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An inversion model based on GEOS-Chem for estimating global and China's terrestrial carbon fluxes in 2019

Advances in Climate Change Research 2023年第1期14卷 49-61页

作者： Chong-Yuan WU Xiao-Ye ZHANG Li-Feng GUO Jun-Ting ZHONG De-Ying WANG Chang-Hong MIAO Xiang GAO Xi-Liang ZHANG Monitoring and Assessment Center for GHGs and Carbon&Key Laboratory of Atmospheric Chemistry of China Meteorological Administration Chinese Academy of Meteorological SciencesBeijing 100081China Zhejiang Institute of Meteorological Science Zhejiang Meteorological BureauHangzhou 310017China Laboratory of Climate Change Mitigation and Carbon Neutrality Henan UniversityZhengzhou 450001China State Key Laboratory of Clean Energy Utilization State Environmental Protection Center for Coal-Fired Air Pollution ControlZhejiang UniversityHangzhou 310027China Institute of Energy Environment and EconomyTsinghua UniversityBeijing 100084China

The 2019 Refinement to the 2006 IPCC Guidelines for National Greenhouse Gas Inventories added the method of assimilating atmospheric CO_(2) concentrations to invert carbon sources and sinks;however,many global carbon inversion models are not publicly *** addition,our regional assimilation inversion system,CCMVS-R(China Carbon monitoring,Verification and Supporting for Regional),needs a global carbon inversion model with higher assimilation efficiency to provide boundary ***,an inversion model based on the global atmospheric chemistry model GEOS-Chem and a more accurate and easier-to-implement ensemble square root Kalman filter(EnSRF)algorithm is constructed and used to infer global and China's carbon fluxes in *** CO_(2) concentrations from ObsPack sites and five additional CO_(2) observational sites from China's Greenhouse Gas Observation Network(CGHGNET)were used for data assimilation to improve the *** inverted annual global terrestrial and oceanic carbon uptake is 2.12 and 2.53 Pg C per year,respectively,accounting for 21.1%and 25.1%of global fossil fuel CO_(2) *** remaining 5.41 Pg C per year in the atmosphere is consistent with the global atmospheric CO_(2) growth rates of 5.44 Pg C per year reported by the National Oceanic and Atmospheric Administration(NOAA),showing that the inversion model can provide a reasonable estimate of global-scale natural carbon *** inverted terrestrial carbon sink of China is 0.37 Pg C per year,accounting for approximately 13%of China's fossil CO_(2) emissions.

关键词： CO_(2) Data assimilation EnSRF GEOS-Chem Terrestrial carbon fluxes

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New insights into the formation of ammonium nitrate from a physical and chemical level perspective

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Frontiers of environmental Science & Engineering 2023年第11期17卷 209-221页

作者： Yuting Wei Xiao Tian Junbo Huang Zaihua Wang Bo Huang Jinxing Liu Jie Gao Danni Liang Haofei Yu Yinchang Feng Guoliang Shi State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control Tianjin Key Laboratory of Urban Transport Emission ResearchCollege of Environmental Science and EngineeringNankai UniversityTianjin 300350China CMA-NKU Cooperative Laboratory for Atmospheric Environment-Health Research(CLAER) College of Environmental Science and EngineeringNankai UniversityTianjin 300350China Institute of Resources Utilization and Rare Earth Development Guangdong Academy of SciencesGuangzhou 510650China Guangzhou Hexin Instrument Co.Ltd. Guangzhou 510530China State Key Laboratory of Precision Measuring Technology and Instruments Tianjin Key Laboratory of Air pollutants Monitoring TechnologySchool of Precision Instrument and Opto-electronics EngineeringTianjin UniversityTianjin 300072China Gigantic Technology(Tianjin)Co.Ltd. Tianjin 300384China Department of Civil Environmental and Construction EngineeringUniversity of Central FloridaOrlandoFL32816USA

