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The “neighbor avoidance effect” of microplastics on bacterial and fungal diversity and communities in different soil horizons

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environmental Science and Ecotechnology 2021年第4期8卷 13-21页

作者： Hong Yu Ying Zhang Wenbing Tan State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing100012China State Environmental Protection Key Laboratory of Simulation and Control of Groundwater Pollution Chinese Research Academy of Environmental SciencesBeijing100012China

Microplastics are a new type of environmental pollutant,and pose a serious threat to soil *** is important to study microplastics effects on soil microorganisms to better understand their effects on terrestrial ***,we collected soil and microplastic samples from corn,pepper,peanut and cucumber fields in Shunyi District,Beijing,China,and used Illumina MiSeq high-throughput sequencing technology to analyze bacterial and fungal community composition and *** focused on microplastic surface and its surrounding“rhizosphere-like”soil in the 0e10 cm(humus)and 10e20 cm(eluvial)deep *** richness and diversity on microplastic surface were significantly lower than those in surrounding“rhizosphere-like”soil,and microbial richness and diversity were reduced to a greater extent in the humus horizon than in the eluvial *** likely enriched the microbes involved in their *** relative abundance levels of Cyanobacteria and Basidiomycota on microplastic surfaces were significantly higher than those in surrounding“rhizosphere-like”soil,while the relative abundance levels of Acidobacteria,Chloreflexi,and Mortierellomycota were higher in“rhizosphere-like”***,the relative abundance levels of pathways related to human diseases,animal pathogen,and fungal parasites were significantly higher on microplastic surfaces than in“rhizosphere-like”*** results show that the microbial diversity,richness,community structure and function between microplastic surfaces and surrounding“rhizosphere-like”soil are significantly different,leading to a“rhizosphere-like neighbor avoidance effect”between microplastic surfaces and the surrounding soil.

关键词： Microplastics Microbial diversity Community structure Rhizosphere Metabolic function

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Toward sustainable food systems: global initiatives and innovations

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Frontiers of Agricultural Science and Engineering 2024年第1期11卷 197-209页

作者： Xiangwen FAN Xiaomeng ZHANG Xiaofei WU Wenqi MA Zhaohai BAI Lin MA State Key Lab Pollution Control&Resource Reuse School of EnvironmentNanjing UniversityNanjing 210023China College of Resources and Environmental Sciences Hebei Agricultural UniversityBaoding 071000China College of Food Science and Biology Hebei University of Science and TechnologyShijiazhuang 050018China

A recent UN Sustainable Development Goals(SDGs) analysis indicated a significant regression in the global SDG goal scores, particularly in SDG 2—Zero Hunger. The emissions of environmental pollution caused by meeting food demands have prompted some countries to intensify their climate change mitigation efforts. These circumstances have introduced significant uncertainty to the future global sustainable food development. Additionally, a notable global challenge is the persistence of hidden hunger, primarily characterized by the insufficient consumption of high-quality animal protein. Addressing this issue would necessitate increased environmental costs to attain high-quality food security. The future food system presents a significant challenge in coordinating food security, food quality and environmental quality. This article presents a comprehensive review and proposes a three-step strategy for future agricultural development based on food security, quality, and environmental aspects. This is a novel food system transfer strategy, as it concurrently addresses both global food security and environmental thresholds. It involves the construction of an efficient food system that operates within the constraints of environmental limits. The objective is to align with global SDG indicators and to maintain natural resource consumption and pollutant emissions within planetary boundaries.

