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Efficient photocatalytic reduction of chromium(Ⅵ) using photoreduced graphene oxide as photocatalyst under visible light irradiation

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Journal of Materials Science & Technology 2021年第32期91卷 17-27页

作者： Mei Yu Jing Shang Yu Kuang Department of Environment and Health State Key Joint Laboratory of Environmental Simulation and Pollution ControlCollege of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China

Graphene oxide(GO),a new and promising material,has been widely used as a co-catalyst in photocatalytic reactions;however,its capacity as a sole photocatalyst has rarely been *** this study,ultraviolet(UV) light irradiation was used as a modification method to obtain reduced GO(rGO) *** samples were used as photocatalysts to examine their visible light photocatalytic activity toward hexavalent chromium(Cr(Ⅵ)) *** force microscopy(AFM),X-ray diffraction(XRD),UV-vis spectrophotometry,Raman spectroscopy,X-ray photoelectron spectroscopy(XPS),and electron spin resonance(ESR) spectroscopy were applied to interpret the surface and structure changes with UV *** oxygen-containing functional groups(OFGs) on the GO surface were reduced to defective carbons andπ-conjugated C=C(sp^(2) domains) under UV light;this led to a decrease in the interlayer distance between GO sheets,GO fragmentation,and increased disorder on the GO *** restoration of sp^(2) domains led to a narrower band gap of GO,which favored the rGO excitation by visible light to generate electron-hole *** rGO pre-irradiated with UV for 1 h(rGO-1),possessing the highest defect density and electron generation efficiency,exhibited the best Cr(Ⅵ) reduction efficiency,which was about three times that of the GO sample;moreover,it outperformed most of the reported GO-based *** addition,low pH and the addition of citric acid as a hole scavenger could further improve the photocatalytic *** study proves that GO or rGO can be used as a sole photocatalyst under visible light to remove environmental pollutants such as heavy-metal ions,and it paves the way for the development of this kind of material and its UV-irradiation modification for further applications.

关键词： Graphene oxide Chromium(Ⅵ) Defect density UV-irradiation modification Photocatalytic reduction

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Black titanium dioxide nanomaterials for photocatalytic removal of pollutants:A review

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Journal of Materials Science & Technology 2022年第17期112卷 239-262页

作者： Ying Liang Guohe Huang Xiaying Xin Yao Yao Yongping Li Jianan Yin Xiang Li Yuwei Wu Sichen Gao State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentBeijing Normal UniversityBeijing 100875China State Key Joint Laboratory of Environmental Simulation and Pollution Control China-Canada Center for EnergyEnvironment and Ecology ResearchUR-BNUSchool of EnvironmentBeijing Normal UniversityBeijing 100875China Department of Environmental Systems Engineering University of ReginaReginaSKS4S 0A2Canada State Key Laboratory of Marine Pollution(SKLMP) City University of Hong KongKowloonHong Kong SARChina Faculty of Engineering and Applied Science University of ReginaReginaSaskatchewanS4S 0A2Canada

Semiconductor photocatalysis is one of the most widely used environment-friendly technologies for removing various *** a well-developed photocatalyst,titanium dioxide(TiO_(2))still has limits in its wide bandgap and rapid recombination rate of photogenerated charge ***,black TiO_(2)appears as a strong candidate in the improvement of sunlight harvesting,because of its excellent absorption capacity and utilization of solar *** extensive applications in both environmental and energy fields,the use of black TiO_(2)as a photocatalyst in pollutant removal is *** primary objective of the review is to comprehensively evaluate the applications of black TiO_(2)in photocatalytic removal of contaminants,including conventional organic contaminants,emerging contaminants,microbes,and heavy *** basic properties,photocatalytic mechanism,and synthesis of black TiO_(2)have been summarized and ***,the stability and recoverability of black TiO_(2)have also been ***,the perspectives of the application of black TiO_(2)in pollutant removal have been further discussed.

