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Challenges and perspectives of air pollution control in China

Frontiers of environmental Science & Engineering 2024年第6期18卷 9-16页

作者： Bin Zhao Shuxiao Wang Jiming Hao State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China

Air pollution is one of the most challenging environmental issues in the *** has achieved remarkable success in improving air quality in last decade as a result of aggressive air pollution control ***,the average fine particulate matter(PM2.5)concentration in China is still about six times of the World Health Organization(WHO)Global Air Quality Guidelines(AQG)and causing significant human health *** emission reductions of multiple air pollutants are required for China to achieve the *** we identify the major challenges in future air quality improvement and propose corresponding control *** main challenges include the persistently high health risk attributed to PM2.5 pollution,the excessively loose air quality standards,and coordinated control of air pollution,greenhouse gases(GHGs)emissions and emerging *** further improve air quality and protect human health,a health-oriented air pollution control strategy shall be implemented by tightening the air quality standards as well as optimizing emission reduction pathways based on the health risks of various *** the meantime,an“oneatmosphere”concept shall be adopted to strengthen the synergistic control of air pollutants and GHGs and the control of non-combustion sources and emerging pollutants shall be enhanced.

关键词： Air pollution China Health impact Air quality standards GHGs Emerging pollutants

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Vehicular volatile organic compounds losses due to refueling and diurnal process in China: 2010–2050

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Journal of environmental Sciences 2015年第7期27卷 88-96页

作者： Xiaofan Yang Huan Liu Hongyang Cui Hanyang Man Mingliang Fu Jiming Hao Kebin He School of Environment State Key Joint Laboratory of Environment Simulation and Pollution Control Tsinghua University State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Collaborative Innovation Center for Regional Environmental Quality

Volatile organic compounds（VOCs） are crucial to control air pollution in major Chinese cities since VOCs are the dominant factor influencing ambient ozone level, and also an important precursor of secondary organic aerosols. Vehicular evaporative emissions have become a major and growing source of VOC emissions in China. This study consists of lab tests, technology evaluation, emissions modeling, policy projections and cost-benefit analysis to draw a roadmap for China for controlling vehicular evaporative emissions. The analysis suggests that evaporative VOC emissions from China＇s light-duty gasoline vehicles were approximately 185,000 ton in 2010 and would peak at 1,200,000 ton in 2040 without control. The current control strategy implemented in China, as shown in business as usual（BAU） scenario, will barely reduce the long-term growth in emissions. Even if Stage II gasoline station vapor control policies were extended national wide（BAU ＋ extended Stage II）, there would still be over 400,000 ton fuel loss in 2050. In contrast, the implementation of on-board refueling vapor recovery（ORVR） on new cars could reduce 97.5% of evaporative VOCs by 2050（BAU ＋ ORVR/BAU ＋ delayed ORVR）. According to the results, a combined Stage II and ORVR program is a comprehensive solution that provides both short-term and long-term benefits. The net cost to achieve the optimal total evaporative VOC control is approximately 62 billion CNY in 2025 and 149 billion CNY in 2050.

关键词： Evaporative VOC emissions China roadmap Vehicle Refueling emission control

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Self-powered decentralized water treatment clean boat with electrochemical fenton system for antibiotic remediation in natural water bodies

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Fundamental Research 2025年

作者： Zhongxin Chen Xiaosong Gu Xiang-Yang Lou Huiling Zhou Jiaxin Liang Yangzi Shangguan Hong Chen School of Environmental Science and Engineering Guangdong Provincial Key Laboratory of Soil and Groundwater Pollution Control State Environmental Protection Key Laboratory of Integrated Surface Water-Groundwater Pollution Control SUSTech Energy Institute for Carbon Neutrality Southern University of Science and Technology Shenzhen 518055 China

