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Photodegradation of soluble microbial products(SMPs) from membrane bioreactor by GO-COOH/TiO2/Ag

Journal of environmental Sciences 2020年第2期32卷 292-300页

作者： Shuyan Yu Xia Huang State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China

This study aimed to explore a new degradation method-photocatalysis technology to polish membrane bioreactor(MBR) effluent, using 2,6-di-tert-butylphenol(2,6-DTBP) as a model soluble microbial product(SMP).2,6-DTBP is one of the predominant SMPs in MBR effluent, which is refractory and difficult to *** study developed a novel carboxylated graphene oxide/titanium dioxide/silver(GO-COOH/TiO2/Ag) nanocomposite to photodegrade 2,***-COOH/TiO2/Ag was successfully synthesized, using L-cysteine as the linker bonding TiO2/Ag to *** structural, morphological and optical properties of the GO-COOH/TiO2/Ag nanocomposite were characterized using various *** to synergistic effects, the GO-COOH/TiO2/Ag nanocomposite exhibited enhanced photocatalytic degradation performance under solar light irradiation when compared to TiO2, Ag and *** remove 25 mg/L 2,6-DTBP, the reaction time for GOCOOH/TiO2/Ag was only 30 min, faster than the 90 min required for pure TiO2 or *** addition, the 200 mg/L GO-COOH/TiO2/Ag nanocomposite aqueous solution showed the best performance under solar light, with 99% removal of 2,*** enhanced capability is likely due to the surface plasmon resonance(SPR) effect contributed by Ag nanoparticles(NPs) doped onto the *** addition, GO-COOH had a high effective surface area, which assisted in degrading the 2,6-DTBP through improved *** stability study showed that the photocatalytic activity of the GO-COOH/TiO2/Ag was stable enough for recycling multiple *** effective degradation performance and excellent stability demonstrates that the GO-COOH/TiO2/Ag nanocomposite can be a promising photocatalyst in the field of effluent SMP photodegradation, which solves the problem of the difficult biodegradation of highly toxic 2,6-DTBP.

关键词： Soluble microbial products (SMPs) 2,6-Di-tert-butylphenol (2,6-DTBP) Carboxylated graphene oxide/titanium dioxide/silver (GO-COOH/TiO2/Ag) nanocomposite Photocatalysis technology

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Microbial Electrosynthesis for Producing Medium Chain Fatty Acids

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Engineering 2022年第9期16卷 141-153页

作者： Na Chu Wen Hao Qinglian Wu Qinjun Liang Yong Jiang Peng Liang Zhiyong Jason Ren Raymond Jianxiong Zeng Fujian Provincial Key Laboratory of Soil Environmental Health and Regulation College of Resources and EnvironmentFujian Agriculture and Forestry UniversityFuzhou 350002China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China College of Architecture and Environment Sichuan UniversityChengdu 610065China Department of Civil and Environmental Engineering&Andlinger Center for Energy and the Environment Princeton UniversityPrincetonNJ 08544USA

Microbial electrosynthesis(MES)employs microbial catalysts and electrochemistry to enhance CO_(2)bioconversion to organics with concurrent waste biorefining *** aim of this review is to comprehensively discuss the current state of the art and prospects of medium chain fatty acids(MCFAs)production in MES from CO_(2)and organic *** mechanisms and development of MCFAs production via conventional fermentation are introduced as *** on MCFAs production in MES are summarized,highlighting the strategy of multiple-electron donors(EDs).Challenges for MCFAs production in MES from CO_(2)are presented,and the primary discussions included methanogenesis inhibition,adenosine triphosphate(ATP)limitations of acetogens,and production of limited EDs via *** applications of electrochemical approaches to promote the bioconversion of actual waste materials with MCFAs production are ***,future directions are explored,including multi-stage reactions,substrate supply,product extraction,and microbial pathways.

