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Green manufacturing for achieving carbon neutrality goal requires innovative technologies:A bibliometric analysis from 1991 to 2022

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Journal of environmental Sciences 2024年第6期140卷 255-269页

作者： Sheng Zhang Xintian Wang Jiayu Xu Qinqin Chen Meng Peng Jiming Hao School of Environment Tsinghua UniversityBeijing 100084China School of Environment&Natural Resources Renmin University of ChinaBeijing 100872China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China

Recent years have seen a significant increase in interest in green manufacturing as a key driver of global carbon-neutral efforts and sustainable *** find the research hotspots of green manufacturing and reveal future research trends,this study reviewed and analyzed research articles from the Web of Science database on green manufacturing from1991 to 2022 using a bibliometric *** findings indicate a significant rise in the number of articles related to green manufacturing since the ***,there has been an increase in the involvement of scholars from developing countries such as China and India in this *** on the literature review and bibliometric cluster analysis on green manufacturing,we believed that future research may continue following the lines of intelligent technology integration,adoption of frontier engineering techniques,and industry development in line with carbon reduction targets.A framework for future green manufacturing development is proposed,with a focus on Chinese *** framework could provide policy implications for developing countries looking to pursue opportunities for development in green manufacturing.

关键词： Green manufacturing Carbon neutrality Sustainable development Innovative technologies China

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Do vehicular emissions dominate the source of C6–C8 aromatics in the megacity Shanghai of eastern China?

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Journal of environmental Sciences 2015年第1期27卷 290-297页

作者： Hongli Wang Qian Wang Jianmin Chen Changhong Chen Cheng Huang Liping Qiao Shengrong Lou Jun Lu Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3) Department of Environmental Science and EngineeringFudan University State Environmental Protection Key Laboratory of Formation and Prevention of Urban Air Pollution Complex Shanghai Academy of Environmental Sciences

The characteristic ratios of volatile organic compounds（VOCs） to i-pentane, the indicator of vehicular emissions, were employed to apportion the vehicular and non-vehicular contributions to reactive species in urban Shanghai. Two kinds of tunnel experiments, one tunnel with more than 90% light duty gasoline vehicles and the other with more than 60% light duty diesel vehicles, were carried out to study the characteristic ratios of vehicle-related emissions from December 2009 to January 2010. Based on the experiments, the characteristic ratios of C6–C8aromatics to i-pentane of vehicular emissions were 0.53 ± 0.08（benzene）, 0.70 ± 0.12（toluene）,0.41 ± 0.09（m,p-xylenes）, 0.16 ± 0.04（o-xylene）, 0.023 ± 0.011（styrene）, and 0.15 ± 0.02（ethylbenzene）, respectively. The source apportionment results showed that around 23.3% of C6–C8 aromatics in urban Shanghai were from vehicular emissions, which meant that the non-vehicular emissions had more importance. These findings suggested that emission control of non-vehicular sources, i.e. industrial emissions, should also receive attention in addition to the control of vehicle-related emissions in Shanghai. The chemical removal of VOCs during the transport from emissions to the receptor site had a large impact on the apportionment results. Generally, the overestimation of vehicular contributions would occur when the VOC reaction rate constant with OH radicals（k OH） was larger than that of the vehicular indicator, while for species with smaller k OH than the vehicular indicator, the vehicular contribution would be underestimated by the method of characteristic ratios.

关键词： Aromatics Characteristic ratio Vehicular emissions Non-vehicular emissions Shanghai

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Effects of acid deposition control in China:a review based on responses of subtropical forests

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Frontiers of environmental Science & Engineering 2024年第6期18卷 115-126页

作者： Danni Xie Xiaodong Ge Lei Duan Jan Mulder School of Land Engineering Chang’an UniversityXi’an 710064China State Key Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China Faculty of Environmental Sciences and Natural Resource Management Norwegian University of Life SciencesBox 5003NO-1432ÅsNorway