关键词： Agricultural green development food system food production optimization transform pathways

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Impacts of Comorbidity and Mental Shock on Organic Micropollutants in Surface Water During and After the First Wave of COVID-19 Pandemic in Wuhan (2019–2021), China

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Engineering 2024年第6期37卷 40-48页

作者： Jian Zhao Jin Kang Xiaofeng Cao Rui Bian Gang Liu Shengchao Hu Xinghua Wu Chong Li Dianchang Wang Weixiao Qi Cunrui Huang Huijuan Liu Jiuhui Qu Center for Water and Ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China Hubei Provincial Research Institute of Environmental Science Wuhan 430072China Key Laboratory of Drinking Water Science and Technology Research Centre for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Sanitary Engineering Department of Water ManagementFaculty of Civil Engineering and GeosciencesDelft University of TechnologyDelft 2600 GAThe Netherlands China Three Gorges Corporation Wuhan 430010China Vanke School of Public Health Tsinghua UniversityBeijing 100084China

The first pandemic wave of coronavirus disease 2019(COVID-19)induced a considerable increase in several antivirals and antibiotics in surface *** common symptoms of COVID-19 are viral and bacterial infections,while comorbidities(e.g.,hypertension and diabetes)and mental shock(e.g.,insomnia and anxiety)are ***,little is known about the long-term impacts of comorbidities and mental shock on organic micropollutants(OMPs)in surface ***,we monitored 114 OMPs in surface water and wastewater treatment plants(WWTPs)in Wuhan,China,between 2019 and *** pandemic-induced OMP pollution in surface water was confirmed by significant increases in 26 OMP *** increases in four antihypertensives and one diabetic drug suggest that the treatment of comorbidities may induce OMP ***,cotinine(a metabolite of nicotine)increased 155 times to 187 ngL1,which might be associated with increased ***,the increases in zolpidem and sulpiride might be the result of worsened insomnia and ***,it is reasonable to note that mental-health protecting drugs/behavior also contributed to OMP *** the observed OMPs,telmisartan,lopinavir,and ritonavir were associated with significantly higher ecological risks because of their limited WWTP-removal rate and high *** study provides new insights into the effects of comorbidities and mental shock on OMPs in surface water during a pandemic and highlights the need to monitor the fate of related pharmaceuticals in the aquatic environment and to improve their removal efficiencies in WWTPs。

关键词： Coronavirus disease 2019 Comorbidities Mental shock Micropollutant Surface water

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Methane and nitrous oxide emissions from municipal wastewater treatment plants in China:A plant-level and technology-specific study

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environmental Science and Ecotechnology 2024年第4期20卷 123-130页

作者： Haiyan Li Liangfang You He Du Bowen Yu Lu Lu Bo Zheng Qiang Zhang Kebin He Nanqi Ren School of Civil and Environmental Engineering Harbin Institute of TechnologyShenzhen518055China Shenzhen Key Laboratory of Ecological Remediation and Carbon Sequestration Institute of Environment and EcologyTsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen518055China Ministry of Education Key Laboratory for Earth System Modeling Department of Earth System ScienceTsinghua UniversityBeijing100084China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing100084China

Wastewater treatment is an important source of greenhouse gases(GHGs).Yet large uncertainties remain in the quantification of GHG emissions from municipal wastewater treatment plants(MWWTPs)in China.A high-resolution and technology-specific emission inventory is still lacking to support mitigation strategies of *** we develop a plant-level and technology-based MWWTP emission inventory for China covering 8703 plants and 19 treatment technology categories by compiling and harmonizing the most up-to-date facility-level ***'s methane(CH_(4))and nitrous oxide(N_(2)O)emissions from MWWTPs in 2020 are estimated to be 150.6 Gg and 22.0 Gg,respectively,with the uncertainty range of-30%to 37%and-30%to 26%at 95%confidence *** find an emission inequality across cities,with the richest cities emitting two times more CH_(4)and N_(2)O per capita from municipal wastewater treatment than the poorest *** emitted CH_(4)and N_(2)O are dominated by Anaerobic/Anoxic/Oxic-,Sequencing Batch Reactor-,Oxidation Ditch-,and Anoxic/Oxic-based MWWTPs of less than 20 years *** the relatively young age structure of China's MWWTPs,the committed emissions highlight the importance of reducing on-site GHG emissions by optimization of operating conditions and innovation *** emission differences among our estimates,previous studies,and the Intergovernmental Panel on Climate Change guidelines are largely attributed to the uncertainties in emission factors,implying the urgent need for more plant-integrated measurements to improve the accuracy of emission accounting.