关键词： Electro-fermentation Microbial electrochemistry Acetogen Chain elongation Electroactive microorganism

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Review on heterogeneous oxidation and adsorption for arsenic removal from drinking water

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Journal of environmental Sciences 2021年第12期33卷 178-188页

作者： Ruiping Liu Jiuhui Qu Key Laboratory of Drinking Water Science and Technology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Center for Water and Ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China

The long term exposure of arsenic via drinking water has resulted in wide occurrence of arsenisim globally, and the oxidation of the non-ionic arsenite(As(Ⅲ)) to negatively-charged arsenate(As(Ⅴ)) is of crucial importance for the promising removal of arsenic. The chemical oxidants of ozone, chlorine, chlorine dioxide, and potassium permanganate may achieve this goal;however, their application in developing countries is sometimes restricted by the complicate operation and high cost. This review paper focuses on the heterogeneous oxidation of As(Ⅲ) by solid oxidants such as manganese oxide, and the adsorption of As(Ⅴ)accordingly. Manganese oxide may be prepared by both chemical and biological methods to achieve good oxidation performance towards As(Ⅲ). Additionally, manganese oxide may be combined with other metal oxides, e.g., iron oxide, to improve the adsorption capability towards As(Ⅴ). Furthermore, manganese oxide may be coated onto porous materials of metal organic frameworks to develop novel adsorbents for arsenic removal. To achieve the application in engineering works, the adsorbents granulation may be achieved by drying and calcination, agglomeration, and the active components may also be in situ coated onto the porous materials to maintain the oxidation and adsorption activities as much as possible. The novel adsorbents with heterogeneous oxidation and adsorption capability may be carefully designed for the removal of arsenic in household purifiers, community-level decentralized small systems, and the large-scale drinking water treatment plants(DWTPs).This review provides insight into the fundamental studies on novel adsorbents, the development of innovative technologies, and the demonstration engineering works involved in the heterogeneous oxidation and adsorption, and may be practically valuable for the arsenic pollution control globally.

关键词： Arsenic Heterogeneous oxidation Adsorption Manganese oxide Drinking water

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Formation of secondary inorganic aerosol in a frigid urban atmosphere

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Frontiers of environmental Science & Engineering 2022年第2期16卷 39-50页

作者： Yuan Cheng Qinqin Yu Jiumeng Liu Youwen Sun Linlin Liang Zhenyu Du Guannan Geng Wanli Ma Hong Qi Qiang Zhang Kebin He State Key Laboratory of Urban Water Resource and Environment School of EnvironmentHarbin Institute of TechnologyHarbin 150090China Key Laboratory of Environmental Optics and Technology Anhui Institute of Optics and Fine MechanicsChinese Academy of SciencesHefei 230031China State Key Laboratory of Severe Weather&CMA Key Laboratory of Atmospheric Chemistry Chinese Academy of Meteorological SciencesBeijing 100081China National Research Center for Environmental Analysis and Measurement Environmental Development Center of the Ministry of Ecology and EnvironmentBeijing 100029China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China Department of Earth System Science Tsinghua UniversityBeijing 100084China

Formation of secondary inorganic aerosol(SIA)was investigated during a six-month long heating season in Harbin,*** sulfate formation was observed at high relative humidity(RH),with the same threshold RH(80%)for both colder and warmer measurement *** to wintertime results from Beijing,the threshold RH was considerably higher in Harbin,whereas the RH-dependent enhancement of sulfur oxidation ratio(SOR)was less *** addition,the high RH events were rarely encountered,and for other periods,the SOR were typically as low as~***,the sulfate formation was considered inefficient in this *** excluding the several cases with high RH,both SOR and the nitrogen oxidation ratio(NOR)exhibited increasing trends as the temperature increased,with the increase of NOR being *** nitrate to sulfate ratio tended to increase with increasing temperature as *** on a semi-quantitative approach,this trend was attributed primarily to the temperature-dependent variations of precursors including SO_(2) and NO_(2).The influence of biomass burning emissions on SIA formation was also *** stronger impact of biomass burning,an enhancement in NOR was observed whereas SOR was largely *** different patterns were identified as the dominant driver of the larger nitrate to sulfate ratios measured at higher concentrations of fine particulate matter.

关键词： Haze Sulfate Nitrate Heterogeneous chemistry Biomass burning

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Enhancing methane production and interspecies electron transfer of anaerobic granular sludge by the immobilization of magnetic biochar

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Chemosphere 2024年 352卷 141332页

作者： Zhuo, Meihui Quan, Xiangchun Yin, Ruoyu Lv, Kai State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Beijing Normal University Beijing 100875 China

