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Estimation for ammonia emissions at county level in China from 2013 to 2018

Science China Earth Sciences 2022年第6期65卷 1116-1127页

作者： Wenling LIAO Mingxu LIU Xin HUANG Tiantian WANG Zhenying XU Fang SHANG Yu SONG Xuhui CAI Hongsheng ZHANG Ling KANG Tong ZHU State Key Joint Laboratory of Environmental Simulation and Pollution Control Department of Environmental SciencePeking UniversityBeijing 100871China Joint International Research Laboratory of Atmospheric and Earth System Sciences School of Atmospheric SciencesNanjing UniversityNanjing 210023China Laboratory for Atmosphere-Ocean Studies Department of Atmospheric and Oceanic ScienceSchool of PhysicsPeking UniversityBeijing 100871China

Ammonia (NH_(3)) can interact with other trace chemicals in the atmosphere,significantly impacting atmospheric chemistry and global climate *** is a largely agricultural country with high consumption of nitrogen fertilizer and large livestock herds,resulting in high NH_(3) *** this study,a comprehensive county-level inventory of Chinese NH_(3) emissions from 2013 to 2018 was *** on previous research,an estimate of NH_(3) emissions from household coal combustion was added to the *** estimation of emissions from open biomass burning was improved by using a method based on fire radiative energy (FRE).The total NH_(3) emissions in China increased from 2013 (9.64 Tg) to 2015 (9.75 Tg),and then decreased to 9.12 Tg in *** from fossil fuels reached a peak value in 2018,accounting for 8.4%of total emissions,while fertilizer application and livestock waste were responsible for fewer emissions than in previous years,accounting for 27.7%and 49.9%of the total from non-fossil fuel sources,*** highest emission rates were in central and southwestern ***,NH_(3) emissions peaked in spring and *** inventory had a 1-km spatial resolution and a monthly temporal resolution,which confirmed its suitability for global and regional air quality simulations.

关键词： Ammonia emission Seasonal variations Spatial distribution Policy Suggestions China

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Recent advances in single-atom catalysts(SACs)for photocatalytic applications

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Materials Reports(Energy) 2024年第3期4卷 1-18页

作者： Tingcha Wei Jing Zhou Xiaoqiang An School of Physics South China Normal UniversityGuangzhou510006China MIIT Key Laboratory of Aerospace Information Materials and Physics College of PhysicsNanjing University of Aeronautics and AstronauticsNanjing211106China Key Laboratory of Songliao Aquatic Environment Ministry of EducationSchool of Municipal and Environmental EngineeringJilin Jianzhu UniversityChangchun130118China Center for Water and Ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing100084China

Artificial photocatalysis represents a hopeful avenue for tackling the global crisis of environmental and energy *** crux of industrial application in photocatalysis lies in efficient photocatalysts that can inhibit the recombination of photogenerated charge carriers,thereby boost the efficiency of chemical *** the past decade,single-atom catalysts(SACs)have been growing extremely rapidly and have become the forefront of photocatalysis owing to their superior utilization of metal atoms and outstanding catalytic *** this work,we provide an overview of the latest advancements and challenges in SACs for photocatalysis,focusing on the photocatalytic mechanisms,encompassing the generation,separation,migration,and surface extraction of photogenerated *** also explore the design,synthesis,and characterization of SACs and introduce the progress of SACs for photocatalytic applications,such as water splitting and CO_(2)***,we offer our personal perspectives on the opportunities and challenges of SACs in photocatalysis,aiming to provide insights into the future studies of SACs for photocatalytic applications.

关键词： Single-atom catalysts Artificial photocatalysis Water splitting CO_(2)reduction

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Solvent-free mechanochemical mild oxidation method to enhance adsorption properties of chitosan

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Frontiers of environmental Science & Engineering 2021年第6期15卷 353-366页

作者： Mohammadtaghi Vakili Wen Qiu Giovanni Cagnetta Jun Huang Gang Yu Green Intelligence Environmental School Yangtze Normal UniversityChongqing 408100China State Key Joint Laboratory of Environment Simulation and Pollution Control(SKJLESPC) Beijing Key Laboratory for Emerging Organic Contaminants Control(BKLEOC)School of EnvironmentTsinghua UniversityBeijing 100084China

Oxidation has been profitably utilized to improve some properties of ***,only solventbased oxidation procedures have been proposed so far,which are hardly feasible at industrial scale in an economic way because of product recovery *** this study,a solvent-free,rapid,and effective oxidation method is *** is based on direct solid-state reaction between chitosan and oxidant powder in a mechanochemical *** prove that by short high energy ball milling(<3 h)it is possible to achieve diverse physicochemical modifications employing different *** from polysaccharidic chain shortening,persulfate provokes high amorphization and induces formation of ketonic groups;percarbonate heightens deacetylation degree,preserving in part crystallinity;calcium peroxide merely deprotonates amino groups and increases amorphization *** tests with the azo-dye reactive red 2 show that adsorption capacity of chitosan co-milled with persulfate(974 mg/g milled product),which is the best performing adsorbent,is twice that of pristine chitosan,while adsorption rate is outstandingly boosted(125 times).

