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Oxidation Mechanism and Toxicity Evolution of Linalool,a Typical Indoor Volatile Chemical Product

environment & Health 2024年第7期2卷 486-498页

作者： Zihao Fu Song Guo Ying Yu Hong-Bin Xie Shiyu Li Daqi Lv Putian Zhou Kai Song Zheng Chen Rui Tan Kun Hu Ruizhe Shen Maosheng Yao Min Hu State Key Joint Laboratory of Environmental Simulation and Pollution Control International Joint Laboratory for Regional Pollution ControlMinistry of Education(IJRC)College of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China Collaborative Innovation Center of Atmospheric Environment and Equipment Technology Nanjing University of Information Science&TechnologyNanjing 210044China Key Laboratory of Industrial Ecology and Environmental Engineering(Ministry of Education) School of Environmental Science and TechnologyDalian University of TechnologyDalian 116024China Institute for Atmospheric and Earth System Research/Physics Faculty of ScienceUniversity of HelsinkiP.O.Box 64FIN-00014 HelsinkiFinland

Linalool,a high-reactivity volatile chemical product(VCP)commonly found in cleaning products and disinfectants,is increasingly recognized as an emerging contaminant,especially in indoor *** the gas-phase oxidation mechanism of linalool is crucial for assessing its impact on atmospheric chemistry and human *** quantum chemical calculations and computational toxicology simulations,we investigated the atmospheric transformation and toxicity evolution of linalool under low and high NO/HO_(2)·levels,representing indoor and outdoor *** findings reveal that linalool can undergo the novel mechanisms involving concerted peroxy(RO_(2)·)and alkoxy radical(RO·)modulated autoxidation,particularly emphasizing the importance of cyclization reactions *** expands the widely known RO_(2)·-dominated H-shift-driven autoxidation and proposes a generalized autoxidation mechanism that leads to the formation of low-volatility secondary organic aerosol(SOA)*** analysis shows that over half of transformation products(TPs)exhibited higher carcinogenicity and respiratory toxicity compared to *** also propose time-dependent toxic effects of TPs to assess their long-term *** results indicate that the strong indoor emission coupled with slow consumption rates lead to significant health risks under an indoor *** results highlight complex indoor air chemistry and health concerns regarding persistent toxic products during indoor cleaning,which involves the use of linalool or other VCPs.

关键词： volatile chemical products(VCPs) peroxy radicals(RO_(2)·) atmospheric autoxidation secondary organic aerosol(SOA) computational toxicology

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The Response of Microbial Compositions and Functions to Chronic Single and Multiple Antibiotic Exposure by Batch Experiment

SSRN

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SSRN 2023年

作者： Li, Siling Chen, Junwen Zhao, Jian Qi, Weixiao Liu, Huijuan Center for Water and Ecology State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua University Beijing100084 China

Understanding the response of the microbial community to external disturbances such as micropollutants is vital for ecological risk evaluation. In this study, the effect of chronic antibiotic exposure on community compositions and functions was investigated by two batch experiments. The first experiment investigated the effect of chronic sulfamethoxazole (SMX) exposure, while the second investigated the combined effect of dissolved organic matter (DOM) sources and multi-antibiotic exposure. The results showed that the community responses to chronic antibiotic exposure depended on the dynamic balance among community resistance, adaptation, recovery, and selection, leading to nonlinear composition diversity variations. The disturbance strength of chronic SMX exposure increased with concentration (0.5–50 μg/L). However, complex sources and structures of coexisting organic matter might delay the disturbance by elevating metabolic activity and generating functional redundancy. Especially, when nutrient was a limiting factor, the disturbance strength by DOM source was greater than that by chronic antibiotic exposure. The resistance of abundant taxa to external distributions resulted in a low explanation of community diversity, while rare taxa played key roles in response to community variation and thereby affected community assembly. Long-term SMX exposure reduced the number of key species and favored the deterministic assembly process by 21%. However, elevated community adaptability might weaken the influence of antibiotic selection. Chronic SMX exposure elevated the relative abundance of sulfonamide resistance genes (sul1, sul2) by a factor of 1.2–4.3, while that of nitrogen-fixing genes (nifH, nifK) and the metabolic pathways related to the toluene, ethylbenzene, and dioxin degradation decreased. However, the combined influence of DOM sources and multi-antibiotic exposure barely caused the difference in the genes linking to element metabolism and drug resistance of mic

关键词： Antibiotics

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Evaluation of laboratory and environmental exposure systems for protein modification upon gas pollutants and environmental factors

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Journal of environmental Sciences 2024年第9期143卷 213-223页