High levels of fine particulate matter(PM_(2.5))is linked to poor air quality and premature deaths,so haze pollution deserves the attention of the *** abundant inorganic components in PM_(2.5),ammonium nitrate(NH_(4)NO_(3))formation includes two processes,the diffusion process(molecule of ammonia and nitric acid move from gas phase to liquid phase)and the ionization process(subsequent dissociation to form ions).In this study,we discuss the impact of meteorological factors,emission sources,and gaseous precursors on NH4NO3 formation based on thermodynamic theory,and identify the dominant factors during clean periods and haze *** show that aerosol liquid water content has a more significant effect on ammonium nitrate formation regardless of the severity of *** dust source is dominant emission source in clean periods;while a combination of coal combustion and vehicle exhaust sources is more important in haze *** the control of ammonia emission is more effective in reducing the formation of ammonium *** findings of this work inform the design of effective strategies to control particulate matter pollution.

关键词： Ammonium nitrate formation Thermodynamic theory Aerosol liquid water content Source apportionment

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Crop antiviral defense:Past and future perspective

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Science China(Life Sciences) 2024年第12期67卷 2617-2634页

作者： Zhirui Yang Guangyao Li Yongliang Zhang Fangfang Li Tao Zhou Jian Ye Xianbing Wang Xiaoming Zhang Zongtao Sun Xiaorong Tao Ming Wu Jianguo Wu Yi Li The State Key Laboratory of Protein and Plant Gene Research School of Life SciencesPeking UniversityBeijing 100871China State Key Laboratory of Plant Environmental Resilience Frontiers Science Center for Molecular Design BreedingCollege of Biological SciencesChina Agricultural UniversityBeijing 100193China State Key Laboratory for Ecological Pest Control of Fujian and Taiwan Crops Vector‐borne Virus Research CenterCollege of Plant ProtectionFujian Agriculture and Forestry UniversityFuzhou 350002China State Key Laboratory for Biology of Plant Diseases and Insect Pests Institute of Plant ProtectionChinese Academy of Agricultural SciencesBeijing 100193China State Key Laboratory for Agro-Biotechnology and Department of Plant Pathology China Agricultural UniversityBeijing100193China State Key Laboratory of Plant Genomics Institute of MicrobiologyChinese Academy of SciencesBeijing100101China State Key Laboratory of Integrated Management of Pest Insects and Rodents Institute of ZoologyChinese Academy of SciencesCAS Center for Excellence in Biotic InteractionsUniversity of Chinese Academy of SciencesBeijing 100049China State Key Laboratory for Managing Biotic and Chemical Threats to the Quality and Safety of Agro-products Key Laboratory of Biotechnology in Plant Protection of MARA and Zhejiang ProvinceInstitute of Plant VirologyNingbo UniversityNingbo 315211China Department of Plant Pathology The Key Laboratory of Plant ImmunityNanjing Agricultural UniversityNanjing 210095China

Viral pathogens not only threaten the health and life of humans and animals but also cause enormous crop yield losses and contribute to global food *** defend against viral pathogens,plants have evolved an intricate immune system to perceive and cope with such *** most of the fundamental studies were carried out in model plants,more recent research in crops has provided new insights into the antiviral strategies employed by crop *** summarize recent advances in understanding the biological roles of cellular receptors,RNA silencing,RNA decay,hormone signaling,autophagy,and ubiquitination in manipulating crop host-mediated antiviral *** potential functions of circular RNAs,the rhizosphere microbiome,and the foliar microbiome of crops in plant-virus interactions will be fascinating research directions in the *** findings will be beneficial for the development of modern crop improvement strategies.

关键词： crops antiviral defense RNA silencing autophagy ubiquitin proteasome system

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Natural variations of maize ZmLecRK1 determine its interaction with ZmBAK1 and resistance patterns to multiple pathogens

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Molecular Plant 2024年第10期17卷 1606-1623页