Decentralized solutions for the low-cost and sustainable treatment of large-scale natural water bodies contaminated with organic pollutants are urgently needed. This study introduces a self-powered clean boat using a photovoltaic (PV)-driven electrochemical Fenton system, featuring a gas diffusion electrode (GDE) and a quasi-solid hydrogel electrolyte. This setup enables in-situ oxygen reduction in low-conductivity lake water, achieving a high H 2 O 2 production rate of 290±10 mg L −1 ·h −1 . The hydrogel, containing Fe 2+ /Fe 3+ pairs, enriches ion concentration, enhances conductivity, and triggers the Fenton reaction to convert H 2 O 2 into •OH radicals for efficient antibiotic degradation. The boat achieved a 99.4% removal rate for tetracycline (TC) at 1 mg L −1 in contaminated water within 3 hours, demonstrating over 98% removal efficiency for other common antibiotics. This system integrates clean energy use, H 2 O 2 production, Fenton reaction activation, and pollutant degradation, addressing the limitations of conventional electrochemical methods in low-conductivity waters. It offers a sustainable solution for decentralized water treatment in pilot-scale experiments with low unique energy consumption (0.43 kWh mg-1) by solar energy.

关键词： Electro-Fenton quasi-solid-state electrolyte self-powered boat antibiotics removal low-conductivity water remediation gas diffusion electrode (GDE)

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Moving policy and regulation forward for single-use plastic alternatives

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Frontiers of environmental Science & Engineering 2021年第3期15卷 191-194页

作者： Wenbing Tan Dongyu Cui Beidou Xi State Key Laboratory of Environmental Criteria and Risk Assessment and State Environmental Protection Key Laboratory of Simulation and Control of Groundwater PollutionChinese Research Academy of Environmental SciencesBeijing 100012China School of Environment Tsinghua UniversityBeijing 100084China

Single-use plastics are often used once or cannot be reused for extended *** are widely consumed with the rapid development of social *** waste generated by single-use plastics threatens ecosystem health by entering the environment and ultimately restricts sustainable human *** innovation of sustainable and environmentally friendly single-use plastic alternative materials and the joint participation of governments,enterprises and the public are promising technologies and management approaches that can solve the problem of single-use plastics *** development of single-use plastic alternative products can be promoted fundamentally only by improving relevant legislation and standards,providing differentiated industrial policies,encouraging scientific and technological innovation and expanding public participation.

关键词： Single-use plastic alternatives Policy Regulation Sustainable development

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Economic analysis of atmospheric mercury emission control for coal-fired power plants in China

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Journal of environmental Sciences 2015年第7期27卷 125-134页

作者： Maria Pia Ancora Lei Zhang Shuxiao Wang Jeremy Schreifels Jiming Hao State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua University Collaborative Innovation Center for Regional Environmental Quality Tsinghua University State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex

Coal combustion and mercury pollution are closely linked, and this relationship is particularly relevant in China, the world＇s largest coal consumer. This paper begins with a summary of recent China-specific studies on mercury removal by air pollution control technologies and then provides an economic analysis of mercury abatement from these emission control technologies at coal-fired power plants in China. This includes a cost-effectiveness analysis at the enterprise and sector level in China using 2010 as a baseline and projecting out to 2020 and2030. Of the control technologies evaluated, the most cost-effective is a fabric filter installed upstream of the wet flue gas desulfurization system（FF ＋ WFGD）. Halogen injection（HI） is also a cost-effective mercury-specific control strategy, although it has not yet reached commercial maturity. The sector-level analysis shows that 193 tons of mercury was removed in 2010 in China＇s coal-fired power sector, with annualized mercury emission control costs of 2.7 billion Chinese Yuan. Under a projected 2030 Emission control（EC） scenario with stringent mercury limits compared to Business As Usual（BAU） scenario, the increase of selective catalytic reduction systems（SCR） and the use of HI could contribute to 39 tons of mercury removal at a cost of 3.8 billion CNY. The economic analysis presented in this paper offers insights on air pollution control technologies and practices for enhancing atmospheric mercury control that can aid decision-making in policy design and private-sector investments.