关键词： Photocatalysis Back TiO_(2) Ti^(3+)self-doping Nanomaterials Pollutant removal

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The development of local ambient air quality standards: A case study of Hainan Province, China

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Eco-environment & Health 2024年第1期3卷 11-20页

作者： Qian Song Nannan Zhang Yanning Zhang Dejia Yin Jiming Hao Shuxiao Wang Shengyue Li Wenshuai Xu Weijun Yan Xinxin Meng Xinghong Xu Xiaochen Wu Donghai Xie Yun Zhu Qipeng Qu Xuan Hou Yueqi Jiang Zhaoxin Dong Haotian Zheng Yisheng Sun Zeqi Li Bin Zhao State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China Institute of Strategic Planning Chinese Academy of Environmental PlanningBeijing 100041China Hainan Research Academy of Environmental Sciences Haikou 571126China Hainan Provincial Ecological and Environmental Monitoring Center Haikou 570206China Hainan Radiation Environmental Monitoring Station Haikou 571126China Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution Control College of Environment and EnergySouth China University of TechnologyGuangzhou Higher Education Mega CenterGuangzhou 510006China

The ambient air quality standard(AAQS)is a vital policy instrument for protecting the environment and human *** Province is at the forefront of China's efforts to protect its ecological environment,with an official goal to achieve world-leading air quality by ***,neither the national AAQS nor the World Health Organization guideline offers sufficient guidance for improving air quality in Hainan because Hainan has well met the former while the latter is excessively ***,the establishment of Hainan's local AAQS becomes ***,research regarding the development of local AAQS is scarce,especially in comparatively more polluted countries such as *** relatively high background values and significant interannual fluctuations in air pollutant concentrations in Hainan present challenges in the development of local *** research proposes a world-class local AAQS of Hainan Province by reviewing the AAQS in major countries or regions worldwide,analyzing the influence of different statistical forms,and carefully evaluating the attainability of the *** the proposed AAQS,the annual mean concentration limit for PM2.5,the annual 95th percentile of daily maximum 8-h mean(MDA8)concentration limit for O_(3),and the peak season concentration limit for O_(3) are set at 10,120,and 85μg/m^(3),*** study indicates that,with effective control policies,Hainan is projected to achieve compliance with the new standard by *** implementation of the local AAQS is estimated to avoid 1,526(1,253–1,789)and 259(132–501)premature deaths attributable to longterm exposure to PM2.5 and O_(3) in Hainan in 2035,respectively.

关键词： Local ambient air quality standard Statistical form Feasibility Health effects Hainan province

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Ammonia removal from low-strength municipal wastewater by powdered resin combined with simultaneous recovery as struvite

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Frontiers of environmental Science & Engineering 2021年第1期15卷 125-134页

作者： Kuo Fang Fei Peng Hui Gong Huanzhen Zhang Kaijun Wang State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China School of Water Resources&Environment China University of GeosciencesBeijing 100083China

Low-strength municipal wastewater is considered to be a recoverable nutrient resource with economic and environmental ***,various technologies for nutrient removal and recovery have been *** this paper,powdered ion exchange resin was employed for ammonia removal and recovery from imitated low-strength municipal *** effects of various working conditions(powdered resin dosage,initial concentration,and pH value)were studied in batch experiments to investigate the feasibility of the approach and to achieve performance *** maximum adsorption capacity determined by the Langmuir model was 44.39 mg/g,which is comparable to traditional ion exchange ***,the effects of co-existing cations(Ca^(2+),Mg^(2+),K^(+))were *** on the above experiments,recovery of ammonia as struvite was successfully achieved by a proposed two-stage crystallization process coupled with a powdered resin ion exchange *** electron microscopy(SEM)and X-ray diffractometry(XRD)results revealed that struvite crystals were successfully gained in alkaline conditions(pH=10).This research demonstrates that a powdered resin and two-stage crystallization process provide an innovative and promising means for highly efficient and easy recovery from low-strength municipal wastewater.

