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Single-atomic tungsten-doped Co_(3)O_(4) nanosheets for enhanced electrochemical kinetics in lithium–sulfur batteries

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Carbon Energy 2023年第8期5卷 31-41页

作者： Sangni Wang Riming Hu Ding Yuan Lei Zhang Chao Wu Tianyi Ma Wei Yan Rui Wang Liang Liu Xuchuan Jiang Hua Kun Liu Shi Xue Dou Yuhai Dou Jiantie Xu National Engineering Laboratory for VOCs Pollution Control Technology and Equipment Guangdong Provincial Key Laboratory of Atmospheric EnvironmentPollution Control School of Environment and EnergySouth China University of TechnologyGuangzhouChina Shandong Institute of Advanced Technology JinanChina School of Materials Science and Engineering Institute for Smart Materials&EngineeringUniversity of JinanJinanChina Institute of Energy Materials Science University of Shanghai for Science and TechnologyShanghaiChina Institute for Superconducting and Electronic Materials University of WollongongWollongongAustralia School of Science RMIT UniversityMelbourneVictoriaAustralia State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Materials Science and EngineeringDonghua UniversityShanghaiChina

The practical application of lithium–sulfur batteries(LSBs)is severely hindered by the undesirable shuttling of lithium polysulfides(LiPSs)and sluggish redox kinetics of sulfur ***,a series of ultrathin singleatomic tungsten-doped Co_(3)O_(4)(Wx-Co_(3)O_(4))nanosheets as catalytic additives in the sulfur cathode for LSBs are rationally designed and *** from the enhanced catalytic activity and optimized electronic structure by W doping,the Wx-Co_(3)O_(4) not only reduces the shuttling of LiPSs but also decreases the energy barrier of sulfur redox reactions of sulfur species,leading to accelerated electrode *** a result,LSB cathodes with the use of 5.0 wt%W0.02-Co_(3)O_(4) as the electrocatalyst show the high reversible capacities of 1217.0 and 558.6 mAh g^(-1) at 0.2 and 5.0 C,respectively,and maintain a high reversible capacity of 644.6 mAh g^(-1) at 1.0 C(1.0 C=1675 mA g^(-1))after 500 *** a high sulfur loading of 5.5 mg cm^(-2) and electrolyte–electrode ratio of 8μL_(electrolyte) mg_(sulfur)^(-1),the 5.0 wt%W_(0.02)-Co_(3)O_(4)-based sulfur cathode also retains a high reversible areal capacity of 3.86 mAh cm^(-2) at 0.1 C after 50 cycles with an initial capacity retention of 84.7%.

关键词： catalytic additives lithium-sulfur batteries single-atomic dopant sluggish redox kinetics

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Efficient photocatalytic NADH regeneration with Rh-loaded Z-scheme mediator-free system

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Chinese Chemical Letters 2024年第2期35卷 496-500页

作者： Yi Zhou Yiling He Ming Gao Ningkai Ding Juying Lei Yanbo Zhou State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process East China University of Science and TechnologyShanghai 200237China National Engineering Research Center of Industrial Wastewater Detoxication and Resource Recovery East China University of Science and TechnologyShanghai 200237China Shanghai Engineering Research Center for Multi-media Environmental Catalysis and Resource Utilization East China University of Science and TechnologyShanghai 200237China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China

Nicotinamide adenine dinucleotide(NADH)regeneration is necessary for the sustainable application of enzymatic *** Rh-based complex[Cp^(*)Rh(bpy)(H)]+has been widely used as an important mediator in NADH regeneration systems,but it is limited by complexity and high ***,a Z-scheme was constructed by loading Rh onto carbon nitride nanosheets/carbon nitride quantum dots(CN-CNQD).The resultant catalyst achieved a high yield of NADH in a mediator-free(M-free)system of 0.283 mmol L^(−1) g^(−1) min^(−1),which is 5.29 times that of pure *** enzyme introduction experiments confirmed that the enzyme active product 1,4-NADH could reach 34.21%selectivity in the M-free *** research revealed that the heterojunction between CNs and CNQDs improved the NADH regeneration activity in the traditional M-involved system,while Rh loading was proved to optimize the yield and selectivity of 1,4-NADH in M-free *** immobilized Rh shows more competitiveness than[Cp^(*)Rh(bpy)(H)]^(+).This study contributes to the construction of an M-free system for further application in greener,lower-cost enzymatic processes.

