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Simultaneous hydrogen production with photo reforming of lactic acid over MXene derived MoS_(2)/TiO_(2)/Ti_(3)C_(2)nanowires

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Chinese Journal of Catalysis 2025年第4期71卷 234-245页

作者： Seemal Mansoor Zixu Hu Yuxin Zhang Muhammad Tayyab Mazhar Khan Zeeshan Akmal Liang Zhou Juying Lei Muhammad Nasir Jinlong Zhang Key Laboratory for Advanced Materials Shanghai Engineering Research Center for Multi–media Environmental Catalysis and Resource UtilizationJoint International Research Laboratory of Precision Chemistry and Molecular EngineeringFeringa Nobel Prize Scientist Joint Research CenterSchool of Chemistry and Molecular EngineeringEast China University of Science&TechnologyShanghai 200237China National Engineering Research Center of Industrial Wastewater Detoxication and Resource Recovery State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical ProcessEast China University of Science and TechnologyShanghai 200237China State Key Laboratory of Urban Water Resource and Environment Harbin Institute of TechnologyHarbin 150090HeilongjiangChina Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China Institute of Materials Research Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055GuangdongChina COMSATS Univ Islamabad Interdisciplinary Res Ctr Biomed Mat IRCBMLahore CampusLahore 54000Pakistan

Developing efficient photocatalysts to address collaborative energy and environmental crises still faces significant *** this report,we present a highly efficient MXene–based photocatalyst,which is combined with MoS_(2)nano patches and TiO_(2)/Ti_(3)C_(2)(TTC)nanowires through hydrothermal *** all the composites tested,the optimized photocatalyst gave a remarkable H_(2)and revolving polylactic acid(PLA)into pyruvic acid(PA).Achieving a remarkable H_(2)evolution rate of 637.1 and 243.2μmol g^(−1)h^(−1),in the presence of TEOA and PLA as a sacrificial reagent under UV-vis(λ≥365 nm)light *** improved photocatalytic activity is a result of the combination of dual cocatalyst on the surface of TTC photocatalyst,which create an ideal synergistic effect for the generation of PA and the production of H_(2)*** MoS_(2)TiO_(2)/Ti_(3)C_(2)(MTT)composite can generate more photoexcited charge carriers,leading to the generation of more active radicals,which may enhance the system's photocatalytic *** work aims at demonstrating its future significance and guide the scientific community towards a more efficient approach to commercializing H_(2)through photocatalysis.

关键词： Photo reforming Polylactic acid Hydrogen evolution Lactic acid Pyruvic acid

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Scrap Iron Filings assisted nitrate and phosphate removal in low C/N waters using mixed microbial culture

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Frontiers of environmental Science & Engineering 2021年第4期15卷 215-228页

作者： Sanjena Narayanasamydamodaran Jian’e Zuo Haiteng Ren Nawnit Kumar State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing100084China State Key Laboratory of Hydroscience and Hydraulic Engineering Tsinghua UniversityBeijing100084China

This study focuses on identifying the factors under which mixed microbial seeds assist bio-chemical denitrification when Scrap Iron Filings(SIF)are used as electron donors and adsorbents in low C/N ratio *** studies were conducted in abiotic and biotic reactors containing fresh and aged SIF under different dissolved oxygen concentrations with NO_(3)^(-)−N and/or PO_(4)^(3−)influent(s)and their nitrate/phosphate removal and by-product formations were *** reactors were seeded with a homogenized mixed microbial inoculum procured from natural sludges which were enriched over 6 months under denitrifying conditions in the presence of *** indicated that when influent containing 40 mg/L of NO_(3)^(-)−N was treated with 5 g SIF,79.9%nitrate reduction was observed in 8 days abiotically and 100%removal was accomplished in 20 days when the reactor was *** abiotic and seeded reactors removed more than 92%PO_(4)^(3−)under high DO conditions in 12 *** and biochemical removal of NO_(3)^(-)−N and abiotic removal of PO_(4)^(3−)were higher under independent NO_(3)^(-)−N/PO_(4)^(3−)loading,while 99%PO_(4)^(3−)was removed biochemically under combined NO_(3)^(-)−N and PO_(4)^(3−)*** study furthers the understandings of nitrate and phosphate removal in Zero Valent Iron(ZVI)assisted mixed microbial systems to encourage the application of SIF-supported bio-chemical processes in the simultaneous removals of these pollutants.