关键词： Ammonia removal and recovery Powdered resin Crystallization process Struvite Co-existing cations

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Effect of CeO_(2) Nanoparticles on the Spread of Antibiotic Resistance in a Reclaimed Water-Soil-Radish System-shenzhen City,Guangdong Province,China,April 2023

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China CDC weekly 2023年第46期5卷 1029-1037,I0005-I0007页

作者： Kaiqiang Yu Bixi Zhao Yuxi Yan Qing Yang Liming Chen Yu Xia School of Environmental Science and Engineering College of EngineeringSouthern University of Science and TechnologyShenzhen CityGuangdong ProvinceChina School of Resource Environment and Life ScienceNingxia Normal UniversityGuyuan CityGansu ProvinceChina State Environmental Protection Key Laboratory of Integrated Surface Water-Groundwater Pollution Control School of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen CityGuangdong ProvinceChina Guangdong Provincial Key Laboratory of Soil and Groundwater Pollution Control School of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen CityGuangdong ProvinceChina

ABSTRACT Introduction:The use of reclaimed water(RW)for irrigation in agricultural practices raises concerns regarding the dissemination of antibiotic resistance genes(ARGs)from soils to edible *** effectiveness of na... 详细信息

关键词： Antibiotic Guangdong claimed

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Spatio-temporal characteristics of genotoxicity in the Yangtze River under the background of COVID-19 pandemic

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Frontiers of environmental Science & Engineering 2024年第11期18卷 121-132页

作者： Xinge Wang Na Li Yingnan Han Xiao Li Weixiao Qi Jian Li Kaifeng Rao Zijian Wang Yanjie Wei Mei Ma Key Laboratory of Drinking Water Science and Technology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China State Key Laboratory of Environmental Aquatic Chemistry Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Yangtze Eco-Environment Engineering Research Center China Three Gorges CorporationBeijing 100038China National Engineering Research Center of Industrial Wastewater Detoxication and Resource Recovery Beijing 100085China University of Chinese Academy of Sciences Beijing 100049China Center for Water and Ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China Engineering Research Center of Groundwater Pollution Control and Remediation Ministry of EducationCollege of Water SciencesBeijing Normal UniversityBeijing 100875China Key Laboratory of Environmental Protection in Water Transport Engineering Ministry of Communications Tianjin Research Institute of Water Transport EngineeringTianjin 300456China

The global spread of viruses can lead to the release of large amounts of disinfectants or antiviral drugs into the water *** resulting disinfection byproducts(DBPs)and residual antiviral drugs,acting as genotoxic substances or their precursors,may pose risks to aquatic animals and drinking water sources;however,to date,no studies have analyzed the changes in genotoxicity in the Yangtze River before and after the *** the present study,water and sediment samples from the Yangtze River were collected during different seasons,just before and after the outbreak of COVID-19,and were assessed using the SOS/umu test(with and without liver S9).The results indicated that water samples exhibited more pronounced genotoxicity than did sediments,with direct genotoxicity being the primary ***,there were significant regional differences,with notably greater genotoxicity observed in the upper Yangtze River than in the lower reaches before the COVID-19 ***,this trend was reversed six to ten months later,suggesting the accumulation of DBPs or antiviral drugs after the COVID-19 ***,the risk quotient indicated that 65%of the water samples posed a high risk for Paramecium caudatum,whereas 71%of the samples posed a medium risk for Danio rerio,thereby representing a potential threat to the ecological security of the Yangtze *** conclusion,this study,at the basin scale,revealed the impacts of COVID-19 on the Yangtze River,highlighting the need to prevent DBPs and pharmaceutical pollution during similar events in the future.

