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Hydrogeochemical characteristics and potential risks within a headwater catchment， Taihu Lake Basin， China

Journal of Earth Science 2024年

作者： Lin Liu Hai Yang Xun Zhou Yuehua Jiang Naizheng Xu Jiangshi Gong Zi Chen Liang Li Jinsong Lv Yang Jin Chinese Academy of Geological Sciences Nanjing Center China Geological Survey Key Laboratory of Watershed Eco-Geological Processes， Ministry of Natural Resources State Environmental Protection Key Laboratory of Source Apportionment and Control of Aquatic Pollution， China University of Geosciences(Wuhan)

The Yuying River catchment is a hilly watershed that serves as a high-quality water source for Taihu Lake. Its hydrochemical characteristics is crucial to the safety of water supplies around Taihu Lake. In order to evaluate the potantial risk to Taihu Lake， samples of rainwater， surface water， and groundwater from the Yuying River catchment were gathered to conduct a comprehensive hydrochemical analysis， the isotope analysis of δ2H， δ18O， and3H. The results showed that the hydrochemical types of the groundwater were mainly HCO3·SO4-Na·Ca and HCO3-Na·Ca. The renewal rate of groundwater in the Yuying River catchment is slightly greater （+10% to +20%） than 34% a-1. The formation process of hydrochemical characteristics was controlled by the process of cation exchange and leaching （mainly based on silicate dissolution）. Combined with historical data， the concentration of NO3-in groundwater of the Yuying River catchment was increased from 2000（4.7 mg/L） to 2019（15.8 mg/L）. Both the constructed land area （increase 377.31%） and NO3-concentration in groundwater （increase 336.17%） elevated about 3 times compared with thoses in 2000. Combined with PCA statistical analysis of nitrate in groundwater of different land use， it was found that the discharge of domestic sewage was the main reason of the abnormal increase of NO3-in the study area. It suggested that the enhanced of human activities （unscientific domestic sewage disposal） has exceeded the self-purification ability of the Yuying river catchment water environment. It is urgent to adopt scientific and effective domestic sewage treatment methods to ensure the water environment and water ecological security of the Yuying river catchment and the downstream Taihu Lake.

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Systematic control technologies for gaseous pollutants from non-ferrous metallurgy

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Journal of environmental Sciences 2023年第1期123卷 65-82页

作者： Hui Liu Fenghua Shen Qingzhu Li Minneng Wen Hongliang Zhang Linhua Jiang Chenghang Zheng Yan Liu Tao Liu Liyuan Chai School of Metallurgy and Environment Central South UniversityChangsha 410083China Chinese National Engineering Research Center for Control&Treatment of Heavy Metal Pollution Changsha 410083China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China College of Environmental Science and Engineering Tongji UniversityShanghai 200092China State Key Lab of Clean Energy Utilization State Environmental Protection Engineering Center for Coal-Fired Air Pollution ControlZhejiang UniversityHangzhou 310027China Key Laboratory of Ecological Metallurgy of Multi-metal Intergrown Ores of Ministry of Education School of MetallurgyNortheastern UniversityShenyang 110819China School of Resource and Environmental Engineering Wuhan University of Science and TechnologyWuhan 430081China

air pollutant emissions represent a critical challenge in the green development of the non-ferrous metallurgy *** work studied the emission characteristics,formation mechanisms,phase transformation and separation of typical air pollutants,such as heavy metal particles,mercury,sulfur oxides and fluoride,during non-ferrous smelting.A series of purification technologies,including optimization of the furnace throat and hightemperature discharge,were developed to collaboratively control and recover fine particles from the flue gas of heavy metal smelting processes,including copper,lead and *** improvements have been realized in wet scrubbing technology for removing mercury,fluoride and SO_(2)from flue ***-liquid sulfidation technology by applying H_(2)S was invented to recycle the acid scrubbing wastewater more efficiently and in an eco-friendly *** on digital technology,a source reduction method was designed for sulfur and fluoride control during the whole aluminum electrolysis *** desulfurization technologies were developed for catalytic reduction of the sulfur content in petroleum coke at low temperature and catalytic reduction of SO_(2)to elemental *** work has established the technology for coupling multi-pollutant control and resource recovery from the flue gas from non-ferrous metallurgy,which provides the scientific theoretical basis and application technology for the treatment of air pollutants in the non-ferrous metallurgy industry.