关键词： Chitosan High energy ball milling Mechanochemistry Oxidation

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Coordinated control of Fine-Particle and Ozone pollution by the Substantial Reduction of Nitrogen Oxides

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Engineering 2022年第8期8卷 13-16页

作者： Biwu Chu Yan Ding Xiang Gao Junhua Li Tingyu Zhu Yunbo Yu Hong He State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Center for Excellence in Regional Atmospheric Environment Institute of Urban EnvironmentChinese Academy of SciencesXiamen 361021China University of the Chinese Academy of Sciences Beijing 100049China Chinese Research Academy of Environmental Sciences Beijing 100012China State Environmental Protection Engineering Center for Coal-Fired Air Pollution Control Zhejiang UniversityHangzhou 310027China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China National Engineering Laboratory for Hydrometallurgical Cleaner Production Technology Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China

*** In recent years,the air quality in China has improved *** many cities,however,the concentration of fine particulate matter(PM_(2.5))remains higher than the secondary-level national ambient air quality standard(NAAQS level-2,35μg·m^(-3),GB3095-2012[1])and much higher than the first-level NAAQS(15μg·m^(-3),GB3095-2012[1])and the World Health Organization(WHO)air quality guidelines(5μg·m^(-3)).

关键词： pollution Ozone ambient

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Air pollutant emissions induced by rural-to-urban migration during China's urbanization(2005-2015)

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environmental Science and Ecotechnology 2022年第2期10卷 45-53页

作者： Guang Shi Xi Lu Hongxia Zhang Haotian Zheng Zhonghua Zhang Shi Chen Jia Xing Shuxiao Wang State Key Joint Laboratory of Environment Simulation and Pollution Control and School of Environment Tsinghua UniversityBeijing100084PR China Institute for Carbon Neutrality Tsinghua UniversityBeijing100084PR China Beijing Laboratory of Environmental Frontier Technologies Tsinghua UniversityBeijing100084PR China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing100084PR China School of Applied Economics Renmin University of ChinaBeijing100872PR China

As the world's most populous country,China has witnessed rapid urbanization in recent decades,with population migration from rural to urban(RU)regions as the major driving *** to the large gap between rural and urban consumption and investment level,large-scale RU migration impacts air pollutant emissions and creates extra uncertainties for air quality ***,we integrated population migration assessment,an environmentally extended inputeoutput model and structural decomposition analysis to evaluate the NOx,SO2 and primary PM2.5 emissions induced by RU migration during China's urbanization from 2005 to *** results show that RU migration increased air pollutant emissions,while the increases in NOx and SO2 emissions peaked in approximately 2010 at 2.4 Mt and 2.2 Mt,accounting for 9.2%and 8.7%of the national emissions,*** primary PM2.5 emissions induced by RU migration also peaked in approximately 2012 at 0.3 Mt,accounting for 2.8%of the national *** indirect emissions embodied in consumption and investment increased,while household direct emissions *** widening gap between urban and rural investment and consumption exerted a major increasing effect on migration-induced emissions;in contrast,the falling emission intensity contributed the most to the decreasing effect benefitting from end-of-pipe control technology applications as well as improving energy *** peak of air pollutant emissions induced by RU migration indicates that although urbanization currently creates extra environmental pressure in China,it is possible to reconcile urbanization and air quality improvement in the future with updating urbanization and air pollution control policies.

关键词： Urbanization Population migration Air pollutant emission reduction Inputeoutput model Structural decomposition analysis

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Grey Prediction Based Input–Output Model for Analyzing Potential Energy-Related Emission Mitigation Pathways: A Case Study of Fujian 14th

Grey Prediction Based Input–Output Model for Analyzing Pote...

引用

14th International Conference on environmental Science and Technology, ICEST 2023

作者： Sun, Z.M. Liu, J. Li, Y.P. School of Environmental Science and Engineering Xiamen University of Technology Xiamen361024 China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Beijing Normal University Beijing100875 China Faculty of Engineering and Applied Science University of Regina ReginaSKS4S 0A2 Canada