Supplementation of conductive materials has been proved to be a promising approach for enhancing microbial interspecies electron transfer (IET) in anaerobic digestion systems. In this study, magnetic bamboo-based biochar was prepared at temperatures of 400–800 °C via a ball milling/carbonization method, and it immobilized in mature anaerobic granular sludge (AGS) aimed to enhance methane production by improving the IET process between syntrophic microbial communities in the AGS. Results showed that the AGS with magnetic biochar immobilization demonstrated increased glucotrophic and acetotrophic methane production by 69.54–77.56 % and 39.96–54.92 %, respectively. Magnetic biochar prepared at 800 °C with a relatively higher Fe content (0.37 g/g magnetic biochar) displayed a stronger electron charge/discharge capacity (36.66 F/g), and its immobilization into AGS promoted methane production most. The conductivity of AGS increased by 52.13–87.32 % after incorporating magnetic biochar. Furthermore, the extracellular polymeric substance (EPS) of AGS showed an increased capacitance and decreased electron transfer resistance possibly due to the binding of magnetic biochar and more riboflavin secretion in EPS, which could contribute to the accelerated IET process in the inner AGS. In addition, the immobilization of magnetic biochar could promote the production of volatile fatty acids by 15.36–22.50 %. All these improvements may jointly lead to the enhanced methane production capacity of AGS. This study provided a fundamental understanding of the role of incorporated magnetic biochar in AGS in promoting anaerobic digestion performance. © 2024 Elsevier Ltd

关键词： Acidogenesis Anaerobic granular sludge Extracellular polymeric substance Interspecies electron transfer Magnetic biochar Methanogenesis

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Screening legacy and emerging organic pollutants in the contaminated soil of Dhaka,Bangladesh

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Emerging Contaminants 2024年第3期10卷 343-353页

作者： Refayat Nigar Shizhen Zhao Xin Liu Huanfang Huang Lele Tian Yuwei Xiao Ahsan Habib Gan Zhang State Key Laboratory of Organic Geochemistry Guangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou510640China Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and Control and Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization Guangzhou510640China Anti-Drug Technology Center of Guangdong Province and National Anti-Drug Laboratory Guangdong Regional Center Guangzhou510230China State Environmental Protection Key Laboratory of Water Environmental Simulation and Pollution Control South China Institute of Environmental SciencesMinistry of Ecology and EnvironmentGuangzhou510530China Department of Chemistry University of DhakaDhaka1000Bangladesh University of Chinese Academy of Sciences Beijing100049China

The current understanding of the legacy and emerging organic pollutants in the soil of Bangladesh remains *** disposal practices,particularly in e-waste,landfills,and industrial operations,may lead to the pervasive presence of persistent organic pollutants(POPs)and polycyclic aromatic hydrocarbons(PAHs)in the *** study aimed to systematically investigate the concentrations,sources,and risk assessment of halogenated flame retardants(HFRs),polychlorinated biphenyls(PCBs),polychlorinated naphthalenes(PCNs),organochlorine pesticides(OCPs),chlorinated paraffins(CPs),and PAHs in the contaminated soil of Dhaka's dumpsites,e-waste,and industrial areas collected in *** total concentration of investigated pollutants averaged at 4790±4040 ng g^(-1)dw,with the following order:P44CPs(4110±4140 ng g^(-1)dw)>P16PAHs(422±491 ng g^(-1)dw)>P16HFRs(190±538 ng g^(-1)dw)>P209PCBs(43.5±73.5 ng g^(-1)dw)>P50PCNs(17.7±21.0 ng g^(-1)dw)>P27OCPs(9.41±9.61 ng g^(-1)dw).The e-waste site exhibited the highest total concentration of the target pollutants,reaching 12,700 ng g1 *** were the predominant contributors,accounting for averages of 81.8%,70.5%,and 68.5%to waste landfills,e-waste,and industrial sites,respectively.A comprehensive analysis of 209 PCB congeners revealed their primary origin from Aroclor PCBs,with minor contributions from unintentionally produced *** highest incremental lifetime carcinogenic risk(ILCR)occurred in e-waste sites,contributed by dioxin-like PCBs,with a maximum value of 5.9×10^(-5)for adults,exceeding the limit 1.0×10^(-6)set by the *** non-carcinogenic hazard quotients(HQs)were much lower,suggesting no significant risk from the investigated *** findings highlight the importance of proper waste management and regulated e-waste recycling to mitigate potential hazardous risks to the Bangladeshi population.

