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A mini-microbial fuel cell for voltage testing of exoelectrogenic bacteria

Frontiers of environmental Science & Engineering 2009年第3期3卷 307-312页

作者： Xiaoxin CAO Xia HUANG Xiaoyuan ZHANG Peng LIANG Mingzhi FAN State Key Joint Laboratory of Environment Simulation and Pollution Control Department of Environmental Science and EngineeringTsinghua UniversityBeijing 100084China

Current methods for testing the electricity generation capacity of isolates are time-and *** paper presents a rapid voltage testing system of exoelectrogenic bacteria called Quickscreen,which is based on a microliter microbial fuel cell(MFC).Geobacter sulfurreducens and Shewanella baltica were used as the model exoelectrogenic bacteria;Escherichia coli that cannot generate electricity was used as a negative *** was found that the electricity generation capacity of the isolates could be determined within about five hours by using Quickscreen,and that its time was relatively rapid compared with the time needed by using larger MFCs.A parallel,stable,and low background voltage was achieved using titanium as a current collector in the blank *** external resistance had little impact on the blank run during the initial *** cathode with a five-hole configuration,used to hydrate the carbon cathode,gave higher cathode potential than that with a one-hole *** discharge and current interrupt methods showed that the anode mostly contributed to the large internal resistance of the Quickscreen ***,the addition of graphite felt decreased the resistance from 18 to 5 kΩ.This device was proved to be useful to rapidly evaluate the electricity generation capacity of different bacteria.

关键词： microbial fuel cell exoelectrogenic bacteria rapid screening

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Intake of tobacco nitrosamines of smokers in various provinces of China and their cancer risk:A meta-analysis

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Journal of environmental Sciences 2024年第7期141卷 249-260页

作者： Xiao Li Zhiwei Ye Jun Wang Pengfei Lin Xiaojin Zhang Shuguang Xie Chao Chen Research Institute for Environmental Innovation(Suzhou) TsinghuaSuzhouJiangsu 215163China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China Shenzhen Key Laboratory of Organic Pollution Prevention and Control State Key Laboratory of Urban Water Resource and EnvironmentHarbin Institute of TechnologyShenzhen 518055China State Key Joint Laboratory of Environmental Simulation and Pollution Control College of Environmental Science and EngineeringPeking UniversityBeijing 100871China

Nitrosamines are a class of carcinogens which have been detected widely in food,water,some pharmaceuticals as well as *** objectives of this paper include reviewing the basic information on tobacco consumption and nitrosamine contents,and assessing the health risks of tobacco nitrosamines exposure to Chinese *** searched the publications in English from“Web of Science”and those in Chinese from the“China National Knowledge Infrastructure”in 2022 and collected 151 literatures with valid *** content of main nitrosamines in tobacco,including 4-(methylnitrosoamino)-1-(3-pyridyl)-1-butanone(NNK),N-nitrosonornicotine(NNN),N-nitrosoanatabine(NAT),N-nitrosoanabasine(NAB),total tobacco-specific nitrosamines(TSNA),and N-nitrosodimethylamine(NDMA)were *** information of daily tobacco consumption of smokers in 30 provinces of China was also ***,the intakes of NNN,NNK,NAT,NAB,TSNAs,and NDMA via tobacco smoke were estimated as 1534ng/day,591 ng/day,685 ng/day,81 ng/day,2543 ng/day,and 484 ng/day by adult smokers in30 provinces,*** cancer risk(CR)values for NNN and NNK inhalation intake were further calculated as 1.44×10^(-5)and 1.95×10^(-4).The CR value for NDMA intake via tobacco smoke(inhalation:1.66×10^(-4))indicates that NDMA is similarly dangerous in tobacco smoke when compared with the *** China,the CR values caused by average nitrosamines intake via various exposures and their order can be estimated as the following:smoke(3.75×10^(-4))>food(1.74×10^(-4))>drinking water(1.38×10^(-5)).Smokers in China averagely suffer 200%of extra cancer risk caused by nitrosamines in tobacco when compared with non-smokers.