For many decades,acid deposition used to pose a significant regional air pollution challenge in *** substantial emission control of anthropogenically derived sulfur and nitrogen containing gasses,both sulfur and nitrogen deposition,as well as the acid rain-affected area,have significantly decreased compared to their peak ***,particularly in the humid subtropics,are sensitive to acid deposition,as evidenced by soil acidification,sulfate and nitrate leaching in stream water,and elevated soil nitrous oxide *** in the total deposition of sulfur and nitrogen,caused a significant decline in sulfate and nitrate leaching from subtropical forest and subsequently in sulfate and nitrate concentrations in stream water,although there was about a 5-year *** delay may be attributed to the desorption of accumulated sulfate and continued elevated mineralization of accumulated nitrogen *** of nitrous oxide,a potent greenhouse gas,also declined in nitrogen-saturated subtropical forest soils,as soil water nitrate concentration ***,subtropical forests in China suffering from elevated acid deposition have begun to ***,the current levels of sulfur and nitrogen deposition continue to exceed the critical loads,i.e.,the assigned threshold levels in accordance with emission control policies,in more than 10%of the country’s land area,respectively,indicating remaining risks of acidification and ***,further emission reductions are urgently needed,also because they will help achieving goals related to air quality and nitrous oxide emissions.

关键词： Acidification Critical load Nitrous oxide Surface water chemistry Recovery

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A review and evaluation of nonroad diesel mobile machinery emission control in China

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Journal of environmental Sciences 2023年第1期123卷 30-40页

作者： Pengju Bie Liang Ji Huanxing Cui Gang Li Shunli Liu Ying Yuan Kebin He Huan Liu State Key Joint Laboratory of ESPC State Environmental Protection Key Laboratory of Sources and Control of Air Pollution ComplexSchool of EnvironmentInternational Joint Laboratory on Low Carbon Clean Energy InnovationTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Vehicle Emission Control and Simulation Chinese Research Academy of Environmental SciencesBeijing 100012China Jinan Automobile Testing Center Co Ltd.Jinan 250102China

China’s emission control for nonroad diesel mobile machinery(NDMM)must deal with a fast increase in stock as well as regulations that are two decades behind those for on-road *** study provides the first large-scale review and evaluation of China’s NDMM policies,along with emission measurements and an investigation on diesel fuel *** sulfur contents of the investigated diesel declined from 430 ppm(median value)in 2011 to6-8 ppm during the 2017-2018 *** emission control of NO_(x)and PM greatly improved with the shift from the China II to China IV standards,as demonstrated by engine tests and field NO_(x)***,the NO_(x)emission factors for non-type-approved engines were approximately twice the limits of the China II *** compliance based on bench tests was not sufficient to control actual emissions because the field-measured NO_(x)emission factors of all machinery ranged from 24%to 225%greater than the respective emission limits for the *** circumstances adversely affected the effectiveness of the regulations and policies for China’s emission control of ***,the policies on new and in-use NDMM,as well as diesel fuel quality,prevented NO_(x)and PM emissions amounting to 4.4 Tg and 297.8 Gg during the period 2008-2017,*** emission management strategy contributed to enhancing the international competitiveness of China’s NDMM industries by promoting advanced *** effective NDMM emission control in the future,portable testing and noncontact remote supervision should be strengthened;also,the issue of noncompliant diesel should be addressed through rigorous control measures and financial penalties.

关键词： Nonroad mobile machinery Emission reduction Emission control policy Emission factor Diesel fuel quality

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Real-world fuel consumption of light-duty passenger vehicles using on-board diagnostic (OBD) systems

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Frontiers of environmental Science & Engineering 2020年第2期14卷 207-216页

作者： Xuan Zheng Sheng Lu Liuhanzi Yang Min Yan Guangyi Xu Xiaomeng Wu Lixin Fu Ye Wu College of Chemistry and Environmental Engineering Shenzhen UniversityShenzhen 518060China School of Environment State Key Joint Laboratory of Environment Simulation and Pollution ControlTsinghua UniversityBeijing 100084China International Council on Clean Transportation Beijing 100084China Shenzhen Research Academy of Environmental Sciences Shenzhen 518001China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China