关键词： Persistent organic pollutants Polycyclic aromatic hydrocarbons Chlorinated paraffins Polychlorinated biphenyls Risk assessment Contaminated soil Bangladesh

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Arsenic release from microbial reduction of scorodite in the presence of electron shuttle in flooded soil

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Journal of environmental Sciences 2023年第4期126卷 113-122页

作者： Yujuan Fang Manjia Chen Chengshuai Liu Leheng Dong Jimei Zhou Xiu Yi Dongqing Ji Jiangtao Qiao Hui Tong School of Water and Environment Chang’an UniversityXi’an 710054China National-Regional Joint Engineering Research Center for Soil Pollution Control and Remediation in South China Guangdong Key Laboratory of Integrated Agro-environmental Pollution Control and ManagementInstitute of Eco-environmental and Soil SciencesGuangdong Academy of SciencesGuangzhou 510650China State Key Laboratory of Environmental Geochemistry Institute of GeochemistryChinese Academy of SciencesGuiyang 550081China College of Agriculture/Tree Peony Henan University of Science and TechnologyLuoyang 471023China

Scorodite (FeAsO_(4)·H_(2)O) is a common arsenic-bearing (As-bearing) iron mineral in nearsurface environments that could immobilize or store As in a bound *** flooded soils,microbe induced Fe(Ⅲ) or As(Ⅴ) reduction can increase the mobility and bioavailability of ***,humic substances can act as electron shuttles to promote this *** dynamics of As release and diversity of putative As(Ⅴ)-reducing bacteria during scorodite reduction have yet to be investigated in detail in flooded ***,the microbial reductive dissolution of scorodite was conducted in an flooded soil in the presence of anthraquinone-2,6-disulfonate (AQDS).Anaeromyxobacter,Dechloromonas,Geothrix,Geobacter,Ideonella,and Zoogloea were found to be the dominant indigenous bacteria during Fe(Ⅲ) and As(Ⅴ) *** increased the relative abundance of dominant species,but did not change the diversity and microbial community of the systems with *** these bacteria,Geobacter exhibited the greatest increase and was the dominant Fe(Ⅲ)-and As(Ⅴ)-reducing bacteria during the incubation with AQDS and *** promoted both Fe(Ⅲ) and As(Ⅴ) reduction,and over 80%of released As(Ⅴ) was microbially transformed to As(Ⅲ).The increases in the abundance of arrA gene and putative arrA sequences of Geobacter were higher with AQDS than without *** a result,the addition of AQDS promoted microbial Fe(Ⅲ) and As(Ⅴ) release and reduction from As-bearing iron minerals into the *** results contribute to exploration of the transformation of As from As-bearing iron minerals under anaerobic conditions,thus providing insights into the bioremediation of As-contaminated soil.

关键词： Scorodite Fe(III)reduction As(V)reduction Arsenate reductase gene(arrA) AQDS

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Local and regional contributions to PM_(2.5) in the Beijing 2022 Winter Olympics infrastructure areas during haze episodes

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Frontiers of environmental Science & Engineering 2021年第6期15卷 499-509页

作者： Yue Wang Mengshuang Shi Zhaofeng Lv Huan Liu Kebin He State Key Joint Laboratory of ESPC State Environmental Protection Key Laboratory of Sources and Control of Air Pollution ComplexInternational Joint Laboratory on Low Carbon Clean Energy InnovationSchool of the EnvironmentTsinghua UniversityBeijing 100084China

The 2022 Winter Olympics is scheduled to take place in Beijing and Zhangjiakou,which were defined as OIAs(Olympic infirastructure areas)in this *** study presents the characteristics and source apportionment of PM_(2.5) in the OIAs,*** entire region of China's Mainland,except for the OIAs,was divided into 9 source regions,including four regions in the BTH(Beijing-Tianjin-Hebei)region,the four provinces surrounding the BTH and the remaining *** CAMx/PSAT,the contributions of the nine regions to the PM_(2.5) concentration in the OIAs were simulated spatially and *** simulated source apportionment results showed that the contribution of regional transportation was 48.78%,and when PM_(2.5) concentration was larger than 75μg/m^(3) central Hebei was the largest contributor with a contribution of 19.18%,followed by Tianjin,northern Hebei,Shanxi,Inner Mongolia,Shandong,southern Hebei,Henan and ***,the contribution from neighboring regions of the OIAs was 47.12%,which was nearly twice that of long-range *** episodes were analyzed,and the results presented the importance of regional transportation during severe PM_(2.5) pollution *** was also found that they were associated with differences in pollution sources between Zhangjiakou and *** transportation was the main factor affecting PM_(2.5) pollution in Zhangjiakou due to its low local *** weather with a low planetary boundary layer height and a low wind velocity prevented the local emitted pollutants in Beijing from being transported outside,and as a result,local emissions constituted a larger contribution in Beijing.