关键词： Photocatalysis NADH regeneration Mediator-free Carbon nitride Z-scheme

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Heterogeneous Image Knowledge Driven Visual Perception

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IEEE/CAA Journal of Automatica Sinica 2024年第1期11卷 255-257页

作者： Lan Yan Wenbo Zheng Fei-Yue Wang IEEE the College of Computer Science and Electronic Engineering Hunan UniversityChangsha 410082China the School of Computer Science and Artificial Intelligence Wuhan University of TechnologyWuhan 430070China the State Key Laboratory for Management and Control of Complex Systems Institute of AutomationChinese Academy of SciencesBeijing 100190China

Dear Editor,This letter is concerned with visual perception closely related to heterogeneous *** the huge challenge brought by different image modalities,we propose a visual perception framework based on heterogeneous image knowledge,i.e.,the domain knowledge associated with specific vision tasks,to better address the corresponding visual perception problems.

关键词： Visual visual knowledge

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Effect of CeO_(2) Nanoparticles on the Spread of Antibiotic Resistance in a Reclaimed Water-Soil-Radish System-Shenzhen City,Guangdong Province,China,April 2023

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China CDC weekly 2023年第46期5卷 1029-1037,I0005-I0007页

作者： Kaiqiang Yu Bixi Zhao Yuxi Yan Qing Yang Liming Chen Yu Xia School of Environmental Science and Engineering College of EngineeringSouthern University of Science and TechnologyShenzhen CityGuangdong ProvinceChina School of Resource Environment and Life ScienceNingxia Normal UniversityGuyuan CityGansu ProvinceChina State Environmental Protection Key Laboratory of Integrated Surface Water-Groundwater Pollution Control School of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen CityGuangdong ProvinceChina Guangdong Provincial Key Laboratory of Soil and Groundwater Pollution Control School of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen CityGuangdong ProvinceChina

ABSTRACT Introduction:The use of reclaimed water(RW)for irrigation in agricultural practices raises concerns regarding the dissemination of antibiotic resistance genes(ARGs)from soils to edible *** effectiveness of na... 详细信息

关键词： Antibiotic Guangdong claimed

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Reverse Time Migration of Ultra-Wideband Ground-Penetrating Radar Based on Multiple Time-Gating Algorithm

Reverse Time Migration of Ultra-Wideband Ground-Penetrating ...

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2024 International Applied Computational Electromagnetics Society Symposium, ACES-China 2024

作者： Wu, Junjie Li, Haixiao Zhou, Yuanguo Cao, Le Wang, Yan Xi'an University of Science and Technology College of Communication and Information Engineering Xi'an China Xi'an University of Science and Technology College of Electrical and Control Engineering Xi'an China Graduate School of Chinese Aeronautical Establishment Yangzhou China Aviation Key Laboratory of Science and Technology on Electromagnetic Environment Effects Shenyang China National Key Laboratory of Electromagnetic Information Control and Effects Shenyang China

ISBN: (纸本)9798350355581

To address the issue of clutter interference in ground-penetrating radar (GPR) imaging using a VNA (Vector Network Analyzer), this paper improves the traditional reverse time migration (RTM) technique for ultra-wideband GPR imaging. The improved method retains the effective signals in the detection wavefield as the valid imaging area and suppresses signals in non-valid areas. Due to variations in the distance between the transmitting and receiving antennas and the number of anomalies in the experiment, the traditional time window cross-correlation is not ideal for this scenario. The improved method automatically applies reasonable windowing to each data channel, avoiding the simultaneous enhancement of clutter interference and effective signals through direct stacking, and preventing the filtering out of effective signals. Experimental results demonstrate that this method, when applied to real measured data and compared with the traditional cross-correlation RTM method, shows advantages in more accurately locating anomalous areas and suppressing clutter interference. This validates that the Multiple Time-Gating Reverse Time Migration (MTG-RTM) method offers better localization and higher imaging accuracy in practical engineering applications. © 2024 IEEE.

关键词： Receiving antennas

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Deciphering decadal urban ozone trends from historical records since 1980

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National science Review 2024年第11期11卷 117-129页

作者： Haolin Wang Xiao Lu Paul I.Palmer Lin Zhang Keding Lu Ke Li Tatsuya Nagashima Ja-Ho Koo Hiroshi Tanimoto Haichao Wang Meng Gao Cheng He Kai Wu Shaojia Fan Yuanhang Zhang School of Atmospheric Sciences Sun Yat-sen University and Key Laboratory of Tropical Atmosphere-Ocean System Ministry of Education Guangdong Provincial Observation and Research Station for Climate Environment and Air Quality Change in the Pearl River Estuary Southern Marine Science and Engineering Guangdong Laboratory (Zhuhai) School of Geo Sciences University of Edinburgh National Centre for Earth Observation University of Edinburgh Laboratory for Climate and Ocean-Atmosphere Studies Department of Atmospheric and Oceanic SciencesSchool of PhysicsPeking University State Key Joint Laboratory of Environmental Simulation and Pollution Control The State Environmental Protection Key Laboratory of Atmospheric Ozone Pollution ControlCollege of Environmental Sciences and Engineering Peking University Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Collaborative Innovation Center of Atmospheric Environment and Equipment Technology School of Environmental Science and Engineering Nanjing University of Information Science &Technology National Institute for Environmental Studies Department of Atmospheric Sciences Yonsei University Department of Geography Hong Kong Baptist University Department of Civil and Environmental Engineering University of California