An increasing discrepancy between real-world and type-approval fuel consumption for light-duty passenger vehicles(LDPVs)has been reported by several ***,real-world fuel consumption is measured primarily by a portable emission measurement *** on-board diagnostic(OBD)approach,which is flexible and offers high-resolution data collection,is a promising fuel consumption monitoring *** LDPVs were tested with a laboratory dynamometer based on a type-approval cycle,the New European Driving Cycle(NEDC).Fuel consumption was measured by the OBD and constant-volume sampling system(CVS,a regulatory method)to verify the accuracy of the OBD *** results of the OBD method and the regulatory carbon balance method exhibited a strong linear correlation(e.g.,R^2=0.906-0.977).Compared with the carbon balance results,the fuel consumption results using the OBD were 7.1%±4.3%lower on ***,the real-world fuel consumption of six LDPVs was tested in Beijing using the *** results showed that the normalized NEDC real-world fliel consumption of the tested vehicles was 13%±17%higher than the type-approval-based fuel *** the OBD values are lower than the actual fuel consumption,using a carbon balance method may result in a larger discrepancy between real-word and type-approval ftiel *** means of the operating mode binning and micro trip methods,a strong relationship(R^2=0.984)was established between the average speed and relative fuel *** congested roads(average vehicle speed less than 25 km/h),the fuel consumption of LDPVs is highly sensitive to changes in average speed.

关键词： Fuel consumption Light-duty passenger vehicles On-board diagnostic systems

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Design and demonstration of a next-generation air quality attainment assessment system for PM_(2.5)and O_3

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Journal of environmental Sciences 2015年第3期27卷 178-188页

作者： Hua Wang Yun Zhu Carey Jang Che-Jen Lin Shuxiao Wang Joshua S.Fu Jian Gao Shuang Deng Junping Xie Dian Ding Xuezhen Qiu Shicheng Long Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution Control College of Environmental and Energy South China University of Technology Guangzhou Higher Education Mega Center State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex School of Environment Tsinghua University USEPA/Office of Air Quality Planning & Standards Department of Civil Engineering Lamar University Department of Civil & Environmental Engineering University of Tennessee Chinese Research Academy of Environmental Sciences

Due to the increasingly stringent standards, it is important to assess whether the proposed emission reduction will result in ambient concentrations that meet the standards. The Software for Model Attainment Test-Community Edition （SMAT-CE） is developed for demonstrating attainment of air quality standards of O3 and PM2.5. SMAT-CE improves computational efficiency and provides a number of advanced visualization and analytical functionalities on an integrated GIS platform. SMAT-CE incorporates historical measurements of air quality parameters and simulated air pollutant concentrations under a number of emission inventory scenarios to project the level of compliance to air quality standards in a targeted future year. An application case study of the software based on the U.S. National Ambient air Quality Standards （NAAQS） shows that SMAT-CE is capable of demonstrating the air quality attainment of annual PM2.5 and 8-hour O3 for a proposed emission control policy.

关键词： air quality standards Attainment test air pollution GIS Emission control

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Variation characteristics of fine particulate matter and its components in diesel vehicle emission plumes

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Journal of environmental Sciences 2021年第9期33卷 138-149页

作者： Xianbao Shen Jiateng Hao Lei Kong Yue Shi Xinyue Cao Jiacheng Shi Zhiliang Yao Xin Li Bobo Wu Yiming Xu Kebin He State Environmental Protection Key Laboratory of Food Chain Pollution Control Beijing Technology and Business UniversityBeijing 100048China Key Laboratory of Cleaner Production and Integrated Resource Utilization of China National Light Industry Beijing Technology and Business UniversityBeijing 100048China School of Ecology and Environment Beijing Technology and Business UniversityBeijing 100048China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China