关键词： N-nitrosamine Tobacco Cancer risk Tobacco specific nitrosamines(TSNAs) N-nitrosodimethylamine(NDMA)

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Efect of dissolved organic matter on sorption and desorption of phenanthrene onto black carbon

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Journal of environmental Sciences 2013年第12期25卷 2378-2383页

作者： Jinghuan Zhang Mengchang He State Key Joint Laboratory of Environment Simulation and Pollution Control Beijing Normal University School of Environment Beijing Normal University College of Environment and Safety Engineering Qingdao University of Science and Technology

Sorption and desorption of phenanthrene （PHE） onto black carbon （BC） extracted from sediments were studied in the presence of three types of dissolved organic matter （DOM）, including L-phenylalanine （L-PH）, peptone and citric acid. The nonlinearity of the sorption isotherms increased in the presence of DOM. The presence of L-PH reduced the sorption capacity and desorption hysteresis because of the solubilization of PHE in L-PH solution. Peptone at 50-500 mg/L also led to a decrease in sorption attributed to solubilization, although the sorbed peptone on the BC surface could slightly increase PHE sorption. Unlike L-PH and peptone, citric acid enhanced the sorption capacity and irreversibility of PHE on BC mainly due to the strong sorption of citric acid on the BC surface. Our results may help to understand the different impacts of DOM on the distribution and transport of PAH in the environment.

关键词： DOM black carbon phenanthrene sorption desorption

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Efficient photocatalytic reduction of chromium(Ⅵ) using photoreduced graphene oxide as photocatalyst under visible light irradiation

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Journal of Materials Science & Technology 2021年第32期91卷 17-27页

作者： Mei Yu Jing Shang Yu Kuang Department of Environment and Health State Key Joint Laboratory of Environmental Simulation and Pollution ControlCollege of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China

Graphene oxide(GO),a new and promising material,has been widely used as a co-catalyst in photocatalytic reactions;however,its capacity as a sole photocatalyst has rarely been *** this study,ultraviolet(UV) light irradiation was used as a modification method to obtain reduced GO(rGO) *** samples were used as photocatalysts to examine their visible light photocatalytic activity toward hexavalent chromium(Cr(Ⅵ)) *** force microscopy(AFM),X-ray diffraction(XRD),UV-vis spectrophotometry,Raman spectroscopy,X-ray photoelectron spectroscopy(XPS),and electron spin resonance(ESR) spectroscopy were applied to interpret the surface and structure changes with UV *** oxygen-containing functional groups(OFGs) on the GO surface were reduced to defective carbons andπ-conjugated C=C(sp^(2) domains) under UV light;this led to a decrease in the interlayer distance between GO sheets,GO fragmentation,and increased disorder on the GO *** restoration of sp^(2) domains led to a narrower band gap of GO,which favored the rGO excitation by visible light to generate electron-hole *** rGO pre-irradiated with UV for 1 h(rGO-1),possessing the highest defect density and electron generation efficiency,exhibited the best Cr(Ⅵ) reduction efficiency,which was about three times that of the GO sample;moreover,it outperformed most of the reported GO-based *** addition,low pH and the addition of citric acid as a hole scavenger could further improve the photocatalytic *** study proves that GO or rGO can be used as a sole photocatalyst under visible light to remove environmental pollutants such as heavy-metal ions,and it paves the way for the development of this kind of material and its UV-irradiation modification for further applications.

关键词： Graphene oxide Chromium(Ⅵ) Defect density UV-irradiation modification Photocatalytic reduction

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Discovery of emerging organic pollutants in the atmosphere through an omics approach

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Frontiers of environmental Science & Engineering 2023年第4期17卷 71-81页

作者： Zhen Cheng Xinghua Qiu Xiaodi Shi Xing Jiang Tong Zhu State Key Joint Laboratory for Environmental Simulation and Pollution Control College of Environmental Sciences and EngineeringCenter for Environment and HealthPeking UniversityBeijing 100871China

Ambient air pollution,containing numerous known and hitherto unknown compounds,is a major risk factor for public *** discovery of harmful components is the prerequisite for pollution control;however,this raises a great challenge on recognizing previously unknown *** we systematically review the analytical techniques on air pollution in the framework of an omics approach,with a brief introduction on sample preparation and analysis,and in more detail,compounds prioritization and *** high-resolution mass spectrometry(HRMS,typically coupled with chromatography),the complicated environmental matrix can be digitalized into“fullcomponent”data.A key step to discover emerging compounds is the prioritization of compounds from massive *** fingerprints,suspect lists and biological effects are the most vital untargeted strategies for comprehensively screening critical and hazardous ***,compressed data of compounds can be identified at various confidence levels according to exact mass and the derived molecular formula,MS libraries,and authentic *** an omics approach on full-component data provides a paradigm for discovering emerging air pollutants;nonetheless,new technological advancements of instruments and databases are warranted for further tracking the environmental behaviors,hence to evaluate the health risk of key pollutants.