ISBN: (纸本)9783031546839

Economic activities release pollutants and carbon (mainly CO2) directly by consuming energy resources and indirectly by using energy-intensive goods. This research put forwards a grey model (GM) (1, 1) based input–output model (GIOM) for simulating pollutants and CO2 emissions in Fujian Province under varied socio-economic development scenarios. Major findings are: (i) in the planning period, Agriculture, forestry, animal husbandry and fishery (AGR) is the main sector for wastewater emissions in the planning period, and manufacturing and materials and energy conversion (MEC) sectors will be the main sectors for emissions of waste gases and CO2 in the planning period;(ii) through the simulation, the total energy consumption in Fujian Province increases by 13.53–51.08%, Metal and nonmetal products (MAN), MEC and Wholesale and retail transportation and warehousing (WRT) are the main energy consumers;(iii) the COD, NH3–N, SO2, and NOx emissions decrease 24.55–70.11%, 24.53–70.83%, 27.11–70.55% and 22.47–72.00% over time, and the CO2 emissions range from an increase of 36.35% to a decrease of 5.98% over time. © The Author(s), under exclusive license to Springer Nature Switzerland AG 2024.

关键词： Carbon dioxide

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Identifying priority areas of Four Major Chinese carps’ species in the Pearl River basin based on the MaxEnt model

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Watershed Ecology and the Environment 2023年第1期5卷 18-23页

作者： Shao, Xiaojing Liu, Xing Cai, Jie Cai, Yanzi Cui, Baoshan Research Center for Monitoring and Environmental Sciences Taihu Basin & East China Sea Ecological Environment Supervision and Administration Authority Ministry of Ecology and Environment of the People's Republic of China Shanghai 200125 China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Beijing Normal University Beijing 100875 China

The Pearl River basin (PRB) is an important producing area and the gene pool of wild resources of Four Major Chinese carps (FMCC). However human activities and climate changes causes the area shrink of the river network in PRB, the pollution aggregation, the serious habitat destroy of aquatic organisms, and the threat of biological resources and their living environment. Based on the accurate location and distribution data of FMCC from the literature and the field survey report of 2015–2016, this study used the MaxEnt model to predict the hot spot distribution area of FMCC in PRB. The simulation results show that the distribution of FMCC in the PRB gradually increases from the upper reaches to the middle and lower reaches. According to the MaxEnt model, the hot spots of FMCC in the PRB are mainly distributed in the south reaches and the lower reaches of the southeast. The model simulation also demonstrates that the hottest spots for the distribution of FMCC species in the PRB are the Yujiang basin, the Qianjiang basin and the lower reaches of the Xijiang basin. This study can provide the scientific guidance for the protection and the restoration of FMCC species in the PRB. © 2022 The Authors

关键词： Biodiversity MaxEnt model Pearl River basin Prior conservation area

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Chemical characteristics and water stability evaluation of groundwater in the CKDu Zone of Sri Lanka

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Journal of environmental Sciences 2024年第12期146卷 67-80页

作者： Dazhou Hu Suresh Indika Madhubhashini Makehelwala COORAY Titus Liying Zhu Zhonghe Pang Hui Zhong Sujithra K.Weragoda K.B.S.N.Jinadasa Rohan Weerasooriya Yuansong Wei State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Laboratory of Water Pollution Control Technology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China Department of Applied Earth Sciences Uva Wellassa UniversityBadulla 90000Sri Lanka China-Sri Lanka Joint Research and demonstration Center for Water Technology Ministry of Water SupplyE.O.E.Pereira MawathaPeradeniya 24000Sri Lanka National Water Supply and Drainage Board Katugastota 20800Sri Lanka Department of Civil Engineering Faculty of EngineeringUniversity of PeradeniyaPeradeniya 20400Sri Lanka National Institute of Fundamental Studies Kandy 20000Sri Lanka

Groundwater is the main source of drinking water for the rural population in the chronic kidney disease of unknown etiology(CKDu)zone of the North Central Province(NCP)in Sri *** this study,a total of 334 groundwater samples(311 dug wells,21 tube wells and 2 springs)during the wet season from two aquifers in the NCP were collected,and inves-tigated their chemical characteristics and evaluate their water quality,including ground-water chemistry,main ion sources,the corrosion and scaling potential of *** results showed that the two hydrochemical types of groundwater in the NCP were mainly of the Ca-HCO_(3),Na·Ca-HCO_(3)types,with the main HCO_(3)−,Na^(+)and Ca^(2+)ions in both types of groundwater originating from silicate and evaporite salt dissolution and influenced by alternating cation adsorption,while the presence of NO_(3)−was mainly ***-uation ofwater stability using namely Langelier saturation index(LSI),Ryznar stability index(RSI),Puckorius scaling index(PSI)and Larson-Skold index(LS),indicated that most ground-water presents corrosion potential and has corrosion behavior tendency of metals to some *** water quality of Polonnaruwa was better than that of Anuradhapura in the NCP,and when the groundwater was worse than the“good”grade,which must be properly treated before it is used as drinking water.