A rapid reaction occurs near the exhaust nozzle when vehicle emissions contact the *** diesel vehicles were studied using a new multipoint sampling system that is suitable for studying the exhaust plume near the exhaust *** variation characteristics of fine particle matter(PM_(2.5)) and its components in diesel vehicle exhaust plumes were *** PM_(2.5) emissions gradually increased with increasing distance from the nozzle in the *** carbon emissions remained basically unchanged, organic carbon and total carbon(TC) increased with increasing *** concentrations of SO_(4)^(2-),NO_(3)^(-) and NH_(4)^(+) (SNA) directly emitted by the vehicles were very low but increased rapidly in the exhaust *** selective catalytic reduction(SCR) reduced 42.7% TC, 40% NO_(3)^(-) emissions, but increased 104% SO_(4)^(2-) and 36% NH_(4)^(+) emissions, *** summary,the SCR reduced 29% primary PM_(2.5) emissions for the tested diesel *** NH_(4)NO_(3) particle formation maybe more important in the plume, and there maybe other forms of formation of NH_(4)^(+) (***4Cl).The generation of secondary organic carbon(SOC) plays a leading role in the generation of secondary PM_(2.5).The SCR enhanced the formation of SOC and SNA in the plume, but comprehensive analysis shows that the SCR more enhanced the SNA formation in the plume, which is mainly new particles formation *** inconsistency between secondary organic aerosol(SOA) and primary organic aerosol definitions is one of the important reasons for the difference between SOA simulation and observation.

关键词： Variation characteristics Diesel vehicle Emission plume PM2.5 Components

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Variability of fuel consumption and CO_(2) emissions of a gasoline passenger car under multiple in-laboratory and on-road testing conditions

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Journal of environmental Sciences 2023年第3期125卷 266-276页

作者： Boya Zhou Liqiang He Shijian Zhang Rui Wang Luowei Zhang Mengliang Li Yu Liu Shaojun Zhang Ye Wu Jiming Hao China Automotive Technology and Research Center Co. Ltd.Tianjin 300300China School of Environment State Key Joint Laboratory of Environment Simulation and Pollution ControlTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China Beijing Laboratory of Environmental Frontier Technologies School of EnvironmentTsinghua UniversityBeijing 100084China

An increasing divergence regarding fuel consumption(and/or CO_(2)emissions) between realworld and type-approval values for light-duty gasoline vehicles(LDGVs) has posed severe challenges to mitigating greenhouse gases(GHGs) and achieving carbon emissions peak and neutrality. To address this divergence issue, laboratory test cycles with more real-featured and transient traffic patterns have been developed recently, for example, the China Lightduty Vehicle Test Cycle for Passenger cars(CLTC-P). We collected fuel consumption and CO_(2)emissions data of a LDGV under various conditions based on laboratory chassis dynamometer and on-road tests. laboratory results showed that both standard test cycles and setting methods of road load affected fuel consumption slightly, with variations of less than 4%. Compared to the type-approval value, laboratory and on-road fuel consumption of the tested LDGV over the CLTC-P increased by 9% and 34% under the reference condition(i.e., air conditioning off, automatic stop and start(STT) on and two passengers). On-road measurement results indicated that fuel consumption under the low-speed phase of the CLTC-P increased by 12% due to the STT off, although only a 4% increase on average over the entire cycle. More fuel consumption increases(52%) were attributed to air conditioning usage and full passenger capacity. Strong correlations(R2> 0.9) between relative fuel consumption and average speed were also identified. Under traffic congestion(average speed below 25 km/hr), fuel consumption was highly sensitive to changes in vehicle speed. Thus,we suggest that real-world driving conditions cannot be ignored when evaluating the fuel economy and GHGs reduction of LDGVs.

关键词： Fuel consumption CO_(2)emissions Light-duty gasoline vehicle(LDGV) Real driving

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air pollution characteristics and their relationship with emissions and meteorology in the Yangtze River Delta region during 2014–2016

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Journal of environmental Sciences 2019年第9期31卷 8-20页

作者： Tao Ma Fengkui Duan Kebin He Yu Qin Dan Tong Guannan Geng Xuyan Liu Hui Li Shuo Yang Siqi Ye Beiyao Xu Qiang Zhang Yongliang Ma State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing Key Laboratory of Indoor Air Quality Evaluation and Control Tsinghua University Beijing 100084 China Ministry of Education Key Laboratory for Earth System Modeling Department of Earth System Science Tsinghua University Beijing 100084 China National Satellite Meteorological Center Beijing 100081 China College of Resources and Environmental Sciences China Agricultural University Beijing 100094 China