关键词： Scrap iron filing Nitrate removal Phosphate removal Mixed culture denitrification Zero valent iron

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Differentiated emission control strategy based on comprehensive evaluation of multi-media pollution:Case of mercury emission control

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Journal of environmental Sciences 2023年第1期123卷 222-234页

作者： Dongwei Lv Qingru Wu Daiwei Ouyang Minneng Wen Gehui Zhang Shuxiao Wang Lei Duan State Key Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China

In order to comprehensively evaluate the environmental impact of multi-media mercury pollution under differentiated emission control strategies in China,a literature review and case studies were carried *** human exposure to methylmercury was assessed through the dietary intake of residents in areas surrounding a typical coal-fired power plant and a zinc(Zn)smelter,located either on acid soil with paddy growth in southern China,or on alkaline soil with wheat growth in northern *** with knowledge on speciated mercury in flue gas and the fate of mercury in the wastewater or solid waste of the typical emitters applying different air pollution control devices,a simplified model was developed by estimating the incremental daily intake of methylmercury from both local and global *** indicated that air pollution control for coal-fired power plants and Zn smelters can greatly reduce health risks from mercury pollution,mainly through a reduction in global methylmercury exposure,but could unfortunately induce local methylmercury exposure by transferring more mercury from flue gas to wastewater or solid waste,then contaminating surrounding soil,and thus increasing dietary intake via ***,tightening air emission control is conducive to reducing the comprehensive health risk,while the environmental equity between local and global pollution control should be fully *** in the south tends to have higher bioconcentration factors than wheat in the north,implying the great importance of strengthening local pollution control in the south,especially for Zn smelters with higher contribution to local pollution.

关键词： Mercury emission Methylmercury Heavy metal Bioconcentration factor Estimated daily intake Health risk assessment

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Metagenomic insights into the profile of antibiotic resistomes in sediments of aquaculture wastewater treatment system

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Journal of environmental Sciences 2022年第3期34卷 345-355页

作者： Jianfei Chen Yuyin Yang Xinshu Jiang Yanchu Ke Tao He Shuguang Xie State Key Joint Laboratory of Environmental Simulation and Pollution Control College of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China State Key Joint Laboratory of Environment Simulation and Pollution Control(SKJLESPC) Beijing Key Laboratory for Emerging Organic Contaminants Control(BKLEOC)School of EnvironmentPOPs Research CenterTsinghua UniversityBeijing 100084China South China Institute of Environmental Sciences(SCIES) Ministry of Ecology and Environment(MEE)Guangzhou 510655China

To meet the rapidly growing global demand for aquaculture products,large amounts of antibiotics were used in aquaculture,which might accelerate the evolution of antibiotic-resistant bacteria(ARB)and the propagation of antibiotic genes(ARGs).In our research,we revealed the ARGs profiles,their co-occurrence with mobile genetic elements(MGEs),and potential hosts in sediments of a crab pond wastewater purification system based on metagenomic *** residual antibiotic seems to increase the propagation of ARGs in the crab pond,but there was no clear relationship between a given antibiotic type and the corresponding resistance *** effect of aquaculture on sediment was not as profound as that of other anthropogentic activities,but increased the relative abundance of sulfon-amide resistance gene.A higher abundance of MGEs,especially plasmid,increased the po-tential ARGs dissemination risk in crab and purification *** and sulfonamide resistance genes had greater potential to transfer because they were more frequently carried by *** horizontal gene transfer was likely to occur among a variety of microorgan-isms,and various ARGs hosts including Pseudomonas,Acinetobacter,Escherichia,and Klebsiella were *** community influenced the composition of ARG hosts,and Pro-teobacteria was the predominant ***,our study provides novel insights into the environmental risk of ARGs in sediments of aquaculture wastewater treatment system.

关键词： Metagenomic sequencing Aquaculture Antibiotic resistome Antibiotic resistance genes(ARGs) Mobile genetic elements(MGEs) ARG hosts

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Mixed sulfur–iron particles packed reactor for simultaneous advanced removal of nitrogen and phosphorus from secondary effluent

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environmental Science and pollution Research 2014年第1期22卷 415-424页

作者： Wang, Shenghui Liang, Peng Wu, Zhongqin Su, Fengfeng Yuan, Lulu Sun, Yanmei Wu, Qing Huang, Xia State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua University Beijing100084 China

A mixed sulfur–iron particles packed reactor (SFe reactor) was developed to simultaneously remove total nitrogen (TN) and total phosphorus (TP) of the secondary effluent from municipal wastewater treatment plants. Lo... 详细信息

关键词： Phosphorus

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Heterogeneous oxidation of SO_2 by O_3-aged black carbon and its dithiothreitol oxidative potential

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Journal of environmental Sciences 2015年第10期27卷 56-62页

作者： Weiwei Xu Qian Li Jing Shang Jia Liu Xiang Feng Tong Zhu State Key Joint Laboratory of Environmental Simulation and Pollution Control College of Environmental Sciences and EngineeringPeking University POTEN Environment Group Co. Ltd.