作者： Zhiwei Pan ShiyiWu Qiaoze Zhu Fobang Liu Yongjian Liang Chenglei Pei Haoyu Jiang Yingyi Zhang Senchao Lai The Key Lab of Pollution Control and Ecosystem Restoration in Industry Clusters Ministry of EducationSchool of Environment and EnergySouth China University of TechnologyGuangzhou 510006China Department of Environmental Science and Engineering Xi’an Jiaotong UniversityXi’an 710049China Guangzhou Sub-branch of Guangdong Ecological and Environmental Monitoring Center Guangzhou 510006China State Key Laboratory of Organic Geochemistry Guangdong Key Laboratory of Environmental Protection and Resources Utilizationand Joint Laboratory of the Guangdong-Hong Kong-Macao Greater Bay Area for the EnvironmentGuangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou 510640China School of Marine Sciences Sun Yat-sen UniversityZhuhai 519082China

Chemical modifications of proteins induced by ambient ozone(O_(3))and nitrogen oxides(NOx)are of public health concerns due to their potential to trigger respiratory *** laboratory and environmental exposure systems have been widely used to investigate their relevant mechanism in the *** bovine serum albumin(BSA)as a model protein,we evaluated the two systems and aimed to reduce the uncertainties of both the reactants and products in the corresponding kinetic *** the laboratory simulation system,the generated gaseous pollutants showed negligible *** layers of BSA were coated on the flow tube with protein extraction recovery of 87.4%.For environmental exposure experiment,quartz fiber filter was selected as the upper filter with low gaseous O_(3)(8.0%)and NO_(2)(1.7%)losses,and cellulose acetate filter was appropriate for the lower filter with protein extraction efficiency of 95.2%.The protein degradation process was observed without the exposure to atmospheric oxidants and contributed to the loss of protein monomer mass fractions,while environmental factors(e.g.,molecular oxygen and ultraviolet)may cause greater protein monomer *** on the evaluation,the study exemplarily applied the two systems to protein modification and both showed that O_(3) promotes the protein oligomerization and nitration,while increased temperature can accelerate the oligomerization and increased relative humidity can inhibit the nitration in the environmental exposure *** developed laboratory and environmental systems are suitable for studying protein modifications formed under different atmospheric conditions.A combination of the two will further reveal the actual mechanism of protein modifications.

关键词： Protein modification laboratory simulation environmental exposure Oligomerization Nitration

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Optimization of Regional Energy-Water Nexus System Under Multiple Uncertainties 15th

Optimization of Regional Energy-Water Nexus System Under Mul...

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15th International Conference on environmental Science and Development, ICESD 2024

作者： Liu, Ruoyan Li, Yongping Huang, Guohe Zhou, Yanxiao Li, Yanfeng State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Beijing Normal University Beijing China Institute for Energy Environment and Sustainable Communities University of Regina ReginaSask Canada

ISBN: (纸本)9783031886829

In this paper, an interval chance-constrained programming (ICCP) method is proposed for collaborative energy-water nexus (EWN) system under multiple uncertainties. This method can solve the uncertainties expressed as probability distribution and interval. An ICCP-based energy-water nexus (ICCP-EWN) model is established, where 15 scenarios are designed for assessing the effect of water cycle coefficients and constraint violation risk. The results show that: (i) coal would remain the main energy sources for future energy supply, but the proportion of clean energy (e.g., natural gas, biomass) in the future power generation structure would significantly increase (about 15.6%);(ii) the water withdrawal of power generation in the energy system would be largest, where thermal power generation would have the largest proportion of water withdrawal, accounting for 85.0%;(iii) the decreasing α level and increasing p level will bring higher system benefits, and the reliability of the system would be reduced. These results can help determine the energy mix of a planned area, improve security of energy supply, and make trade-off between system benefits and the risk of violating constraints. © The Author(s), under exclusive license to Springer Nature Switzerland AG 2025.

关键词： Normal distribution

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Annual nonmethane hydrocarbon trends in Beijing from 2000 to 2019

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Journal of environmental Sciences 2022年第2期34卷 210-217页

作者： Dan Yao Guiqian Tang Jie Sun Yinghong Wang Yuan Yang Yiming Wang Baoxian Liu Hong He Yuesi Wang Center for Excellence in Regional Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China School of Environment Tsinghua UniversityBeijing 100084China Beijing Key Laboratory of Airborne Particulate Matter Monitoring Technology Beijing Municipal Environmental Monitoring CenterBeijing 100048China Uniuersity of Chinese Academy of Sciences Beijing 100049China