作者： Zhenju Li Junbin Chen Chuang Liu Shengfeng He Mingyu Wang Lei Wang Vijai Bhadauria Shiwei Wang Wenyu Cheng Hui Liu Xiaohong Yang Mingliang Xu You-Liang Peng Wangsheng Zhu State Key Laboratory of Maize Bio-breeding/College of Plant Protection/Ministry of Agriculture and Rural Affairs Key Laboratory of Surveillance and Management for Plant Quarantine Pests China Agricultural UniversityBeijing 100193P.R.China Institute of Plant Protection and Microbiology Zhejiang Academy of Agricultural SciencesZhejiang 310021P.R.China Yazhouwan National Laboratory SanyaHainan 572024P.R.China Ministry of Agriculture and Rural Affairs Key Laboratory for Crop Pest Monitoring and Green Control College of Plant ProtectionChina Agricultural UniversityBeijing 100193P.R.China State Key Laboratory of Plant Environmental Resilience College of Agronomy and BiotechnologyNational Maize Improvement CenterCenter for Crop Functional Genomics and Molecular BreedingChina Agricultural UniversityBeijing 100193P.R.China

Maize(Zea mays)is one of the most important crops in the world,but its yield and quality are seriously affected by diverse *** broad-spectrum resistance genes is crucial for developing effective strategies to control the disease in *** a genome-wide study in maize,we identified a G-type lectin receptor kinase ZmLecRK1,as a new resistance protein against Pythium aphanidermatum,one of the causal pathogens of stalk rot in *** analysis showed that the specific ZmLecRK1 allele can confer resistance to multiple pathogens in *** cell death and disease resistance phenotype mediated by the resistant variant of ZmLecRK1 requires the co-receptor ZmBAK1.A naturally occurring A404S variant in the extracellular domain of ZmLecRK1 determines the ZmLecRK1-ZmBAK1 interaction and the formation of ZmLecRK1-related protein ***,the ZmLecRK1 susceptible variant was found to possess the amino acid S404 that is present in the ancestral variants of ZmLecRK1 and conserved among the majority of grass species,while the resistance variant of ZmLecRK1 with A404 is only present in a few maize inbred *** of S by A at position 404 in ZmLecRK1-like proteins of sorghum and rice greatly enhances their ability to induce cell *** transcriptomic analysis reveals that ZmLecRK1 likely regulates gene expression related to the pathways in cell wall organization or biogenesis in response to pathogen *** together,these results suggest that the ZmLecRK1 resistance variant enhances its binding affinity to the co-receptor ZmBAK1,thereby enhancing the formation of active complexes for defense in *** work highlights the biotechnological potential for generating disease-resistant crops by precisely modulating the activity of ZmLecRK1 and its homologs through targeted base editing.

关键词： natural variation G-type lectin receptor-like kinase co-receptor BAK1 broad-spectrum resistance genome-wide association study maize

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Enhanced secondary pollution offset reduction of primary emissions during COVID-19 lockdown in China

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National Science Review 2021年第2期8卷 51-59页

作者： Xin Huang Aijun Ding Jian Gao Bo Zheng Derong Zhou Ximeng Qi Rong Tang Jiaping Wang Chuanhua Ren Wei Nie Xuguang Chi Zheng Xu Liangduo Chen Yuanyuan Li Fei Che Nini Pang Haikun Wang Dan Tong Wei Qin Wei Cheng Weijing Liu Qingyan Fu Baoxian Liu Fahe Chai Steven J.Davis Qiang Zhang Kebin He School of Atmospheric Sciences Nanjing University Chinese Research Academy of Environmental Sciences Department of Earth System Science Tsinghua University State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua University Department of Earth System Science University of California Jiangsu Environmental Monitoring Center Jiangsu Provincial Academy of Environment Science Shanghai Environmental Monitoring Center Beijing Key Laboratory of Airborne Particulate Matter Monitoring Technology Beijing Municipal Environmental Monitoring Center

To control the spread of the 2019 novel coronavirus(COVID-19), China imposed nationwide restrictions on the movement of its population(lockdown) after the Chinese New Year of 2020, leading to large reductions in economic activities and associated emissions. Despite such large decreases in primary pollution, there were nonetheless several periods of heavy haze pollution in eastern China, raising questions about the well-established relationship between human activities and air quality. Here, using comprehensive measurements and modeling, we show that the haze during the COVID lockdown was driven by enhancements of secondary pollution. In particular, large decreases in NOx emissions from transportation increased ozone and nighttime NO3radical formation, and these increases in atmospheric oxidizing capacity in turn facilitated the formation of secondary particulate matter. Our results, afforded by the tragic natural experiment of the COVID-19 pandemic, indicate that haze mitigation depends upon a coordinated and balanced strategy for controlling multiple pollutants.