Ozone（O3） is an important atmospheric oxidant. Black carbon（BC） particles released into the atmosphere undergo an aging process via O3 oxidation. O3-aged BC particles may change their uptake ability toward trace reducing gases such as SO2 in the atmosphere,leading to different environmental and health effects. In this paper, the heterogeneous reaction process between O3-aged BC and SO2 was explored via in-situ diffuse reflectance infrared Fourier transform spectroscopy（DRIFTS）. Combined with ion chromatography（IC）,DRIFTS was used to qualitatively and quantitatively analyze the sulfate product. The results showed that O3-aged BC had stronger SO2 oxidation ability than fresh BC, and the reactive species/sites generated on the surface had an important role in the oxidation of *** humidity or 254 nm UV（ultraviolet） light illumination enhanced the oxidation uptake of SO2 on O3-aged BC. The oxidation potentials of the BC particles were detected via dithiothreitol（DTT） assay. The DTT activity over BC was decreased in the process of SO2 reduction, with the consumption of oxidative active sites.

关键词： Black carbon Ozone SO2 Heterogeneous reaction Oxidative potential Dithiothreitol assay

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Efectiveness of national air pollution control policies on the air quality in metropolitan areas of China

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Journal of environmental Sciences 2014年第1期26卷 13-22页

作者： Shuxiao Wang Jia Xing Bin Zhao Carey Jang Jiming Hao State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua University State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex US Environmental Protection Agency Research Triangle Park Collaborative Innovation Center for Regional Environmental Quality Tsinghua University

Understanding the effectiveness of national air pollution controls is important for control policy design to improve the future air quality in China. This study evaluated the effectiveness of major national control policies implemented recently in China through a modeling analysis. The sulfur dioxide （SO2） control policy during the llth Five Year Plan period （2006-2010） had succeeded in reducing the national SO2 emission in 2010 by 14% from its 2005 level, which correspondingly reduced ambient SO2 and sulfate （SO42-） concentrations by 13%-15% and 8%-10% respectively over east China. The nitrogen oxides （NOx） control policy during the 12th Five Year Plan period （2011-2015） targets the reduction of the national NOx emission in 2015 by 10% on the basis of 2010. The simulation results suggest that such a reduction in NOx emission will reduce the ambient nitrogen dioxide （NO2）, nitrate （NO3-）, 1-hr maxima ozone （03） concentrations and total nitrogen deposition by 8%, 3%-14%, 2% and 2%--4%, respectively over east China. The application of new emission standards for power plants will further reduce the NO2, NO3-, 1-hr maxima 03 concentrations and total nitrogen deposition by 2%-4%, 1%-%, 0-2% and 1%-2%, respectively. Sensitivity analysis was conducted to evaluate the inter-provincial impacts of emission reduction in Beijing-Tianjin-Hebei and the Yangtze River Delta, which indicated the need to implement joint regional air pollution control.

关键词： air pollution control sulfur dioxide nitrogen oxides power plant

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Contrasting trends of PM2.5 and surface-ozone concentrations in China from 2013 to 2017

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National Science Review 2020年第8期7卷 1331-1339页

作者： Yonghong Wang Wenkang Gao Shuai Wang Tao Song Zhengyu Gong Dongsheng Ji Lili Wang Zirui Liu Guiqian Tang Yanfeng Huo Shili Tian Jiayun Li Mingge Li Yuan Yang Biwu Chu Tuukka Pet?j? Veli-Matti Kerminen Hong He Jiming Hao Markku Kulmala Yuesi Wang Yuanhang Zhang State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry (LAPC) Institute of Atmospheric Physics Chinese Academy of Sciences Institute for Atmospheric and Earth System Research University of Helsinki China National Environmental Monitoring Center (CNEMC) Anhui Institute of Meteorological Sciences State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental Sciences Chinese Academy of Sciences Center for Excellence in Regional Atmospheric Environment Institute of Urban Environment Chinese Academy of Sciences State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua University State Key Joint Laboratory of Environmental Simulation and Pollution Control College of Environmental Sciences and Engineering Peking University