High loads of ground-level ozone have occurred with the implementation of the Air pollution Prevention and control Action ***,the long temporal variation in precursor nonmethane hydrocarbons(NMHCs)has rarely been *** this study,we examined the evolution of NMHCs in Beijing based on ambient measurements from 2000 to *** results indicated that the annual variation of ambient NMHCs during 2000 and 2019 could be divided into two *** mixing ratios of NMHCs rapidly rose during 2000 and 2009(1.76 ppbv/year)but exhibited a downward trend from 2009 to 2019 at rate of 0.80 ppbv/***,the notable decrease in alkenes and aromatics after 2009 led to a sharp decrease in the propylene-equivalent concentration(PEC)(-0.80 ppbv/year).Implementation of emission reduction measures in Beijing have effectively reduced the contribution of vehicle-related sources,but the contribution of solvent usage and fuel consumption increased,which will become the focus of VOC control in Beijing in the future.

关键词： Beijing NMHCs Reactivity Temporal variation

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Corrigendum to "Landscape ecological risk assessment and driving factors analysis based on optimal spatial scales in Luan River Basin, China" [Ecol. Indic. 169 (2024) 112821] (Ecological Indicators (2024) 169, (S1470160X24012780), (10.1016/***.2024.112821))

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Ecological Indicators 2025年 173卷

作者： Yang, Nijuan Zhang, Ting Li, Jianzhu Feng, Ping Yang, Nina State Key Laboratory of Hydraulic Engineering Intelligent Construction and Operation Tianjin University Tianjin300350 China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Tsinghua University Beijing100084 China

The authors regret "the incorrect use of Figure 1 in the paper. The original figure has now been replaced with the revised figure."[Figure presented] Revised Figure 1 The authors would like to apologise for ...

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Global methyl halide emissions from biomass burning during 2003-2021

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environmental Science and Ecotechnology 2023年第2期14卷 79-86页

作者： Xiaoyi Hu Di Chen Liting Hu Bowei Li Xinhe Li Xuekun Fang College of Environmental&Resource Sciences Zhejiang UniversityHangzhouZhejiang310058PR China State Key Joint Laboratory for Environmental Simulation and Pollution Control College of Environmental Sciences and EngineeringPeking UniversityBeijing100871PR China Center for Global Change Science Massachusetts Institute of TechnologyCambridgeMA02139USA

Methyl halides(CH3Cl,CH3Br,and CH3I)are ozone-depleting *** burning(BB)is an important source of methyl *** temporal variations and global spatial distribution of BB methyl halide emissions are ***,global methyl halide emissions from BB during 2003e2021 were estimated based on satellite data.A significant decreasing trend(p<0.01)in global methyl halide emissions from BB was found between 2003 and 2021,with CH3Cl emissions decreasing from 302 to 220 Gg yr^(-1),CH3Br emissions decreasing from 16.5 to 11.7 Gg yr^(-1),and CH3I emissions decreasing from 8.9 to 6.1 Gg yr^(-1).From a latitudinal perspective,the northern high-latitude region(60e90N)was the only latitude zone with significant increases in BB methyl halide emissions(p<0.01).Based on an analysis of the drivers of BB methyl halide emissions,emissions from cropland,grassland,and shrubland fires were more correlated with the burned area,while BB emissions from forest fires were more correlated with the emissions per unit burned *** non-BB emissions of CH3Cl increased from 4749 Gg yr^(-1)in 2003 to 4882 Gg yr^(-1)in 2020,while those of CH3Br decreased from 136 Gg yr^(-1)in 2003 to 118 Gg yr^(-1)in 2020(global total CH3I emissions are not available).The finding indicates that global CH3Cl and CH3Br emissions from sources besides BB increased and decreased during *** on our findings,not only searching for unknown sources is important,but also re-evaluating known sources is necessary for addressing methyl halide emissions.

关键词： Methyl halides Biomass burning Emission inventory Global budget Ozone depletion

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Biodiversity conservation and ecological restoration of vulnerable ecosystems in the Anthropocene

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Journal of Plant Ecology 2024年第5期17卷 1-4页

作者： Zhonghua Ning Tian Xie Xinxin Wang Zhenchang Zhu Cong Chen Baoshan Cui Key Laboratory of Ecological Protection in the Yellow River Basin of National Forestry and Grassland Administration School of Ecology and Nature ConservationBeijing Forestry UniversityBeijing 100083China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentBeijing Normal UniversityBeijing 100875China Ministry of Education Key Laboratory for Biodiversity Science and Ecological Engineering National Observations and Research Station for Wetland Ecosystems of the Yangtze EstuarySchool of Life ScienceFudan UniversityShanghai 200433China School of Ecology Environment and ResourcesGuangdong University of TechnologyGuangzhou 510006China Research and Development Center for Watershed Environmental Eco-engineering Advanced Institute of Natural SciencesBeijing Normal UniversityZhuhai 519087China

This editorial summarizes the contributions to the Special Issue Biodiversity conservation and ecological restoration of vulnerable ecosystems in the Anthropocene',established under the Journal of Plant Ecology.