关键词： COVID-19 haze pollution ozone emission reduction secondary pollution

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Biochar technology cannot offset land carbon emissions in Guangdong province, China

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Carbon Research 2024年第1期3卷 1-14页

作者： Wang, Funing Zhou, Wenneng Wang, Xili Zhao, Qing Han, Mengjie State Key Lab of Clean Energy Utilization Institute of Carbon Neutrality State Environmental Protection Engineering Center for Coal-Fired Air Pollution Control Zhejiang University Hangzhou310027 China Jiaxing Research Institute Zhejiang University Jiaxing314000 China Guangdong Provincial Key Laboratory of Water Quality Improvement and Ecological Restoration for Watersheds School of Ecology Environment and Resources Guangdong University of Technology Guangzhou510006 China Economic & amp Information center Zhejiang310006 China Department of Earth System Science Ministry of Education Key Laboratory for Earth System Modeling Institute for Global Change Studies Tsinghua University Beijing100084 China Guangdong Key Laboratory of Integrated Agro-environmental Pollution Control and Management Institute of Eco-environmental and Soil Sciences Guangdong Academy of Sciences Guangzhou510650 China National-Regional Joint Engineering Research Center for Soil Pollution Control and Remediation in South China Guangzhou510650 China

As a highly developed region, Guangdong province has substantial industrial emissions. Its subtropical monsoon climate, characterized by abundant hydrothermal conditions, contributes to a substantial biomass potential. The adoption of potential biomass-based carbon dioxide removal (CDR) technologies, such as biochar, presents an opportunity to mitigate emissions and work towards carbon neutrality in the future. However, the current state of the land carbon balance and the CDR potential of biochar in Guangdong province remains unclear. We first calculated the land carbon balance based on inventory data. Then we estimated the CDR potential of biochar derived from agricultural residues, forestry residues, and bioenergy crops cultivated on marginal lands in Guangdong province using life cycle analysis (LCA). Results show that Guangdong province has not yet achieved carbon neutrality, with a net emission (carbon emissions remaining after offsetting by carbon sinks) of 925.63 Tg CO2e (CO2 equivalent, 1Tg = 106 t) in 2021. Emissions from energy consumption account for the highest proportion, contributing 83.8% of total emissions. In the highest biomass utilization scenario, the maximum CDR potential of biochar derived from all biomass types reaches 84.30 Tg CO2e yr-1, which could offset 9.11% of net carbon emissions in Guangdong province. Our findings provide crucial guidance for setting emission reduction targets and implementing effective mitigation strategies in Guangdong province under temperature warming. Graphical Abstract: (Figure presented.) © The Author(s) 2024.

关键词： Carbon capture and utilization

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Impact of anthropogenic heat emissions on meteorological parameters and air quality in Beijing using a high-resolution model simulation

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Frontiers of environmental Science & Engineering 2022年第4期16卷 47-57页

作者： Hengrui Tao Jia Xing Gaofeng Pan Jonathan Pleim Limei Ran Shuxiao Wang Xing Chang Guojing Li Fei Chen Junhua Li Aviation University of Air Force Changchun 130022China School of Environment and State Key Joint Laboratory of Environment Simulation and Pollution Control Tsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China Research Triangle Park Environmental Protection AgencyNC 27711USA East Remote Sensing Laboratory United States Department of AgricultureNC 20250USA Unit No.96941 of Chinese People's Liberation Army Beijing 100041China Unit No.31010 of Chinese People's Liberation Army Beijing 100081China