关键词： Methane Nitrous oxide Emissions Municipal wastewater treatment plants

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Extruded monolith MnO_(x)-CeO_(2)-TiO_(2) catalyst for NH_(3)-SCR of low temperature flue gas from an industry boiler:Deactivation and recovery

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Journal of Rare Earths 2023年第9期41卷 1336-1343,I0002页

作者： Wei Shi Jingjing Liu Ying Zhu Lin Zhao Yonggang Wang Zhaohuan Cheng Xueping Peng Xiaoyan Shi Yunbo Yu Hong He State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing100085China University of Chinese Academy of Sciences Beijing 100049China Center for Excellence in Regional Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China Tianjin Cement Industry Design&Research Institute Co LtdTianjin 300400China

The selective catalytic reduction(SCR) of NO_(x) with NH_(3)(NH_(3)-SCR) technology has been widely applied for reducing NO_(x) emissions from stationary and mobile *** this work,the extruded monolith MnO_(x)-CeO_(2)-TiO_(2) catalyst was installed in a cement kiln for NH_(3)-SCR of NO_(x),where the flue gas temperature was 110-140℃.It is found that the monolith catalyst is severely deactivated after operating for about 200 h with almost no NO_(x) conversion at 160℃ under GHSV of 50000 h^(-1),while the fresh monolith catalyst remains 60% NO_(x) *** electron microscopy-energy dispersive spectroscopy(SEM-EDS),X-ray photoelectron spectroscopy(XPS),temperature-programmed desorption of SO_(2)(SO_(2)-TPD) and thermogravimetric-differential thermal analysis(TG-DTG) experiments reveal that both MnO_(x) and CeO_(2) oxides in monolith are severely sulfated to manganese sulfate and cerium sulfate,and the external monolith walls are covered by massive ceria sulfate and little ammonium *** situ diffuse reflectance infrared Fourier trans form spectroscopy(DRIFTS) analysis demonstrates that the formation of nitrates at low temperatures is inhibited due to the occupation of active sites in MnO_(x)-CeO_(2)-TiO_(2) by sulfates,resulting in the decrease of low temperature *** washing with water,the activity of deactivated monolith catalyst can be partially recovered,together with significant loss of manganese and cerium from monolith.

关键词： Low temperature NH_(3)-SCR MnO_(x)-CeO_(2)-TiO_(2) Extruded monolith catalysts Deactivation Recovery Rare earths

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Phthalate levels in Chinese residences:Seasonal and regional variations and the implication on human exposure

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National Science Open 2023年第6期2卷 65-79页

作者： Yatai Li Jing Hou Zukun Wang Xilei Dai Yuexia Sun Junjie Liu Yingjun Liu Key Joint Laboratory of Environmental Simulation and Pollution Control College of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China College of Public Health Zhengzhou UniversityZhengzhou 450001China Tianjin Key Lab of Indoor Air Environmental Quality Control School of Environmental Science and EngineeringTianjin UniversityTianjin 300072China College of Design and Engineering National University of SingaporeSingapore 117566Singapore Center for Environment and Health Peking UniversityBeijing 100871China

Indoor pollution of manmade semivolatile organic compounds(SVOCs)such as phthalates are a growing threat to human *** we summarize the dust-phase phthalate concentrations in Chinese residences reported from 2011 to 2021and simulate corresponding airborne concentrations based on equilibrium *** simulation considers seasonal and regional variations in indoor temperature and PM_(2.5)concentration,in contrast to the common practice of using constant *** show that variations in these two environmental factors lead to up to ten-and six-fold variations in the monthly median gas-and particle-phase concentrations of phthalates,respectively,in residences in individual climate *** higher-vaporpressure species di-n-butyl phthalate and di-isobutyl phthalate,the resultant seasonal and regional variations in aggregate nondiet intake can reach six-and three-fold,*** results have important implications on exposure assessment of SVOCs and epidemiological evaluation of their health effects.