关键词： Non-ferrous smelting Gaseous pollutant Flue gas purification Acid wastewater Heavy metal

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Observation-based sources evolution of non-methane hydrocarbons (NMHCs) in a megacity of China

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Journal of environmental Sciences 2023年第2期124卷 794-805页

作者： Yarong Peng Hongli Wang Qian Wang Shengao Jing Jingyu An Yaqin Gao Cheng Huang Rusha Yan Haixia Dai Tiantao Cheng Qiang Zhang Meng Li Jianlin Hu Zhihao Shi Li Li Shengrong Lou Shikang Tao Qinyao Hu Jun Lu Changhong Chen Department of Environmental Science and Engineering Shanghai Key Laboratory of Atmospheric Particle Pollution and PreventionInstitute of Atmospheric SciencesFudan UniversityShanghai 200438China State Environmental Protection Key Laboratory of Formation and Prevention of Urban Air Pollution Complex Shanghai Academy of Environmental SciencesShanghai 200233China Department of Atmospheric and Oceanic Sciences Institute of Atmospheric SciencesFudan UniversityShanghai 200438China Department of Earth System Science Ministry of Education Key Laboratory for Earth System ModelingTsinghua UniversityBeijing 100084China Big Data Institute for Carbon Emission and Environmental Pollution Fudan UniversityShanghai 200438China School of Environmental Science and Engineering Nanjing University of Information Science&TechnologyNanjing 210044China

Both concentrations and emissions of many air pollutants have been decreasing due to implement of control measures in China,in contrast to the fact that an increase in emissions of non-methane hydrocarbons(NMHCs)has been *** study employed seven years continuous NMHCsmeasurements and the related activities data of Shanghai,a megacity in China,to explore evolution of emissions and effectiveness of air pollution control *** mixing ratio of NMHCs showed no statistical interannual changes,of which their compositions exhibited marked *** resulted in a decreasing trend of ozone formation potential by 3.8%/year(p<0.05,the same below),which should be beneficial to ozone pollution mitigation as its production in Shanghai is in the NMHCs-limited *** alkanes,aromatics and acetylene changed by+3.7%/year,-5.9%/year and-7.4%/year,respectively,and alkenes showed no apparent *** sources were apportioned by a positive matrix factorization ***,vehicular emissions(-5.9%/year)and petrochemical industry emissions(-7.1%/year)decreased significantly,but the decrease slowed down;significant reduction in solvent usage(-9.0%/year)appeared after 2010;however,emissions of natural gas(+12.6%/year)and fuel evaporation(with an increasing fraction)became more *** inconsistency between observations and inventories was found in interannual trend and speciation as well as source contributions,emphasizing the need for further validation in NMHCs emission *** study confirms the effectiveness of measures targeting mobile and centralized emissions from industrial sources and reveals a need focusing on fugitive emissions,which provided new insights into future air policies in polluted region.

关键词： Characteristics source apportionment Observation-based Interannual trend Shanghai

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Forest Mercury Deposition Observation in Chongqing: Evaluating Effectiveness of Mercury pollution control over the Past Decade in Southwestern China

ACS ES&T Air

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ACS ES&T air 2025年第2期2卷 286-294页

作者： Ziyi Zhan Dongwei Lv Huang Zhou Qingru Wu Yuying Cui Lei Duan State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Tsinghua University 100084 Beijing China School of the Environment Nanjing University 210023 Nanjing China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Tsinghua University 100084 Beijing China；State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Tsinghua University 100084 Beijing China