关键词： CKDu zone Rock weathering Cation alternating adsorption Water stability Water quality assessment

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Evaluation of laboratory and environmental exposure systems for protein modification upon gas pollutants and environmental factors

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Journal of environmental Sciences 2024年第9期143卷 213-223页

作者： Zhiwei Pan ShiyiWu Qiaoze Zhu Fobang Liu Yongjian Liang Chenglei Pei Haoyu Jiang Yingyi Zhang Senchao Lai The Key Lab of Pollution Control and Ecosystem Restoration in Industry Clusters Ministry of EducationSchool of Environment and EnergySouth China University of TechnologyGuangzhou 510006China Department of Environmental Science and Engineering Xi’an Jiaotong UniversityXi’an 710049China Guangzhou Sub-branch of Guangdong Ecological and Environmental Monitoring Center Guangzhou 510006China State Key Laboratory of Organic Geochemistry Guangdong Key Laboratory of Environmental Protection and Resources Utilizationand Joint Laboratory of the Guangdong-Hong Kong-Macao Greater Bay Area for the EnvironmentGuangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou 510640China School of Marine Sciences Sun Yat-sen UniversityZhuhai 519082China

Chemical modifications of proteins induced by ambient ozone(O_(3))and nitrogen oxides(NOx)are of public health concerns due to their potential to trigger respiratory *** laboratory and environmental exposure systems have been widely used to investigate their relevant mechanism in the *** bovine serum albumin(BSA)as a model protein,we evaluated the two systems and aimed to reduce the uncertainties of both the reactants and products in the corresponding kinetic *** the laboratory simulation system,the generated gaseous pollutants showed negligible *** layers of BSA were coated on the flow tube with protein extraction recovery of 87.4%.For environmental exposure experiment,quartz fiber filter was selected as the upper filter with low gaseous O_(3)(8.0%)and NO_(2)(1.7%)losses,and cellulose acetate filter was appropriate for the lower filter with protein extraction efficiency of 95.2%.The protein degradation process was observed without the exposure to atmospheric oxidants and contributed to the loss of protein monomer mass fractions,while environmental factors(e.g.,molecular oxygen and ultraviolet)may cause greater protein monomer *** on the evaluation,the study exemplarily applied the two systems to protein modification and both showed that O_(3) promotes the protein oligomerization and nitration,while increased temperature can accelerate the oligomerization and increased relative humidity can inhibit the nitration in the environmental exposure *** developed laboratory and environmental systems are suitable for studying protein modifications formed under different atmospheric conditions.A combination of the two will further reveal the actual mechanism of protein modifications.

关键词： Protein modification laboratory simulation environmental exposure Oligomerization Nitration

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Variation characteristics of fine particulate matter and its components in diesel vehicle emission plumes

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Journal of environmental Sciences 2021年第9期33卷 138-149页

作者： Xianbao Shen Jiateng Hao Lei Kong Yue Shi Xinyue Cao Jiacheng Shi Zhiliang Yao Xin Li Bobo Wu Yiming Xu Kebin He State Environmental Protection Key Laboratory of Food Chain Pollution Control Beijing Technology and Business UniversityBeijing 100048China Key Laboratory of Cleaner Production and Integrated Resource Utilization of China National Light Industry Beijing Technology and Business UniversityBeijing 100048China School of Ecology and Environment Beijing Technology and Business UniversityBeijing 100048China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China

A rapid reaction occurs near the exhaust nozzle when vehicle emissions contact the *** diesel vehicles were studied using a new multipoint sampling system that is suitable for studying the exhaust plume near the exhaust *** variation characteristics of fine particle matter(PM_(2.5)) and its components in diesel vehicle exhaust plumes were *** PM_(2.5) emissions gradually increased with increasing distance from the nozzle in the *** carbon emissions remained basically unchanged, organic carbon and total carbon(TC) increased with increasing *** concentrations of SO_(4)^(2-),NO_(3)^(-) and NH_(4)^(+) (SNA) directly emitted by the vehicles were very low but increased rapidly in the exhaust *** selective catalytic reduction(SCR) reduced 42.7% TC, 40% NO_(3)^(-) emissions, but increased 104% SO_(4)^(2-) and 36% NH_(4)^(+) emissions, *** summary,the SCR reduced 29% primary PM_(2.5) emissions for the tested diesel *** NH_(4)NO_(3) particle formation maybe more important in the plume, and there maybe other forms of formation of NH_(4)^(+) (***4Cl).The generation of secondary organic carbon(SOC) plays a leading role in the generation of secondary PM_(2.5).The SCR enhanced the formation of SOC and SNA in the plume, but comprehensive analysis shows that the SCR more enhanced the SNA formation in the plume, which is mainly new particles formation *** inconsistency between secondary organic aerosol(SOA) and primary organic aerosol definitions is one of the important reasons for the difference between SOA simulation and observation.

关键词： Variation characteristics Diesel vehicle Emission plume PM2.5 Components

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