Although much attention has been paid to investigating and controlling air pollution in China, the trends of air-pollutant concentrations on a national scale have remained unclear. Here, we quantitatively investigated the variation of air pollutants in China using long-term comprehensive data sets from 2013 to 2017, during which Chinese government made major efforts to reduce anthropogenic emission in polluted regions. Our results show a significant decreasing trend in the PM2.5concentration in heavily polluted regions of eastern China, with an annual decrease of ～7% compared with measurements in 2013. The measured decreased concentrations of SO2, NO2and CO（a proxy for anthropogenic volatile organic compounds） could explain a large fraction of the decreased PM2.5concentrations in different regions. As a consequence, the heavily polluted days decreased significantly in corresponding regions. Concentrations of organic aerosol,nitrate, sulfate, ammonium and chloride measured in urban Beijing revealed a remarkable reduction from 2013 to 2017, connecting the decreases in aerosol precursors with corresponding chemical components closely. However, surface-ozone concentrations showed increasing trends in most urban stations from 2013 to 2017, which indicates stronger photochemical pollution. The boundary-layer height in capital cities of eastern China showed no significant trends over the Beijing–Tianjin–Hebei, Yangtze River Delta and Pearl River Delta regions from 2013 to 2017, which confirmed the reduction in anthropogenic emissions. Our results demonstrated that the Chinese government was successful in the reduction of particulate matter in urban areas from 2013 to 2017, although the ozone concentration has increased significantly, suggesting a more complex mechanism of improving Chinese air quality in the future.

关键词： air pollution clean-air action particulate matter surface ozone China chemical composition

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Accelerating exploitation and integration of global renewable energy

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Innovation 2025年

作者： Wang, Jianxiao Chen, Xinjiang Zhuang, Minghao Li, Yan Ruan, Ziwen Wang, Yuhan Zhang, Ning Song, Jie He, Kebin Lu, Xi National Engineering Laboratory for Big Data Analysis and Applications Peking University Beijing100871 China Department of Industrial Engineering and Management College of Engineering Peking University Beijing100871 China Peking University Ordos Research Institute of Energy Ordos017000 China State Key Laboratory of Nutrient Use and Management College of Resources and Environmental Sciences China Agricultural University Beijing100193 China College of Environmental Science and Engineering Tongji University Shanghai200092 China School of Environment State Key Joint Laboratory of Environment Simulation and Pollution Control Tsinghua University Beijing100084 China State Key Lab of Power Systems Department of Electrical Engineering Tsinghua University Beijing100084 China Institute for Carbon Neutrality Tsinghua University Beijing100084 China

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Comparison of changes of typical river segment ecosystem service value in LRGR

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Chinese Science Bulletin 2007年第A02期52卷 262-272页

作者： WEI GuoLiang CUl BaoShan YANG ZhiFeng BAI JunHong WANG Juan HU Bo State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Beijing Normal UniversityBeijing 100875 China

来自 Lancang 河和 Yuanjiang 河的河片断生态系统的陆地使用变化从 1985 ～ 2000 被学习以便比较他们服务价值的变化并且分析开车机制基于 eco 经济并且 GIS 方法。结果显示出那个森林在两个的区域河片断生态系统被减少。在 Lancang 河... 详细信息

来自 Lancang 河和 Yuanjiang 河的河片断生态系统的陆地使用变化从 1985 ～ 2000 被学习以便比较他们服务价值的变化并且分析开车机制基于 eco 经济并且 GIS 方法。结果显示出那个森林在两个的区域河片断生态系统被减少。在 Lancang 河(LR ) 片断生态系统的减少的森林主要与 56.0% 的变换率被转变成大地，当在 Yuanjiang 河(年) 片断生态系统的减少的森林主要与 42.5% 的变换率被转变成住处土地时。变化数量和在 LR 片断生态系统的每种陆地使用类型的区域的变化率比在 YR 片断生态系统的那些大得多。LR 片断生态系统的全部的服务价值与 15.3% 的变化率被减少，当年片断生态系统的与 0.6% 的变化率被增加时。Manwan 水力发出的电力开发是与 93% 的贡献率导致了 LR 片断生态系统的服务价值的变化的主要人为的开车因素。农业活动是在有 59% 的贡献率的 YR 片断生态系统的最重要的开车因素。沉积交通服务源于 Manwan 水力发出的电力工程建设的价值的损失应该负责水的服务价值的重要减少，甚至为整个 LR 片断生态系统。在学习区域的森林和草地的生态系统服务系数比在中国的平均水平高得多，那么是间接价值的比率指导两个的价值河片断生态系统。在人的活动的影响下面，为提供产品的河生态系统的能力被提高，当维持自然生态系统健康被削弱时。

关键词：纵向岭谷区河流生态环境评估方法

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