关键词： 2022 Winter Olympics PM_(2.5) Source apportionment

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Progress in quantitative research on the relationship between atmospheric oxidation and air quality

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Journal of environmental Sciences 2023年第1期123卷 350-366页

作者： Yuesi Wang Xin Jin Zirui Liu Gehui Wang Guiqian Tang Keding Lu Bo Hu Shanshan Wang Guohui Li Xinqin An Chao Wang Qihou Hu Lingyan He Fenfen Zhang Yuanhang Zhang State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry(LAPC) Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China College of Earth and Planetary Sciences University of Chinese Academy of SciencesBeijing 100049China 3 State Key Joint Laboratory or Environmental Simul ation and Pollution Control College of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China Key Lab of Geophysical Information System of the Ministry of Education School of Geographic SciencesEast China Normal UniversityShanghai 200241China Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention(LAP3) Department of Environmental Science and EngineeringFudan UniversityShanghai 201203China Key Lab of Aerosol Chemistry and Physics State Key Laboratory of Loess and Quaternary GeologyInstitute of Earth EnvironmentChinese Academy of SciencesXi’an 710061China Institute of Atmospheric Composition and Environmental Meteorology Chinese Academy of Meteorological SciencesBeijing 100081China Key Lab of Environmental Optics and Technology Anhui Institute of Optics and Fine MechanicsHefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China

Atmospheric oxidizing capacity(AOC)is an essential driving force of troposphere chemistry and self-cleaning,but the definition of AOC and its quantitative representation remain *** by national demand for air pollution control in recent years,Chinese scholars have carried out studies on theories of atmospheric chemistry and have made considerable progress in AOC *** paper will give a brief review of these ***,AOC indexes were established that represent apparent atmospheric oxidizing ability(AOIe)and potential atmospheric oxidizing ability(AOIp)based on aspects of macrothermodynamics and microdynamics,respectively.A closed study refined the quantitative contributions of heterogeneous chemistry to AOC in Beijing,and these AOC methods were further applied in Beijing-Tianjin-Hebei and key areas across the *** addition,the detection of ground or vertical profiles for atmospheric OH·,HO_(2)·,NO_(3)·radicals and reservoir molecules can now be obtained with domestic instruments in diverse ***,laboratory smoke chamber simulations revealed heterogeneous processes involving reactions of O_(3)and NO_(2),which are typical oxidants in the surface/interface atmosphere,and the evolutionary and budgetary implications of atmospheric oxidants reacting under multispecies,multiphase and multi-interface conditions were ***,based on the GRAPES-CUACE adjoint model improved by Chinese scholars,simulations of key substances affecting atmospheric oxidation and secondary organic and inorganic aerosol formation have been *** numerical simulations of AOIe and AOIp were performed,and regional coordination of AOC was *** optimized plan for controlling O_(3)and PM2.5was analyzed by scenario simulation.

关键词： Atmospheric oxidizing capacity(AOC) Quantitative index Free radicals Observation and modeling Air quality

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Enhancing Methane Production and Interspecies Electron Transfer of Anaerobic Granular Sludge by the Immobilization of Magnetic Biochar

SSRN

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SSRN 2023年

Supplementation of conductive materials has been proved to be a promising approach for enhancing microbial interspecies electron transfer (IET) in anaerobic digestion systems. In this study, magnetic bamboo-based biochar synthesized at temperatures of 400–800 ºC via a ball milling/carbonization method was immobilized in mature anaerobic granular sludge (AGS), which aimed to enhance methane production by improving the IET process between syntrophic microbial communities in the inner AGS. Results showed that the immobilization of magnetic biochar in the inner AGS increased glucotrophic and acetotrophic methane production by 69.54–77.56% and 39.96–54.92%, respectively. Magnetic biochar prepared at 800 ºC possessed superior electron charge/discharge capacity (36.66 F/g) with more Fe serving as electroactive sites (0.37 g/g magnetic biochar), which showed the highest promotion of methane production of AGS. After immobilization with magnetic biochar, the conductivity of AGS increased by 52.13–87.32%. Furthermore, both the binding of magnetic biochar with extracellular polymeric substance (EPS) and the increase of riboflavin in EPS helped to increase the capacitance and decrease the electron transfer resistance of the EPS, which could support the establishment of an efficient IET process in the inner AGS. In addition, the immobilization of magnetic biochar could promote the production of volatile fatty acids by 15.36–22.50%. All these improvements may jointly lead to the enhanced methane production capacity of AGS. This study provided a fundamental understanding of the role of incorporated magnetic biochar in AGS in promoting anaerobic digestion performance. © 2023, The Authors. All rights reserved.

关键词： Anaerobic digestion

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