Ozone pollution is a major environmental threat to human health. Timely assessment of ozone trends is crucial for informing environmental policy. Here we show that for the most recent decade（2013–2022） in the northern hemisphere, warm-season（April–September） mean daily 8-h average maximum ozone increases much faster in urban regions with top ozone levels(mainly in the North China Plain, 1.2 ± 1.3 ppbv year-1) than in other, low-ozone regions(0.2 ± 0.9 ppbv year-1). These trends widen the ozone differences across urban regions, and increase extreme pollution levels and health threats from a global perspective. Comparison of historical trends in different urban regions reveals that ozone increases in China during 2013–2022 differ in magnitude and mechanisms to historical periods in other regions since *** reflects a unique chemical environment characterized by exceptionally high nitrogen oxides and aerosol concentrations, where reducing ozone precursor emissions leads to substantial ozone *** increase in China has slowed down in 2018–2022 compared to 2013–2017, driven by ongoing emission reductions, but with ozone-favorable weather conditions. Historical ozone evolution in Japan and South Korea indicates that ozone increases should be suppressed with continuous emission *** temperature and associated wildfires have also reversed ozone decreases in the USA and Europe,with anthropogenic ozone control slowing down in recent decades.

关键词： air quality surface ozone trends

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Habitual Daily Intake of Fried Foods Raises Transgenerational Inheritance Risk of Heart Failure Through NOTCH1-Triggered Apoptosis

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Research 2025年第1期2024卷 647-664页

作者： Anli Wang Xuzhi Wan Fanghuan Zhu Haoyin Liu Xiaoran Song Yingyu Huang Li Zhu Yang Ao Jia Zeng Binjie Wang Yuanzhao Wu Zhongshi Xu Jiye Wang Weixuan Yao Haoyu Li Pan Zhuang Jingjing Jiao Yu Zhang Department of Gastroenterology The First Affiliated HospitalZhejiang University School of MedicineZhejiang Key Laboratory for Agro-Food ProcessingCollege of Biosystems Engineering and Food ScienceZhejiang UniversityHangzhouZhejiangChina Department of Endocrinology The Second Affiliated HospitalDepartment of NutritionSchool of Public HealthZhejiang University School of MedicineHangzhouZhejiangChina Key Laboratory of Drug Prevention and Control Technology of Zhejiang Province Department of Criminal Science and TechnologyZhejiang Police CollegeHangzhouZhejiangChina

Consumption of fried foods is highly prevalent in the Western dietary *** diet has been unfavorably linked with high risk of developing cardiovascular *** failure(HF)as a cardiovascular disease subtype is a growing global pandemic with high morbidity and ***,the causal relationship between long-term fried food consumption and incident HF remains *** population-based study revealed that frequent fried food consumption is strongly associated with 15%higher risk of *** causal relationship may be ascribed to the dietary acrylamide exposure in fried *** cross-sectional study evidenced that acrylamide exposure is associated with an increased risk of ***,we discover and demonstrate that chronic acrylamide exposure may induce HF in zebrafish and ***,we reveal that acrylamide induces energy metabolism disturbance in heart due to the mitochondria dysfunction and metabolic ***,acrylamide exposure induces myocardial apoptosis via inhibiting NOTCH1-phosphatidylinositol 3-kinase/AKT *** addition,acrylamide exposure could affect heart development during early life stage,and the adverse effect of acrylamide exposure is a threat for next generation via epigenetic change evoked by DNA methyltransferase 1(DNMT1).In this study,we reveal the adverse effects and underlying mechanism of fried foods and acrylamide as a typical food processing contaminant on HF from population-based observations to experimental ***,these results both epidemiologically and mechanistically provide strong evidence to unravel the mechanism of acrylamide-triggered HF and highlight the significance of reducing fried food consumption for lower the risk of HF.