With rapid economic growth and urbanization, the Yangtze River Delta(YRD) region in China has experienced serious air pollution challenges. In this study, we analyzed the air pollution characteristics and their relationship with emissions and meteorology in the YRD region during 2014–2016. In recent years, the concentrations of all air pollutants, except O3,decreased. Spatially, the PM2.5, PM10, SO2, and CO concentrations were higher in the northern YRD region, and NO2 and O3 were higher in the central YRD region. Based on the number of non-attainment days(i.e., days with air quality index greater than 100), PM2.5 was the largest contributor to air pollution in the YRD region, followed by O3, PM10, and ***, particulate matter pollution has declined gradually, while O3 pollution *** conditions mainly influenced day-to-day variations in pollutant concentrations. PM2.5 concentration was inversely related to wind speed, while O3 concentration was positively correlated with temperature and negatively correlated with relative *** air quality improvement in recent years was mainly attributed to emission *** 2014–2016, PM2.5, PM10, SO2, NOx, CO, NH3, and volatile organic compound(VOC)emissions in the YRD region were reduced by 26.3%, 29.2%, 32.4%, 8.1%, 15.9%, 4.5%, and0.3%, respectively. Regional transport also contributed to the air pollution. During regional haze periods, pollutants from North China and East China aggravated the pollution in the YRD region. Our findings suggest that emission reduction and regional joint prevention and control helped to improve the air quality in the YRD region.

关键词： air pollution Spatiotemporal variation Meteorological condition Emission inventory Regional transport Yangtze River Delta

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Constructing multi-active sites of LDH-derived MnCoFe layered mixed oxide catalysts for simultaneous removal of NO and toluene

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Applied Catalysis B: Environment and Energy 2025年 377卷

作者： Xinhua He Boxiong Shen Jiaqi Gao Yaqin Ji Meihong Wu Fumei Wang Tianjin Key Laboratory of Clean Energy and Pollution Control School of Energy and Environmental Engineering Hebei University of Technology Tianjin 300401 China The State Environmental Protection Key Laboratory of Urban Air Particulate Matter Pollution Prevention and Control College of Environmental Science and Engineering Nankai University Tianjin 300350 China

Nitrogen oxides (NOx) and toluene are air pollutants emitted from fossil fuel combustion and industrial processes. Simultaneous removal of NOx and toluene using the NH 3 -selective catalytic reduction (SCR) unit has proved to be a promising technology. Composite metal oxides have been widely studied for the simultaneous catalytic abatement of NOx and toluene. However, the catalytic applications of this process and the synergetic effect of multi-metal centers on their reactivity are unclear. In this study, mixed metal oxide catalysts with a two-dimensional layered structure, composed of Mn-Co-Fe-layered double oxide (LDO), were prepared by the co-precipitation method for the simultaneous removal of NO and toluene. The MnCoFe-LDO catalyst demonstrated the best synergistic catalytic performance, with 91 % NO conversion and 93 % toluene conversion, along with over 90 % selectivity for both N 2 and CO 2 at 200 ℃. The synergistic interaction between Mn, Co and Fe facilitated electron transfer during the redox process and increased reactive oxygen species and acid sites, resulting in the effective simultaneous removal of toluene and NO. The transformation of Mn 3+ + Co 3+ to Mn 4+ + Co 2+ promoted NO reduction, while the transformation of Mn 3+ + Fe 3+ to Mn 4+ + Fe 2+ promoted toluene oxidation. Density of states (DOS) analysis further demonstrated that the efficient assembly of Mn, Co and Fe elements improved the electron conduction efficiency and facilitated rapid electron transfer. The mechanism revealed mutual inhibition between the SCR reaction and toluene oxidation due to both toluene and NH 3 being more readily adsorbed on Co sites, engaging in competitive adsorption with approximate adsorption energies. The interaction of NH 3 , NO 2 , and nitrate with benzaldehyde and benzoic acid formed inactive by-products, such as nitrile and amide, which hindered the deep oxidation of toluene, reduction of NO, and conversion of benzyl alcohol to benzaldehyde as the rate-limit

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