关键词： SVOCs indoor air temperature dust

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Cerium-tungsten oxides supported on activated red mud for the selective catalytic reduction of NO_(x)

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Green Energy & Environment 2023年第1期8卷 173-182页

作者： Qiuzhun Chen Dong Wang Chuan Gao Bin Wang Shengli Niu Gaiju Zhao Yue Peng Junhua Li Chunmei Lu John Crittenden National Engineering Laboratory for Coal-Burning Pollutants Emission Reduction School of Energy and Power EngineeringShandong UniversityJinan250061China State Key Joint Laboratory of Environment Simulation and Pollution Control National Engineering Laboratory for Multi Flue Gas Pollution Control Technology and EquipmentSchool of EnvironmentTsinghua UniversityBeijing100084China Brook Byers Institute for Sustainable Systems and School of Civil and Environmental Engineering Georgia Institute of Technology828 West Peachtree StreetAtlantaGA30332United States Energy Institute Qilu University of Technology(Shandong Academy of Sciences)Jinan250013ShandongChina

Activated red mud(RM)has been proved to be a promising base material for the selective catalysis reduction(SCR)of *** inherent low reducibility and acidity limited its low-temperature *** this work,molybdenum oxide,tungsten oxide,and cerium oxide were used to reconfigure the redox sites and acid sites of red mud based *** activated red mud was reconfigured by cerium-tungsten oxide(Ce-W@RM),the NOx conversion kept above 90%at 219-480℃.The existence of Ce^(3+)/Ce^(4+) redox electron pairs provided more surface adsorbed oxygen(O_(α)) and served as a redox *** interactions between Ce,W species and Fe oxide in red mud occurred,which led to the formation of unsaturated chemical bond and promoted the activation of adsorbed NH_(3) ***_(3) and Ce_(2)(WO_(4))_(3)(formed by solid-state reaction between Ce and W species)could provide more Brønsted acid sites(W-O modes of WO_(3),W=O or W-O-W modes of Ce_(2)(WO_(4))_(3)).CeO_(2) species could provide more Lewis acid *** Langmuir-Hinshelwood(L-H)routes and Eley-Rideal(E-R)routes occurred in the low-temperature SCR reaction on the Ce-W@RM ***_(4)^(+) species on Brønsted acid sites,NH_(3) species on Lewis acid sites,bidentate nitrate and bridging nitrate species were key active intermediates species.

关键词： Air pollution control NOx Selective catalytic reduction Cerium Tungsten

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Estimation for ammonia emissions at county level in China from 2013 to 2018

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Science China Earth Sciences 2022年第6期65卷 1116-1127页

作者： Wenling LIAO Mingxu LIU Xin HUANG Tiantian WANG Zhenying XU Fang SHANG Yu SONG Xuhui CAI Hongsheng ZHANG Ling KANG Tong ZHU State Key Joint Laboratory of Environmental Simulation and Pollution Control Department of Environmental SciencePeking UniversityBeijing 100871China Joint International Research Laboratory of Atmospheric and Earth System Sciences School of Atmospheric SciencesNanjing UniversityNanjing 210023China Laboratory for Atmosphere-Ocean Studies Department of Atmospheric and Oceanic ScienceSchool of PhysicsPeking UniversityBeijing 100871China