关键词： Yangtze River COVID-19 Genotoxicity Spatio-temporal characteristics

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Chemical characteristics,oxidative potential,and sources of PM_(2.5)in wintertime in Lahore and Peshawar,Pakistan

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Journal of environmental Sciences 2021年第4期33卷 148-158页

作者： Mushtaq Ahmad Qing Yu Jing Chen Siming Cheng Weihua Qin Yuepeng Zhang State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentBeijing Normal UniversityBeijing 100875China Department of Environmental Sciences University of PeshawarPeshawar 25120Pakistan

The chemical characteristics,oxidative potential,and sources of PM_(2.5)were analyzed at the urban sites of Lahore and Peshawar,Pakistan in February *** species,water soluble ions,and metal elements were measured to investigate the chemical composition and sources of PM_(2.5).The dithiothreitol(DTT)consumption rate was measured to evaluate the oxidative potential of PM_(2.5).Both cities showed a high exposure risk of PM_(2.5)regarding its oxidative potential(DTT v).Carbonaceous and some of the elemental species of PM_(2.5)correlated well with DTT v in both Lahore and ***,the DTT v of PM_(2.5)in Lahore showed significant positive correlation with most of the measured water soluble ions,however,ions were DTT-inactive in *** to the higher proportions of carbonaceous species and metal elements,Peshawar showed higher mass-normalized DTT activity of PM_(2.5)compared to Lahore although the average PM_(2.5)concentration in Peshawar was *** high concentrations of toxic metals also posed serious non-carcinogenic and carcinogenic risks to the residents of both *** component analysis coupled with multiple linear regression was applied to investigate different source contributions to PM_(2.5)and its oxidative *** sources of traffic and road dust resuspension and coal combustion,direct vehicle emission,and biomass burning and formation of secondary aerosol were identified as the major sources of PM_(2.5)in both *** findings of this study provide important data for evaluation of the potential health risks of PM_(2.5)and for formulation of efficient control strategies in major cities of Pakistan.

关键词： Air pollution DTT Health risk Oxidative potential Source apportionment

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Modeling of wintertime regional formation of secondary organic aerosols around Beijing: sensitivity analysis and anthropogenic contributions

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Carbon Research 2023年第1期2卷 1-19页

作者： Zhang, Yuepeng Huang, Huiying Qin, Weihua Yu, Qing Sun, Yuewei Cheng, Siming Ahmad, Mushtaq Ouyang, Wei Soyol-Erdene, Tseren-Ochir Chen, Jing State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Beijing Normal University Beijing100875 China Center of Atmospheric Environmental Studies Beijing Normal University Beijing100875 China Department of Environmental and Forest Engineering School of Engineering and Applied Sciences National University of Mongolia Ulaanbaatar14201 Mongolia

Modeling of secondary organic aerosol (SOA) has remained a big challenge due to the various precursors and complex processes involved. In this study, the WRF-CAMx model was used to predict the ambient SOA concentrations in urban Beijing as well as the North China Plain (NCP) during a polluted period in winter. To identify the major uncertainties and improve the model performance, a series of model tests were performed to assess the sensitivity of model prediction to the key factors. Then the sources of SOA in Beijing were identified using the optimized model. Both the volatility basis set (VBS) approach and the two-product approach were used for SOA simulation. Although the modeled SOA was underpredicted compared with the SOA estimated through filter-based measurements, the VBS scheme produced higher SOA than the traditional two-product scheme. According to the sensitivity tests with the VBS scheme, the emissions of volatile organic compounds (VOC) and intermediate volatility organic compounds (IVOC) as well as the oxidant levels were the key factors that affected SOA prediction. Based on the optimized simulation scenario, the potential contributions from different anthropogenic sources and source areas were identified, with over 80% of SOA in urban Beijing from regional transport of SOA or its precursors from the surrounding areas during the polluted period. Residential emission in the North China Plain appeared as the dominant source of SOA in urban Beijing from the perspective of regional contribution. Graphical Abstract: [Figure not available: see fulltext.] © 2023, The Author(s).