As the largest Hg reservoir in terrestrial ecosystems, forests provide valuable insights into atmospheric Hg levels through observations of mercury deposition. In this study, we conducted a one-year observation of Hg deposition, by both throughfall and litterfall, in a forest located in Chongqing, an industrial hub in southwestern China, in 2021. We compared the results with observations made at the same sampling site in 2010–2011. The results showed that there were significant decreases in both Hg concentrations (from 115 μg·kg–1to 80.2 μg·kg–1for litterfall and from 68.4 ng·L–1to 4.01 ± 2.09 ng·L–1for throughfall) and Hg deposition fluxes (from 89.8 μg·m–2·yr–1to 19.9 μg·m–2·yr–1for total deposition, decreasing by 77.8%) in the forest from 2010 to 2021. The decrease in deposition might result from the synergistic effect of reduction in both anthropogenic (inventory-listed or nonquantitative) and re-emission sources. Over the decade since the initiation of theMinamata Convention on Mercury, atmospheric Hg levels have decreased significantly, mainly due to the co-benefits of conventional air pollutant control, indicating the effectiveness of China’s Hg pollution control policies.

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Impact of anthropogenic heat emissions on meteorological parameters and air quality in Beijing using a high-resolution model simulation

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Frontiers of environmental Science & Engineering 2022年第4期16卷 47-57页

作者： Hengrui Tao Jia Xing Gaofeng Pan Jonathan Pleim Limei Ran Shuxiao Wang Xing Chang Guojing Li Fei Chen Junhua Li Aviation University of Air Force Changchun 130022China School of Environment and State Key Joint Laboratory of Environment Simulation and Pollution Control Tsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China Research Triangle Park Environmental Protection AgencyNC 27711USA East Remote Sensing Laboratory United States Department of AgricultureNC 20250USA Unit No.96941 of Chinese People's Liberation Army Beijing 100041China Unit No.31010 of Chinese People's Liberation Army Beijing 100081China

Anthropogenic heat emissions(AHE)play an important role in modulating the atmospheric thermodynamic and kinetic properties within the urban planetary boundary layer,particularly in densely populated megacities like *** this study,we estimate the AHE by using a Large-scale Urban Consumption of energY(LUCY)model and further couple LUCY with a high-resolution regional chemical transport model to evaluate the impact of AHE on atmospheric environment in *** areas with high AHE,the 2-m temperature(T_(2))increased to varying degrees and showed distinct diurnal and seasonal variations with maxima in night and *** increase in 10-m wind speed(WS_(10))and planetary boundary layer height(PBLH)exhibited slight diurnal variations but showed significant seasonal ***,the systematic continuous precipitation increased by 2.1 mm due to the increase in PBLH and water vapor in upper *** contrast,the precipitation in local thermal convective showers increased little because of the limited water ***,the PM_(2.5) reduced in areas with high AHE because of the increase in WS_(10) and PBLH and continued to reduce as the pollution levels *** contrast,in areas where prevailing wind direction was opposite to that of thermal circulation caused by AHE,the WS_(10) reduced,leading to increased PM_(2.5).The changes of PM_(2.5) illustrated that a reasonable AHE scheme might be an effective means to improve the performance of PM_(2.5) ***,high AHE aggravated the O_(3) pollution in urban areas due to the reduction in NO_(x).

关键词： Anthropogenic heat emissions LUCY High-resolution Meteorological parameters air quality

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Understand the local and regional contributions on air pollution from the view of human health impacts

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Frontiers of environmental Science & Engineering 2021年第5期15卷 133-143页

作者： Yueqi Jiang Jia Xing Shuxiao Wang Xing Chang Shuchang Liu Aijun Shi Baoxian Liu Shovan Kumar Sahu State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing100084China Beijing Municipal Research Institute of Environment Protection Beijing100037China Beijing Key Laboratory of Airborne Particulate Matter Monitoring Technology Beijing Municipal Environmental Monitoring CenterBeijing100048China