关键词： Atmospheric mercury Coal-fired power plants China Cost-effectiveness Activated carbon and halogen injection

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Molecular characterization of methanogenic microbial communities for degrading various types of polycyclic aromatic hydrocarbon

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Journal of environmental Sciences 2019年第12期31卷 97-106页

作者： Quanhui Ye Chengyue Liang Xunwen Chen Tingting Fang Yun Wang Hui Wang State Key Joint Laboratory on Enuironment Simulation and Pollution Control School o/EnuironmentTsinghua UniversityBeijing 100084China Guangdong Provincial Key Laboratory of Soil and Groundwater Pollution Control School of Environmental Science and EngineeringSouthern University of Science and Technology of ChinaShenzhen 518055China State Environmental Protection Key Laboratory of Integrated Surface Water-Groundwater Pollution Control School of Environmental Science and EngineeringSouthern University of Science and TechnologyShenzhen 518055China

Knowledge on methanogenic microbial communities associated with the degradation of polycyclic aromatic hydrocarbons(PAHs)is crucial to developing strategies for PAHs *** this study,the linkage between the type of PAHs and microbial community structure was fully investigated through 16 S rRNA gene sequencing on four PAH-degrading *** degradation products were also *** results indicated that naphthalene(Nap)/2-methylnaphthalene(2-Nap),phenanthrene(Phe)and anthracene(Ant)sculpted different microbial *** them,Nap and 2-Nap selected for similar degrading bacteria(i.e.,Alicycliphilus and Thauera)and methanogens(Methanomethylovorans and Methanobacterium).Nap and 2-Nap were probably activated via carboxylation,producing 2-naphthoic *** contrast,Phe and Ant shaped different bacterial and archaeal communities,with Arcobacter and Acinetobacter being Phe-degraders and Thiobacillus *** archaea Methanobacterium and Methanomethylovorans predominated Phe-degrading and Ant-degrading culture,*** findings can improve our understanding of natural PAHs attenuation and provide some guidance for PAHs bioremediation in methanogenic environment.

关键词： Polycyclic aromatic hydrocarbons Microbial community structure Degradation products Degrading bacteria Carboxylation

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Synergetic PM_(2.5) and O_(3) control strategy for the Yangtze River Delta,China

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Journal of environmental Sciences 2023年第1期123卷 281-291页

作者： Zhaoxin Dong Jia Xing Fenfen Zhang Shuxiao Wang Dian Ding Hongli Wang Cheng Huang Haotian Zheng Yueqi Jiang Jiming Hao State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China State Environmental Protection Key Laboratory of the Formation and Prevention of Urban Air Pollution Complex Shanghai Academy of Environmental SciencesShanghai 200233China

PM_(2.5)concentrations have dramatically reduced in key regions of China during the period 2013-2017,while O_(3)has *** there is an urgent demand to develop a synergetic regional PM_(2.5)and O_(3)control *** study develops an emission-to-concentration response surface model and proposes a synergetic pathway for PM_(2.5)and O_(3)control in the Yangtze River Delta(YRD)based on the framework of the Air Benefit and Cost and Attainment Assessment System(ABaCAS).Results suggest that the regional emissions of NOx,SO_(2),NH3,VOCs(volatile organic compounds)and primary PM_(2.5)should be reduced by 18%,23%,14%,17%and 33%compared with 2017 to achieve 25%and 5% decreases of PM_(2.5)and O_(3)in 2025,and that the emission reduction ratios will need to be 50%,26%,28%,28% and 55%to attain the National Ambient Air Quality *** effectively reduce the O_(3) pollution in the central and eastern YRD,VOCs controls need to be strengthened to reduce O_(3)by 5%,and then NOx reduction should be accelerated for air quality ***,control of primary PM_(2.5)emissions shall be prioritized to address the severe PM_(2.5)pollution in the northern *** most cities in the YRD,the VOCs emission reduction ratio should be higher than that for NOx in Spring and *** control should be increased in summer rather than winter when a strong VOC-limited regime ***,regarding the emission control of industrial processes,on-road vehicle and residential sources shall be prioritized and the joint control area should be enlarged to include Shandong,Jiangxi and Hubei Province for effective O_(3)control.