Anthropogenic heat emissions(AHE)play an important role in modulating the atmospheric thermodynamic and kinetic properties within the urban planetary boundary layer,particularly in densely populated megacities like *** this study,we estimate the AHE by using a Large-scale Urban Consumption of energY(LUCY)model and further couple LUCY with a high-resolution regional chemical transport model to evaluate the impact of AHE on atmospheric environment in *** areas with high AHE,the 2-m temperature(T_(2))increased to varying degrees and showed distinct diurnal and seasonal variations with maxima in night and *** increase in 10-m wind speed(WS_(10))and planetary boundary layer height(PBLH)exhibited slight diurnal variations but showed significant seasonal ***,the systematic continuous precipitation increased by 2.1 mm due to the increase in PBLH and water vapor in upper *** contrast,the precipitation in local thermal convective showers increased little because of the limited water ***,the PM_(2.5) reduced in areas with high AHE because of the increase in WS_(10) and PBLH and continued to reduce as the pollution levels *** contrast,in areas where prevailing wind direction was opposite to that of thermal circulation caused by AHE,the WS_(10) reduced,leading to increased PM_(2.5).The changes of PM_(2.5) illustrated that a reasonable AHE scheme might be an effective means to improve the performance of PM_(2.5) ***,high AHE aggravated the O_(3) pollution in urban areas due to the reduction in NO_(x).

关键词： Anthropogenic heat emissions LUCY High-resolution Meteorological parameters Air quality

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Plant virology in the 21st century in China:Recent advances and future directions

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Journal of Integrative Plant Biology 2024年第3期66卷 579-622页

作者： Jianguo Wu Yongliang Zhang Fangfang Li Xiaoming Zhang Jian Ye Taiyun Wei Zhenghe Li Xiaorong Tao Feng Cui Xianbing Wang Lili Zhang Fei Yan Shifang Li Yule Liu Dawei Li Xueping Zhou Yi Li State Key Laboratory for Ecological Pest Control of Fujian and Taiwan Crops Vector-borne Virus Research CenterCollege of Plant ProtectionFujian Agriculture and Forestry UniversityFuzhou 350002China State Key Laboratory of Plant Environmental Resilience and Ministry of Agriculture Key Laboratory of Soil Microbiology College of Biological SciencesChina Agricultural UniversityBeijing 100193China State Key Laboratory for Biology of Plant Diseases and Insect Pests Institute of Plant ProtectionChinese Academy of Agricultural SciencesBeijing 100193China State Key Laboratory of Integrated Management of Pest Insects and Rodents Institute of ZoologyChinese Academy of SciencesBeijing 100101China CAS Center for Excellence in Biotic Interactions University of Chinese Academy of SciencesBeijing 100049China State Key Laboratory of Plant Genomics Institute of MicrobiologyChinese Academy of SciencesBeijing 100101China State Key Laboratory of Rice Biology Institute of BiotechnologyZhejiang UniversityHangzhou 310058China Department of Plant Pathology The Key Laboratory of Plant ImmunityNanjing Agricultural UniversityNanjing 210095China State Key Laboratory for Managing Biotic and Chemical Threats to the Quality and Safety of Agro-products Institute of Plant VirologyNingbo UniversityNingbo 315211China MOE Key Laboratory of Bioinformatics Center for Plant BiologySchool of Life SciencesTsinghua UniversityBeijing 100084China State Key Laboratory of Protein and Plant Gene Research School of Life SciencesPeking UniversityBeijing 100871China

Plant viruses are a group of intracellular pathogens that persistently threaten global food *** advances in plant virology have been achieved by Chinese scientists over the last 20 years,including basic research and technologies for preventing and controlling plant viral ***,we review these milestones and advances,including the identification of new crop-infecting viruses,dissection of pathogenic mechanisms of multiple viruses,examination of multilayered interactions among viruses,their host plants,and virus-transmitting arthropod vectors,and in-depth interrogation of plantencoded resistance and susceptibility ***,various plant virus-based vectors have also been successfully developed for gene function studies and target gene expression in *** also recommend future plant virology studies in China.