关键词： Sensitivity analysis

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Constructing extrinsic oxygen vacancy on the surface of photocatalyst as CO_(2)and electrons reservoirs to improve photocatalytic CO_(2)reduction activity

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Journal of environmental Sciences 2024年第6期140卷 37-45页

作者： Zaiyong Jiang Hao Li Zhimin Yuan Zheng Wang Maohong Fan Wenkang Miao Hong He State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China School of Chemistry&Chemical Engineering and Environmental Engineering Weifang UniversityWeifangShandong 261061China Departments of Chemical and Petroleum Engineering University of WyomingLaramieWY 82071USA Materials Genome Institute Shanghai UniversityShanghai 200444China

Constructing own oxygen vacancies in the photocatalysts is a very promising method to improve their photocatalytic CO_(2)reduction ***,some catalysts have excellent stabilities,making it difficult for them to construct their own oxygen *** simplify the above difficulty of stable photocatalysts,constructing extrinsic oxygen vacancies on their surface as a novel idea is ***,a stable TiO_(2)nanosheet is chosen as a research object,we uniformly deposited BiOCl quantum dots on their surface via a simple adsorption-deposition *** is found that BiOCl quantum dots are able to simultaneously self-transform into defective BiOCl with many oxygen vacancies when the photocatalyst is performed photocatalytic CO_(2)*** extrinsic oxygen vacancies can act as“CO_(2)and photo-generated electrons reservoirs”to improve CO_(2)capture and accelerate the separation of photogenerated electrons and *** the above reasons,the modified TiO_(2)showed obvious enhancement of photocatalytic CO_(2)reduction compared to pristine TiO_(2)and *** work may open a new avenue to broaden the use of oxygen vacancies in the process of photocatalytic CO_(2)reduction.

关键词： Oxygen vacancy BiOCl Photocatalyst CO_(2)reduction TiO_(2)

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Cost-Effective Mapping of Hyperlocal Air pollution Using Large-Scale Mobile Monitoring and Land-Use Machine Learning

ACS ES&T Air

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ACS ES&T Air 2025年第2期2卷 151-161页

作者： Tie Zheng Yifan Wen Sheng Xiang Pan Yang Xuan Zheng Yan You Shaojun Zhang Ye Wu School of Environment State Key Joint Laboratory of Environment Simulation and Pollution Control Tsinghua University Beijing 100084 China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Beijing Normal University Beijing 100875 China State Key Laboratory of Pollution Control and Resource Reuse Tongji University Shanghai 200092 China；College of Environmental Science and Engineering Tongji University Shanghai 200092 China College of Chemistry and Environmental Engineering Shenzhen University Shenzhen 518060 China Macao Environmental Research Institute Macau University of Science and Technology Macau 999078 China；National Observation and Research Station of Coastal Ecological Environments in Macao Macao Environmental Research Institute Macau University of Science and Technology Macao 999078 China School of Environment State Key Joint Laboratory of Environment Simulation and Pollution Control Tsinghua University Beijing 100084 China；State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084 China；Beijing Laboratory of Environmental Frontier Technologies Beijing 100084 China

The advent of large-scale mobile monitoring using fast-response instruments has enabled hyperlocal mapping (≤100 m) of traffic-related air pollution (TRAP), with important implications for air quality management. However, most related studies have been confined within small areas due to the high cost and labor intensity. This study pioneers a cost-effective TRAP mapping method by incorporating large-scale mobile monitoring and land-use machine learning (LUML). Here, over 4.6 million 1 Hz high-frequency measurements (∼1300 h) were collected on a part of major roadways in the Chinese megacity of shenzhen. Unmeasured locations were estimated by LUML models to reduce measurement costs and labor intensity. Various ML algorithms and varying spatial aggregation segment lengths were incorporated to optimize the model performance. Hyperlocal maps of NO, NO2, and PM2.5were predicted across the entire road network covering over 1700 km2. Based on our results, LU-RF (random forest) for mapping NO and NO2and LU-GBM (Gradient Boosting Machine) for mapping PM2.5, demonstrated superior performance. Deep learning models, in contrast, did not yield comparable results. Finer partitioning of road segments (≤100 m) improved NO prediction performance, but worsened that for NO2and PM2.5. By deployment of optimal ML algorithms and segment lengths, the TRAP mapping accuracy increased by 20–80% compared to conventional land-use regression models. This study provides a promising and cost-effective approach to hyperlocal air pollution mapping and management in cities worldwide.

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