关键词： PM_(2.5) O_(3) Response surface model Synergistic control pathway Cost-benefit analysis

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Aerosol exposure assessment during reclaimed water utilization in China and risk evaluation in case of Legionella

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Frontiers of environmental Science & Engineering 2022年第7期16卷 173-183页

作者： Menghao Chen Liangliang Shi Gang Liu Xiaojin Wu Yun Lu State Key Joint Laboratory of Environmental Simulation and Pollution Control State Environment Protection Key Laboratory of Microorganism Application and Risk ControlSchool of EnvironmentTsinghua UniversityBeijing100084China

Reclaimed water utilization provides an effective way to alleviate water ***,the residual pathogens in the recycled water like Legionella,could be spread into the air as aerosols through water-to-air transmission *** the aerosols by the people nearby increases their susceptibility to *** estimating the health risks associated with the potential exposure of airborne Legionella emitted from the urban use of reclaimed water in China,nationwide questionnaire was designed to investigate the exposure habits of Chinese population in different *** microbial risk assessment(QMRA)served as the suitable explanatory tool to estimate the *** results indicated that annual infection probability of populations exposed to Legionella for three scenarios,0.0764(95%CI:0.0032−0.6880)for road cleaning,1.0000(95%CI:0.1883−1.0000)for greenfield irrigation,0.9981(95%CI:0.0784−1.0000)for landscape fountain,were markedly higher than the threshold recommended by WHO(10^(−4) per person per year(pppy))according to the concentration distribution of Legionella in the reclaimed *** age-,educational background-,region-and gender-specific data in annual infection probability also showed different tendencies for some *** study provides some detailed information on the health risks from the water reuse in China and will be useful to promote the safe application of reclaimed water in water-deficient areas.

关键词： Legionella QMRA Reclaimed water Aerosol Water reuse

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Mercury mass flow in iron and steel production process and its implications for mercury emission control

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Journal of environmental Sciences 2016年第5期28卷 293-301页

作者： Fengyang Wang Shuxiao Wang Lei Zhang Hai Yang Wei Gao Qingru Wu Jiming Hao State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua UniversityBeijing 100084 China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084 China

The iron and steel production process is one of the predominant anthropogenic sources of atmospheric mercury emissions worldwide. In this study, field tests were conducted to study mercury emission characteristics and mass flows at two iron and steel plants in China. It was found that low-sulfur flue gas from sintering machines could contribute up to41% of the total atmospheric mercury emissions, and desulfurization devices could remarkably help reduce the emissions. Coal gas burning accounted for 17%–49% of the total mercury emissions, and therefore the mercury control of coal gas burning, specifically for the power plant burning coal gas to generate electricity, was significantly important. The emissions from limestone and dolomite production and electric furnaces can contribute29.3% and 4.2% of the total mercury emissions from iron and steel production. More attention should be paid to mercury emissions from these two processes. Blast furnace dust accounted for 27%–36% of the total mercury output for the whole iron and steel production process. The recycling of blast furnace dust could greatly increase the atmospheric mercury emissions and should not be conducted. The mercury emission factors for the coke oven,sintering machine and blast furnace were 0.039–0.047 g Hg/ton steel, and for the electric furnace it was 0.021 g Hg/ton steel. The predominant emission species was oxidized mercury, accounting for 59%–73% of total mercury emissions to air.

关键词： Iron and steel plant Mercury Emission characteristics Mass flow Emission control

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An optimized two-step derivatization method for analyzing diethylene glycol ozonation products using gas chromatography and mass spectrometry

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Journal of environmental Sciences 2017年第3期29卷 313-321页

作者： Ran Yu Lei Duan Jingkun Jiang Jiming Hao State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China

The ozonation of hydroxyl compounds （e.g., sugars and alcohols） gives a broad range of products such as alcohols, aldehydes, ketones, and carboxylic adds. This study developed and optimized a two-step derivatization procedure for analyzing polar products of aldehydes and carboxylic acids from the ozonation of diethylene glycol （DEG） in a non-aqueous environment using gas chromatography-mass spectrometry. Experiments based on Central Composite Design with response surface methodology were carried out to evaluate the effects of derivatization variables and their interactions on the analysis. The most desirable derivati- zation conditions were reported, i.e., oximation was performed at room temperature overnight with the o-（2,3,4,5,6-pentafluorobenzyl） hydroxyl amine to analyte molar ratio of 6, silylation reaction temperature of 70℃, reaction duration of 70 min, and N,O-bis（trimethylsilyl）- trifluoroacetamide volume of 12.5 μL. The applicability of this optimized procedure was verified by analyzing DEG ozonation products in an ultrafine condensation particle counter simulation system.

关键词： Gas chromatography-massspectrometryResponse surface methodologyCentral Composite DesignDiethylene glycol ozonation

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