关键词： China emerging plant viruses plant virology plant resistance/susceptibility to viral infection plant-virus transmission vector interactions plant virus-based vectors viral pathogenesis

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Volatile organic compounds in wintertime North China Plain:Insights from measurements of proton transfer reaction time-of-flight mass spectrometer(PTR-ToF-MS)

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Journal of environmental Sciences 2022年第4期34卷 98-114页

作者： Xianjun He Bin Yuan Caihong Wu Sihang Wang Chaomin Wang Yibo Huangfu Jipeng Qi Nan Ma Wanyun Xu Ming Wang Wentai Chen Hang Su Yafang Cheng Min Shao Institute for Environmental and Climate Research Jinan UniversityGuangzhou 511443China Guangdong-Hongkong-Macao Joint Laboratory of Collaborative Innovation for Environmental Quality Guangzhou 511443China State Key Laboratory of Severe Weather&Key Laboratory for Atmospheric Chemistry of China Meteorology Administration Chinese Academy of Meteorological SciencesBeijing 100081China Collaborative Innovation Center of Atmospheric Environment and Equipment Technology Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution ControlSchool of Environmental Science and EngineeringNanjing University of Information Science&TechnologyNanjing 210044China Nanjing Intelligent Environmental Science and Technology Co. Ltd.Nanjing 211800China Max Planck Institute for Chemistry Mainz 55128Germany

The characteristics of wintertime volatile organic compounds(VOCs)in the North China Plain(NCP)region are complicated and remain *** measurements were conducted by a proton transfer reaction time-of-flight mass spectrometer(PTR-ToF-MS)at a rural site in the NCP from November to December *** ions measured by PTRToF-MS were quantified and the overall VOC compositions were investigated by combining the measurements of PTR-ToF-MS and gas chromatography-mass spectrometer/flame ionization detector(GC-MS/FID).The measurement showed that although atmospheric VOCs concentrations are often dominated by primary emissions,the secondary formation of oxygenated VOCs(OVOCs)is non-negligible in the wintertime,i.e.,OVOCs accounts for 42%±7%in the total VOCs(151.3±75.6 ppbV).We demonstrated that PTR-MS measurements for isoprene are substantially overestimated due to the interferences of *** chemical changes of organic carbon in a pollution accumulation period were investigated,which suggests an essential role of fragmentation reactions for large,chemically reduced compounds during the heavy-polluted stage in wintertime *** changes of emission ratios of VOCs between winter 2011 and winter 2018 in the NCP support the positive effect of“coal to gas”strategies in curbing air *** high abundances of some key species(*** aromatics)indicate the strong emissions of coal combustion in wintertime of *** ratio of naphthalene to C8 aromatics was proposed as a potential indicator of the influence of coal combustion on VOCs.

关键词： North China Plain Volatile organic compound Wintertime PTR-ToF-MS

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laboratory and field evaluation of a low-cost optical particle sizer

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Journal of environmental Sciences 2024年第8期142卷 215-225页

作者： Mingzhen Tang Yicheng Shen Yanzhen Ge Jian Gao Chong Wang Liqing Wu Shuchun Si State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing 100012China Jinan Grid-Based Supervision Center of Ecological and Environmental Protection Jinan 250100China Tai’an Ecological Environment Protection Control Center Tai’an 271000China School of Physics Shandong UniversityJinan 250013China

Low-cost sensors are widely used to collect high-spatial-resolution particulate matter data that traditional reference monitoring devices *** addition to the mass concentration,the number concentration and size distribution are also fundamental in determining the origin and hazard level of particulate ***,low-cost optical sensors have been improved to establish optical particle sizers(OPSs).In this study,a low-cost OPS,the Nova SDS029,is introduced,and it is evaluated in comparison to two reference instruments—the GRIMM 11-D and the TSI *** first tested the sizing accuracy using polystyrene latex ***,we assessed the mass and number size distribution accuracy in three application scenarios:indoor smoking,ambient air quality,and mobile *** evaluations suggest that the low-cost SDS029 rivals research-grade optical sizers in many *** example,(1)the particle diameters obtained with the SDS029 are close to the reference instruments(usually<10%)in the 0.3-5μm range;(2)the number of particles and mass concentration are highly correlated(r≥0.99)with the values obtained with the reference instruments;and(3)the SDS029 slightly underestimates the number concentration,but the derived PM_(2.5)values are closer to monitoring station than the reference *** successful application of the SDS029 in multiple scenarios suggests that a plausible particle size distribution can be obtained in an easy and cost-efficient *** believe that low-cost OPSs will increasingly be used to map the sources and risk levels of particles at the city scale.

关键词： Optical particle sizer Particle size distribution Low-cost sensor Evaluation Field application

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