关键词： Air pollution Emerging pollutants Full-component High-resolution mass spectrometry Omics approach

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Vertical distribution of rare earth elements in a wetland soil core from the Sanjiang Plain in China

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Journal of Rare Earths 2012年第7期30卷 731-738页

作者：程红光郝芳华欧阳威刘少卿林春野杨文静 State Key Joint Laboratory of Environmental Simulationand Pollution Control School of EnvironmentBeijing Normal University

The objective of this study was to investigate the vertical distribution of rare earth elements （REEs） in a natural wetland soil core to understand the influence of natural and anthropogenic activities on geochemical behavior of REEs. A natural wetland soil core of 95 cm was collected from the Sanjiang Plain in China and sliced into 5 cm slices for analyses of REEs, Fe, Al, Mn, Sc, Y, and soil organic matter （SOM）. Results indicated that SOM was accumulated in the upper part of the soil core （0 to 20 cm depth）, while Fe and Mn was reductively leached from the upper part of the soil core and accumulated in the low part. The content of total REEs ranged from 137.9 to 225.9 mg/kg in the soil core. Content profiles obtained for all REEs were almost identical except for Ce. The highest contents of REEs generally occurred at about 20 cm depth, but enrichment factor （EF） of REEs except Ce was usually the highest in the surface horizon. Average EF ranged from 1.1 for La to 2.1 for Gd. The pronounced shift in EF occurred at about 40 cm depth and it gradually increased from 40 cm depth to surface （except for Ce）, probably suggesting anthropogenic atmospheric deposition of REEs. In comparison with chondrite, Eu was depleted in all horizons, while Ce was negatively anomalous in the top horizons and positively anomalous in the bottom horizons. This positive anomaly of Ce in the bottom horizons was due to its preferential adsorption on Fe and Mn oxides, relative to other REEs. Although both natural and anthropogenic activi-ties influence the geochemical behaviors of REEs in soils, enrichment or mobility of REEs is low in the natural wetland soil core of the San-jiang Plain.

关键词： wetland soil core rare earth element distribution enrichment factor

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Reduction of wastewater toxicity and change of microbial community in a hydrolysis acidification reactor pre-treating trimethylolpropane wastewater

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Frontiers of environmental Science & Engineering 2018年第6期12卷 119-131页

作者： Xin Xing Yin Yu Hongbo Xi Guangqing Song Yajiao Wang Jiane Zuo Yuexi Zhou State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China Research Center of Water Pollution Control Technology Chinese Research Academy of Environmental SciencesBeijing 100012China

Trimethylolpropane (TMP) wastewater is one of the most toxic petrochemical wastewater. Toxicants with high concentrations in TMP wastewater often inhibit the activity of microorganisms associated with biological treatment processes. The hydrolysis acidification process (HAP) is widely used to pretreat petrochemical wastewater. However, the effects of HAP on the reduction of wastewater toxicity and the relevant underlying mechanisms have rarely been reported. In this study, an HAP reactor was operated for 240 days, fed with actual TMP wastewater diluted by tap water in varying ratios. The toxicity of TMP wastewater was assessed with the inhibition ratio of oxygen uptake rate. When the organic loading rates were lower than 7.5 kg COD/m3/d, the toxicity of TMP wastewater was completely eliminated. When the actual TMP wastewater was directly fed into the reactor, the toxicity of TMP wastewater decreased from 100% to 34.9%. According to the results of gas chromatographymass spectrometry analysis, four main toxicants contained in TMP wastewater, namely, formaldehyde, 2-ethylacrolein, TMP and 2-ethylhexanol, were all significantly removed, with removal efficiencies of 93.42%, 95.42%, 72.85% and 98.94%, respectively. Compared with the removal efficiency of CODCr, the reduction rate of toxicity is markedly higher by HAP. In addition, the change of microbial community in the HAP reactor, along the operation period, was studied. The results revealed that, compared with the seed sludge, Firmicutes became the dominant phylum (abundance increased from 0.51% to 57.08%), followed by Proteobacteria and Bacteroidetes (abundance increased from 59.75% to 25.99% and from 4.70% to 8.39%, respectively).

关键词： Trimethylolpropane wastewater Hydrolysis acidification process Toxicity Oxygen uptake rate 16S rDNA

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Superhigh adsorption of perfluorooctane sulfonate on aminated polyacrylonitrile fibers with the assistance of air bubbles

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Chemical Engineering Journal 2017年 315卷 108-114页

作者： Meng, Pingping Deng, Shubo Wang, Bin Huang, Jun Wang, Yujue Yu, Gang State Key Joint Laboratory of Environment Simulation and Pollution Control Beijing Key Laboratory for Emerging Organic Contaminants Control School of Environment Tsinghua University Beijing100084 China