Ammonia (NH_(3)) can interact with other trace chemicals in the atmosphere,significantly impacting atmospheric chemistry and global climate *** is a largely agricultural country with high consumption of nitrogen fertilizer and large livestock herds,resulting in high NH_(3) *** this study,a comprehensive county-level inventory of Chinese NH_(3) emissions from 2013 to 2018 was *** on previous research,an estimate of NH_(3) emissions from household coal combustion was added to the *** estimation of emissions from open biomass burning was improved by using a method based on fire radiative energy (FRE).The total NH_(3) emissions in China increased from 2013 (9.64 Tg) to 2015 (9.75 Tg),and then decreased to 9.12 Tg in *** from fossil fuels reached a peak value in 2018,accounting for 8.4%of total emissions,while fertilizer application and livestock waste were responsible for fewer emissions than in previous years,accounting for 27.7%and 49.9%of the total from non-fossil fuel sources,*** highest emission rates were in central and southwestern ***,NH_(3) emissions peaked in spring and *** inventory had a 1-km spatial resolution and a monthly temporal resolution,which confirmed its suitability for global and regional air quality simulations.

关键词： Ammonia emission Seasonal variations Spatial distribution Policy Suggestions China

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Recent advances in single-atom catalysts(SACs)for photocatalytic applications

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Materials Reports(Energy) 2024年第3期4卷 1-18页

作者： Tingcha Wei Jing Zhou Xiaoqiang An School of Physics South China Normal UniversityGuangzhou510006China MIIT Key Laboratory of Aerospace Information Materials and Physics College of PhysicsNanjing University of Aeronautics and AstronauticsNanjing211106China Key Laboratory of Songliao Aquatic Environment Ministry of EducationSchool of Municipal and Environmental EngineeringJilin Jianzhu UniversityChangchun130118China Center for Water and Ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing100084China

Artificial photocatalysis represents a hopeful avenue for tackling the global crisis of environmental and energy *** crux of industrial application in photocatalysis lies in efficient photocatalysts that can inhibit the recombination of photogenerated charge carriers,thereby boost the efficiency of chemical *** the past decade,single-atom catalysts(SACs)have been growing extremely rapidly and have become the forefront of photocatalysis owing to their superior utilization of metal atoms and outstanding catalytic *** this work,we provide an overview of the latest advancements and challenges in SACs for photocatalysis,focusing on the photocatalytic mechanisms,encompassing the generation,separation,migration,and surface extraction of photogenerated *** also explore the design,synthesis,and characterization of SACs and introduce the progress of SACs for photocatalytic applications,such as water splitting and CO_(2)***,we offer our personal perspectives on the opportunities and challenges of SACs in photocatalysis,aiming to provide insights into the future studies of SACs for photocatalytic applications.

关键词： Single-atom catalysts Artificial photocatalysis Water splitting CO_(2)reduction

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Solvent-free mechanochemical mild oxidation method to enhance adsorption properties of chitosan

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Frontiers of environmental Science & Engineering 2021年第6期15卷 353-366页

作者： Mohammadtaghi Vakili Wen Qiu Giovanni Cagnetta Jun Huang Gang Yu Green Intelligence Environmental School Yangtze Normal UniversityChongqing 408100China State Key Joint Laboratory of Environment Simulation and Pollution Control(SKJLESPC) Beijing Key Laboratory for Emerging Organic Contaminants Control(BKLEOC)School of EnvironmentTsinghua UniversityBeijing 100084China

Oxidation has been profitably utilized to improve some properties of ***,only solventbased oxidation procedures have been proposed so far,which are hardly feasible at industrial scale in an economic way because of product recovery *** this study,a solvent-free,rapid,and effective oxidation method is *** is based on direct solid-state reaction between chitosan and oxidant powder in a mechanochemical *** prove that by short high energy ball milling(<3 h)it is possible to achieve diverse physicochemical modifications employing different *** from polysaccharidic chain shortening,persulfate provokes high amorphization and induces formation of ketonic groups;percarbonate heightens deacetylation degree,preserving in part crystallinity;calcium peroxide merely deprotonates amino groups and increases amorphization *** tests with the azo-dye reactive red 2 show that adsorption capacity of chitosan co-milled with persulfate(974 mg/g milled product),which is the best performing adsorbent,is twice that of pristine chitosan,while adsorption rate is outstandingly boosted(125 times).

关键词： Chitosan High energy ball milling Mechanochemistry Oxidation

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