based on the profile data of S5010 ***/methodology/approach - Combined with the body shape variation of the stingray in the propulsion process, the parametric study of the aerodynamic shape of the original design airfoil is carried out to explore the influence of a single parameter change on the aerodynamic performance of the airfoil. Then, according to the influence law of single parameter variation on the aerodynamic performance of the airfoil, the original airfoil is synthetically deformed by changing multiple *** - By comparing the aerodynamic performance of the multi-parameter deformed airfoil with the original airfoil, it is found that the lift coefficient of the multi-parameter deformed airfoil changes from negative to positive value when AOA = 0 degrees. When AOA = 2 degrees, the lift coefficient growth rate is the largest, which is 47.27%, and the lift-to-drag ratio is increased by 50.00%. At other angles of attack, the lift, drag, and torque coefficients of the multi-parameter deformed airfoil are optimized to some ***/value - Combined the body shape variation of the stingray in the propulsion process, the parametric study of the aerodynamic shape of the original design airfoil is carried out to explore the influence of a single parameter change on the aerodynamic performance of the airfoil.

关键词： Micro air vehicle Airfoil design Parameter optimization Deformed airfoil Aerodynamic performance

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Lattice Boltzmann simulation of wetting gradient accelerating droplets merging and shedding on a circumferential surface

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engineering APPLICATIONS OF COMPUTATIONAL FLUID MECHANICS 2022年第1期16卷 1796-1812页

作者： Chen, Lu Gao, Ming Liang, Jia Wang, Dongmin Hao, Liang Zhang, Lixin Univ Shanghai Sci & Technol Sch Power Engn Shanghai Key Lab Multiphase Flow & Heat Transfer Shanghai Peoples R China

A lattice Boltzmann method (LBM) based on Shan-Chen pseudo-potential model is used to investigate the process of droplets merging and shedding on a gradient wetting circular surface. The effects of wetting gradient, radius, and radius ratio on droplet merging and shedding were mainly explored. The results show that applying a wetting gradient on the circumferential surface can accelerate the process of droplet merging and shedding. The velocity of droplets merging and shedding increase with the increase of the wetting gradient. The more hydrophilic the original surface, the better the optimization effect of accelerating drainage is by applying a wetting gradient. The radius and radius ratio significantly affect droplets merging and shedding on the gradient wetting surface. The larger the radius and radius ratio, the shorter the droplets merging and shedding time.

关键词： Droplets lattice boltzmann method wetting gradient circumferential surface shedding

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Pore-Scale Simulation of Tortuosity in the Catalyst Layer of Proton Exchange Membrane Fuel Cells

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JOURNAL OF ENERGY engineering 2024年第4期150卷 04024015-04024015页

作者： He, Yusong Hao, Liang Bai, Minli Dalian Univ Technol Sch Energy & Power Engn Key Lab Ocean Energy Utilizat & Energy Conservat Minist Educ Dalian 116024 Liaoning Peoples R China Univ Shanghai Sci & Technol Sch Energy & Power Engn Shanghai Key Lab Multiphase Flow & Heat Transfer P Shanghai 200093 Peoples R China

The porous structures of the catalyst layer (CL) for proton exchange membrane (PEM) fuel cells were reconstructed using the sphere-based simulated annealing (SA) method, in which different carbon sphere diameters, carbon phase fractions, ionomer loadings, and porosities were achieved to simulate different samples. The pore-scale simulation model based on the random walk algorithm was developed to evaluate the tortuosity in the CL. The results show that the carbon phase fraction, particularly the carbon sphere diameter, significantly influences the tortuosities in both pores and ionomer. Larger carbon spheres contribute to tightening the solid phase and enlarging the pore size within the CL, thereby affecting the pore structure and the ionomer distribution. The tortuosity obtained from the random walk algorithm aligns well with those from pore-scale diffusion and flow simulations using the Lattice-Boltzmann method (LBM). The random walk algorithm has the highest efficiency of the three methods in calculating the tortuosity of the CL when the porosity is less than 0.2, demonstrating its wider applicability. This study further proposes formulas for predicting the tortuosities in both pores and ionomer, which are closer to actual CLs than empirical equations. In addition, the present work confirms that the structural randomness resulting from the reconstruction method used in this work has little effect on the tortuosity, indicating that a small number of reconstructed samples suffice for investigating transport processes in the CL. Overall, our research contributes to the prediction of the properties of real porous media in energy engineering. This manuscript reports on the reconstruction of the catalyst layer in proton exchange membrane fuel cells using the simulated annealing method under some appropriate assumptions. A pore-scale simulation using a random walk algorithm was performed to compute the tortuosity both in the pores and in the ionomer, which is compared w

关键词： Pore-scale simulation Proton exchange membrane (PEM) fuel cells Catalyst layer (CL) Tortuosity

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A New Structure of Cooling Wall Tube for Supercritical CO_(2)Coal-Fired power Plants

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Journal of Thermal Science 2023年第3期32卷 1239-1250页

作者： WANG Yanjuan GAO Shuo JIANG Qiongqiong LI Yi LIU Qibin XU Jinliang The Beijing Key Laboratory of Multiphase Flow and Heat Transfer North China Electric Power UniversityBeijing 102206China Institute of Engineering Thermophysics Chinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

In terms of developing supercritical CO_(2)(sCO_(2))coal-fired power plants,enhancing cooling wall performance is one of significant factors to improve system *** this paper,a new cooling wall tube structure is proposed to match the non-uniform heat flux(NUH)with the thermal resistance by changing the cooling wall tube eccentricity.A three-dimensional multi-physical coupling model of cooling wall is constructed to compare the novel structure to the conventional *** properties of fluid dynamics,thermal stress,coupled heat transfer and cooling wall deformation are *** contrast to the traditional structure,the maximum temperature and circumferential temperature difference(CTD)of the proposed structure can be reduced by 2%and 27.4%,*** essential working parameters related to the performances of the cooling wall tube are *** maximum temperature of the new structure is reduced by 8-13 K and the maximum thermal stress is reduced by about 10%-15%under all the simulated working conditions when the eccentricity changes from 0 to *** proposed structure can effectively reduce the maximum temperature and circumferential temperature gradient under ***,a novel insight is put out for the design and optimization of the cooling wall tube in coal-fired power plants.

关键词： supercritical carbon dioxide cooling wall tube thermal-hydraulic structural coupling supereritical heat transfer

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