关键词： Biodiversity ecosystems restoration

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Antibiotic resistance genes in manure-amended paddy soils across eastern China:Occurrence and influencing factors

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Frontiers of environmental Science & Engineering 2022年第7期16卷 101-111页

作者： Yuwei Guo Xian Xiao Yuan Zhao Jianguo Liu Jizhong Zhou Bo Sun Yuting Liang School of Environmental and Safety Engineering Changzhou UniversityChangzhou213164China State Key Laboratory of Soil and Sustainable Agriculture Institute of Soil ScienceChinese Academy of SciencesNanjing210008China Institute for Environmental Genomics Department of Microbiology and Plant Biologyand School of Civil Engineering and Environmental SciencesUniversity of OklahomaNormanOK73019USA State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing100084China Earth and Environmental Sciences Lawrence Berkeley National LaboratoryBerkeleyCA94270USA

Pig manure,rich in antibiotics and metals,is widely applied in paddy fields as a soil conditioner,triggering the proliferation of antibiotic resistance genes(ARGs)in ***,comprehensive studies on the effects of manure fertilization on the abundance of ARGs and their influencing factors are still ***,pig manure and manure-amended and inorganic-amended soils were collected from 11 rice-cropping regions in eastern China,and the accumulation of antibiotics,metals,and ARGs was assessed *** results showed that manure fertilization led to antibiotic residues and increased the metal content(i.e.,Zn,Cu,Ni,and Cr).Tetracycline and sulfonamide resistance genes(tetM,tetO,sul1,and sul2)were also significantly enhanced with manure *** to variance partitioning analysis,the most important factors that individually influenced ARGs were soil physicochemical properties,accounting for 12%of the *** correlations between soil nutrients and ARGs indicated that manure application enhanced the growth of resistant microorganisms by supplying more *** and antibiotics contributed 9%and 5%to the variations in ARGs,*** co-occurrence also increased the enrichment of ARGs,as their interactions accounted for 2%of the variation in ***,Cu was significantly related to most ARGs in the soil(r=0.26–0.52,p<0.05).Sulfapyridine was significantly related to sul2,and tetracycline resistance genes were positively related to *** study highlighted the risks of antibiotic and ARG accumulation with manure fertilization and shed light on the essential influencing factors of ARGs in paddy soils.

关键词： Pig manure Antibiotics Metals Antibiotic resistance genes Paddy fields

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An Ecological-Network Input–Output Clustering Model for Analyzing CO2 Emission System 7th

An Ecological-Network Input–Output Clustering Model for Ana...

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Proceedings of 2022 7th International Conference on environmental Engineering and Sustainable Development (CEESD 2022)

作者： Wang, P.P. Huang, G.H. Li, Y.P. State Key Joint Laboratory of Environmental Simulation and Pollution Control China-Canada Center for Energy Environment and Ecology Research UR-BNU School of Environment Beijing Normal University Beijing100875 China Faculty of Engineering and Applied Science University of Regina ReginaSKS4S 0A2 Canada

ISBN: (纸本)9783031281921

Excessive carbon dioxide (CO2) emission has been challenges to regional sustainable development. In this study, an ecological-network input–output clustering (ENIOC) model is developed to analyze CO2 emission system. ENIOC can recognize the complex characteristics and relationships within CO2 emission system from network and statistical perspectives. ENIOC is applied to Jiangsu. Some major findings are as follows: (i) electricity-heat supply and metal smelting industries are dominant CO2 emission contributors (i.e., 16.4% and 12.3% of the total CO2 emission, respectively);also, they provide plenty of carbon-intensive products for supporting construction and heavy industries;(ii) the CO2 emission system is relatively unstable;optimize the structure of key pathways (e.g., mining → metal smelting → metal products) could mitigate CO2 emission across the supply chain;(iii) CO2 mitigation policy should focus on the sectors in cluster 2 (e.g., chemical, metal product and equipment industries) to reduce their dependency on carbon-intensive products from other sectors;CO2 mitigation policy also should focus on metal smelting and electricity-heat supply industries (i.e., the sectors in cluster 3) to improve their efficiencies of energy use. © 2023, The Author(s), under exclusive license to Springer Nature Switzerland AG.

关键词： Carbon dioxide

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