The source-receptor matrix of PM_(2.5)concentration from local and regional sources in the Beijing-Tianjin-Hebei(BTH)and surrounding provinces has been created in previous ***,because the spatial distribution of concentration does not necessarily match with that of the population,such concentration-based source-receptor matrix may not fully reflect the importance of pollutant control effectiveness in reducing the PM_(2.5)-related health *** demonstrate that,we study the source-receptor matrix of the PM_(2.5)-related deaths instead,with inclusion of the spatial correlations between the concentrations and the *** advanced source apportionment numerical model combined with the integrated exposure-response functions is used for BTH and surrounding regions in *** observed that the relative contribution to PM_(2.5)-related deaths of local emissions was 0.75%to 20.77%larger than that of PM_(2.5)*** results address the importance of local emissions control for reducing health impacts of PM_(2.5)particularly for local *** of regional transport to PM_(2.5)-related deaths in rural area was 22%larger than that in urban area due to the spatial pattern of regional transport which was more related to the rural *** resulted in an environmental inequality in the sense that people staying in rural area with access to less educational resources are subjected to higher impacts from regional transport as compared with their more resourceful and knowledgeable urban *** unexpected benefit from the multi-regional joint controls is suggested for its effectiveness in reducing the regional transport of PM_(2.5)pollution thus mitigating the associated environmental inequality.

关键词： PM_(2.5) Regional transport Local emissions Health impact environmental inequality

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Trends and drivers of anthropogenic NOx emissions in China since 2020

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environmental Science and Ecotechnology 2024年第5期21卷 287-293页

作者： Hui Li Bo Zheng Yu Lei Didier Hauglustaine Cuihong Chen Xin Lin Yi Zhang Qiang Zhang Kebin He Shenzhen Key Laboratory of Ecological Remediation and Carbon Sequestration Institute of Environment and EcologyTsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China State Environmental Protection Key Laboratory of Environmental Planning and Policy Simulation and Center of Air Quality Simulation and System Analysis Chinese Academy of Environmental PlanningBeijing 100041China Laboratoire des Sciences du Climat et de l’Environnement LSCE/IPSLCEA-CNRS-UVSQUniversite Paris-SaclayGif-sur-YvetteFrance Center for Satellite Application on Ecology and Environment Ministry of Ecology and Environment of ChinaBeijing 100094China Institute of Future Human Habitats Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China Ministry of Education Key Laboratory for Earth System Modeling Department of Earth System ScienceTsinghua UniversityBeijing 100084China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China

Nitrogen oxides(NOx),significant contributors to air pollution and climate change,form aerosols and ozone in the ***,timely,and transparent information on NOx emissions is essential for decision-making to mitigate both haze and ozone ***,a comprehensive understanding of the trends and drivers behind anthropogenic NOx emissions from Chinadthe world's largest emitterdhas been lacking since 2020 due to delays in emissions *** we show a consistent decline in China's NOx emissions from 2020 to 2022,despite increased fossil fuel consumption,utilizing satellite observations as constraints for NOx emission estimates through atmospheric *** reduction is corroborated by data from two independent spaceborne instruments:the TROPOspheric Monitoring Instrument(TROPOMI)and the Ozone Monitoring Instrument(OMI).Notably,a reduction in transport emissions,largely due to the COVID-19 lockdowns,slightly decreased China's NOx emissions in *** subsequent years,2021 and 2022,reductions in NOx emissions were driven by the industry and transport sectors,influenced by stringent air pollution *** satellite-based inversion system developed in this study represents a significant advancement in the real-time monitoring of regional air pollution emissions from space.

关键词： China's NOx emissions pollution control Socio-economic drivers Atmospheric inversion

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On the optimality of Kalman filter for fault detection 4

On the optimality of Kalman filter for fault detection

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4th IEEE International Conference on Digital Twins and Parallel Intelligence, DTPI 2024

作者： Zhou, Jinming Zhu, Yucai Yang, Chao Zhu, Yun Yin, Feng Zhejiang University State Key Laboratory of Industrial Control Technology College of Control Science and Engineering Hangzhou310027 China Zhejiang University State Key Lab of Clean Energy Utilization State Environmental Protection Center for Coal-Fired Air Pollution Control Hangzhou310027 China Zhejiang Baima Lake Laboratory Co. Ltd Hangzhou310051 China

ISBN: (纸本)9798350349252

Kalman filter is widely used for residual generation in fault detection. It leads to optimality in fault detection using some performance indices and also leads to statistically sound residual evaluation and threshold setting. This paper shows that these nice features do not necessarily imply an optimal fault detection performance. Based on a performance index related to fault detection rate and false alarm rate, several occasions where Kalman filter should not be used are pointed out;further the residual evaluation and threshold setting are discussed, in which it is pointed out that in stochastic setting an optimal statistical test of Kamlan filter is not related to optimality of commonly used detection performance indicators. The theoretical analysis is verified through Monte Carlo simulations and Tennessee Eastman process (TEP) dataset. © 2024 IEEE.