The role of air bubbles in the adsorption of perfluorooctane sulfonate (PFOS) is normally overlooked, and particularly the influence of air bubbles on PFOS adsorption onto hydrophilic adsorbents remains unclear. In this study, for the first time we propose that air bubbles originally existing in solution or being formed during shaking play an important role in the adsorption of PFOS on the aminated polyacrylonitrile fibers (APANFs). The APANFs possess a superhigh adsorption capacity of 15.0 mmol/g for PFOS at pH 3 with the assistance of air bubbles. The contribution of air bubbles to PFOS adsorption increases with the decrease of initial PFOS concentrations and the increase of solution pH. The adsorbed amount of PFOS on the APANFs deceases by 79% when 0.026 mmol/L PFOS solution at pH 6 is degassed at 0.01 atm for 24 h. By contrast, degassing the APANFs shows no influence on PFOS adsorption, suggesting the dominant contribution of air bubbles in solution rather than on the APANFs. PFOS is adsorbed on the APANFs via not only the electrostatic attraction and micelles, but also the adsorbed air bubbles with accumulated PFOS at gas-liquid interfaces. A new schematic sorption model of PFOS on the APANFs with the assistance of air bubbles is proposed, and this finding is helpful for developing PFOS removal strategy and understanding PFOS transport and fate in aquatic environments. © 2017 Elsevier B.V.

关键词： Adsorption

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Quantification of multi-antibiotic resistant opportunistic pathogenic bacteria in bioaerosols in and around a pharmaceutical wastewater treatment plant

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Journal of environmental Sciences 2018年第10期30卷 53-63页

作者： Mengyu Zhang Jiane Zuo Xin Yu Xuchuan Shi Lei Chen Zaixing Li State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Tsinghua University School of Environmental Science and Engineering Hebei University of Science and Technology

Pharmaceutical wastewater treatment plants（WWTPs） are thought to be a ＂seedbed＂ and reservoirs for multi-antibiotic resistant pathogenic bacteria which can be transmitted to the air environment through aeration. We quantified airborne multi-antibiotic resistance in a full-scale plant to treat antibiotics-producing wastewater by collecting bioaerosol samples from December2014 to July 2015. Gram-negative opportunistic pathogenic bacteria（GNOPB） were isolated, and antibiotic susceptibility tests against 18 commonly used antibiotics, including 11 β-lactam antibiotics, 3 aminoglycosides, 2 fluoroquinolones, 1 furan and 1 sulfonamide, were *** than 45% of airborne bacteria isolated from the pharmaceutical WWTP were resistant to three or more antibiotics, and some opportunistic pathogenic strains were resistant to 16 antibiotics, whereas 45.3% and 50.3% of the strains isolated from residential community and municipal WWTP showed resistance to three or more antibiotics. The calculation of the multiple antibiotic resistance（MAR） index demonstrated that the air environment in the pharmaceutical WWTP was highly impacted by antibiotic resistance, while the residential community and municipal WWTP was less impacted by antibiotic resistance. In addition, we determined that the dominant genera of opportunistic pathogenic bacteria isolated from all bioaerosol samples were Acinetobacter, Alcaligenes, Citrobacter, Enterobacter, Escherichia, Klebsiella, Pantoea, Pseudomonas and Sphingomonas. Collectively, these results indicate the proliferations and spread of antibiotic resistance through bioaerosols in WWTP treating cephalosporin-producing wastewater, which imposed a potential health risk for the staff and residents in the neighborhood, calling for administrative measures to minimize the air-transmission hazard.

关键词： Multi-antibiotic resistance Gram-negative opportunistic pathogenic bacteria Bioaerosols Pharmaceutical wastewater treatment plants

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A review of atmospheric mercury emissions, pollution and control in China

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Frontiers of environmental Science & Engineering 2014年第5期8卷 631-649页

作者： Shuxiao WANG Lei ZHANG Long WANG Qingru WU FengyangWANG Jiming HAO State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Tsinghua University Beijing 100084 China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084 China

Mercury, as a global pollutant, has significant impacts on the environment and human health. The current state of atmospheric mercury emissions, pollution and control in China is comprehensively reviewed in this paper. With about 500-800 t of anthropogenic mercury emissions, China contributes 25%-40% to the global mercury emissions. The dominant mercury emission sources in China are coal combustion, non-ferrous metal smelting, cement production and iron and steel production. The mercury emissions from natural sources in China are equivalent to the anthropogenic mercury emissions. The atmospheric mercury concentration in China is about 2-10 times the background level of North Hemisphere. The mercury deposition fluxes in remote areas in China are usually in the range of 10-50μg·m^-2·yr^-1. To reduce mercury emissions, legislations have been enacted for power plants, non-ferrous metal smelters and waste incinerators. Currently mercury contented in the flue gas is mainly removed through existing air pollution control devices for sulfur dioxide, nitrogen oxides, and particles. Dedicated mercury control technologies are required in the future to further mitigate the mercury emissions in China.

关键词： atmospheric mercury emissions pollution,control China

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