关键词： fried foods acrylamide western dietary pattern heart failure transgenerational inheritance notch triggered apoptosis

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Immoral post detection using a one-dimensional convolutional neural network-based LSTM network

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Multimedia Tools and Applications 2025年 1-20页

作者： Saqia, Bibi Khan, Khairullah Rahman, Atta Ur Khan, Aurangzeb Jain, Deepak Kumar Department of Computer Science University of Science and Technology Bannu28100 Pakistan Riphah Institute of Systems Engineering Riphah International University Islamabad46000 Pakistan Key Laboratory of Intelligent Control and Optimization for Industrial Equipment of Ministry of Education Dalian University of Technology Dalian116024 China Symbiosis Institute of Technology Symbiosis International University Pune India

In text mining and Natural Language Processing (NLP), extracting emotions from textual data is gaining rapid attraction. The proliferation of online content and the freedom of expression on social media platforms has compelled the advancement of more sophisticated methods for the automatic identification of unwanted content. The One-Dimensional Convolutional Neural Network (1D-CNN) performs best for feature extraction, while the Long Short-Term Memory Network (LSTM) is well-known for extracting sequential features and classification of textual data. This study proposes a novel solution by combining 1D-CNN with LSTM. Utilizing a context-aware model, this study aims to enhance the detection of immoral posts, including hate speech and other forms of immoral content on social media platforms. Various posts are extracted from social media, which are then processed using Glove word embedding models. It depicts the word representations in the text, which yields the form of a real-valued vector determining the words' meaning. The 1D convolution utilizes a filter window over the input time-series data to extract features. Relying on the acquired parameters of the filters, they act as feature extractors. This feature extraction technique allows the model to distinguish detailed patterns and nuances from the textual contents of posts. The sequential processing capabilities of the LSTM network enable an in-depth examination of the text, capturing temporal relationships and context, which is critical for successful content categorization. To validate the proposed model, we utilized a benchmark dataset, called the Twitter dataset. The proposed model achieved the highest accuracy of 95.37% and outperforms state-of-the-art works. © The Author(s), under exclusive licence to Springer science+Business Media, LLC, part of Springer Nature 2025.

关键词： Convolutional neural networks

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Design and Experimental Validation of a Worm-Like Tensegrity Robot for In-Pipe Locomotion

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Journal of Bionic engineering 2023年第2期20卷 515-529页

作者： Xiaolin Dai Yixiang Liu Wei Wang Rui Song Yibin Li Jie Zhao School of Control Science and Engineering Shandong UniversityJinan250061China Engineering Research Center of Intelligent Unmanned System of Ministry of Education Jinan250061China Shandong Research Institute of Industrial Technology Jinan250061China State Key Laboratory of Robotics and System Harbin Institute of TechnologyHarbin150080China

Traditional rigid-body in-pipe robots usually have complex and heavy structures with limited flexibility and *** soft in-pipe robots have great improvements in flexibility,they still have manufacturing difficulties due to their reliance on high-performance soft *** structure is a kind of self-stressed spatial structure consisting discrete rigid struts connected by a continuous net of tensional flexible strings,which combines the advantages of both rigid structures and soft *** applying tensegrity structures into robotics,this paper proposes a novel worm-like tensegrity robot for moving inside ***,a robot module capable of body deformation is designed based on the concept of tensegrity and its deformation performance is ***,the optimal parameters of the module are obtained based on the tensegrity *** deformation ability of the tensegrity module is tested ***,the worm-like tensegrity robot that can crawl inside pipes is developed by connecting three modules in *** performance and load capacity are tested on the prototype of the worm-like tensegrity robot by experiments of moving in horizontal pipe,vertical pipe,and elbow *** results demonstrate the effectiveness of the proposed design and suggest that the robot has high compliance,mobility,and adaptability although with simple structure and low cost.

关键词： Bio-inspired robot Soft robot application Tensegrity structure Pipe crawling

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A Production Plan and Error Feedback DBN-DNN based prediction method for LDG Generation in steel industry 41

A Production Plan and Error Feedback DBN-DNN based predictio...

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第41届中国控制会议

作者： Xu Han Feng Jin Jun Zhao Wei Wang Key Laboratory of Intelligent Control and Optimization for Industrial Equipment (Dalian University of Technology) Ministry of Education School of Control Science and Engineering Dalian University of Technology

ISBN: (数字)9789887581536

ISBN: (纸本)9781665482561

Linz Donawiz converter Gas(LDG) is a kind of important secondary energy source in iron and steel *** prediction of LDG generation may provide guidance for scheduling *** this paper,a two-stage method for predicting LDG generation is *** to the characteristics of LDG generation data,an improved k-means clustering integrating dynamic time warping is proposed to divide the time series data into typical characteristic ***,an error feedback deep belief network(EF-DBN-DNN) model is established to predict the starting time of LDG generation by considering the relationship between production plan and the actual performance,Actual data of LDG system in an iron and steel enterprise are employed to verify the effectiveness of the proposed method,and the results show that the prediction accuracy of the proposed one is suitable for practical application.

关键词： LDG generation production plan improved k-means clustering error feedback DBN-DNN

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