关键词： Kalman filters

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Size distribution and chemical characteristics of particles from crop residue open burning in North China

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Journal of environmental Sciences 2021年第11期33卷 66-76页

作者： Tingkun Li Qili Dai Xiaohui Bi Jianhui Wu Yufen Zhang Yinchang Feng State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control College of Environmental Science and EngineeringNankai UniversityTianjin300350China.

Crop residue open burning is an important emission source of ambient particles in *** study analyzed the particle emission characteristics of crop residue open burning through combustion experiments with a novel open combustion simulation device using three typical crop straws in north China(corn,wheat,and rice).Particle samples size ranging from 0.006–9.890μm were collected by an Electrical Low Pressure Impactor plus,a high size-resolution instrument capable of dividing particles into 14 size *** size distributions of organic carbon(OC),elemental carbon(EC),water-soluble ions,and elements were analyzed,and source chemical profiles were constructed for PM0.1,PM1,PM2.5,and *** number concentration of particles was concentrated in the Aiken nuclei mode(0.006–0.054μm),accounting for 75%of the total number,whereas the mass concentration was concentrated in the accumulation mode(0.054–0.949μm),accounting for 85.43%of the mass ***,EC,Cl−,and K(include total K and water-soluble K)were the major chemical components of the particles,whose mass percentage distributions differed from those of other *** fivemain components exhibited a bell-shaped size distribution in the 0.006–9.890μm range,whereas the other components exhibited a U-shaped *** the chemical profiles for PM0.1–PM10,OC was the most important component at 10–30%,followed by EC at 2%–8%.The proportions of K^(+),Cl^(−),and K varied substantially in different experimental groups,ranging from 0–15%,and K+and Cl−were significantly correlated(r=0.878,α=0.000).

关键词： Crop residue Open burning Size distribution source profile Electrical Low Pressure Impactor plus(ELPI+)

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Arsenic Removal from Groundwater Using Iron Pyrite:Influence Factors and Removal Mechanism

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Journal of Earth Science 2023年第3期34卷 857-867页

作者： Muhammad Yousuf Jat Baloch Chunli Su Shakeel Ahmed Talpur Javed Iqbal Kulvinder Bajwa School of Environmental Studies China University of GeosciencesWuhan 430078China State Environmental Protection Key Laboratory of Source Apportionment and Control of Aquatic Pollution Ministry of Ecology and EnvironmentWuhan 430078China College of New Energy and Environment Jilin UniversityChangchun 130021China University School for Graduates Studies Chaudhary Devi Lal University125055 Sirsa HaryanaIndia

Iron pyrite has been reported as a kind of potential material for arsenic(As)removal from the groundwater because it exhibits a strong attraction in groundwater for both arsenite and arsenate *** this study,batch adsorption experiments were carried out to determine the optimum conditions for As adsorption by the iron pyrite adsorbent,including the initial concentration,adsorbent dosage ratio,pH,temperature and stirring *** characterization methods were employed to identify the mechanism of As *** removal efficiency for As(Ⅲ)was observed 93%at pH=7,and for As(Ⅴ)was 95%observed at pH=*** model resulted in the maximum adsorption capacity(q_(m))for As(Ⅲ)and As(Ⅴ)were 571.7 and 671.1μg/g,respectively,as well as the experiments were found to be favorable as separation factor R_(L)<*** value of“n”2.68 and 2.47 for As(Ⅲ)and As(Ⅴ)obtained by Freundlich model(n>1)indicates favorable *** pseudo-first and second-order kinetic models also fitted *** addition of oxalate on the adsorbent surface plays an important role for the recycling of Fe(Ⅱ)/Fe(Ⅲ)to minimize the arsenic *** surface area,ion exchange mechanism and structure of adsorbent confirmed that addition of oxalate could enhance the surface area of adsorbent.

关键词： arsenic groundwater pyrite adsorption oxalate hydrochemistry

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